Columnar dipolar clusters defying gravity

A striking and highly versatile feature of magnetic (nano)particles is their ability to be manipulated at will at a distance by external fields. In this paper, the influence of gravity on the self-assembly of dipolar particles near a surface in the presence of a strong vertical magnetic field is investigated theoretically. A rich ground-state phase diagram stems from the effects of the number of particles N and gravity. Two distinct regimes are discovered for the gravity-mediated breakup of a standing chain. When N is small, there is a chain fragmentation (with two widely separated repulsive chain fragments) above a critical value for the gravity, whereas for higher chains, ribbonization (with two cohesive chain fragments) sets in. In both scenarios, simple algebraic decays for the transition gravity as a function of N are analytically predicted and accurately corroborate the exact numerical results. Further intricate chain fragmentations and internal ribbon transformations operate upon further increasing the gravity until all N constitutive particles lie on the surface. Our findings shed additional light on various recent experiments and computer simulations on magnetic colloids and granular media.

Automated summary

This paper theoretically investigates the influence of gravity on the self-assembly of dipolar particles near a surface in the presence of a strong vertical magnetic field and discovers different phenomena such as chain fragmentation and ribbonization. Additionally, it predicts the relationship between gravity and the number of particles, which is in good agreement with experimental data.