期刊
ORGANIC CHEMISTRY FRONTIERS
卷 9, 期 13, 页码 3473-3479出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2qo00466f
关键词
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资金
- Taishan Scholars Construction Projects of Shandong [tsqn201812075]
- Natural Science Foundation of Shandong Province for Distinguished Young Scholars [ZR2020JQ07]
- Youth Innovation Science and Technology Plan of Colleges and Universities in Shandong Province [2019KJC003]
- Natural Science Foundation of China [21702115]
- Natural Science Foundation of Shandong Province, China [ZR2017BB028, ZR2019PB020, ZR2019MB010]
- Qingdao University of Science Technology
An efficient solvent-free radical oxyamination reaction has been demonstrated for the modification of carbonyl compounds adjacent to different chalcogens (e.g., S, O, and Se). This method does not require the use of a transition metal catalyst, chemical oxidant, or photocatalyst, and exhibits a wide substrate scope and high functional group tolerance.
An efficient radical C(sp(3))-H alpha-oxyamination of carbonyls adjacent to different chalcogens (e.g., S, O, and Se) at the alpha-position is demonstrated. This radical oxyamination process proceeds under solvent-free conditions without the use of a transition metal catalyst, chemical oxidant or photocatalyst and exhibits a wide substrate scope of chalcogen-containing carbonyls with high functional group tolerance.
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