期刊
JOURNAL OF THE SERBIAN CHEMICAL SOCIETY
卷 87, 期 3, 页码 345-354出版社
SERBIAN CHEMICAL SOC
DOI: 10.2298/JSC210520050A
关键词
renewable energy; cyclic voltammetry; proton-coupled electron transfer
资金
- Scientific Research Deanship at University of Hail, Kingdom of Saudi Arabia [RG-20072]
The study demonstrates the impressive HER catalytic activity of Cu(II) complexes based on pyridoxal semicarbazone and thiosemicarbazone. The catalytic activity of these complexes is not only determined by the central metal, but also influenced by the coordinating ligand.
The growing global demand for renewable energy sources has pushed renewable, green energy sources to the forefront, among which the production of hydrogen gas from water occupies a significant place. To realize this goal, researchers across the globe are developing various systems that could swiftly catalyze the hydrogen evolution reaction (HER) in the highest possible yield. In the present work, the electrocatalytic HER performances of pyridoxal semi- carbazone-and thiosemicarbazone-based Cu(II) complexes, i.e., ([Cu(PLSC)Cl-2] and [Cu(PLTSC-H)H2O]Br center dot H2O) are reported. It has been unambiguously demonstrated that the complexes exhibit enviable level of HER catalytic act-ivity. The catalytic activity of the complexes was not only the function of cen-tral metal but it was also controlled by the nature of the coordinating ligand.
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