期刊
ACS SENSORS
卷 1, 期 7, 页码 842-846出版社
AMER CHEMICAL SOC
DOI: 10.1021/acssensors.6b00209
关键词
ricin; surface-enhanced raman spectroscopy; glycopolymers; film over nanospheres; DFT modeling
资金
- National Science Foundation through the University of Minnesota Materials Science Research and Engineering Center [DMR-1420013]
- NSF through the MRSEC program
- NSF through the NNIN program
- NSF GRFP [DGE-1324585]
- MRSEC program at Northwestern University [DMR-1121262]
A novel sensing scheme is exemplified through the detection of ricin B-chain (RBC) in water and liquid food matrices: surface-enhanced Raman spectroscopy (SERS) coupled with an N-acetyl-galactosamine glycopolymer capture layer. The sensing scheme's detection limit was well below that of the predicted oral exposure limit. Theoretical predictions of the normal Raman spectrum of the glycomonomer give insight into polymer-RBC intermolecular interactions.
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