☆ 4.7 Review

A review on the application of perovskite as peroxymonosulfate activator for organic pollutants removal

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2022)

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Article Engineering, Environmental

Anionic ligands driven efficient ofloxacin degradation over LaMnO3 suspended particles in water due to the enhanced peroxymonosulfate activation

Yulun Nie et al.

Summary: This study explored the effects of organic ligands on the PMS activation performance of inorganic metal-based particles, revealing significant differences in the degradation efficiency of OFX depending on the type of ligand present. The study found that different molecular structures of organic ligands played a key role in influencing the activation process and subsequent degradation efficiency.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Enhanced redox activity and oxygen vacancies of perovskite triggered by copper incorporation for the improvement of electro-Fenton activity

Liangbo Xie et al.

Summary: ABO3 perovskite oxides doped with cation substitutions have been shown to alter the electronic and structural properties of perovskites. In this study, Cu was incorporated into LaCoO3 perovskite to act as a heterogeneous EF catalyst for the almost complete removal of the target pollutant ciprofloxacin within 120 minutes. The results demonstrated that the incorporation of Cu improved EF activity by enhancing redox activity and oxygen vacancies of LaCoxCu1_xO3_delta, leading to the activation of hydrogen peroxide and increased production of hydroxyl radicals and superoxide free radicals. Additionally, the degradation mechanism of LaCoxCu1_xO3_delta was investigated, highlighting the important role of cation substitutions in perovskite oxides for improving heterogeneous EF activity.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Applied

Adsorption behavior and mechanism of mixed heavy metal ions by zeolite adsorbent prepared from lithium leach residue

Yingwei Lv et al.

Summary: In this study, zeolite NaA was prepared from lithium leach residue (LLR) using the traditional hydrothermal synthesis method, and its adsorption performance on Pb2+ and Cd2+ in heavy metal wastewater was investigated. The results showed that zeolite NaA exhibited excellent adsorption properties for Pb2+ and Cd2+, and the adsorption process followed the Langmuir model and pseudo-second-order model. The adsorption mechanism was attributed to ion exchange and hydroxyl groups on the zeolite NaA surface.

MICROPOROUS AND MESOPOROUS MATERIALS (2022)

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Review Engineering, Chemical

A review on heavy metal ions adsorption from water by layered double hydroxide and its composites

Xiaofang Feng et al.

Summary: This study provides a comprehensive review of the recent developments in the use of functionalized layered double hydroxide (LDH) as heavy metal adsorption materials, highlighting the lack of research on LDH-based nanomaterials in heavy metal removal.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Engineering, Environmental

Enhanced heterogeneous activation of peroxymonosulfate by Ruddlesden-Popper-type La2CoO4+δ nanoparticles for bisphenol A degradation

Mohaned Hammad et al.

Summary: The study presents a facile and efficient synthesis method for high-performance La2CoO4+delta nanoparticles using a spray-flame technique, demonstrating significant catalytic activity and chemical stability in PMS-assisted oxidation of organic pollutants. Results show that the La2CoO4+delta catalyst exhibits higher catalytic degradation efficiency in the PMS system and maintains low cobalt leaching, highlighting its potential as a stable and active heterogeneous catalyst.

CHEMICAL ENGINEERING JOURNAL (2022)

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Review Chemistry, Applied

Perovskite-type lanthanum ferrite based photocatalysts: Preparation, properties, and applications

Muhammad Humayun et al.

Summary: This article discusses the use of LaFeO3 as a photocatalyst in addressing solar energy conversion and environmental purification. It focuses on the characteristics, applications, and strategies for enhancing the activity of LaFeO3.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Applied

Heterogeneous activation of persulfate by lanthanum strontium cobaltite for sulfamethoxazole degradation

C. Gkika et al.

Summary: This study investigates the degradation of sulfamethoxazole (SMX) using La0.8Sr0.2CoO3-δ (LSC) perovskite oxide activated by sodium persulfate (SPS). LSC showed high activity in catalyzing SPS and resulted in complete SMX degradation. Experiments in bottled water and secondary treated wastewater revealed the existence of retarding phenomena in SMX degradation, prompting further investigation.

CATALYSIS TODAY (2021)

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Article Engineering, Environmental

Perovskite LaFexCo1-xO3-λ deposited SiO2 catalytic membrane for deeply cleaning wastewater

Longfei Zhang et al.

Summary: A perovskite LaFexCo1-xO3-lambda deposited SiO2 catalytic membrane (PCM) was prepared with modified functional layer containing Fe, which exhibited excellent catalytic oxidation and membrane separation abilities. The PCM showed promising performance in water treatment, with high water yield and degrading efficiency for pollutants.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Engineering, Environmental

A review of the innovations in metal- and carbon-based catalysts explored for heterogeneous peroxymonosulfate (PMS) activation, with focus on radical vs . non-radical degradation pathways of organic contaminants

Mona Kohantorabi et al.

Summary: This review summarizes the rapid development of heterogeneous catalysts for peroxymonosulfate (PMS) activation in sulfate radical-based AOPs, covering various catalysts and discussing their roles in the activation mechanism.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Composition-engineered LaCoO3-based monolithic catalysts for easily operational and robust peroxymonosulfate activation

Qihui Pan et al.

Summary: This study reports the construction of perovskite oxide catalysts on monolithic supports for peroxymonosulfate (PMS) activation to eliminate organic pollutants in wastewater for the first time. The resulting monolithic catalysts showed large sizes, highly porous architectures, and compositionally favorable active components, leading to easy catalyst recycling, rapid mass transfer, and high catalytic performance in degradation of antibiotic pollutants. Optimizing the introduction amount of Ca and Ti resulted in improved catalytic activity and reduced cobalt leaching compared to unmodified catalysts.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

New insights into Sr-O bonds enhances Co/Fe catalytic activity in SrCoFe perovskite for boosted peroxymonosulfate activation

Dan Yu et al.

Summary: The study identified the crucial role of Sr-O bond in boosting the catalytic activity of SrCo0.81Fe0.19O2.78 perovskite, where oxygen vacancy, Fe4+/Fe3+, and Co3+/Co2+ redox cycles synergistically enhanced catalytic activity. The Sr-O ionic bond was found to provide electrons for CoO and Fe-O covalent bonds, accelerating Fe4+/Fe3+ and Co3+/Co2+ redox cycles for PMS activation, leading to efficient removal of antibiotics.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Chemical

Interface engineered perovskite oxides for enhanced catalytic oxidation: The vital role of lattice oxygen

Xue Ma et al.

Summary: In this study, nanocomposites of La1.15NiO3 were synthesized through a facile one-pot method, showing high catalytic activity and excellent stability in advanced oxidation processes. The performance improvement is mainly attributed to the generation of more oxygen vacancies and reactive oxygen species in La1.15NiO3.

CHEMICAL ENGINEERING SCIENCE (2021)

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Article Chemistry, Physical

Microwave-assisted synthesis of blue-emitting cesium bismuth bromine perovskite nanocrystals without polar solvent

Heng Pan et al.

Summary: A microwave-assisted method was used to synthesize non-toxic and stable Cs3Bi2Br9 perovskite nanocrystals with efficient blue emission. The passivation of surface trap-states by BiOBr led to a significant increase in photoluminescence quantum yield. These lead-free perovskite nanocrystals show great potential for solid-state lighting applications.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Engineering, Environmental

Enhanced catalytic activity of series LaCuxFe1-xO3 (x=0.2, 0.4, 0.6, 0.8) perovskite-like catalyst for the treatment of highly toxic ABS resin wastewater: Phytotoxicity study, parameter optimization andreaction pathways

Arvind Kumar et al.

Summary: In this study, ABS resin wastewater was treated using LaCuxFe1xO3 perovskite-like catalyst activated with PMS. High removal efficiency of acrylonitrile and TOC was achieved under optimized conditions, and the reaction kinetics, catalyst reusability, and reaction pathways were investigated.

PROCESS SAFETY AND ENVIRONMENTAL PROTECTION (2021)

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Article Environmental Sciences

Highly efficient removal of bisphenol A by a novel Co-doped LaFeO3 perovskite/PMS system in salinity water

Jiana Jing et al.

Summary: The newly synthesized LaCo0.5Fe0.5O3 microns were effective in degrading BPA, even in the presence of 50 mM Cl- in salty water. Reactive chlorine species and radicals generated by LaCo0.5Fe0.5O3 activation of PMS played a crucial role in promoting the degradation of BPA.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Engineering, Chemical

Mechanistic approach of SO4•-/•OH radical toward target pollutants degradation simultaneously enhanced activity and stability of perovskite-like catalyst SrCuxNi1-xO3

Arvind Kumar et al.

Summary: This study systematically investigated the degradation of highly toxic pollutants ACN and ACM by activating with PMS and series perovskite-like catalysts. Catalyst 0.6SCN showed the highest catalytic activity, achieving 96% removal of ACN and 81% removal of ACM with 86% PMS consumption. The in-situ generated reactive species were responsible for the synergistic removal of ACN and ACM in the 0.6SCN/PMS system, as revealed by EPR and quenching experimental studies. Overall, the operating cost of the treatment process was assessed at 50.62$/m(3) in the 0.6SCN/PMS system.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Chemical

Enhanced activation of peroxymonosulfate by Sr-doped LaFeO3 perovskite for Orange I degradation in the water

Ying Zhao et al.

Summary: A-site doping of perovskite with Sr in LaFeO3 perovskites enhanced catalytic activity and stability, leading to improved PMS activation and Orange I degradation. The modified surface properties resulted in efficient electron transfer and ROS generation, ensuring continuous catalytic performance. LSFO-40 showed great potential for practical wastewater treatment with negligible inhibitory effects under a wide pH range and co-existing anions.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Chemistry, Physical

Understanding oxygen-deficient La2CuO4-δ perovskite activated peroxymonosulfate for bisphenol A degradation: The role of localized electron within oxygen vacancy

Hanxiao Chen et al.

Summary: An A(2)BO(4)-type oxygen-deficient perovskite (La2CuO4-delta, LCO) shows superior low-temperature reducibility and more abundant oxygen vacancies (OVs) compared to CuO oxide, and was successfully used in peroxymonosulfate (PMS) activation for more than 96% BPA removal within 60 mM over a wide pH range. The activation mechanism involves surface Cu(II)/Cu (I) redox couple, lattice oxygen (O2-)/O-2, and direct activation of PMS by OVs with localized electrons.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Environmental

Cation deficiency tuned LaCoO3-δ perovskite for peroxymonosulfate activation towards bisphenol A degradation

Ping Liang et al.

Summary: This study prepared cation deficient LaCoO3-delta perovskite oxides to regulate their catalytic activity towards peroxymonosulfate (PMS) activation. It was found that B-site cation deficiency promotes catalytic performance and can efficiently mineralize organic compounds.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Enhanced Fenton-like efficiency by the synergistic effect of oxygen vacancies and organics adsorption on FexOy-d-g-C3N4 with Fe-N complexation

Yumeng Wang et al.

Summary: The d-g-C3N4-Fe composite material was prepared via a self-assembly and calcination process, demonstrating high degradation efficiency for hydroxyl-containing and hydrophobic pollutants. The Fe(III)-pi interaction on the catalyst surface can oxidize pollutants and decrease the consumption of H2O2, while the role of OVs depends on pollutant adsorption patterns.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Engineering, Environmental

Peroxymonosulfate/LaCoO3 system for tetracycline degradation: Performance and effects of co-existing inorganic anions and natural organic matter

Xue Yang et al.

Summary: The activation of peroxymonosulfate (PMS) by LaCoO3 is an efficient method for degrading tetracycline (TC) by generating reactive oxygen species (ROS). The presence of inorganic anions and low concentration of natural organic matter can enhance the degradation efficiency, while LaCoO3 shows stable reusability.

JOURNAL OF WATER PROCESS ENGINEERING (2021)

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Review Engineering, Environmental

Strategies for improving perovskite photocatalysts reactivity for organic pollutants degradation: A review on recent progress

Kexin Wei et al.

Summary: This review summarizes recent progress in tuning strategies and coupling Advanced Oxidation Processes (AOPs) methods to improve perovskite photocatalyst reactivity for water decontamination. It introduces general principles of designing perovskite photocatalysts for water decontamination and discusses diverse strategies to enhance perovskite photocatalytic activity. Additionally, it presents the rapid development of coupling various AOPs with perovskite for improved water remediation and discusses remaining challenges and future directions for practical perovskite photocatalytic water purification.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Copper in LaMnO3 to promote peroxymonosulfate activation by regulating the reactive oxygen species in sulfamethoxazole degradation

Panpan Gao et al.

Summary: This study investigated the role of copper in promoting PMS activation performance of LaMnO3 for efficient degradation of SMX in water treatment. The results showed that Cu-LaMnO3 could regulate the production of reactive oxygen species (ROS) and achieve radical dominant PMS activation mechanism, leading to enhanced catalytic activity compared to LaMnO3 alone. This study provides new insights for improving the catalytic activity of perovskites in PMS activation in water treatment.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Review Chemistry, Physical

Synthesis and application of perovskite-based photocatalysts in environmental remediation: A review

Huifang Wang et al.

Summary: This review paper comprehensively discusses the recent advances of perovskite-based materials in environmental remediation, providing suggestions for future challenges and utilization. It emphasizes the importance of photocatalysis in utilizing solar energy and its potential for cleaning up the environment.

JOURNAL OF MOLECULAR LIQUIDS (2021)

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Article Biotechnology & Applied Microbiology

Recent developments on hybrid perovskite materials for solar energy conversion and environmental protection

Andreas Kaltzoglou et al.

Summary: Halide perovskites have shown promising progress in solar cells and photocatalysis, with power conversion efficiency exceeding 25%. However, current focus is on improving the stability of these materials. Additionally, their photocatalytic efficiency has led to new applications in CO2 reduction, H-2 evolution, organic synthesis, and pollutants photodecomposition. Best materials and engineering methods have brought devices closer to commercial use than ever before.

CURRENT OPINION IN CHEMICAL ENGINEERING (2021)

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Review Chemistry, Multidisciplinary

Towards the environmentally friendly solution processing of metal halide perovskite technology

Minh Tam Hoang et al.

Summary: Metal halide perovskite materials show unique properties for optoelectrical devices, but the use of hazardous solvents limits their commercialization. Developing environmentally-friendly solvents is critical for the commercial uptake of perovskite technology.

GREEN CHEMISTRY (2021)

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Article Engineering, Environmental

Enhanced performance of LaFeO3 perovskite for peroxymonosulfate activation through strontium doping towards 2,4-D degradation

Cheng Cheng et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Room-Temperature Synthesis of High-Entropy Perovskite Oxide Nanoparticle Catalysts through Ultrasonication-Based Method

Francis Okejiri et al.

CHEMSUSCHEM (2020)

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Fabrication of GdFO3-Carbon nanotubes nanocomposites for enhanced photocatalytic applications

Aysha Daud et al.

CERAMICS INTERNATIONAL (2020)

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Postsynthesis Oxygen Nonstoichiometric Regulation: A New Strategy for Performance Enhancement of Perovskites in Advanced Oxidation

Jie Miao et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Critical role of oxygen vacancies in heterogeneous Fenton oxidation over ceria-based catalysts

Nuanqin Zhang et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2020)

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Article Chemistry, Physical

Effective promotion of oxygen reduction activity by rare earth doping in simple perovskite cathodes for intermediate-temperature solid oxide fuel cells

Wenwen Zhang et al.

JOURNAL OF POWER SOURCES (2020)

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3D hollow sphere-like Cu-incorporated LaAlO3 perovskites for peroxymonosulfate activation: Coaction of electron transfer and oxygen defect

Ting Chen et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Carbamazepine degradation by heterogeneous activation of peroxymonosulfate with lanthanum cobaltite perovskite: Performance, mechanism and toxicity

Huichao Guo et al.

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MXene-Ti3C2 assisted one-step synthesis of carbon-supported TiO2/Bi4NbO8Cl heterostructures for enhanced photocatalytic water decontamination

Daixun Jiang et al.

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Enhanced activation of peroxydisulfate by CuO decorated on hexagonal boron nitride for bisphenol A removal

Wen-Da Oh et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Surface oxygen vacancy inducing peroxymonosulfate activation through electron donation of pollutants over cobalt-zinc ferrite for water purification

Hongxiang Zhang et al.

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Mechanism insight of dual synergistic effects of plasmonic Pd-SrTiO3for enhanced solar energy photocatalysis

Ping Feng Lim et al.

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Strategy for Modifying Layered Perovskites toward Efficient Solar Light-Driven Photocatalysts for Removal of Chlorinated Pollutants

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Metal-organic frameworks-derived perovskite catalysts for efficient degradation of 2, 4-dichlorophenol via peroxymonosulfate activation

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A facile, environmentally friendly synthesis of strong photo-emissive methylammonium lead bromide perovskite nanocrystals enabled by ionic liquids

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Sonia Rani et al.

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The role of oxygen vacancies of ABO3 perovskite oxides in the oxygen reduction reaction

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ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Review Engineering, Environmental

Design and application of heterogeneous catalysts as peroxydisulfate activator for organics removal: An overview

Wen-Da Oh et al.

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Promoted peroxymonosulfate activation into singlet oxygen over perovskite for ofloxacin degradation by controlling the oxygen defect concentration

Panpan Gao et al.

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Efficient degradation of diclofenac by LaFeO3-Catalyzed peroxymonosulfate oxidation-kinetics and toxicity assessment

Yongfang Rao et al.

CHEMOSPHERE (2019)

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Heterogeneous activation of peroxymonosulfate via a Ag-La0.8Ca0.2Fe0.94O3-δ perovskite hollow fibre membrane reactor for dye degradation

Teng Ma et al.

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Influence of carbonate on sequestration of U(VI) on perovskite

Songhua Lu et al.

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A review of recent advances in catalytic combustion of VOCs on perovskite-type catalysts

Meng Zang et al.

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Stable and Highly Efficient Photocatalysis with Lead-Free Double-Perovskite of Cs2AgBiBr6

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Oxygen vacancy mediated La1-xCexFeO3-δ perovskite oxides as efficient catalysts for CWAO of acrylic acid by A-site Ce doping

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Enhanced activation of peroxymonosulfte by LaFeO3 perovskite supported on Al2O3 for degradation of organic pollutants

Shaohua Wu et al.

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A framework for optimizing oxygen vacancy formation in doped perovskites

Christopher L. Hanselman et al.

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Facile synthesis of perovskite LaFeO3 ferroelectric nanostructures for heavy metal ion removal applications

Martha Purnachander Rao et al.

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Enhanced degradation of atrazine by nanoscale LaFe1-xCuxO3-δ perovskite activated peroxymonosulfate: Performance and mechanism

Guoying Wang et al.

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Ordered Mesoporous Cobalt Containing Perovskite as a High-Performance Heterogeneous Catalyst in Activation of Peroxymonosulfate

Xinsheng Luo et al.

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A systematic investigation on morphology tailoring, defect tuning and visible-light photocatalytic functionality of Ti-based perovskite nanostructures

Reshalaiti Hailili et al.

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Effective steering of charge flow through synergistic inducing oxygen vacancy defects and p-n heterojunctions in 2D/2D surface-engineered Bi2WO6/BiOI cascade: Towards superior photocatalytic CO2 reduction activity

Xin Ying Kong et al.

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Efficient degradation of atrazine by LaCoO3/Al2O3 catalyzed peroxymonosulfate: Performance, degradation intermediates and mechanism

Renjing Zhang et al.

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Effect of Fe and Bi doping on LaCoO3 structural, magnetic, electric and catalytic properties

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Crystal structure and photocatalytic properties of perovskite MSn(OH)6 (M = Cu and Zn) composites with d10-d10 configuration

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Low temperature crystal growth of lead-free complex perovskite nano-structure by using sol-gel hydrothermal process

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Mechanochemical synthesis of inorganic halide perovskites: evolution of phase-purity, morphology, and photoluminescence

Francisco Palazon et al.

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Will organic-inorganic hybrid halide lead perovskites be eliminated from optoelectronic applications?

Zijun Yi et al.

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Insights into perovskite-catalyzed peroxymonosulfate activation: Maneuverable cobalt sites for promoted evolution of sulfate radicals

Xiaoguang Duan et al.

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Effect of the metal type in perovskites prepared by modified proteic method in dye adsorption from aqueous medium

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Enhanced photocatalytic activity of layered perovskite oxides Sr(2.7-x)Ca(x)Ln(0.3)Fe(2)O(7-delta) for MB degradation

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