期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 20, 期 21, 页码 4314-4319出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2ob00439a
关键词
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资金
- National Science Foundation [1856522]
- National Institutes of Health, National Institute of General Medical Sciences [R01 GM128659]
Resin-immobilized catalysts prepared through chirality-driven self-assembly allow for regeneration under mild conditions and quantitative in situ catalyst exchange. The uniqueness of the methodology was demonstrated by preparing a catalyst for TEMPO oxidation and enabling a two-step sequential TEMPO oxidation/aldol condensation sequence with facile catalyst exchange.
Resin-immobilized catalysts were prepared through chirality-driven self-assembly. The method allows the resin-immobilized catalyst to be regenerated under mild conditions and in situ catalyst exchange to be carried out quantitatively. The uniqueness of the methodology was demonstrated by the preparation of a catalyst for TEMPO oxidation as well as a two-step sequential TEMPO oxidation/aldol condensation sequence enabled by facile catalyst exchange.
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