期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 10, 期 6, 页码 1372-1376出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ee00751e
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资金
- Swedish Energy Agency
- Knut and Alice Wallenberg Foundation
- Aforsk Foundation [14-452]
- StandUP for energy
- Olle Engkvist Builder Foundation
- China Scholarship Council (CSC)
- CAPES Foundation
In this work, we report a highly efficient organic polymer nano-photocatalyst for light driven proton reduction. The system renders an initial rate of hydrogen evolution up to 50 +/- 0.5 mmol g(-1) h(-1), which is the fastest rate among all other reported organic photocatalysts. We also experimentally and theoretically prove that the nitrogen centre of the benzothiadiazole unit plays a crucial role in the photocatalysis and that the Pdots structure holds a close to ideal geometry to enhance the photocatalysis.
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