☆ 4.8 Review

Manganese-catalyzed hydrogenation, dehydrogenation, and hydroelementation reactions

CHEMICAL SOCIETY REVIEWS (2022)

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Article Chemistry, Applied

Hydrogenation of Esters by Manganese Catalysts

Xiao-Gen Li et al.

Summary: The hydrogenation of esters catalyzed by a manganese complex of phosphine-aminopyridine ligand was developed. A variety of esters, including biomass-derived esters and lactones, can be efficiently hydrogenated to primary alcohols with yields of 63-98%. The manganese catalyst showed high activity for the hydrogenation of methyl benzoate, with turnover numbers (TON) as high as 45,000. Investigation of catalyst intermediates revealed that the amido manganese complex is the active species for the reaction.

ADVANCED SYNTHESIS & CATALYSIS (2022)

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Article Chemistry, Physical

Manganese-Catalyzed Hydrogenation of Sclareolide to Ambradiol

Viktoriia Zubar et al.

Summary: The hydrogenation of (+)-Sclareolide to (-)-ambradiol catalyzed by a manganese pincer complex was achieved with high yield. The catalyst is easy to prepare, and the reaction conditions are relatively mild, with reproducible experimental results.

CHEMCATCHEM (2022)

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Article Chemistry, Multidisciplinary

Manganese(i)-catalyzed access to 1,2-bisphosphine ligands

Luo Ge et al.

Summary: Chiral bisphosphine ligands play a key role in transition-metal-catalyzed asymmetric synthesis. However, the commonly used transition metals are expensive and scarce, and the synthesis of chiral phosphine ligands is complex. In this study, a catalytic asymmetric hydrophosphination reaction using a chiral complex of earth-abundant manganese(i) was developed. This reaction provides a short and efficient synthetic route to access easily obtainable and structurally tunable chiral bisphosphines, which can be used in asymmetric catalysis with earth-abundant metal-based organometallic catalysts.

CHEMICAL SCIENCE (2022)

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Article Chemistry, Physical

E-Selective Manganese-Catalyzed Semihydrogenation of Alkynes with H2 Directly Employed or In Situ-Generated

Ronald A. Farrar-Tobar et al.

Summary: This study describes the selective semihydrogenation of alkynes using a Mn(I) alkyl catalyst, leading to good to excellent yields of E-alkenes. Mechanistic investigations reveal that the initially formed Z-isomer undergoes fast isomerization to the thermodynamically more stable E-isomer.

ACS CATALYSIS (2022)

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Article Chemistry, Multidisciplinary

Evaluation of Manganese Catalysts for the Hydrogenative Deconstruction of Commercial and End-of-Life Polyurethane Samples

Laurynas Gausas et al.

Summary: Polyurethane (PU) is a commonly used thermoset plastic with complex structure, leading to challenges in recycling. The study shows that catalytic hydrogenation of PU materials using a manganese catalyst can effectively deconstruct PU into original monomer components for efficient recovery.

CHEMSUSCHEM (2022)

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Article Chemistry, Multidisciplinary

Hydrogenative Depolymerization of Polyurethanes Catalyzed by a Manganese Pincer Complex

Viktoriia Zubar et al.

Summary: This report discusses the promising method of utilizing plastic waste through chemical recycling, specifically hydrogenative depolymerization using a Mn pincer complex catalyst. The key to success lies in the combination of the catalyst with elevated temperatures and appropriate solvents to ensure sufficient solubility of the polymers. The process successfully depolymerizes a wide range of polyurethane samples, releasing polyetherols and diaminotoluene in high yields.

CHEMSUSCHEM (2022)

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Article Chemistry, Physical

Manganese-Catalyzed Reformation of Vicinal Glycols toα-HydroxyCarboxylic Acids with the Liberation of Hydrogen Gas

Satyadeep Waiba et al.

Summary: In this study, a sustainable catalytic pathway was developed to convert readily available feedstocks into valuable α-hydroxycarboxylic acid molecules. A bench stable metal complex was used as the catalyst, enabling the selective transformation of vicinal glycols into α-hydroxycarboxylic acids at low temperature. The protocol showed high efficiency and applicability for various types of vicinal glycols, with significant potential in the synthesis of bioactive molecules and biodegradable polymers.

ACS CATALYSIS (2022)

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Article Chemistry, Multidisciplinary

Manganese catalyzed asymmetric transfer hydrogenation of ketones

Guang-Ya Zhang et al.

Summary: The study investigated the asymmetric transfer hydrogenation of a wide range of ketones catalyzed by manganese complex and chiral PxNy-type ligand under mild conditions. By using 2-propanol as a hydrogen source and combining [MnBr(CO)(5)] with chiral, 22-membered macrocyclic ligand (R,R,R',R')-CyP2N4 (L5) with 2% catalyst loading, various ketones could be enantioselectively hydrogenated to afford highly valuable chiral alcohols with up to 95% ee.

CHINESE CHEMICAL LETTERS (2021)

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Review Chemistry, Applied

Recent Trends and Prospects in Homogeneous Manganese-Catalysed Epoxidation

Rose Mary Philip et al.

Summary: Epoxidation of alkenes is an important reaction in organic chemistry with significant potential in producing biochemically relevant compounds. Recent studies have focused on catalytic epoxidation using homogeneous manganese catalysts, particularly with porphyrin, Schiff base, Salen, and other ligands, showing advantages in green chemistry. The use of greener approaches, such as photo-catalysis, has been highlighted in recent reports, aiming to provide researchers with a better understanding of the reaction and catalyst selection.

ADVANCED SYNTHESIS & CATALYSIS (2021)

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Article Chemistry, Applied

Selective Construction of C-C and C=C Bonds by Manganese Catalyzed Coupling of Alcohols with Phosphorus Ylides

Xin Liu et al.

Summary: The manganese catalyzed coupling of alcohols with phosphorus ylides was found to be controllable in terms of selectivity for forming carbon-carbon single and double bonds by adjusting ligands and reaction conditions. Compared to previous methods using precious metal complexes, this system utilizes earth abundant manganese catalysts, allowing for C-C and C=C bond formation in a sequential one-pot reaction. Mechanistic studies revealed that C-C bonds were generated through a borrowing hydrogen pathway, while C=C bond formation followed an acceptorless dehydrogenative coupling pathway.

ADVANCED SYNTHESIS & CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Asymmetric Hydrogenation of Quinolines Enabled by π-π Interaction

Chenguang Liu et al.

Summary: The article reports on the non-noble metal-catalyzed asymmetric hydrogenation of N-heteroaromatics, quinolines. A new chiral pincer manganese catalyst showed outstanding catalytic activity in the reaction, producing high yields and enantioselectivities. The precise regulation of enantioselectivity was ensured by a pi-pi interaction, achieving competitive turnover numbers with noble metal catalysts.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Four-Coordinated Manganese(II) Disilyl Complexes for the Hydrosilylation of Aldehydes and Ketones with 1,1,3,3-Tetramethyldisiloxane

Kyoka Saito et al.

Summary: The article discusses a method of catalytic hydrosilylation using manganese complexes, with improved catalytic efficiency achieved by modifying the structure of the complex and combining it with isocyanide.

CHEMCATCHEM (2021)

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Article Chemistry, Inorganic & Nuclear

Manganese-Catalyzed Hydroboration of Terminal Olefins and Metal-Dependent Selectivity in Internal Olefin Isomerization- Hydroboration

Subhash Garhwal et al.

Summary: The study reports a manganese complex that shows high selectivity for terminal alkenes in hydroboration reactions, in contrast to cobalt which exhibits different selectivity towards internal alkenes, leading to different reaction pathways and product structures.

INORGANIC CHEMISTRY (2021)

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Article Chemistry, Organic

Manganese Catalyzed Direct Amidation of Esters with Amines

Zhengqiang Fu et al.

Summary: The development of a new transition metal catalyzed amide forming reaction with a wide substrate scope and low catalyst loading represents a novel approach to overcome the limitations of traditional methods.

JOURNAL OF ORGANIC CHEMISTRY (2021)

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Article Chemistry, Organic

N-Alkylation of Amines with Alcohols Catalyzed by Manganese(II) Chloride or Bromopentacarbonylmanganese(I)

Dongyue Wei et al.

Summary: A manganese-catalyzed N-alkylation reaction has been demonstrated, providing access to diverse secondary amines in moderate-to-high yields. The catalytic system is practical, scalable, and suitable for synthesizing heterocycles with potential activity against Alzheimer's disease.

JOURNAL OF ORGANIC CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Manganese-catalysed divergent silylation of alkenes

Jie Dong et al.

Summary: This study presents a new method for manganese-catalysed dehydrosilylation and hydrosilylation of alkenes, utilizing a ligand-tuned metalloradical reactivity strategy. The reaction is redox-neutral and atom-economical, with broad substrate scope and excellent functional group tolerance, suitable for various synthetic applications on a gram scale.

NATURE CHEMISTRY (2021)

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Article Chemistry, Inorganic & Nuclear

Cationic PCP and PCN NHC Core Pincer-Type Mn(I) Complexes: From Synthesis to Catalysis

Ruqaya Buhaibeh et al.

Summary: The coordination chemistry of NHC core pincer-type PCP and PCN ligands with a Mn(I) center was studied, revealing that Mn(I) complexes with bidentate and tridentate ligands exhibit different catalytic activities based on ligand structure.

ORGANOMETALLICS (2021)

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Article Multidisciplinary Sciences

Robust and efficient hydrogenation of carbonyl compounds catalysed by mixed donor Mn(I) pincer complexes

Wenjun Yang et al.

Summary: In this study, a highly efficient manganese pincer pre-catalyst was reported, displaying high TOF values (up to 41,000 h(-1)) and stability (TON up to 200,000) at loadings as low as 5-200 ppm. The crucial role of catalyst activation step for the catalytic performance and stability of the system was highlighted, with activation using hydride donor promoters significantly improving catalytic performance and eliminating induction times. Manganese-based hydrogenation catalysts are shown to be sensitive to high temperatures, but this pre-catalyst offers a promising alternative.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Dehydrogenation of Formic Acid to CO2 and H2 by Manganese(I)-Complex: Theoretical Insights for Green and Sustainable Route

Tiziana Marino et al.

Summary: This study presents a detailed computational investigation on a recently synthesized Mn(I)-dependent complex, which shows good catalytic performance in the dehydrogenation of formic acid. The calculated results confirm the robustness of the complex and its ability to reproduce experimental data, potentially inspiring the design of new efficient catalysts for hydrogen production.

CATALYSTS (2021)

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Review Chemistry, Multidisciplinary

Homogeneous manganese-catalyzed hydrogenation and dehydrogenation reactions

Yujie Wang et al.

Summary: The development of novel and efficient earth-abundant metal catalysts, with manganese as a rising star in catalytic hydrogenation and dehydrogenation reactions, has made significant progress since 2016. This review provides a comprehensive overview of homogeneous Mn-catalyzed hydrogenation and dehydrogenation reactions, emphasizing mechanistic understanding and future development trends in this promising field.

CHEM (2021)

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Article Chemistry, Applied

Catalytic Formal Hydroamination of Allylic Alcohols Using Manganese PNP-Pincer Complexes

Leandro Duarte de Almeida et al.

Summary: Several manganese-PNP pincer catalysts were used in the formal hydroamination of allylic alcohols to selectively obtain gamma-amino alcohols in high yields under mild conditions.

ADVANCED SYNTHESIS & CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

Manganese(I)-Catalyzed H-P Bond Activation via Metal-Ligand Cooperation

Juana M. Perez et al.

Summary: Chiral Mn(I) complexes have been shown to activate H-P bonds, providing a general method for the hydrophosphination of internal and terminal alpha,beta-unsaturated nitriles. Metal-ligand cooperation, a previously unconsidered strategy for catalytic H-P bond activation, plays a key role in the mechanistic action of the Mn(I)-based catalyst. Computational studies support a stepwise mechanism for the hydrophosphination reaction and offer insights into the origin of enantioselectivity.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Dehydrogenative Silylation of Alkenes Following Two Parallel Inner-Sphere Pathways

Stefan Weber et al.

Summary: A novel manganese(I)-catalyzed dehydrogenative silylation reaction was reported, using an alkyl bisphosphine manganese(I) complex as the most active precatalyst. The reaction efficiently converted a variety of aromatic and aliphatic alkenes to their corresponding products with high selectivity at room temperature. Insights into the mechanism were provided based on experimental data and DFT calculations, revealing two parallel reaction pathways.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Inorganic & Nuclear

Manganese-Catalyzed C(α)-Alkylation of Oxindoles with Secondary Alcohols via Borrowing Hydrogen

Jagannath Rana et al.

Summary: The general and efficient C(alpha)-alkylation of oxindoles with unactivated secondary alcohols as alkylating agents catalyzed by a newly developed NNN-Mn(II) complex demonstrates the importance of the NH moiety in the complex and M-L cooperation during the catalytic transformation.

ORGANOMETALLICS (2021)

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Article Chemistry, Physical

Phosphine-Free Manganese Catalyst Enables Selective Transfer Hydrogenation of Nitriles to Primary and Secondary Amines Using Ammonia-Borane

Koushik Sarkar et al.

Summary: Primary and secondary amines were synthesized via nitrile hydrogenation using a borrowing hydrogenation strategy catalyzed by phosphine-free manganese complexes. The method is chemodivergent, allowing control over the final product by adjusting catalyst structure and reaction polarity. The protocol operates without the need for externally added base or high-pressure dihydrogen gas, providing a practical and efficient route to a variety of amines.

ACS CATALYSIS (2021)

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Article Chemistry, Applied

Manganese-Catalyzed Selective Hydrogenative Cross-Coupling of Nitriles and Amines to Form Secondary Imines

Xiao-Gen Li et al.

Summary: Manganese complexes with tridentate PNN ligands have been synthesized as catalysts for hydrogenative cross-coupling reaction of nitriles and amines to form secondary imines. This reaction yielded a variety of unsymmetrical secondary imines in good yields with excellent selectivity. Investigation of catalyst intermediates suggested that an amido manganese complex may be the active catalyst species for this reaction.

ADVANCED SYNTHESIS & CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Hydroborations with Broad Scope

Pradip Ghosh et al.

Summary: The reductive transformations of easily available oxidized matter play a crucial role in synthetic manipulation and chemical valorization. The use of liquid reducing agents and simple setups in catalytic hydrofunctionalization adds to its practicality. Metal-catalyzed hydroborations offer a productive platform for reductive valorizations of stable C=X electrophiles, as demonstrated in this study with the pre-catalyst Mn(hmds)(2) for the reduction of various functional groups under mild conditions, including successful depolymerizations.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Hydrogenation of CO2 to Methanol with Mn-PNP-Pincer Complexes in the Presence of Lewis Acids: the Formate Resting State Unleashed

David A. Kuss et al.

Summary: Balancing the interaction between the acidic additive and the catalyst to remove the formate ligand can unleash the full catalytic potential in the hydrogenation of CO2 to methanol. This optimized process using MACHO-Ph and Ti((OPr)-Pr-i)(4) as the most active system allows for a liquid phase conversion of CO2/H-2 with high efficiency.

CHEMCATCHEM (2021)

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Article Chemistry, Multidisciplinary

Hydroboration of Nitriles, Esters, and Carbonates Catalyzed by Simple Earth-Abundant Metal Triflate Salts

Ranjeesh Thenarukandiyil et al.

Summary: Earth-abundant metals have become increasingly important in homogeneous catalysis, particularly in the hydroboration reactions of challenging substrates like nitriles, carbonates, and esters. The use of manganese(II) triflate salt in combination with potassium tert-butoxide and pinacolborane enables efficient hydroboration of these substrates with near quantitative yields in less than three hours at room temperature, showcasing a simple and effective methodology for these transformations. Further studies indicate that other earth-abundant metal triflate salts can also facilitate this reaction, expanding the scope of this catalytic process.

CHEMISTRY-AN ASIAN JOURNAL (2021)

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Article Chemistry, Inorganic & Nuclear

Carbon Dioxide Hydrogenation to Formate Catalyzed by a Bench-Stable, Non-Pincer-Type Mn(I) Alkylcarbonyl Complex

Sylwia Kostera et al.

Summary: The catalytic reduction of carbon dioxide using a non-precious-metal precatalyst is efficient and selective in forming formate under mild conditions. Mechanistic insight into the catalytic reaction is provided by means of density functional theory calculations.

ORGANOMETALLICS (2021)

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Article Chemistry, Inorganic & Nuclear

Manganese-Catalyzed Hydrogenation of Ketones under Mild and Base-free Conditions

Stefan Weber et al.

Summary: This paper investigated several Mn(I) complexes as catalysts for the homogeneous hydrogenation of ketones. The most active precatalyst was identified, and the reaction was carried out under base-free conditions at room temperature. Temperature-dependent selectivity for different compounds was observed in the reduction process.

ORGANOMETALLICS (2021)

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Article Chemistry, Multidisciplinary

Manganese-New prominent actor in transfer hydrogenation catalysis

Karim Azouzi et al.

Summary: This review comprehensively covers transfer hydrogenation processes catalyzed by manganese organometallic complexes, with a focus on reduction reactions of various substances and ligand design for Mn-catalyzed asymmetric transfer hydrogenation reactions.

CURRENT OPINION IN GREEN AND SUSTAINABLE CHEMISTRY (2021)

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Article Chemistry, Applied

Manganese Catalyzed Hydrogenation of Azo (N=N) Bonds to Amines

Uttam Kumar Das et al.

Summary: The first example of homogeneously catalyzed hydrogenation of the N=N bond of azo compounds has been reported using a complex of an earth-abundant-metal. The hydrogenation reaction is catalyzed by a manganese pincer complex, proceeds under mild conditions, and yields amines, which makes this methodology a sustainable alternative route for the conversion of azo compounds. A plausible mechanism involving metal-ligand cooperation and hydrazine intermediacy is proposed based on mechanistic studies.

ADVANCED SYNTHESIS & CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

Hydroboration of Terminal Alkenes and trans-1,2-Diboration of Terminal Alkynes Catalyzed by a Manganese(I) Alkyl Complex

Stefan Weber et al.

Summary: The Mn-catalyzed hydroboration of terminal alkenes and the 1,2-diboration of terminal alkynes with pinacolborane have been successfully achieved. The most active pre-catalyst is a bench-stable alkyl bisphosphine Mn-I complex. The catalytic process involves migratory insertion of a CO ligand into the Mn-alkyl bond to yield an acyl intermediate, which further undergoes B-H bond cleavage or C-H bond cleavage for alkenes and alkynes, respectively, forming active Mn-I boryl and acetylide catalysts.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Inorganic & Nuclear

Homogeneously catalyzed acceptorless dehydrogenation of alcohols: A progress report

Monica Trincado et al.

Summary: This paper reviews recent advances in homogeneously catalyzed acceptorless alcohol dehydrogenation, highlighting the importance of metal-ligand cooperativity in catalyzing the reaction and the potential positive impact of introducing multifunctional cooperative ligands.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Chemistry, Inorganic & Nuclear

Deciphering the Mechanistic Details of Manganese-Catalyzed Formic Acid Dehydrogenation: Insights from DFT Calculations

Neethinathan Johnee Britto et al.

Summary: A comprehensive density functional theory investigation revealed the detailed mechanistic landscape of aqueous-phase formic acid dehydrogenation catalyzed by a pyridyl-imidazoline-based Mn(I) catalyst. The stepwise mechanism was found to be kinetically and thermodynamically favorable for the production of a Mn-formate intermediate. The beta-hydride elimination process was identified as the rate-determining step, confirming experimental observations.

INORGANIC CHEMISTRY (2021)

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Article Chemistry, Organic

Manganese(I) Catalyzed α-Alkenylation of Amides Using Alcohols with Liberation of Hydrogen and Water

Biplab Keshari Pandia et al.

Summary: The unprecedented manganese-catalyzed direct alpha-alkenylation of amides using alcohols was reported, providing alpha,beta-unsaturated amides in moderate to good yields with excellent selectivity. Mechanistic studies showed that the selective olefination is facilitated by metal-ligand cooperation, resulting in water and dihydrogen as the only byproduct, making this catalytic transformation attractive, sustainable, and environmentally benign.

JOURNAL OF ORGANIC CHEMISTRY (2021)

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Article Chemistry, Organic

Recent advances in homogeneous base-metal-catalyzed transfer hydrogenation reactions

Daler Baidilov et al.

Summary: Catalytic transfer hydrogenation has become an appealing alternative for direct hydrogenation reactions due to its simplicity and mild reaction conditions. Research is now focused on developing sustainable catalysts using abundant first-row transition metals, with many novel examples appearing in the literature in recent decades.

TETRAHEDRON (2021)

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Article Chemistry, Organic

Homogeneous first-row transition metal catalyst for sustainable hydrogen production and organic transformation from methanol, formic acid, and bio-alcohols

Jagannath Rana et al.

Summary: Recent advances in homogeneous first-row transition-metal catalyzed for hydrogen production and important organic transformations focus on earth-abundant 3d base-metal complexes, showing promise for sustainable catalysis development.

TETRAHEDRON (2021)

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Article Chemistry, Organic

Manganese catalyzed enantio- and regioselective hydrogenation of α, β-unsaturated ketones using an imidazole-based chiral PNN tridentate ligand

Ze Wang et al.

Summary: This study demonstrates an enantioselective 1,2-reduction of alpha,beta-unsaturated ketones using a chiral pincer Mn catalyst, leading to the synthesis of chiral allyl alcohols with high catalytic activity and enantioselectivity. The process also provides a novel synthesis route for key pharmaceutical intermediates of cannabidiol.

TETRAHEDRON LETTERS (2021)

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Article Chemistry, Physical

Manganese-Catalyzed Anti-Markovnikov Hydroamination of Allyl Alcohols via Hydrogen-Borrowing Catalysis

Kuhali Das et al.

Summary: This article presents a method for selective formal anti-Markovnikov hydroamination of allyl alcohols, enabling the synthesis of valuable gamma-amino alcohol building blocks. Catalyzed by a phosphine-free Earth's abundant manganese(I) complex, a wide range of hydroamination reactions were successfully conducted with excellent functional group tolerance. The mechanistic studies highlighted the importance of metal-ligand bifunctionality and ligand backbone hemilability for the success of this catalysis.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Mechanistic Study of Metal-Ligand Cooperativity in Mn(II)-Catalyzed Hydroborations: Hemilabile SNS Ligand Enables Metal Hydride-Free Reaction Pathway

Matthew R. Elsby et al.

Summary: The study describes the chemoselective hydroboration of carbonyls using the paramagnetic bis-amido Mn[(SNSMe)-N-Me](2) complex (1). It was found that the bifunctional amido bis(thioether) ligand L plays a crucial role in the success of the reaction, while also ruling out the possibility of side reactions.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Amino Acid Derived Chiral Aminobenzimidazole Manganese Catalysts for Asymmetric Transfer Hydrogenation of Ketones

Lixian Wang et al.

Summary: A series of Mn(I) catalysts with chiral bidentate benzimidazoles derived from easily available amino acids have been developed for asymmetric transfer hydrogenation (ATH), showing high activity and enantioselectivity. These phosphine-free chiral Mn catalysts can efficiently convert bulky substrates into drug intermediate alcohols, with a possible mechanism and enantiocontrol model proposed based on experimental and DFT studies.

ACS CATALYSIS (2021)

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Review Chemistry, Organic

Acceptorless Dehydrogenative Coupling Reactions by Manganese Pincer Complexes

Pinaki Nad et al.

Summary: Acceptorless dehydrogenative coupling reactions using manganese catalyst is a promising and sustainable method for constructing carbon-carbon and carbon-heteroatom bonds. The methodology is highly atom economical, producing water and hydrogen as byproducts, and provides a unique opportunity for constructing various synthons and biologically important motifs. Recent progress in this field has been made with manganese catalysis based on pincer ligands for various homogeneous transformations.

ASIAN JOURNAL OF ORGANIC CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Acceptorless Dehydrogenation of Methanol to Carbon Monoxide and Hydrogen using Molecular Catalysts

Akash Kaithal et al.

Summary: The acceptorless dehydrogenation of methanol to carbon monoxide and hydrogen using homogeneous molecular complexes, particularly those containing ruthenium and manganese with the MACHO ligand framework, showed promising catalytic activities. The metal complex was found to mediate the initial fast dehydrogenation of methanol to formaldehyde and methyl formate followed by subsequent slow decarbonylation, resulting in gas mixtures with varying CO/H2 ratios.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Redox-active ligand based Mn(i)-catalyst for hydrosilylative ester reduction

Soumi Chakraborty et al.

Summary: A new Mn(i) catalyst with a redox-active ligand is reported for the efficient hydrosilylation of esters to alcohols, with mechanistic investigations showing a strong cooperation between the ligand and metal in initiating the reaction through a ligand-based single electron transfer (SET) process activating the Si-H bond.

CHEMICAL COMMUNICATIONS (2021)

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Article Chemistry, Organic

Transfer hydrogenation of N-heteroarenes with 2-propanol and ethanol enabled by manganese catalysis

Yingjie Gong et al.

Summary: A convenient manganese-catalyzed transfer hydrogenation method using alcohols as hydrogen sources for N-heteroarenes was presented. The use of a specific manganese pincer complex allowed for good to excellent isolated yields, with even biomass-derived ethanol being a viable option for the process. Detailed DFT calculations supported an outer sphere hydrogenation mechanism with hydride transfer as the rate-determining step.

ORGANIC CHEMISTRY FRONTIERS (2021)

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Article Chemistry, Multidisciplinary

Manganese catalyzed switchable C-alkylation/alkenylation of fluorenes and indene with alcohols

Avijit Mondal et al.

Summary: The study successfully demonstrated the selective C-alkylation and olefination of fluorene and indene with alcohols using manganese catalyst, providing insights into the potential use of earth-abundant, nontoxic transition metals in place of rare noble metals in catalysis.

CHEMICAL COMMUNICATIONS (2021)

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Review Chemistry, Multidisciplinary

Advancements in multifunctional manganese complexes for catalytic hydrogen transfer reactions

Kuhali Das et al.

Summary: Catalytic hydrogen transfer reactions are essential for the production of diverse molecular scaffolds, with manganese emerging as a viable alternative due to its abundance and sustainability. Strategies such as metal-ligand bifunctionality and hemilability play crucial roles in achieving desired catalytic activity and selectivity. The use of multifunctional ligand-based manganese complexes in various organic transformations has been detailed, highlighting the importance of ligand design for successful HT reactions.

CHEMICAL COMMUNICATIONS (2021)

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Article Chemistry, Physical

Synthesis of 1,3-diketones from esters via liberation of hydrogen

Guoying Zhang et al.

Summary: The study presents a method for catalytic dehydrogenative rearrangement of esters into 1,3-diketones, mediated by both a base-acid catalyst and a dehydrogenation catalyst based on manganese. This approach allows for the conversion of green or sustainable and inexpensive ester starting materials into highly attractive 1,3-diketones for organic synthesis, with hydrogen as the only by-product.

CHEM CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

Indirect reduction of CO2 and recycling of polymers by manganese-catalyzed transfer hydrogenation of amides, carbamates, urea derivatives, and polyurethanes

Xin Liu et al.

Summary: A manganese pincer complex is reported as a versatile catalyst for the transfer hydrogenation of amides, carbamates, urea derivatives, and polyurethanes, leading to the corresponding alcohols, amines, and methanol. This method represents an approach to the indirect reduction of CO2 and shows the first examples of reduction of carbamates and urea derivatives as well as C-N bond cleavage in amides by transfer hydrogenation. The general applicability of this methodology is demonstrated by successful reduction of various compounds with good to excellent yields.

CHEMICAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Reduction of Carboxylic Acids to Alcohols via Manganese(I) Catalyzed Hydrosilylation

Emanuele Antico et al.

Summary: The study demonstrated the reduction of carboxylic acids to alcohols using [MnBr(CO)(5)] as the catalyst and PhSiH3 as the reducing agent under mild conditions. The reaction could be performed with low catalyst loading or using the lowest reported amount of silane, showing promise for green and sustainable synthetic strategies in industrial production.

JACS AU (2021)

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Article Chemistry, Multidisciplinary

Alcohol-Assisted Hydrogenation of Carbon Monoxide to Methanol Using Molecular Manganese Catalysts

Akash Kaithal et al.

Summary: Alcohol-assisted hydrogenation of carbon monoxide to methanol was achieved using homogeneous molecular complexes. The best performance was observed with a molecular manganese complex, with a turnover number of 4023 and turnover frequency of 857 h(-1) under optimized conditions. The reaction proceeds via formate ester as the intermediate, resulting in high selectivity for methanol formation and no accumulation of formate ester.

JACS AU (2021)

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Review Chemistry, Organic

Recent advances in sustainable synthesis of N-heterocycles following acceptorless dehydrogenative coupling protocol using alcohols

Milan Maji et al.

Summary: This review summarizes recent advances in the synthesis of heterocycles using the ADC approach, which involves transition metal-catalyzed acceptorless dehydrogenative coupling using alcohols as greener substrates. Homogeneous and heterogeneous catalysis are both discussed in this review, showcasing environmentally benign methodologies for producing N-heterocycles.

ORGANIC CHEMISTRY FRONTIERS (2021)

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Article Chemistry, Multidisciplinary

Manganese catalyzed C-alkylation of methyl N-heteroarenes with primary alcohols

Akash Jana et al.

Summary: A new study reports the alkylation of nine different classes of methyl-substituted N-heteroarenes using an environmentally friendly catalyst. The compounds are synthesized with high yields and selectivities, with water as the sole byproduct.

CHEMICAL COMMUNICATIONS (2021)

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Article Chemistry, Physical

Enantioselective direct, base-free hydrogenation of ketones by a manganese amido complex of a homochiral, unsymmetrical P-N-P′ ligand

Chris S. G. Seo et al.

Summary: The use of manganese in homogeneous hydrogenation catalysis has shown great promise in terms of enantioselectivity, activity, and tolerance for base-sensitive substrates. NMR structural analysis and computational analysis have provided insights into the reaction mechanism and the influence of reactant structure on product enantiomeric selectivity.

CATALYSIS SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Carbon monoxide and hydrogen (syngas) as a C1-building block for selective catalytic methylation

Akash Kaithal et al.

Summary: A catalytic reaction using syngas as feedstock for the selective beta-methylation of alcohols was developed, with carbon monoxide and hydrogen gas as key components. The complex molecular structure involving earth-abundant manganese enables the generation of formaldehyde from syngas. This new syngas conversion method provides a pathway for installing methyl branches at carbon centers and synthesizing biologically active compounds, fine chemicals, and advanced biofuels.

CHEMICAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Manganese(I)-Catalyzed β-Methylation of Alcohols using Methanol as C1 Source

Akash Kaithal et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Applied

Manganese-Catalysed Dehydrogenative Coupling - An Overview

K. R. Rohit et al.

ADVANCED SYNTHESIS & CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed β-Methylation of Alcohols by Methanol

Martin Schlagbauer et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Biomimetic Hydrogenation Catalyzed by a Manganese Model of [Fe]-Hydrogenase

Hui-Jie Pan et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Physical

Manganese Catalyzed Acceptorless Dehydrogenative Coupling Reactions

Satyadeep Waiba et al.

CHEMCATCHEM (2020)

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Article Chemistry, Multidisciplinary

Simple manganese carbonyl catalyzed hydrogenation of quinolines and imines

Zelong Wang et al.

CHINESE CHEMICAL LETTERS (2020)

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Article Chemistry, Organic

Manganese-Catalyzed One-Pot Conversion of Nitroarenes into N-Methylarylamines Using Methanol

Benjamin G. Reed-Berendt et al.

EUROPEAN JOURNAL OF ORGANIC CHEMISTRY (2020)

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Article Chemistry, Inorganic & Nuclear

Synthesis and characterization of N,N-chelate manganese complexes and applications in C-N coupling reactions

Kuhali Das et al.

INORGANICA CHIMICA ACTA (2020)

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Article Chemistry, Inorganic & Nuclear

The Importance of Metal-Ligand Cooperativity in the Phosphorus-Nitrogen PN3P Platform: A Computational Study on Mn-Catalyzed Pyrrole Synthesis

Daniel Lupp et al.

ORGANOMETALLICS (2020)

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Article Chemistry, Inorganic & Nuclear

A Highly Selective Manganese-Catalyzed Synthesis of Imines under Phosphine-Free Conditions

Huining Chai et al.

ORGANOMETALLICS (2020)

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Article Multidisciplinary Sciences

Reversible interconversion between methanol-diamine and diamide for hydrogen storage based on manganese catalyzed (de)hydrogenation

Zhihui Shao et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Physical

Manganese-Catalyzed α-Olefination of Nitriles with Secondary Alcohols

Vinita Yadav et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

A Phosphine-Free Manganese Catalyst Enables Stereoselective Synthesis of (1+n)-Membered Cycloalkanes from Methyl Ketones and 1,n-Diols

Akash Jana et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

Development of a practical non-noble metal catalyst for hydrogenation of N-heteroarenes

Veronica Papa et al.

NATURE CATALYSIS (2020)

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Article Chemistry, Applied

Bench-Stable Manganese NHC Complexes for the Selective Reduction of Esters to Alcohols with Silanes

Sara C. A. Sousa et al.

ADVANCED SYNTHESIS & CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed anti-Selective Asymmetric Hydrogenation of α-Substituted β-Ketoamides

Linli Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Sustainable and Selective Alkylation of Deactivated Secondary Alcohols to Ketones by Non-bifunctional Pincer N-heterocyclic Carbene Manganese

Xiao-Bing Lan et al.

CHEMSUSCHEM (2020)

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Article Chemistry, Organic

Manganese(I)-Catalyzed Sustainable Synthesis of Quinoxaline and Quinazoline Derivatives with the Liberation of Dihydrogen

Akash Mondal et al.

JOURNAL OF ORGANIC CHEMISTRY (2020)

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Article Chemistry, Organic

Manganese-Catalyzed Regioselective Dehydrogenative C- versus N-Alkylation Enabled by a Solvent Switch: Experiment and Computation

Jannik C. Borghs et al.

ORGANIC LETTERS (2020)

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Article Chemistry, Organic

Hydrogenation or Dehydrogenation of N-Containing Heterocycles Catalyzed by a Single Manganese Complex

Viktoriia Zubar et al.

ORGANIC LETTERS (2020)

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Article Chemistry, Organic

Chemoselective Hydroboration of Propargylic Alcohols and Amines Using a Manganese(II) Catalyst

Aleksandra Brzozowska et al.

ORGANIC LETTERS (2020)

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Article Chemistry, Organic

Hydrosilylation of Esters Catalyzed by Bisphosphine Manganese(I) Complex: Selective Transformation of Esters to Alcohols

Rakesh R. Behera et al.

ORGANIC LETTERS (2020)

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Article Chemistry, Physical

Mild and Selective Carbon Dioxide Hydroboration to Methoxyboranes Catalyzed by Mn(I) PNP Pincer Complexes

Sylwia Kostera et al.

CHEMCATCHEM (2020)

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Article Chemistry, Physical

Asymmetric transfer hydrogenation of ketones promoted by manganese(I) pre-catalysts supported by bidentate aminophosphines

Karim Azouzi et al.

CATALYSIS COMMUNICATIONS (2020)

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Article Chemistry, Physical

Hydrogenation of Alkenes Catalyzed by a Non-pincer Mn Complex

S. M. Wahidur Rahaman et al.

CHEMCATCHEM (2020)

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Article Chemistry, Organic

Chemoselective Hydrogenation of Alkynes to (Z)-Alkenes Using an Air-Stable Base Metal Catalyst

Viktoriia Zubar et al.

ORGANIC LETTERS (2020)

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Article Chemistry, Organic

Methanol as the Hydrogen Source in the Selective Transfer Hydrogenation of Alkynes Enabled by a Manganese Pincer Complex

Jan Sklyaruk et al.

ORGANIC LETTERS (2020)

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Article Chemistry, Organic

Benzimidazole fragment containing Mn-complex catalyzed hydrosilylation of ketones and nitriles

Kasturi Ganguli et al.

TETRAHEDRON (2020)

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Article Chemistry, Physical

Toward Amines, Imines, and Imidazoles: A Viewpoint on the 3d Transition-Metal-Catalyzed Homogeneous Hydrogenation of Nitriles

Jorge A. Garduno et al.

ACS CATALYSIS (2020)

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Review Polymer Science

Polyurethane Recycling and Disposal: Methods and Prospects

Aleksandra Kemona et al.

POLYMERS (2020)

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Article Chemistry, Inorganic & Nuclear

Highly Selective Hydroboration of Carbonyls by a Manganese Catalyst: Insight into the Reaction Mechanism

Srikanth Vijjamarri et al.

ORGANOMETALLICS (2020)

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Article Chemistry, Inorganic & Nuclear

Manganese Diphosphine and Phosphinoamine Complexes Are Effective Catalysts for the Production of Biofuel Alcohols via the Guerbet Reaction

Ashley M. King et al.

ORGANOMETALLICS (2020)

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Review Chemistry, Multidisciplinary

Strategies and mechanisms of metal-ligand cooperativity in first-row transition metal complex catalysts

Matthew R. Elsby et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Inorganic & Nuclear

Hydrosilylation of Aldehydes by a Manganese α-Diimine Complex

Veeranna Yempally et al.

INORGANICS (2020)

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Article Chemistry, Physical

C1-Symmetric PNP Ligands for Manganese-Catalyzed Enantioselective Hydrogenation of Ketones: Reaction Scope and Enantioinduction Model

Liyao Zeng et al.

ACS CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Manganese and rhenium-catalyzed selective reduction of esters to aldehydes with hydrosilanes

Duo Wei et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Manganese catalyzed selective hydrogenation of cyclic imides to diols and amines

Uttam Kumar Das et al.

GREEN CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Manganese-catalysed transfer hydrogenation of esters

Conor L. Oates et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Manganese complex-catalysed α-alkylation of ketones with secondary alcohols enables the synthesis of β-branched carbonyl compounds

Satyadeep Waiba et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Physical

Chemoselective semihydrogenation of alkynes catalyzed by manganese(i)-PNP pincer complexes

Marcel Garbe et al.

CATALYSIS SCIENCE & TECHNOLOGY (2020)

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Article Chemistry, Physical

Manganese(i) κ2-NNcomplex-catalyzed formic acid dehydrogenation

Alexander Leval et al.

CATALYSIS SCIENCE & TECHNOLOGY (2020)

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Article Chemistry, Multidisciplinary

Scope and mechanism of nitrile dihydroboration mediated by a β-diketiminate manganese hydride catalyst

Thao T. Nguyen et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Hydrogen production from formic acid catalyzed by a phosphine free manganese complex: investigation and mechanistic insights

Alexander Leval et al.

GREEN CHEMISTRY (2020)

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Article Chemistry, Inorganic & Nuclear

1-D manganese(ii)-terpyridine coordination polymers as precatalysts for hydrofunctionalisation of carbonyl compounds

Guoqi Zhang et al.

DALTON TRANSACTIONS (2020)

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Article Chemistry, Multidisciplinary

C-Alkylation of Secondary Alcohols by Primary Alcohols through Manganese-Catalyzed Double Hydrogen Autotransfer

Osama El-Sepelgy et al.

CHEMSUSCHEM (2019)

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Review Chemistry, Organic

Recent advances in homogeneous borrowing hydrogen catalysis using earth-abundant first row transition metals

Benjamin G. Reed-Berendt et al.

ORGANIC & BIOMOLECULAR CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Phosphine-NHC Manganese Hydrogenation Catalyst Exhibiting a Non-Classical Metal-Ligand Cooperative H2 Activation Mode

Ruqaya Buhaibeh et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Palladium-Catalyzed Methylation of Nitroarenes with Methanol

Lin Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Lutidine-Based Chiral Pincer Manganese Catalysts for Enantioselective Hydrogenation of Ketones

Linli Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Physical

Transfer Hydrogenation of Carbonyl Groups, Imines and N-Heterocycles Catalyzed by Simple, Bipyridine-Based MnI Complexes

Abhishek Dubey et al.

CHEMCATCHEM (2019)

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Article Chemistry, Physical

Manganese-Catalyzed Transfer Hydrogenation of Aldimines

Duo Wei et al.

CHEMCATCHEM (2019)

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Article Chemistry, Physical

Design of Manganese Phenol Pi-complexes as Shvo-type Catalysts for Transfer Hydrogenation of Ketones

Nikita Shvydkiy et al.

CHEMCATCHEM (2019)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Selective Upgrading of Ethanol with Methanol into Isobutanol

Yaqian Liu et al.

CHEMSUSCHEM (2019)

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Article Chemistry, Organic

Manganese-Catalyzed N-Alkylation of Sulfonamides Using Alcohols

Benjamin G. Reed-Berendt et al.

JOURNAL OF ORGANIC CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Manganese(III) Porphyrin-Catalyzed Dehydrogenation of Alcohols to form Imines, Tertiary Amines and Quinolines

Kobra Azizi et al.

CHEMISTRY-A EUROPEAN JOURNAL (2019)

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Article Chemistry, Multidisciplinary

Cobalt-Catalyzed Aqueous Dehydrogenation of Formic Acid

Wei Zhou et al.

CHEMISTRY-A EUROPEAN JOURNAL (2019)

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Article Chemistry, Multidisciplinary

Manganese-Mediated Formic Acid Dehydrogenation

Nickolas H. Anderson et al.

CHEMISTRY-A EUROPEAN JOURNAL (2019)

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Article Chemistry, Organic

Sustainable Alkylation of Nitriles with Alcohols by Manganese Catalysis

Jannik C. Borghs et al.

JOURNAL OF ORGANIC CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

A catalytically active [Mn]-hydrogenase incorporating a non-native metal cofactor

Hui-Jie Pan et al.

NATURE CHEMISTRY (2019)

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Article Chemistry, Organic

A Highly Active PN3 Manganese Pincer Complex Performing N-Alkylation of Amines under Mild Conditions

Leonard Homberg et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Organic

Visible-Light-Initiated Manganese-Catalyzed E-Selective Hydrosilylation and Hydrogermylation of Alkynes

Hao Liang et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Organic

Sustainable Synthesis of Quinazoline and 2-Aminoquinoline via Dehydrogenative Coupling of 2-Aminobenzyl Alcohol and Nitrile Catalyzed by Phosphine-Free Manganese Pincer Complex

Kalicharan Das et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Organic

Highly Enantioselective Synthesis of Chiral Benzhydrols via Manganese Catalyzed Asymmetric Hydrogenation of Unsymmetrical Benzophenones Using an Imidazole-Based Chiral PNN Tridentate Ligand

Fei Ling et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Organic

Manganese(I)-Catalyzed α-Alkenylation of Ketones Using Primary Alcohols

Suhas Shahaji Gawali et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Inorganic & Nuclear

Phosphine-Free Well-Defined Mn(I) Complex-Catalyzed Synthesis of Amine, Imine, and 2,3-Dihydro-1H-perimidine via Hydrogen Autotransfer or Acceptorless Dehydrogenative Coupling of Amine and Alcohol

Kalicharan Das et al.

ORGANOMETALLICS (2019)

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Article Chemistry, Applied

Mn(I) and Fe(II)/PN(H)P Catalysts for the Hydrogenation of Ketones: A Comparison by Experiment and Calculation

Alessandro Passera et al.

ADVANCED SYNTHESIS & CATALYSIS (2019)

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Article Chemistry, Physical

Efficient and Practical Transfer Hydrogenation of Ketones Catalyzed by a Simple Bidentate Mn-NHC Complex

Robbert van Putten et al.

CHEMCATCHEM (2019)

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Article Chemistry, Multidisciplinary

Manganese Catalyzed Hydrogenation of Carbamates and Urea Derivatives

Uttam Kumar Das et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Direct Synthesis of Amides by Acceptorless Dehydrogenative Coupling of Benzyl Alcohols and Ammonia Catalyzed by a Manganese Pincer Complex: Unexpected Crucial Role of Base

Prosenjit Daw et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Mechanistic Studies of Hydride Transfer to Imines from a Highly Active and Chemoselective Manganate Catalyst

Frederik Freitag et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Physical

Hydrogen Storage Technology: Development of Effective Catalysts for Hydrogen Storage Technology Using Formic Acid (Adv. Energy Mater. 23/2019)

Naoya Onishi et al.

Advanced Energy Materials (2019)

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Article Chemistry, Multidisciplinary

Manganese(I)-Catalyzed Cross-Coupling of Ketones and Secondary Alcohols with Primary Alcohols

Suhas Shahaji Gawali et al.

ACS OMEGA (2019)

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Article Chemistry, Multidisciplinary

Base Metal-Catalyzed Direct Olefinations of Alcohols with Sulfones

Satyadeep Waiba et al.

ACS OMEGA (2019)

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Article Chemistry, Physical

The atomic-resolution crystal structure of activated [Fe]-hydrogenase

Gangfeng Huang et al.

NATURE CATALYSIS (2019)

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Article Chemistry, Physical

Ethylene glycol as an efficient and reversible liquid-organic hydrogen carrier

You-Quan Zou et al.

NATURE CATALYSIS (2019)

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Article Chemistry, Physical

Manganese-Catalyzed Transfer Hydrogenation of Nitriles with 2-Butanol as the Hydrogen Source

Jorge A. Garduno et al.

CHEMCATCHEM (2019)

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Article Chemistry, Organic

Nonbifunctional Outer-Sphere Strategy Achieved Highly Active α-Alkylation of Ketones with Alcohols by N-Heterocyclic Carbene Manganese (NHC-Mn)

Xiao-Bing Lan et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Inorganic & Nuclear

Manganese(I)-Catalyzed Transfer Hydrogenation and Acceptorless Dehydrogenative Condensation: Promotional Influence of the Uncoordinated N-Heterocycle

Chong Zhang et al.

ORGANOMETALLICS (2019)

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Article Chemistry, Inorganic & Nuclear

Mechanistic Complexity of Asymmetric Transfer Hydrogenation with Simple Mn-Diamine Catalysts

Robbert van Putten et al.

ORGANOMETALLICS (2019)

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Article Chemistry, Physical

Rethinking Basic Concepts-Hydrogenation of Alkenes Catalyzed by Bench-Stable Alkyl Mn(I) Complexes

Stefan Weber et al.

ACS CATALYSIS (2019)

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Article Chemistry, Applied

Old Concepts, New Application - Additive-Free Hydrogenation of Nitriles Catalyzed by an Air Stable Alkyl Mn(I) Complex

Stefan Weber et al.

ADVANCED SYNTHESIS & CATALYSIS (2019)

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Article Chemistry, Multidisciplinary

Molecularly Defined Manganese Catalyst for Low-Temperature Hydrogenation of Carbon Monoxide to Methanol

Pavel Ryabchuk et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Direct Synthesis of Cycloalkanes from Diols and Secondary Alcohols or Ketones Using a Homogeneous Manganese Catalyst

Akash Kaithal et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Unmasking the Ligand Effect in Manganese-Catalyzed Hydrogenation: Mechanistic Insight and Catalytic Application

Yujie Wang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Inorganic & Nuclear

β-Amino Phosphine Mn Catalysts for 1,4-Transfer Hydrogenation of Chalcones and Allylic Alcohol Isomerization

Vipulan Vigneswaran et al.

ORGANOMETALLICS (2019)

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Article Chemistry, Multidisciplinary

Catalytic C1 Alkylation with Methanol and Isotope-Labeled Methanol

Jan Sklyaruk et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Review Chemistry, Physical

Manganese-Catalyzed C-H Olefination Reactions

Yuanyuan Hu et al.

CHEMCATCHEM (2019)

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Review Chemistry, Multidisciplinary

First-Row Transition Metal (De)Hydrogenation Catalysis Based On Functional Pincer Ligands

Lukas Alig et al.

CHEMICAL REVIEWS (2019)

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Review Chemistry, Multidisciplinary

3d-Metal Catalyzed N- and C-Alkylation Reactions via Borrowing Hydrogen or Hydrogen Autotransfer

Torsten Irrgang et al.

CHEMICAL REVIEWS (2019)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Multicomponent Synthesis of Pyrroles through Acceptorless Dehydrogenation Hydrogen Autotransfer Catalysis: Experiment and Computation

Jannik C. Borghs et al.

CHEMSUSCHEM (2019)

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Article Chemistry, Organic

Manganese-Catalyzed Acceptorless Dehydrogenative Coupling of Alcohols With Sulfones: A Tool To Access Highly Substituted Vinyl Sulfones

Satyadeep Waiba et al.

JOURNAL OF ORGANIC CHEMISTRY (2019)

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Article Chemistry, Organic

Selective Hydroboration of Carboxylic Acids with a Homogeneous Manganese Catalyst

Milan K. Barman et al.

JOURNAL OF ORGANIC CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Mechanism of the Manganese-Pincer-Catalyzed Acceptorless Dehydrogenative Coupling of Nitriles and Alcohols

Jesus A. Luque-Urrutia et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Organic

Sustainable Manganese-Catalyzed Solvent-Free Synthesis of Pyrroles from 1,4-Diols and Primary Amines

Jannik C. Borghs et al.

ORGANIC LETTERS (2019)

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Article Chemistry, Physical

Dehydrogenative Cross-Coupling of Primary Alcohols To Form Cross-Esters Catalyzed by a Manganese Pincer Complex

Uttam Kumar Das et al.

ACS CATALYSIS (2019)

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Article Chemistry, Physical

Non-Pincer Mn(I) Organometallics for the Selective Catalytic Hydrogenation of Nitriles to Primary Amines

Jorge A. Garduno et al.

ACS CATALYSIS (2019)

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Article Chemistry, Physical

Carbon Dioxide Reduction to Methanol Catalyzed by Mn(I) PNP Pincer Complexes under Mild Reaction Conditions

Federica Bertini et al.

ACS CATALYSIS (2019)

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Article Chemistry, Physical

PN3(P)-Pincer Complexes: Cooperative Catalysis and Beyond

Huaifeng Li et al.

ACS CATALYSIS (2019)

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Article Chemistry, Inorganic & Nuclear

Cooperative Mn(i)-complex catalyzed transfer hydrogenation of ketones and imines

Kasturi Ganguli et al.

DALTON TRANSACTIONS (2019)

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Article Chemistry, Inorganic & Nuclear

Manganese-catalyzed direct C-C coupling of -C-H bonds of amides and esters with alcohols via hydrogen autotransfer

Jagannath Rana et al.

DALTON TRANSACTIONS (2019)

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Article Chemistry, Multidisciplinary

Development and mechanistic investigation of the manganese(iii) salen-catalyzed dehydrogenation of alcohols

SimoneV. Samuelsen et al.

CHEMICAL SCIENCE (2019)

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Article Chemistry, Multidisciplinary

Manganese catalyzed α-methylation of ketones with methanol as a C1 source

Antoine Bruneau-Voisine et al.

CHEMICAL COMMUNICATIONS (2019)

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Article Chemistry, Inorganic & Nuclear

Diastereoselective diazenyl formation: the key for manganese-catalysed alcohol conversion into (E)-alkenes

Luis Miguel Azofra et al.

DALTON TRANSACTIONS (2019)

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Article Chemistry, Multidisciplinary

Room temperature N-heterocyclic carbene manganese catalyzed selective N-alkylation of anilines with alcohols

Ming Huang et al.

CHEMICAL COMMUNICATIONS (2019)

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Article Chemistry, Organic

A pincer ligand enabled ruthenium catalyzed highly selective N-monomethylation of nitroarenes with methanol as the C1 source

Shaochun Zhang et al.

ORGANIC CHEMISTRY FRONTIERS (2019)

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Article Chemistry, Physical

Hydrosilylation of carbonyl and carboxyl groups catalysed by Mn(i) complexes bearing triazole ligands

Oriol Martinez-Ferrate et al.

CATALYSIS SCIENCE & TECHNOLOGY (2019)

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Article Chemistry, Physical

Manganese PNP-pincer catalyzed isomerization of allylic/homo-allylic alcohols to ketones - activity, selectivity, efficiency

Tian Xia et al.

CATALYSIS SCIENCE & TECHNOLOGY (2019)

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Review Chemistry, Multidisciplinary

Isoelectronic Manganese and Iron Hydrogenation/Dehydrogenation Catalysts: Similarities and Divergences

Nikolaus Gorgas et al.

ACCOUNTS OF CHEMICAL RESEARCH (2018)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Hydrofunctionalization of Alkenes

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Manganese-Catalyzed Dehydrogenative Alkylation or -Olefination of Alkyl-Substituted N-Heteroarenes with Alcohols

Guoying Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

Manganese-Catalyzed Direct Olefination of Methyl-Substituted Heteroarenes with Primary Alcohols

Milan K. Barman et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

N-Substituted Hydrazones by Manganese-Catalyzed Coupling of Alcohols with Hydrazine: Borrowing Hydrogen and Acceptorless Dehydrogenation in One System

Uttam Kumar Das et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Physical

Practical (asymmetric) transfer hydrogenation of ketones catalyzed by manganese with (chiral) diamines ligands

Ding Wang et al.

CATALYSIS COMMUNICATIONS (2018)

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Manganese N-Heterocyclic Carbene Complexes for Catalytic Reduction of Ketones with Silanes

Mara Pinto et al.

CHEMCATCHEM (2018)

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Manganese catalyzed reductive amination of aldehydes using hydrogen as a reductant

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CHEMICAL COMMUNICATIONS (2018)

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Intermolecular Metal-Catalyzed Reductive Coupling of Dienes, Allenes, and Enynes with Carbonyl Compounds and Imines

Michael Holmes et al.

CHEMICAL REVIEWS (2018)

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Review Chemistry, Multidisciplinary

Advances in One-Pot Synthesis through Borrowing Hydrogen Catalysis

Avelino Corma et al.

CHEMICAL REVIEWS (2018)

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Catalytic (de)hydrogenation promoted by non-precious metals - Co, Fe and Mn: recent advances in an emerging field

Georgy A. Filonenko et al.

CHEMICAL SOCIETY REVIEWS (2018)

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Review Chemistry, Multidisciplinary

Manganese-Catalyzed Hydrosilylation Reactions

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CHEMISTRY-AN ASIAN JOURNAL (2018)

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Selective Synthesis of 2-Substituted and 1,2-Disubstituted Benzimidazoles Directly from Aromatic Diamines and Alcohols Catalyzed by Molecularly Defined Nonphosphine Manganese(I) Complex

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JOURNAL OF ORGANIC CHEMISTRY (2018)

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Review Chemistry, Physical

Liquid organic hydrogen carriers for transportation and storing of renewable energy - Review and discussion

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JOURNAL OF POWER SOURCES (2018)

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Manganese-Catalyzed Direct Conversion of Ester to Amide with Liberation of H-2

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ORGANIC LETTERS (2018)

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Manganese Catalyzed Hydrogenation of Enantiornerically Pure Esters

Magnus B. Widegren et al.

ORGANIC LETTERS (2018)

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Advances in Homogeneous Catalysis for Low Temperature Methanol Reforming in the Context of the Methanol Economy

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TOPICS IN CATALYSIS (2018)

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Manganese-Catalyzed beta-Alkylation of Secondary Alcohols with Primary Alcohols under Phosphine-Free Conditions

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ACS CATALYSIS (2018)

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Highly Selective N-Monomethylanilines Synthesis From Nitroarene and Formaldehyde via Kinetically Excluding of the Thermodynamically Favorable N,N-Dimethylation Reaction

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ACS CATALYSIS (2018)

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Article Chemistry, Physical

Catalytic Upgrading of Ethanol to n-Butanol via Manganese-Mediated Guerbet Reaction

Naveen V. Kulkarni et al.

ACS CATALYSIS (2018)

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Chemoselective Hydrogenation of Aldehydes under Mild, Base-Free Conuditions: Manganese Outperforms Rhenium

Mathias Glatz et al.

ACS CATALYSIS (2018)

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Review Chemistry, Physical

High-Purity Hydrogen Generation via Dehydrogenation of Organic Carriers: A Review on the Catalytic Process

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ACS CATALYSIS (2018)

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Highly Chemo- and Stereoselective Transfer Semihydrogenation of Alkynes Catalyzed by a Stable, Well-Defined Manganese(II) Complex

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ACS CATALYSIS (2018)

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Mechanistic insights into catalytic CO2 hydrogenation using Mn(I)-complexes with pendant oxygen ligands

Shubhajit Das et al.

CATALYSIS SCIENCE & TECHNOLOGY (2018)

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Exploring the mechanisms of aqueous methanol dehydrogenation catalyzed by defined PNP Mn and Re pincer complexes under base-free as well as strong base conditions

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CATALYSIS SCIENCE & TECHNOLOGY (2018)

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A general and efficient Mn-catalyzed acceptorless dehydrogenative coupling of alcohols with hydroxides into carboxylates

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ORGANIC CHEMISTRY FRONTIERS (2018)

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Phosphine-Free NNN-Manganese Complex Catalyzed alpha-Alkylation of Ketones with Primary Alcohols and Friedlander Quinoline Synthesis

Milan K. Barman et al.

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Direct Conversion of Alcohols into Alkenes by Dehydrogenative Coupling with Hydrazine/Hydrazone Catalyzed by Manganese

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Hydrogenation of CO2-Derived Carbonates and Polycarbonates to Methanol and Diols by Metal-Ligand Cooperative Manganese Catalysis

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Catalytic Hydrogenation of Cyclic Carbonates using Manganese Complexes

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Manganese Catalyzed Hydrogenation of Organic Carbonates to Methanol and Alcohols

Amit Kumar et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Aminotriazole Mn(I) Complexes as Effective Catalysts for Transfer Hydrogenation of Ketones

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CHEMCATCHEM (2018)

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Phosphine free Mn-complex catalysed dehydrogenative C-C and C-heteroatom bond formation: a sustainable approach to synthesize quinoxaline, pyrazine, benzothiazole and quinoline derivatives

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Diverse Fates of -Silyl Radical under Manganese Catalysis: Hydrosilylation and Dehydrogenative Silylation of Alkenes

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CHINESE JOURNAL OF CHEMISTRY (2018)

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A β-diketiminate manganese catalyst for alkene hydrosilylation: substrate scope, silicone preparation, and mechanistic insight

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CHEMICAL SCIENCE (2018)

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Manganese Catalyzed alpha-Alkylation of Nitriles with Primary Alcohols

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ACS CATALYSIS (2018)

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Manganese-Catalyzed and Base-Switchable Synthesis of Amines or Imines via Borrowing Hydrogen or Dehydrogenative Condensation

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ACS CATALYSIS (2018)

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Highly Selective, Efficient Deoxygenative Hydrogenation of Amides Catalyzed by a Manganese Pincer Complex via Metal-Ligand Cooperation

You-Quan Zou et al.

ACS CATALYSIS (2018)

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Synthesis of Pyrazines and Quinoxalines via Acceptorless Dehydrogenative Coupling Routes Catalyzed by Manganese Pincer Complexes

Prosenjit Daw et al.

ACS CATALYSIS (2018)

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Manganese-Catalyzed Dual-Deoxygenative Coupling of Primary Alcohols with 2-Arylethanols

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Benyzl Alcohol Dehydrogenative Coupling Catalyzed by Defined Mn and Re PNP Pincer Complexes - A Computational Mechanistic Study

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EUROPEAN JOURNAL OF INORGANIC CHEMISTRY (2018)

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Hydrogenation of Nitriles and Ketones Catalyzed by an Air-Stable Bisphosphine Mn(I) Complex

Stefan Weber et al.

ORGANIC LETTERS (2018)

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Article Chemistry, Organic

Sustainable Alkylation of Unactivated Esters and Amides with Alcohols Enabled by Manganese Catalysis

Yoon Kyung Jang et al.

ORGANIC LETTERS (2018)

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Catalytic Formic Acid Dehydrogenation and CO2 Hydrogenation Using Iron (PNP)-P-R Pincer Complexes with Isonitrile Ligands

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Asymmetric Transfer Hydrogenation of Ketones with Well-Defined Manganese(I) PNN and PNNP Complexes

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ORGANOMETALLICS (2018)

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Manganese-catalyzed hydroboration of carbon dioxide and other challenging carbonyl groups

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NATURE COMMUNICATIONS (2018)

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Homogeneous Catalysis by Cobalt and Manganese Pincer Complexes

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ACS CATALYSIS (2018)

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Manganese-Catalyzed alpha-Alkylation of Ketones, Esters, and Amides Using Alcohols

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ACS CATALYSIS (2018)

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Mn(II)-catalysed alkylation of methylene ketones with alcohols: direct access to functionalised branched products

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CHEMICAL COMMUNICATIONS (2018)

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Hydrogenation of Carbonyl Derivatives Catalysed by Manganese Complexes Bearing Bidentate Pyridinyl-Phosphine Ligands

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Unexpected concerted two-proton transfer for amination of formic acid to formamide catalysed by Mn bipyridinol complexes

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Stereoselective Transfer Semi-Hydrogenation of Alkynes to E-Olefins with N-Heterocyclic Silylene-Manganese Catalysts

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CHEMISTRY-A EUROPEAN JOURNAL (2018)

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Manganese catalyzed N-alkylation of anilines with alcohols: ligand enabled selectivity

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ORGANIC & BIOMOLECULAR CHEMISTRY (2018)

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Dichotomy of Manganese Catalysis via Organometallic or Radical Mechanism: Stereodivergent Hydrosilylation of Alkynes

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Review Chemistry, Multidisciplinary

Liquid Organic Hydrogen Carriers (LOHCs): Toward a Hydrogen -free Hydrogen Economy

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ACCOUNTS OF CHEMICAL RESEARCH (2017)

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A Stable Manganese Pincer Catalyst for the Selective Dehydrogenation of Methanol

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Manganese-Catalyzed Hydrogenation of Esters to Alcohols

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Molecularly Defined Manganese Pincer Complexes for Selective Transfer Hydrogenation of Ketones

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CHEMSUSCHEM (2017)

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Homogeneous Catalysis by Manganese-Based Pincer Complexes

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EUROPEAN JOURNAL OF ORGANIC CHEMISTRY (2017)

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Introducing and energy analysis of a novel cryogenic hydrogen liquefaction process configuration

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2017)

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Mono-N-methylation of anilines with methanol catalyzed by a manganese pincer-complex

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Manganese-Catalyzed Upgrading of Ethanol into 1-Butanol

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2017)

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Mechanistic Investigation of Bis(imino)pyridine Manganese Catalyzed Carbonyl and Carboxylate Hydrosilylation

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Manganese-Catalyzed Aminomethylation of Aromatic Compounds with Methanol as a Sustainable C1 Building Block

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Synthesis of Cyclic Imides by Acceptorless Dehydrogenative Coupling of Diols and Amines Catalyzed by a Manganese Pincer Complex

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Manganese Catalyzed α-Olefination of Nitriles by Primary Alcohols

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Transfer Hydrogenation of Carbonyl Derivatives Catalyzed by an Inexpensive Phosphine-Free Manganese Precatalyst

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ORGANIC LETTERS (2017)

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Cobalt-Catalyzed α-Alkylation of Ketones with Primary Alcohols

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ORGANIC LETTERS (2017)

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Iron-Catalyzed Amide Formation from the Dehydrogenative Coupling of Alcohols and Secondary Amines

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Hydrosilylation of Aldehydes and Formates Using a Dimeric Manganese Precatalyst

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Carbon dioxide hydrogenation catalysed by well-defined Mn(I) PNP pincer hydride complexes

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Efficient and selective hydrogenation of amides to alcohols and amines using a well-defined manganese-PNN pincer complex

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Convenient iron-catalyzed reductive aminations without hydrogen for selective synthesis of N-methylamines

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NATURE COMMUNICATIONS (2017)

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Bio-Inspired Mn(I) Complexes for the Hydrogenation of CO2 to Formate and Formamide

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Manganese-Catalyzed Sequential Hydrogenation of CO2 to Methanol via Formamide

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ACS CATALYSIS (2017)

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Manganese Pincer Complexes for the Base-Free, Acceptorless Dehydrogenative Coupling of Alcohols to Esters: Development, Scope, and Understanding

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Facile Ruthenium(II)-Catalyzed α-Alkylation of Arylmethyl Nitriles Using Alcohols Enabled by Metal-Ligand Cooperation

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Manganese-Catalyzed Direct Deoxygenation of Primary Alcohols

Jonathan O. Bauer et al.

ACS CATALYSIS (2017)

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Nitrogen-Containing Liquid Organic Hydrogen Carriers: Progress and Prospects

Robert H. Crabtree

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Supported Palladium Nanoparticle Catalyzed α-Alkylation of Ketones Using Alcohols as Alkylating Agents

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A Manganese Pre-Catalyst: Mild Reduction of Amides, Ketones, Aldehydes, and Esters

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Direct Synthesis of Amides by Dehydrogenative Coupling of Amines with either Alcohols or Esters: Manganese Pincer Complex as Catalyst

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Atmosphere-Controlled Chemoselectivity: Rhodium-Catalyzed Alkylation and Olefination of Alkylnitriles with Alcohols

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Efficient and Selective N-Methylation of Nitroarenes under Mild Reaction Conditions

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Review Chemistry, Multidisciplinary

The Emergence of Manganese-Based Carbonyl Hydrosilylation Catalysts

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Manganese-Catalyzed Asymmetric Hydrosilylation of Aryl Ketones

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Manganese(I)-Catalyzed Enantioselective Hydrogenation of Ketones Using a Defined Chiral PNP Pincer Ligand

Marcel Garbe et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Oxidative Transformations of Biosourced Alcohols Catalyzed by Earth-Abundant Transition Metals

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Mechanism-Based Enantiodivergence in Manganese Reduction Catalysis: A Chiral Pincer Complex for the Highly Enantioselective Hydroboration of Ketones

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Homogeneous Transition Metal Catalysis of Acceptorless Dehydrogenative Alcohol Oxidation: Applications in Hydrogen Storage and to Heterocycle Synthesis

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CHEMICAL REVIEWS (2017)

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Tandem Transformation of Nitro Compounds into N-Methylated Amines: Greener Strategy for the Utilization of Methanol as a Methylating Agent

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Non-Pincer-Type Manganese Complexes as Efficient Catalysts for the Hydrogenation of Esters

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Manganese-Catalyzed Sustainable Synthesis of Pyrroles from Alcohols and Amino Alcohols

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Enantioselective Transfer Hydrogenation of Ketones Catalyzed by a Manganese Complex Containing an Unsymmetrical Chiral PNP′ Tridentate Ligand

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Improved and General Manganese-Catalyzed N-Methylation of Aromatic Amines Using Methanol

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CHEMISTRY-A EUROPEAN JOURNAL (2017)

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A Highly Active Manganese Catalyst for Enantioselective Ketone and Ester Hydrogenation

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Manganese-Catalyzed N-Formylation of Amines by Methanol Liberating H2: A Catalytic and Mechanistic Study

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Hydrogen autotransfer and related dehydrogenative coupling reactions using a rhenium(I) pincer catalyst

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CHEMICAL COMMUNICATIONS (2017)

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Hydrogenation of ketones with a manganese PN3P pincer pre-catalyst

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Manganese-Catalyzed Multicomponent Synthesis of Pyrimidines from Alcohols and Amidines

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Review Chemistry, Multidisciplinary

C-Alkylation of Ketones and Related Compounds by Alcohols: Transition-Metal-Catalyzed Dehydrogenation

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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CHEMSUSCHEM (2016)

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Cobalt-Catalyzed N-Alkylation of Amines with Alcohols

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ORGANIC LETTERS (2016)

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Photo-Triggered Click Chemistry for Biological Applications

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TOPICS IN CURRENT CHEMISTRY (2016)

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Highly Selective Hydroboration of Alkenes, Ketones and Aldehydes Catalyzed by a Well-Defined Manganese Complex

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Manganese-Catalyzed Hydrogen-Autotransfer C-C Bond Formation: α-Alkylation of Ketones with Primary Alcohols

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Highly Active and Selective Manganese C=O Bond Hydrogenation Catalysts: The Importance of the Multidentate Ligand, the Ancillary Ligands, and the Oxidation State

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Hydrogenation of Esters to Alcohols Catalyzed by Defined Manganese Pincer Complexes

Saravanakumar Elangovan et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Direct Olefination of Alcohols with Sulfones by Using Heterogeneous Platinum Catalysts

S. M. A. Hakim Siddiki et al.

CHEMISTRY-A EUROPEAN JOURNAL (2016)

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Divergent Coupling of Alcohols and Amines Catalyzed by Isoelectronic Hydride MnI and FeII PNP Pincer Complexes

Matthias Mastalir et al.

CHEMISTRY-A EUROPEAN JOURNAL (2016)

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Review Chemistry, Organic

Recent Advances of Manganese Catalysis for Organic Synthesis

Jonathan R. Carney et al.

EUROPEAN JOURNAL OF ORGANIC CHEMISTRY (2016)

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Pd-, Ni-, Fe-, and Co-Catalyzed Cross-Couplings Using Functionalized Zn-, Mg-, Fe-, and In-Organometallics

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Nitrile-Containing Pharmaceuticals: Efficacious Roles of the Nitrile Pharmacophore

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Well-Defined N-Heterocyclic Carbene Based Ruthenium Catalysts for Direct Amide Synthesis from Alcohols and Amines

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ORGANOMETALLICS (2010)

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Editorial Material Multidisciplinary Sciences

Radical Ligands Confer Nobility on Base-Metal Catalysts

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SCIENCE (2010)

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Continuous Hydrogen Generation from Formic Acid: Highly Active and Stable Ruthenium Catalysts

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Chemical and Physical Solutions for Hydrogen Storage

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2009)

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2009)

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Structural and Functional Analogues of the Active Sites of the [Fe]-, [NiFe]-, and [FeFe]-Hydrogenases

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Direct Dehydrogenative Amide Synthesis from Alcohols and Amines Catalyzed by gamma-Alumina Supported Silver Cluster

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CHEMISTRY-A EUROPEAN JOURNAL (2009)

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Review Chemistry, Multidisciplinary

Coming of Age: Sustainable Iron-Catalyzed Cross-Coupling Reactions

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CHEMSUSCHEM (2009)

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The crystal structure of C176A mutated [Fe]-hydrogenase suggests an acyl- iron ligation in the active site iron complex

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FEBS LETTERS (2009)

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Ruthenium-Catalyzed N-Alkylation of Amines and Sulfonamides Using Borrowing Hydrogen Methodology

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Ruthenium-Catalyzed Oxidation of Alcohols into Amides

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ORGANIC LETTERS (2009)

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The Promise and Challenge of Iron-Catalyzed Cross Coupling

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ACCOUNTS OF CHEMICAL RESEARCH (2008)

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Amide Synthesis from Alcohols and Amines by the Extrusion of Dihydrogen

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The crystal structure of [Fe]-hydrogenase reveals the geometry of the active site

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SCIENCE (2008)

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New highlights in the synthesis and reactivity of 1,4-dihydropyrazine derivatives

Mathilde Chaignaud et al.

TETRAHEDRON (2008)

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C-C bond formation from alcohols and malonate half esters using borrowing hydrogen methodology

Simon J. Pridmore et al.

TETRAHEDRON LETTERS (2008)

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A novel salt-free ruthenium-catalyzed alkylation of aryl amines

Dirk Hollmann et al.

TETRAHEDRON LETTERS (2008)

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Synthesis, biological activity, and crystal structure of potent nonnucleoside inhibitors of HIV-1 reverse transcriptase that retain activity against mutant forms of the enzyme

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Direct synthesis of amides from alcohols and amines with liberation of H2

Chidambaram Gunanathan et al.

SCIENCE (2007)

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Borrowing hydrogen in the activation of alcohols

Malai Haniti S. A. Hamid et al.

ADVANCED SYNTHESIS & CATALYSIS (2007)

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Synthesis of symmetrical and unsymmetrical pyrazines

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Alkylation of active methylene compounds with alcohols catalyzed by an iridium complex

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CHEMICAL COMMUNICATIONS (2007)

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Environmentally friendly one-pot synthesis of α-alkylated nitriles using hydrotalcite-supported metal species as multifunctional solid catalysts

Ken Motokura et al.

CHEMISTRY-A EUROPEAN JOURNAL (2006)

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Efficient solvent-free selective monoalkylation of arylacetonitriles with mono-, bis-, and tris-primary alcohols catalyzed by a Cp*Ir complex

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RuCl2(DMSO)4 catalyzes the β-alkylation of secondary alcohols with primary alcohols through a hydrogen autotransfer process

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Green chemistry: The development of cross-dehydrogenative coupling (CDC) for chemical synthesis

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PURE AND APPLIED CHEMISTRY (2006)

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A solid-phase self-organized catalyst of nanopalladium with main-chain viologen polymers:: α-Alkylation of ketones with primary alcohols

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ORGANIC LETTERS (2006)

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The path forward for biofuels and biomaterials

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Borrowing hydrogen: iridium-catalysed reactions for the formation of C-C bonds from alcohols

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ORGANIC & BIOMOLECULAR CHEMISTRY (2006)

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Olefin-metathesis catalysts for the preparation of molecules and materials (Nobel lecture)

Robert H. Grubbs

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2006)

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Novel pyrazines from the myxobacterium Chondromyces crocatus and marine bacteria

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EUROPEAN JOURNAL OF ORGANIC CHEMISTRY (2005)

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Chromium- and manganese-salen promoted epoxidation of alkenes

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CHEMICAL REVIEWS (2005)

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Recyclable palladium catalyst for highly selective alpha alkylation of ketones with alcohols

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2005)

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An efficient direct α-alkylation of ketones with primary alcohols catalyzed by [Ir(cod)Cl]2/PPh3/KOH system without solvent

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2004)

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Cp*Ir complex-catalyzed N-heterocyclization of primary amines with diols:: A new catalytic system for environmentally benign synthesis of cyclic amines

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ORGANIC LETTERS (2004)

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A ruthenium-grafted hydrotalcite as a multifunctional catalyst for direct α-alkylation of nitriles with primary alcohols

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2004)

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Platinum group metals in catalysis: Fabrication of catalysts and catalyst precursors

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ORGANIC PROCESS RESEARCH & DEVELOPMENT (2003)

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Transition-metal-based Lewis acid and base ambiphilic catalysts of iridium hydride complexes: Multicomponent synthesis of glutarimides

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2003)

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Development of Pd-Cu catalyzed cross-coupling of terminal acetylenes with sp2-carbon halides

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JOURNAL OF ORGANOMETALLIC CHEMISTRY (2002)

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Kinetic study of the hydrosilylation of acetophenone by [Rh(cod)Cl]2/(R)-BINAP

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ORGANOMETALLICS (2002)

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Esomeprazole - A review of its use in the management of acid-related disorders

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DRUGS (2002)

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An unusual type of ruthenium-catalyzed transfer hydrogenation of ketones with alcohols accompanied by C-C coupling

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JOURNAL OF ORGANIC CHEMISTRY (2001)

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Electronic structure of bis(o-iminobenzosemiquinonato)metal complexes (Cu, Ni, Pd).: The art of establishing physical oxidation states in transition-metal complexes containing radical ligands

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Transition-metal complex-catalyzed reduction of amides with hydrosilanes: a facile transformation of amides to amines

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TETRAHEDRON LETTERS (2001)

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Article Chemistry, Organic

Conjugate reduction of α,β-unsaturated ketones using an MnIII catalyst, phenylsilane and isopropyl alcohol

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TETRAHEDRON LETTERS (2000)

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Design, synthesis, and biological evaluation of tricyclic nucleosides (dimensional probes) as analogues of certain antiviral polyhalogenated benzimidazole ribonucleosides

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Hydrosilylation of ketones catalyzed by tricarbonyl(naphthalene)manganese cation

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Synthesis and biological activities of novel antiallergic agents with 5-lipoxygenase inhibiting action

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BIOORGANIC & MEDICINAL CHEMISTRY (2000)

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