期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 10, 期 20, 页码 10837-10843出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2ta01544g
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资金
- National Key Research and Development Program Nanotechnology Specific Project [2020YFA0210900]
- National Natural Science Foundation of China [21908255, 22078371, 22108315, 21938001, 22078072, 21961160741]
- Guangdong Provincial Key RD Programme [2019B110206002]
- Special fund for Local Science and Technology Development by the Central Government
- Local Innovative and Research Teams Project of the Guangdong Pearl River Talents Program [2017BT01C102]
- Guangdong Natural Science Funds for Distinguished Young Scholar [2022B1515020035]
- NSF of Guangdong Province [2020A1515011141]
- Science and Technology Key Project of Guangdong Province, China [2020B010188002]
- Basic and Applied basic research program of Guangzhou City [202102020461]
- Guangdong Basic and Applied Basic Research Foundation [2020A1515110864]
Pt1/Co3O4-c catalysts exhibit great catalytic activities in hydrolytic dehydrogenation, with electron depletion of single-atomic Pt species tailored by supports.
The Pt1/Co3O4-c catalysts exhibit great catalytic activities in hydrolytic dehydrogenation of ammonia borane (AB) with a specific rate of 6035 molH2 molPt-1 min-1 at room temperature. In situ DRIFTS spectra and theoretical calculations illustrate the chemisorption form of H3N-BH3MIDLINE HORIZONTAL ELLIPSISPt1/Co3O4-c due to the electron depletion of single-atomic Pt species tailoring by supports.
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