期刊
CHEMICAL COMMUNICATIONS
卷 58, 期 54, 页码 7507-7510出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc02650c
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资金
- NSFC [92061101, 21871141, 21871142, 22071109]
- Excellent Youth Foundation of NSF of Jiangsu Province [BK20211593]
- Guangdong Basic and Applied Basic Research Foundation [2021A1515110429]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- Foundation of Jiangsu Collaborative Innovation Center of Biomedical Functional Materials
A viologen-functionalized metal-organic framework (MOF), MIL-125-RV2+, was obtained by modifying MIL-125-NH2 with viologen molecules. MIL-125-RV2+ is the first viologen-based MOF used for photocatalytic CO2 reduction reaction (CO2RR), exhibiting excellent photocatalytic activity and high selectivity for HCOO-.
Here, a viologen-functionalized metal-organic framework (MOF), MIL-125-RV2+, was obtained by modification of MIL-125-NH2 with viologen molecules. MIL-125-RV2+, the first viologen-based MOF for photocatalytic CO2RR, exhibited excellent photocatalytic activity and high selectivity for HCOO-. The strategy of using photoresponsive color-changing organics to functionalize the MOF is significant for achieving efficient CO2RR.
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