☆ 4.8 Review

In Situ/Operando Raman Techniques in Lithium-Sulfur Batteries

SMALL STRUCTURES (2022)

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Review Chemistry, Physical

Host Materials Anchoring Polysulfides in Li-S Batteries Reviewed

Lei Zhou et al.

Summary: Lithium-sulfur batteries are seen as a viable alternative to future energy storage devices due to their high theoretical energy density. However, the main challenge lies in the leakage and migration of sulfur species. Recent research has focused on developing sulfur host materials that can effectively anchor polysulfides for improved battery performance.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Ferroelectric polarization accelerates lithium-ion diffusion for dendrite-free and highly-practical lithium-metal batteries

Lanxin Xue et al.

Summary: In this study, a ferroelectric decoration layer of BiFeO3 nanoparticles was applied on a commercial separator to construct a polarization field, accelerating Li-ion migratory process and effectively eliminating barren areas near the anode surface. This facilitated dense and smooth nucleation of lithium deposition, resulting in long-term stability and high Coulombic efficiency. The use of BFO/PP separator in Li-S pouch cells also showed significant improvements in specific capacity and capacity decay over cycles, demonstrating the potential for highly practical Li metal batteries.

NANO ENERGY (2021)

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Article Chemistry, Physical

Diluted High Concentration Electrolyte with Dual Effects for Practical Lithium-Sulfur Batteries

Zhipeng Jiang et al.

Summary: A modified diluted high concentration electrolyte (MDHCE) was designed for practical Li-S batteries to achieve high energy density and stable cycling. The MDHCE enables high stability and fast Li-ion transport at the hybrid interface, improving the reversibility of Li anode and kinetics of S cathode. The practicality of MDHCE was further demonstrated in a 0.4 Ah Li-S pouch cell with no obvious capacity fading and steady Coulombic efficiency of 99.6%.

ENERGY STORAGE MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Status and Prospects of MXene-Based Lithium-Sulfur Batteries

Qian Zhao et al.

Summary: MXenes, with their metallic conductivity, strong chemical adsorption ability to polysulfides, and effective catalytic effect, show promising potential for high-performance Li-S batteries. Their use in sulfur cathode, interlayer between cathode and separator, and Li anode can enhance electrochemical performance and address challenges in Li-S battery application.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

3D Holey Graphene/Polyacrylonitrile Sulfur Composite Architecture for High Loading Lithium Sulfur Batteries

Tao Wang et al.

Summary: The 3DHG/PS composite cathode for lithium sulfur batteries enhances electron and ion transport speed and reduces volume expansion issues, effectively lowering the fading rate. Moreover, the avoidance of soluble lithium polysulfides formation further reduces the shuttling effect, demonstrating high capacity and rate performance.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

ZnS-SnS@NC Heterostructure as Robust Lithiophilicity and Sulfiphilicity Mediator toward High-Rate and Long-Life Lithium-Sulfur Batteries

Weiqi Yao et al.

Summary: By optimizing the lithiophilicity and sulfiphilicity, the ZnS-SnS@NC heterostructure demonstrates excellent sulfur electrochemistry with high reversibility, high rate performance, and long cycle life. This work provides a feasible scheme for the rational design of bimetal sulfides heterostructures and promotes the development of other electrochemical applications.

ACS NANO (2021)

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Article Energy & Fuels

A high-energy-density and long-life initial-anode-free lithium battery enabled by a Li2O sacrificial agent

Yu Qiao et al.

Summary: Anode-free batteries are promising for high-energy applications, but face challenges with cycling stability due to limited lithium sources. In this study, researchers preloaded Li2O onto the cathode of an initial-anode-free cell to provide additional lithium for offsetting irreversible lithium loss during long-term cycling. By utilizing O-2(-) species released through Li2O oxidation and a fluorinated ether additive, a LiF-based layer was constructed at the cathode/electrolyte interface to passivate the cathode surface and inhibit the detrimental oxidative decomposition of ether solvents. As a result, a long-life 2.46 Ah initial-anode-free pouch cell with a gravimetric energy density of 320 Wh kg(-1) was achieved, maintaining 80% capacity after 300 cycles.

NATURE ENERGY (2021)

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Article Materials Science, Multidisciplinary

Intermetallic interphases in lithium metal and lithium ion batteries

Ke Sun et al.

Summary: A robust electrode-electrolyte interface is crucial for battery systems, especially in the development of new battery technologies. The introduction of artificial Li-alloying intermetallic interphases has significantly improved the stability and performance of lithium metal batteries and solid-state batteries.

INFOMAT (2021)

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Article Materials Science, Multidisciplinary

A flexible metallic TiC nanofiber/vertical graphene 1D/2D heterostructured as active electrocatalyst for advanced Li-S batteries

Yongshang Zhang et al.

Summary: This study developed a flexible Li-S battery architecture based on electrocatalyzed cathodes, which successfully improved the conversion kinetics between sulfur species by enhancing both ion and electron transportation as well as affinity to polysulfides, leading to homogeneous deposition of Li2S in the catalyzed cathodes. The highly active electro-electrocatalysts-based cells exhibited remarkable rate capability and high specific capacity, even under ultra-high sulfur loading and low electrolyte/sulfur ratio conditions.

INFOMAT (2021)

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Article Chemistry, Multidisciplinary

An artificial hybrid interphase for an ultrahigh-rate and practical lithium metal anode

Anjun Hu et al.

Summary: An artificial hybrid SEI layer composed of lithium-antimony alloy and lithium fluoride was constructed to reduce electron tunneling between the Li anode and SEI, resulting in uniform Li deposition and stable Li plating/stripping behaviors at an ultrahigh rate. This work uncovers the internal mechanism of Li+ transport within the SEI component, providing a pathway to stabilize the Li anode under practical high-rate conditions.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Materials Science, Multidisciplinary

Strategies to anode protection in lithium metal battery: A review

Jiawei Li et al.

Summary: Lithium metal batteries show great potential for energy storage, but safety concerns and poor cycling performance due to lithium dendrite growth have led to research on suppressing dendrite growth through strategies such as constructing artificial solid electrolyte interface, current collector modification, separator film improvement, and electrolyte additive.

INFOMAT (2021)

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Review Materials Science, Multidisciplinary

Enabling the thermal stability of solid electrolyte interphase in Li-ion battery

Chenxi Zu et al.

Summary: The thermal safety of lithium-ion batteries is crucial for various applications, and thermal runaway can lead to hazardous incidents and battery pack failures. To enhance the thermal stability of battery systems, building a thermally stable solid/cathode electrolyte interface and incorporating functional components such as stable lithium salts and high boiling point solvents are key measures. In addition, techniques like in-situ polymerization/solidification can enhance the overall stability of the battery system.

INFOMAT (2021)

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Article Chemistry, Physical

Strong intermolecular polarization to boost polysulfide conversion kinetics for high-performance lithium-sulfur batteries†

Yin Hu et al.

Summary: The introduction of CoIn2S4 nanostructured particles as a catalyst boosts the polysulfide conversion kinetics in the Li-S battery, allowing for improved performance at high rates. This study provides insights into a new catalytic mechanism and opens up new pathways for constructing highly practical Li-S batteries.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Hydrogen-substituted graphdiyne/graphene as an sp/sp2 hybridized carbon interlayer for lithium-sulfur batteries

Suzhen Kong et al.

Summary: An all-carbon interlayer with high specific surface area was designed and prepared to overcome the shuttle effect in lithium-sulfur batteries by coating graphene and hydrogen-substituted graphdiyne on a cathode. The material exhibited excellent cycling stability by enabling fast physical adsorption and chemical anchoring of lithium polysulfides, mitigating the shuttling problem and promoting conversion reaction.

NANOSCALE (2021)

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Article Materials Science, Multidisciplinary

Design aspects of electrolytes for fast charge of Li-ion batteries

Sheng S. Zhang

Summary: This article discusses and proposes the design aspects of electrolytes for fast charging of lithium-ion batteries, highlighting how fast charging can exacerbate parasitic reactions and structural degradation of the electrolytes.

INFOMAT (2021)

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Review Chemistry, Multidisciplinary

Present and Future of Surface-Enhanced Raman Scattering

Judith Langer et al.

ACS NANO (2020)

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Article Chemistry, Physical

1T-MoS2 nanotubes wrapped with N-doped graphene as highly-efficient absorbent and electrocatalyst for Li-S batteries

Bo Yu et al.

JOURNAL OF POWER SOURCES (2020)

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Article Chemistry, Physical

Graphene quantum dots as the nucleation sites and interfacial regulator to suppress lithium dendrites for high-loading lithium-sulfur battery

Yin Hu et al.

NANO ENERGY (2020)

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Article Chemistry, Multidisciplinary

Biomimetic Molecule Catalysts to Promote the Conversion of Polysulfides for Advanced Lithium-Sulfur Batteries

Xinwei Ding et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Physical

Ultrathin Lithium Aluminate Nanoflake-Inlaid Sulfur as a Cathode Material for Lithium-Sulfur Batteries with High Areal Capacity

Arnab Ghosh et al.

ACS APPLIED ENERGY MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Coordinating Adsorption and Catalytic Activity of Polysulfide on Hierarchical Integrated Electrodes for High-Performance Flexible Li-S Batteries

Jianbo Li et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Review Materials Science, Multidisciplinary

Interfacial structure design of MXene-basednanomaterials for electrochemical energy storage and conversion

Jianmin Luo et al.

INFOMAT (2020)

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Review Chemistry, Physical

Challenges and Key Parameters of Lithium-Sulfur Batteries on Pouch Cell Level

Susanne Doerfler et al.

JOULE (2020)

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Review Materials Science, Multidisciplinary

One-dimensional and two-dimensional synergized nanostructures for high-performing energy storage and conversion

Xin Li et al.

INFOMAT (2020)

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Article Materials Science, Multidisciplinary

A compact inorganic layer for robust anode protection in lithium-sulfur batteries

Yu-Xing Yao et al.

INFOMAT (2020)

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Review Materials Science, Multidisciplinary

Mechanistic understanding of the role separators playing in advanced lithium-sulfur batteries

Zhaohuan Wei et al.

INFOMAT (2020)

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Review Materials Science, Multidisciplinary

Recent progress in graphene-based electrodes for flexible batteries

Chunlong Dai et al.

INFOMAT (2020)

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Review Chemistry, Multidisciplinary

Recent Advances in Hollow Porous Carbon Materials for Lithium-Sulfur Batteries

Ang Fu et al.

SMALL (2019)

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Article Chemistry, Physical

A robust 2D organic polysulfane nanosheet with grafted polycyclic sulfur for highly reversible and durable lithium-organosulfur batteries

Hao Hu et al.

NANO ENERGY (2019)

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Article Nanoscience & Nanotechnology

Single-Atom Coated Separator for Robust Lithium-Sulfur Batteries

Kun Zhang et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Physical

Superior cycling life of Li-S batteries with high sulfur loading enabled by a bifunctional layered-MoO3 cathode

Ruihan Zhang et al.

JOURNAL OF POWER SOURCES (2019)

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Review Chemistry, Physical

Harnessing the unique properties of 2D materials for advanced lithium-sulfur batteries

Bin Li et al.

NANOSCALE HORIZONS (2019)

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Editorial Material Multidisciplinary Sciences

How lithium dendrites form in liquid batteries

Jie Xiao

SCIENCE (2019)

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Article Multidisciplinary Sciences

Lithiophilic montmorillonite serves as lithium ion reservoir to facilitate uniform lithium deposition

Wei Chen et al.

NATURE COMMUNICATIONS (2019)

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Review Materials Science, Multidisciplinary

A review of rechargeable batteries for portable electronic devices

Yeru Liang et al.

INFOMAT (2019)

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Article Chemistry, Multidisciplinary

Direct tracking of the polysulfide shuttling and interfacial evolution in all-solid-state lithium-sulfur batteries: a degradation mechanism study

Yue-Xian Song et al.

ENERGY & ENVIRONMENTAL SCIENCE (2019)

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Article Materials Science, Multidisciplinary

Expediting redox kinetics of sulfur species by atomic-scale electrocatalysts in lithium-sulfur batteries

Bo-Quan Li et al.

INFOMAT (2019)

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Review Chemistry, Multidisciplinary

In situ optical spectroscopy characterization for optimal design of lithium-sulfur batteries

Li Zhang et al.

CHEMICAL SOCIETY REVIEWS (2019)

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Article Chemistry, Physical

The Role of Metal Disulfide Interlayer in Li-S Batteries

Andrea Paolella et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2018)

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Review Chemistry, Multidisciplinary

Development and Challenges of Functional Electrolytes for High-Performance Lithium-Sulfur Batteries

Lili Wang et al.

ADVANCED FUNCTIONAL MATERIALS (2018)

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News Item Multidisciplinary Sciences

ELECTROCHEMISTRY Lithium-sulfur batteries poised for leap

Robert F. Service

SCIENCE (2018)

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Article Chemistry, Physical

Direct impregnation of SeS2 into a MOF-derived 3D nanoporous Co-N-C architecture towards superior rechargeable lithium batteries

Jiarui He et al.

JOURNAL OF MATERIALS CHEMISTRY A (2018)

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Article Chemistry, Physical

Regulating the polysulfide redox conversion by iron phosphide nanocrystals for high-rate and ultrastable lithium-sulfur battery

Shaozhuan Huang et al.

NANO ENERGY (2018)

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Article Chemistry, Multidisciplinary

Confined Lithium-Sulfur Reactions in Narrow-Diameter Carbon Nanotubes Reveal Enhanced Electrochemical Reactivity

Chengyin Fu et al.

ACS NANO (2018)

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Review Materials Science, Multidisciplinary

Revisiting Scientific Issues for Industrial Applications of Lithium-Sulfur Batteries

Bo Liu et al.

ENERGY & ENVIRONMENTAL MATERIALS (2018)

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Review Chemistry, Physical

Sulfur Hosts against the Shuttle Effect

Yazhou Wang et al.

SMALL METHODS (2018)

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Review Chemistry, Multidisciplinary

In situ/operando characterization techniques for rechargeable lithium-sulfur batteries: a review

Jian Tan et al.

NANOSCALE (2017)

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Review Chemistry, Physical

Effective strategies for stabilizing sulfur for advanced lithium-sulfur batteries

Ogechi Ogoke et al.

JOURNAL OF MATERIALS CHEMISTRY A (2017)

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Article Chemistry, Physical

Thiol-based electrolyte additives for high-performance lithium-sulfur batteries

Heng-Liang Wu et al.

NANO ENERGY (2017)

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Article Energy & Fuels

Burning lithium in CS2 for high-performing compact Li2S-graphene nanocapsules for Li-S batteries

Guoqiang Tan et al.

NATURE ENERGY (2017)

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Article Chemistry, Physical

Investigation of the reaction mechanism of lithium sulfur batteries in different electrolyte systems by in situ Raman spectroscopy and in situ X-ray diffraction

W. Zhu et al.

SUSTAINABLE ENERGY & FUELS (2017)

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Review Chemistry, Multidisciplinary

Anode Improvement in Rechargeable Lithium-Sulfur Batteries

Tao Tao et al.

ADVANCED MATERIALS (2017)

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Review Chemistry, Physical

A Toolbox for Lithium-Sulfur Battery Research: Methods and Protocols

Ge Zhang et al.

SMALL METHODS (2017)

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Article Chemistry, Physical

In Situ Chemical Imaging of Solid-Electrolyte Interphase Layer Evolution in Li-S Batteries

Manjula I. Nandasiri et al.

CHEMISTRY OF MATERIALS (2017)

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Review Chemistry, Multidisciplinary

Nanostructured Metal Oxides and Sulfides for Lithium-Sulfur Batteries

Xue Liu et al.

ADVANCED MATERIALS (2017)

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Article Chemistry, Physical

In operando scanning electron microscopy and ultraviolet-visible spectroscopy studies of lithium/sulfur cells using all solid-state polymer electrolyte

Hugues Marceau et al.

JOURNAL OF POWER SOURCES (2016)

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Article Chemistry, Multidisciplinary

Nitrogen Rich Hierarchically Organized Porous Carbon/Sulfur Composite Cathode Electrode for High Performance Li/S Battery: A Mechanistic Investigation by Operando Spectroscopic Studies

Bhaghavathi Parambath Vinayan et al.

ADVANCED MATERIALS INTERFACES (2016)

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Review Nanoscience & Nanotechnology

Nanostructure-based plasmon-enhanced Raman spectroscopy for surface analysis of materials

Song-Yuan Ding et al.

NATURE REVIEWS MATERIALS (2016)

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Article Nanoscience & Nanotechnology

In Situ Raman Spectroscopy of Sulfur Speciation in Lithium-Sulfur Batteries

Heng-Liang Wu et al.

ACS APPLIED MATERIALS & INTERFACES (2015)

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Article Chemistry, Physical

Conductive Lewis Base Matrix to Recover the Missing Link of Li2S8 during the Sulfur Redox Cycle in Li-S Battery

Jia-Jia Chen et al.

CHEMISTRY OF MATERIALS (2015)

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Article Physics, Atomic, Molecular & Chemical

The Quest for Polysulfides in Lithium-Sulfur Battery Electrolytes: An Operando Confocal Raman Spectroscopy Study

Julien Hannauer et al.

CHEMPHYSCHEM (2015)

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Review Chemistry, Multidisciplinary

Lithium sulfur batteries, a mechanistic review

M. Wild et al.

ENERGY & ENVIRONMENTAL SCIENCE (2015)

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Article Chemistry, Physical

On the reasons for low sulphur utilization in the lithium-sulphur batteries

V. S. Kolosnitsyn et al.

JOURNAL OF POWER SOURCES (2015)

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Article Chemistry, Multidisciplinary

Electrochemical (De)Lithiation of 1D Sulfur Chains in Li-S Batteries: A Model System Study

Chun-Peng Yang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2015)

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Article Chemistry, Multidisciplinary

Following the Transient Reactions in Lithium-Sulfur Batteries Using an In Situ Nuclear Magnetic Resonance Technique

Jie Xiao et al.

NANO LETTERS (2015)

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Article Multidisciplinary Sciences

A highly efficient polysulfide mediator for lithium-sulfur batteries

Xiao Liang et al.

NATURE COMMUNICATIONS (2015)

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Article Multidisciplinary Sciences

Two-dimensional layered transition metal disulphides for effective encapsulation of high-capacity lithium sulphide cathodes

Zhi Wei Seh et al.

NATURE COMMUNICATIONS (2014)

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Article Chemistry, Multidisciplinary

Mechanistic insights into operational lithium-sulfur batteries by in situ X-ray diffraction and absorption spectroscopy

Michael A. Lowe et al.

RSC ADVANCES (2014)

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Article Nanoscience & Nanotechnology

Mesoporous Carbon-Carbon Nanotube-Sulfur Composite Microspheres for High-Areal-Capacity Lithium-Sulfur Battery Cathodes

Terrence Xu et al.

ACS APPLIED MATERIALS & INTERFACES (2013)

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Article Electrochemistry

In-Situ Raman Investigation of Polysulfide Formation in Li-S Cells

M. Hagen et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2013)

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Article Biochemical Research Methods

Surface analysis using shell-isolated nanoparticle-enhanced Raman spectroscopy

Jian Feng Li et al.

NATURE PROTOCOLS (2013)

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Review Biochemical Research Methods

Surface-enhanced Raman spectroscopy (SERS): progress and trends

Dana Cialla et al.

ANALYTICAL AND BIOANALYTICAL CHEMISTRY (2012)

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Review Geochemistry & Geophysics

Raman spectroscopy for fluid inclusion analysis

Maria Luce Frezzotti et al.

JOURNAL OF GEOCHEMICAL EXPLORATION (2012)

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Article Chemistry, Multidisciplinary

In Operando X-ray Diffraction and Transmission X-ray Microscopy of Lithium Sulfur Batteries

Johanna Nelson et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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Article Electrochemistry

Lithium-sulfur batteries: Problems and solutions

V. S. Kolosnitsyn et al.

RUSSIAN JOURNAL OF ELECTROCHEMISTRY (2008)

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