☆ 4.1 Review

Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review

ENVIRONMENTAL SCIENCE-ATMOSPHERES (2022)

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Review Chemistry, Analytical

PFAS on atmospheric aerosol particles: a review

Jennifer A. Faust

Summary: Per- and polyfluoroalkyl substances (PFAS) are persistent organic pollutants that pose a concern to human health. They can be transported over long distances through sorption to aerosol particles in the atmosphere. Comprehensive monitoring and further research are needed to understand the distribution and evolution of PFAS.

ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS (2023)

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Article Chemistry, Physical

Computer Simulation of the Surface of Aqueous Ionic and Surfactant Solutions

Maria Lbadaoui-Darvas et al.

Summary: The interest in studying the surface of aqueous solutions of simple salts has increased in the past two decades, leading to progress and new unresolved questions. Computer simulation methods and intrinsic surface analysis methods have facilitated research in this field, raising new interesting questions. In addition to reviewing methodological advances, the focus is on the surface studies of two specific systems.

JOURNAL OF PHYSICAL CHEMISTRY B (2022)

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Article Engineering, Environmental

Per- and Polyfluoroalkyl Substances in Outdoor and Indoor Dust from Mainland China: Contributions of Unknown Precursors and Implications for Human Exposure

Bin Wang et al.

Summary: The concentrations of PFASs in indoor and outdoor dust samples in mainland China were analyzed. The study found high levels of emerging PFASs and unknown PFAA precursors in both indoor and outdoor dust. The estimated daily intake of PFAAs through indoor dust exceeded the daily threshold set by the European Food Safety Authority for toddlers.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Multidisciplinary

Tight Coupling of Surface and In-Plant Biochemistry and Convection Governs Key Fine Particulate Components over the Amazon Rainforest

Manish Shrivastava et al.

Summary: Combining aircraft measurements and model simulations, this study reveals the important role of in-plant biochemistry in fine particulate formation and atmosphere-biosphere- climate interactions over the Amazon rainforest. The study shows that direct emissions of certain gases formed by in-plant biochemical reactions explain a significant portion of sub-micrometer aerosol particles in the upper troposphere.

ACS EARTH AND SPACE CHEMISTRY (2022)

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Article Environmental Sciences

Molecular size of surfactants affects their degree of enrichment in the sea spray aerosol formation

Lingrui Liu et al.

Summary: This study investigated the impact of different molecular weights of ethylene glycol and polyethylene glycol on the properties of sea spray aerosol (SSA), showing that molecular weight affects the production efficiency of SSA and alters the structure of SSA.

ENVIRONMENTAL RESEARCH (2022)

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Review Geochemistry & Geophysics

Ice-Nucleating Particles That Impact Clouds and Climate: Observational and Modeling Research Needs

Susannah M. Burrows et al.

Summary: Atmospheric ice-nucleating particles play a critical role in precipitation formation and cloud radiative properties. However, our understanding of these particles is still limited. There is a need to bridge observations and models to improve the predictability of ice-nucleating particle abundance.

REVIEWS OF GEOPHYSICS (2022)

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Article Chemistry, Multidisciplinary

Morphology and Viscosity Changes after Reactive Uptake of Isoprene Epoxydiols in Submicrometer Phase Separated Particles with Secondary Organic Aerosol Formed from Different Volatile Organic Compounds

Ziying Lei et al.

Summary: The reactive uptake of VOC-derived semivolatile oxidation products on inorganic-organic submicron particles was studied, and it was found that the viscosity and morphology of the particles changed significantly after the uptake. The changes were highly dependent on the VOC precursor, and the impact on air quality and climate predictions could be altered.

ACS EARTH AND SPACE CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

In situ analysis of the bulk and surface chemical compositions of organic aerosol particles

Yuqin Qian et al.

Summary: Probing the chemical compositions of organic aerosol particles is crucial for understanding their growth mechanisms. However, methods to directly probe chemical species at aerosol particle surfaces are lacking. In this study, a new in situ spectroscopy technique is demonstrated to directly identify the chemical structures of molecules present on organic aerosol particle surfaces. This opens a new avenue in revealing the surface compositions and chemical aging in the formation of secondary organic aerosols in the atmosphere, as well as chemical analysis of indoor and outdoor viral aerosol particles.

COMMUNICATIONS CHEMISTRY (2022)

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Review Environmental Sciences

Single-particle Raman spectroscopy for studying physical and chemical processes of atmospheric particles

Zhancong Liang et al.

Summary: Studying the properties and processes of atmospheric particles at a single-particle level is valuable for understanding their fate and environmental impacts. Single-particle Raman spectroscopy is a practical analytical technique that can non-destructively characterize individual particles under atmospheric pressure.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2022)

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Review Chemistry, Analytical

Aerosol Droplet Surface Measurement Methods

Derrick M. Mott et al.

Summary: In recent years, there has been a surge in the development of analysis techniques aimed at studying the surface tension properties of aerosol droplets, which are thought to play a crucial role in weather patterns. The review focuses on the most relevant and influential studies, with an emphasis on historical trends and how current techniques are poised to revolutionize the field.

ANALYTICAL SCIENCES (2021)

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Review Chemistry, Multidisciplinary

Criegee Intermediates Beyond Ozonolysis: Synthetic and Mechanistic Insights

Zahid Hassan et al.

Summary: Criegee intermediates (CIs) have regained attention in modern chemistry due to their roles in chemical synthesis, climate control, and atmospheric chemistry. This Minireview summarizes key aspects of CIs, highlighting recent findings and potential for further investigations in this exciting field.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Physical

Atomic Force Microscopy: An Emerging Tool in Measuring the Phase State and Surface Tension of Individual Aerosol Particles

Hansol D. Lee et al.

Summary: Atmospheric aerosols are suspended particulate matter with varying composition, size, and mixing state. Understanding their impact on climate, atmosphere, and human health poses challenges, necessitating experimental methods to measure their dynamic properties. The recent emergence of atomic force microscopy as an experimental tool in physical, analytical, and atmospheric chemistry enables such measurements to be conducted on individual aerosol particles.

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 72 (2021)

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Review Environmental Sciences

Overview of biological ice nucleating particles in the atmosphere

Shu Huang et al.

Summary: Biological particles in the Earth's atmosphere play a crucial role as ice nucleating particles, influencing cloud and precipitation formation, and regional climate. Research has shown the ice nucleating properties and controlling factors of biological particles from various sources, yet there remain uncertainties and open questions for further investigations in this field.

ENVIRONMENT INTERNATIONAL (2021)

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Article Engineering, Environmental

Microscopic Evidence for Phase Separation of Organic Species and Inorganic Salts in Fine Ambient Aerosol Particles

Weijun Li et al.

Summary: Phase separation in aerosol particles reflects surface properties and organic component aging. Most particles >100 nm have inorganic aerosol core with OM coating. Rural particles show higher frequency of phase separation, indicating aging enhances it.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Chemical

Photochemistry of single optically trapped oleic acid droplets

Evelyne A. Parmentier et al.

Summary: The photodegradation of optically trapped oleic acid droplets by visible light was studied, showing that the oxygen amount and droplet size have minimal influence on the reaction rate. However, higher laser power and shorter wavelength significantly increased the reaction rate, suggesting that mechanisms involving the photoexcitation of oleic acid are dominant pathways. This study highlights the importance of considering direct photodegradation when using optical traps or spectroscopic methods to study aerosol particles containing fatty acids.

JOURNAL OF AEROSOL SCIENCE (2021)

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Article Environmental Sciences

Composition dependent density of ternary aqueous solutions of ionic surfactants and salts Capturing the effect of surfactant micellization in atmospheric droplet model solutions

Silvia M. Calderon et al.

Summary: Surfactants in atmospheric aerosols play a significant role in cloud droplet formation. By studying the properties of aqueous surfactant-salt solutions, it is possible to model the formation of atmospheric droplets in marine environments.

JOURNAL OF ATMOSPHERIC CHEMISTRY (2021)

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Article Chemistry, Physical

Chemistry and Photochemistry of Pyruvic Acid at the Air-Water Interface

Keaten J. Kappes et al.

Summary: The study investigates the chemistry and photochemistry of pyruvic acid at the air-water interface, showing that surface chemistry leads to substantial oligomer formation.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Engineering, Environmental

Sea Spray Aerosols Contain the Major Component of Human Lung Surfactant

Emmanuel Van Acker et al.

Summary: Marine phytoplankton release DPPC, influencing the composition of SSAs, with potential implications for human health. The airborne exposure to DPPC from SSAs may not directly affect human health, but it could facilitate the effects of other marine bioactive compounds. By analyzing environmental variables, it was found that wave height is a key predictor of DPPC air concentration and that DPPC content in SSAs is positively correlated with enriched aerosolization of Mg2+ and Ca2+.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Environmental

Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles

Weijun Li et al.

Summary: This study demonstrates that secondary aerosol particles exhibit a liquid-liquid phase-separated structure, with the thickness of the organic shell having a significant impact on the hygroscopic growth and phase transition process of the particles. The thicker the organic shell, the lower the hygroscopicity of the particles at low relative humidity, and the phase transition of the core from solid to liquid occurs earlier.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Environmental Sciences

Characterization of seawater and aerosol particle surfactants using solid phase extraction and mass spectrometry

Tret C. Burdette et al.

Summary: The study identified different classes of surface active organic molecules in ocean and aerosol particles, with varying proportions of anionic and cationic surfactants in atmospheric aerosol particles and estuarine water.

JOURNAL OF ENVIRONMENTAL SCIENCES (2021)

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Article Environmental Sciences

Role of Sea Surface Microlayer Properties in Cloud Formation

Brianna N. Hendrickson et al.

Summary: The study suggests that sea salt in marine aerosols is the key factor driving cloud formation potential, while organic material from ocean surface waters has minimal impact on the cloud condensation nuclei properties of aerosols. The cloud formation potential of mixed organic and sea salt marine aerosols will be slightly weakened or remain unchanged compared to sea spray aerosols.

FRONTIERS IN MARINE SCIENCE (2021)

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Article Chemistry, Physical

Hydration and Hydrogen Bond Order of Octadecanoic Acid and Octadecanol Films on Water at 21 and 1 °C

Maria G. Vazquez de Vasquez et al.

Summary: The research investigates the temperature-dependent hydration structure of long-chain fatty acids and alcohols at air-water interfaces using a combination of techniques including surface-sensitive infrared reflection-absorption spectroscopy (IRRAS) and ab initio molecular dynamics simulations. Results show that temperature affects the molecular structures of headgroup hydration shells, with high surface concentration of alcohols exhibiting the largest surface potential. This study provides insights into the complex surface potential and spectral signatures involved in ice templating behavior of fatty acids and alcohols.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Chemistry, Physical

Prediction of Phase State of Secondary Organic Aerosol Internally Mixed with Aqueous Inorganic Salts

Zechen Yu et al.

Summary: This study developed a regression model to predict aerosol phase separation relative humidity for various organic and inorganic mixes, showing that organic compounds with lower oxygen to carbon ratios, higher molecular weights, and higher aerosol acidity have greater phase separation relative humidity. Conversely, a larger fraction of inorganic nitrate led to lower phase separation relative humidity. The resulting model was demonstrated for three different SOA systems, showing liquid-liquid phase separation at relative humidity below 80%.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Chemistry, Physical

Low-Temperature Water Uptake of Individual Marine and Biologically Relevant Atmospheric Particles Using Micro-Raman Spectroscopy

Liora E. Mael et al.

Summary: The study found that at lower temperatures, some atmospheric particles begin to uptake water through mechanisms different from simple sugars, indicating that at lower temperatures, particles adsorb water on the surface rather than dissolve and absorb water. Furthermore, repeated water uptake cycles cause changes in the morphology of particles, promoting water uptake at lower relative humidity.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Molecular Chirality and Cloud Activation Potentials of Dimeric α-Pinene Oxidation Products

Aleia Bellcross et al.

Summary: The study shows that the surface activity of atmospherically relevant α-pinene-derived dimers is influenced by terminal functional groups and backbone stereochemistry, with a link established between molecular chirality and cloud activation potential of secondary organic aerosol particles. There is a roughly 10% difference in surface activity between diastereomers, with the more hydrophobic dimers exhibiting increased surface activity.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Physical

Core level photoelectron spectroscopy of heterogeneous reactions at liquid-vapor interfaces: Current status, challenges, and prospects

Remi Dupuy et al.

Summary: This article reviews the progress made in the study of liquid-vapor interfaces over the past few decades, discusses the challenges that need to be overcome in the research process, and looks forward to the future development direction.

JOURNAL OF CHEMICAL PHYSICS (2021)

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Article Chemistry, Physical

Important Oxidants and Their Impact on the Environmental Effects of Aerosols

Maofa Ge et al.

Summary: This paper reviews the latest research results of important oxidants in the atmosphere, such as HONO, NO3, N2O5, and CIs, and discusses the environmental effects of secondary particles formed through corresponding oxidation processes. Furthermore, it also provides some perspectives for future research.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Biochemical Research Methods

Investigation of the Acid-Mediated Photosensitized Reactions of Amphiphilic α-Keto Acids at the Air-Water Interface Using Field-Induced Droplet Ionization Mass Spectrometry

Chu Gong et al.

Summary: This study shows that the acid-mediated photochemistry of alpha-keto acids at the air-water interface is significantly different from those in bulk solution, contributing to the formation of HULIS. The research highlights the uniqueness of photochemistry at the air-water interface and suggests that further studies in this area could present rich opportunities.

JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY (2021)

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Article Environmental Sciences

Source profiles and emission factors of organic and inorganic species in fine particles emitted from the ultra-low emission power plant and typical industries

Xin Zeng et al.

Summary: Accurate source markers, profiles, and species-based emission factors are crucial for source apportionment and emission inventory research. This study collected PM2.5 from eight stationary sources, revealing dominant chemical species and identifying indicative chemical components and species ratios through statistical equations and randomForest. The study contributes to identifying emission sources of PM2.5, especially for subtypes of stationary sources, and to improving emission inventories continuously.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Multidisciplinary Sciences

Atmospheric aging enhances the ice nucleation ability of biomass-burning aerosol

Lydia G. Jahl et al.

Summary: Recent research has found that ice-nucleating particles in biomass-burning aerosol are driven by the production of mineral phases, and atmospheric aging can enhance the ice activity of these particles. Removing organic carbon particle coatings can increase the ice activity of biomass-burning aerosol by more than an order of magnitude.

SCIENCE ADVANCES (2021)

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Article Chemistry, Physical

In situ determination of the structure and composition of Langmuir monolayers at the air/water interface by neutron and X-ray reflectivity and ellipsometry

Armando Maestro et al.

Summary: This review paper focuses on the structure and composition of Langmuir monolayers (LMs) at the air/water interface using various experimental techniques. From the first experiment by Angels Pockels in her home kitchen to the present day, LMs of different materials have been extensively studied and are important model systems in biology, physics, and chemistry.

ADVANCES IN COLLOID AND INTERFACE SCIENCE (2021)

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Article Engineering, Environmental

Unexpected Oligomerization of Small α-Dicarbonyls for Secondary Organic Aerosol and Brown Carbon Formation

Yixin Li et al.

Summary: Experimental results show that the oligomerization of small alpha-dicarbonyls on sub-micrometer aerosols leads to the formation of secondary organic aerosol (SOA) and brown carbon (BrC) more efficiently upon exposure to atmospherically relevant concentrations. Carbenium ion-mediated nucleophilic addition, interfacial electric field-induced attraction, and synergetic oligomerization involving organic/inorganic species are identified as the key mechanisms for the distinct aerosol growth and light absorption in the presence of methylglyoxal.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Environmental

Photoinduced Release of Volatile Organic Compounds from Fatty Alcohols at the Air-Water Interface: The Role of Singlet Oxygen Photosensitized by a Carbonyl Group

Jingyi Lin et al.

Summary: The study reveals the significant impact of oxygen content on the total yields of VOCs during the photoinduced interfacial reaction of NOL, with O-1(2) playing a crucial role in VOC formation. The photoactivity of NOL is greatly enhanced in the presence of air compared to nitrogen, primarily due to the generation of O-1(2).

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Chemical

Surfactant Modeling Using Classical Density Functional Theory and a Group Contribution PC-SAFT Approach

Philipp Rehner et al.

Summary: Modeling of surfactants requires incorporation of the amphiphilic nature of molecules to describe key properties. A possible approach is to model surfactant molecules as heteronuclear chains. The model presented in this study is able to reproduce the significant enrichment of surfactant molecules at interfaces and the reduction of interfacial tensions, considering binary interaction parameters and the polarity of the surfactant head groups.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Impact of Tetrabutylammonium on the Oxidation of Bromide by Ozone

Shuzhen Chen et al.

Summary: The reaction of ozone with sea-salt derived bromide is enhanced by the presence of the cationic surfactant tetrabutylammonium (TBA), leading to increased concentrations of bromide and the bromide ozonide reaction intermediate at the aqueous interface. The enhanced interfacial reactivity is attributed to the positively charged nitrogen group in TBA, as well as its surface activity.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation

Nurun Nahar Lata et al.

Summary: This study investigated the physicochemical properties and ice nucleation activity of free tropospheric particles collected at a remote observatory in the North Atlantic Ocean. It was found that particles with different transport patterns had significant differences in size-resolved chemical composition, mixing state, and phase state. Particles with higher viscosity were found to be more ice active in the deposition mode at specific temperatures. This research provides a better understanding of the role of long-range transported free tropospheric aerosols in ice cloud formation.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Ozonolysis of Oleic Acid Aerosol Revisited: Multiphase Chemical Kinetics and Reaction Mechanisms

Thomas Berkemeier et al.

Summary: The chemical processing of organic aerosol particles plays a crucial role in atmospheric chemistry, climate, and public health. Heterogeneous oxidation of oleic acid particles by ozone is a commonly studied model system. However, there are systematic differences and inconsistencies in existing kinetic data and mechanistic analyses, which can be reconciled with consistent sets of multiphase chemical kinetic parameters through inverse modeling. Further experimental evidence is needed to uniquely determine these parameters and it is suggested that secondary reactions involving Criegee intermediates are essential for resolving discrepancies found in earlier studies.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Response of the Reaction Probability of N2O5 with Authentic Biomass-Burning Aerosol to High Relative Humidity

Lydia G. Jahl et al.

Summary: The study investigated the heterogeneous kinetics of N2O5(g) reactive uptake and ClNO2(g) product yields in biomass-burning smoke, revealing that high chloride fuels drive N2O5 reactive uptake and organic coatings do not limit the reaction in high-chloride fuels at high relative humidity. The experiments showed substantial nitryl chloride yield in high-chloride biomass-burning aerosol, approaching 100% at 86% relative humidity. The complex chemical composition and morphology of biomass-burning aerosol, as well as the solid phase state of chloride salts at relative humidity below 80%, limit the ability for N2O5 to react with the aerosol and produce ClNO2(g).

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Modeling the Size Distribution and Chemical Composition of Secondary Organic Aerosols during the Reactive Uptake of Isoprene-Derived Epoxydiols under Low-Humidity Condition

Mega Octaviani et al.

Summary: The study evaluates mechanistic IEPOX-SOA models through controlled experiments, finding that IEPOX multiphase chemistry can increase particle size and concentration, while the model can also predict particle number and diameter at the end of the experiment.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Physical

Shining New Light on the Kinetics of Water Uptake by Organic Aerosol Particles

Matus E. Diveky et al.

Summary: The uptake of water vapor by various organic aerosols plays a crucial role in applications such as medical delivery of pharmaceutical aerosols and cloud formation in the atmosphere. The mass accommodation coefficient, alpha(M), defines the probability of gas-phase molecules sticking to a surface, but accurate values are lacking for many systems. Experimental techniques, including photothermal single-particle spectroscopy (PSPS), have been used to study interfacial water transport and evaluate alpha(M) values for different organics.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Chemistry, Physical

Water-Air Interfaces as Environments to Address the Water Paradox in Prebiotic Chemistry: A Physical Chemistry Perspective

Alexandra M. Deal et al.

Summary: The asymmetric water-air interface provides a dynamic aqueous environment for abiotic synthesis reactions, promoting condensation reactions such as peptide synthesis, phosphorylation, and oligomerization. Photochemistry at water-air interfaces may have been a significant source of prebiotic molecular complexity, while the interfaces can also promote spontaneous reduction and oxidation reactions, potentially providing protometabolic pathways. Life likely began within a relatively short time frame, and water-air interfaces offer promising environments for simultaneous and efficient biomolecule production.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Chemistry, Physical

Ice Nucleation Activity of Perfluorinated Organic Acids

Ralph Schwidetzky et al.

Summary: Perfluorooctanoic acid (PFOA) can initiate heterogeneous ice nucleation at temperatures as high as -16 degrees C, potentially impacting cloud glaciation and the removal of persistent pollutants by wet deposition in the atmosphere.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

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Article Multidisciplinary Sciences

Coexistence of three liquid phases in individual atmospheric aerosol particles

Yuanzhou Huang et al.

Summary: Individual atmospheric particles can contain mixtures of primary organic aerosol (POA), secondary organic aerosol (SOA), and secondary inorganic aerosol (SIA), with the potential to have three distinct liquid phases. The presence of these phases is influenced by the elemental oxygen-to-carbon (O:C) ratio of the SOA, impacting equilibration timescales and potential effects on cloud formation and atmospheric chemistry.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

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Article Chemistry, Multidisciplinary

Simulation of Monoterpene SOA Formation by Multiphase Reactions Using Explicit Mechanisms

Zechen Yu et al.

Summary: The study simulated the formation of terpene secondary organic aerosol using a unified partitioning aerosol phase reaction model. By predicting oxygenated products and classifying them into groups based on volatility and reactivity, the model revealed three formation pathways including partitioning, oligomerization, and aqueous phase reactions. The model also included a peroxy radical autoxidation mechanism to form less volatile products.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Fluorescence Aerosol Flow Tube Spectroscopy to Detect Liquid-Liquid Phase Separation

Paul E. Ohno et al.

Summary: This study develops a method using fluorescence aerosol flow tube spectroscopy to characterize liquid-liquid phase separation in aerosols, and finds that the SRH values for submicron particles are lower than those for supermicron particles. The experiment uses fluorescence emission from probe molecules in particles to determine the relative humidity at which LLPS occurs.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Aerosol Marine Primary Carbohydrates and Atmospheric Transformation in the Western Antarctic Peninsula

Sebastian Zeppenfeld et al.

Summary: The study found higher concentrations of combined carbohydrates in both particulate and dissolved phases in seawater compared to dissolved free carbohydrates, with moderate enrichment factors in SML samples. In atmospheric particles, combined carbohydrates were mainly found in particles of two size modes and were strongly correlated with Na-aerosol and wind speed. The aerosol monosaccharide compositions in the atmosphere were significantly different from those in seawater, suggesting selective consumption and release of polysaccharides by bacteria in the atmosphere.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Engineering, Chemical

Water uptake and optical properties of mixed organic-inorganic particles

Lucy Nandy et al.

Summary: Atmospheric aerosol particles can consist of mixtures of inorganic and organic species, which can affect their water uptake and optical properties. Simplifying assumptions commonly made in chemical transport models for organic-inorganic mixtures can lead to significant errors in growth factor and single scattering albedo, especially for higher organic mass fractions.

AEROSOL SCIENCE AND TECHNOLOGY (2021)

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Article Chemistry, Analytical

'Measuring the Chemical Evolution of Levitated Particles: A Study on the Evaporation of Multicomponent Organic Aerosol

Ravleen Kaur Kohli et al.

Summary: Single-particle levitation methods provide an effective platform for probing the physical properties of atmospheric aerosol through micrometer-sized particles. By using high-resolution mass spectrometry, accurate measurements of the evolving size and composition of evaporating multicomponent levitated particles in real time were reported, providing insights into the evaporation dynamics and activity of organic components in suspended particles. Through compositionally resolved evaporation measurements and thermodynamic models, the LQ-EDB-MS platform demonstrates high precision and reproducibility, offering an effective methodology for future studies on chemical aging and gas-particle partitioning in suspended particles.

ANALYTICAL CHEMISTRY (2021)

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Article Environmental Sciences

Surfactant effect on the hygroscopicity of aerosol particles at relative humidity ranging from 80% to 99.5%: Internally mixed adipic acid-ammonium sulfate particles

Chao Zhang et al.

Summary: In this study, the hygroscopicity of aerosol particles composed of adipic acid and ammonium sulfate at 80-99.5% relative humidity was investigated using experimental and theoretical methods. A new model (Model 3 (UNIFAC)) was developed to account for the reduction of surface tension and the effects of bulk-surface partitioning of adipic acid on particle hygroscopicity. Results showed that the change in water activity had a greater impact on particle hygroscopicity than surface tension.

ATMOSPHERIC ENVIRONMENT (2021)

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Article Environmental Sciences

The possible role of the surface active substances (SAS) in the airborne transmission of SARS-CoV-2

Irena Ciglenecki et al.

Summary: This study examines the potential role of surface active substances (SAS) in stabilizing respiratory aerosols in a closed space, with enhanced concentrations observed indoors. The findings suggest that SAS may play a crucial role in stabilizing respiratory droplets and prolonging the viability of viruses inside droplets, such as SARS-CoV-2.

ENVIRONMENTAL RESEARCH (2021)

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Article Engineering, Environmental

Phase Behavior of Hydrocarbon-like Primary Organic Aerosol and Secondary Organic Aerosol Proxies Based on Their Elemental Oxygen-to-Carbon Ratio

Fabian Mahrt et al.

Summary: The research found that internal mixtures of POA and SOA in the atmosphere almost always formed two phases when the O/C ratio of the POA was less than 0.11. When the O/C ratio of the POA was between 0.11 and 0.29, the mixtures mostly resulted in particles with one liquid phase. However, depending on the types of SOA and POA surrogates, two liquid phases were also observed in some cases, and an increase in phase-separated particles was observed when increasing the relative humidity within this O/C range.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Environmental

Effect of Inorganic Salts on N-Containing Organic Compounds Formed by Heterogeneous Reaction of NO2 with Oleic Acid

Huifan Deng et al.

Summary: The study found that the processing of nitrogen oxides on fatty acids in urban grime and organic aerosol particles in the atmosphere can lead to the formation of HONO and other nitrogen-containing organic compounds. Under low humidity conditions, the uptake coefficient of NO2 on pure oleic acid decreases with increasing relative humidity.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Engineering, Environmental

Using Micro-Raman Spectroscopy to Investigate Chemical Composition, Mixing States, and Heterogeneous Reactions of Individual Atmospheric Particles

Mingjin Wang et al.

Summary: This study used micro-Raman spectroscopy to measure the chemical composition of individual atmospheric particles in Beijing air, identifying components such as (NH4)2SO4, NH4NO3, minerals, carbonaceous species, and NaNO3, which represent the main components of aerosol particles. The research also found possible reaction pathways of CaCO3 particles in the atmosphere, as well as internal mixtures of soot and inorganic material in 23% of soot-containing particles and organic and inorganic materials in 57% of organics-containing particles. Micro-Raman spectroscopy was shown to be a powerful tool for measuring the chemical composition of individual atmospheric particles with a diameter of >= 1.0 µm.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Physical

Seeded Crystal Growth of Internally Mixed Organic-Inorganic Aerosols: Impact of Organic Phase State

Shuichi B. Ushijima et al.

Summary: Atmospheric aerosols are complex mixtures of inorganic and organic components. This study focused on the efflorescence of (NH4)2SO4/organic particles and found that poly(ethylene glycol) 400 did not inhibit seeded crystal growth, while raffinose inhibited heterogeneous efflorescence at lower humidities. Lower humidity led to increased viscosity, preventing the diffusion of water and ions, and thus inhibiting efflorescence of aerosols. The observed efflorescence at higher humidity suggests that collisions can induce efflorescence of mixed aerosols.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Chemistry, Physical

Contribution of Different Molecules and Moieties to the Surface Tension in Aqueous Surfactant Solutions. II: Role of the Size and Charge Sign of the Counterions

Gyorgy Hantal et al.

Summary: The study investigates the impact of counterion type and charge sign on the surface tension of surfactant solutions, highlighting the key role of counterion hardness in this respect. The findings indicate that while charge inversion significantly affects surface tension contributions of different species, the overall surface tension of the system remains relatively unchanged due to compensating free energy changes.

JOURNAL OF PHYSICAL CHEMISTRY B (2021)

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Article Chemistry, Physical

Conjugate Acid-Base Interaction Driven Phase Transition at a 2D Air-Water Interface

R. Rajagopal et al.

Summary: The study introduces a lattice model to explain a recent observation of a cooperative surface adsorption effect for an organic acid system at an air-water interface, attributing the enhancement in acidity-dependent p-methylbenzoic acid to interactions between the acid and its conjugate base anion, which competes with repulsion between the conjugate bases. The research reveals an analogy to well-studied magnetic systems, showing how attractions between different molecular species can lead to a phase transition at the interface.

JOURNAL OF PHYSICAL CHEMISTRY B (2021)

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Article Chemistry, Physical

Thermodynamic Investigation of Droplet-Droplet and Bubble-Droplet Equilibrium in an Immiscible Medium

Hikmat Binyaminov et al.

Summary: This study examines the influence of interfacial tensions between different phases on the equilibrium morphology of multiphase systems, focusing on a simple model composed of liquid drops and bubbles. Using Gibbsian composite-system thermodynamics, equilibrium conditions and the system's free energy equation are derived and numerically solved. The effects of parameters on the system's geometry and stability are explored, with potential applications in various fields such as microfluidics, atmospheric physics, and oil recovery.

JOURNAL OF PHYSICAL CHEMISTRY B (2021)

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Article Chemistry, Physical

Cation-Driven Lipopolysaccharide Morphological Changes Impact Heterogeneous Reactions of Nitric Acid with Sea Spray Aerosol Particles

Christopher Lee et al.

Summary: This study found that the presence of divalent cations in sea spray aerosol particles reduces their reactivity with HNO3 compared to particles dominated by monovalent cations, due to changes in particle phase and morphology caused by cation interactions.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

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Article Environmental Sciences

Unraveling interfacial properties of organic-coated marine aerosol with lipase incorporation

Minglan Xu et al.

Summary: In this study, the effect of Burkholderia cepacia lipase on the surface properties of stearic acid monolayer at the air-water interface was investigated, revealing a significant expansion of the stearic acid film and reduction in molecular ordering as a result of lipase incorporation. The findings suggest that hydrophobic interaction plays a key role in the disorder of stearic acid monolayer in the presence of lipase, providing insights into lipid-enzyme interfacial interactions.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Chemistry, Multidisciplinary

Differences in Photosensitized Release of VOCs from Illuminated Seawater versus Freshwater Surfaces

Laura T. Stirchak et al.

Summary: Recent studies have shown that photochemical reactions at the air-water interface are a source of volatile organic compounds (VOCs) to the atmosphere. Different photochemical pathways were observed for VOC formation from illuminated seawater coated with nonanoic acid compared to freshwater. The presence of halides, metals, and pH differences between freshwater and seawater may contribute to the differences in product formation.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ

Ying Li et al.

Summary: SOA's glass transition temperature and viscosity play important roles in the formation and evolution of atmospheric particulate matter; the Tg and viscosity of dry SOA are mainly influenced by different species at different locations and seasons; significant vertical variations exist in SOA, with winter exhibiting glass transition at lower altitudes.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Enhanced Ice Nucleation of Simulated Sea Salt Particles with the Addition of Anthropogenic Per- and Polyfluoroalkyl Substances

Martin J. Wolf et al.

Summary: The research demonstrates that adding common fluorinated pollutants to seawater can enhance the ice nucleation activity of simulated sea spray particles, especially in conditions relevant to cirrus cloud formation. Further studies are needed to investigate the interactions of fluorinated pollutants with other marine organic matter to determine the impacts of particle composition on the ice nucleation activity of ambient sea spray.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Ice Nucleating Activity and Residual Particle Morphology of Bulk Seawater and Sea Surface Microlayer

Priyatanu Roy et al.

Summary: Laboratory experiments using microfluidic technology to simulate the ocean-atmosphere environment were used to analyze the ice nucleating characteristics of INPs in sea spray aerosols. The study found different morphologies of dried residual particles, with a higher quantity of particles in the sea surface microlayer compared to bulk samples. Additionally, the study noted that different morphologies of particles had different ice nucleation spectra.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Morphology of Organic Carbon Coatings on Biomass-Burning Particles and Their Role in Reactive Gas Uptake

Leif G. Jahn et al.

Summary: Inorganic salts and organic carbon in biomass-burning aerosols undergo complex chemical reactions during atmospheric aging, with organic carbon particle coatings and deliquescence limitations of chloride salts potentially affecting the occurrence and extent of chloride displacement reactions.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Zinc-Carboxylate Binding in Mixed Octadecanoic Acid and Octadecanol Monolayers on Proxy Seawater Solution Surfaces

Nicole C. Auvil et al.

Summary: The study found that the ratio of fatty alcohols to fatty acids in organic coatings on sea spray aerosol affects the binding affinity of Zn2+-carboxylate on the surface. It was observed that Zn2+-carboxylate binding at the surface is significantly enhanced compared to bulk solution, and the addition of fatty alcohols can reduce the apparent binding affinity.

ACS EARTH AND SPACE CHEMISTRY (2021)

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Article Environmental Sciences

A predictive thermodynamic framework of cloud droplet activation for chemically unresolved aerosol mixtures, including surface tension, non-ideality, and bulk-surface partitioning

Nonne L. Prisle

Summary: This study presents a thermodynamically consistent framework for self-contained and predictive calculations of droplet growth and activation in atmospheric aerosols with consideration of surface adsorption, surface tension reduction, and non-ideal water activity. The model couples Kohler theory with the Gibbs adsorption and Szyszkowski-type surface tension equations to quantify composition-dependent properties for chemically unresolved mixtures. The impact of surface activity on cloud condensation nuclei (CCN) activation is systematically explored, showing that the effects of surface-active species on droplet growth and activation can be accurately predicted.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Ice nucleation on surrogates of boreal forest SOA particles: effect of water content and oxidative age

Ana A. Piedehierro et al.

Summary: The study reveals that surrogates of boreal forest secondary organic aerosol (SOA) particles only promote homogeneous ice formation, and the effect of homogeneous freezing is influenced by preconditioning humidity rather than the oxidative age of the SOA.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

An organic crystalline state in ageing atmospheric aerosol proxies: spatially resolved structural changes in levitated fatty acid particles

Adam Milsom et al.

Summary: The study reveals the existence of crystalline acid-soap complexes in organic aerosols and emphasizes that the atmospheric lifetime of organic species in aerosols highly depends on their phase state. These findings have significant implications for climate, urban air quality, and the long-range transport of pollutants.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds

Andreas Tilgner et al.

Summary: The acidity of aqueous atmospheric solutions plays a crucial role in the partitioning of trace gases, aqueous-phase chemistry, and environmental impacts. Atmospheric research has made significant progress in understanding the feedbacks between acidity and multiphase chemistry, highlighting the need for further investigations and advancements in measurements and modeling tools.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Opinion: Papers that shaped tropospheric chemistry

Paul S. Monks et al.

Summary: This paper examines the impact of published papers on the development of atmospheric chemistry, identifying major milestones through their influence on science, legislation, and environmental events. It also discusses the methods of identifying papers with the most significant impact on the field, along with the advantages and disadvantages of various approaches.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Ice nucleation ability of ammonium sulfate aerosol particles internally mixed with secondary organics

Barbara Bertozzi et al.

Summary: The study investigated the ice nucleation ability of internally mixed particles composed of crystalline ammonium sulfate (AS) and secondary organic material (SOM) at temperatures between -50 and -65 degrees C. The results show that the ice nucleation ability of mixed AS / SOM particles is strongly dependent on particle morphology. Further research is needed to investigate the impact of atmospheric aging and cloud processing on the morphology and related ice nucleation ability of internally mixed particles.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Chemistry, Physical

The persistence of a proxy for cooking emissions in megacities: a kinetic study of the ozonolysis of self-assembled films by simultaneous small and wide angle X-ray scattering (SAXS/WAXS) and Raman microscopy

Adam Milsom et al.

Summary: Cooking emissions play a significant role in urban organic aerosol emissions, with their kinetic behavior depend on film thickness and potential formation of inert crust. The study also suggests the presence of unreacted proxies after extensive ozone exposure, indicating a potential impact on the atmospheric lifetimes of aerosol components.

FARADAY DISCUSSIONS (2021)

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Article Chemistry, Multidisciplinary

Direct observation and assessment of phase states of ambient and lab-generated sub-micron particles upon humidification

Zezhen Cheng et al.

Summary: This study introduces a new analytical platform that directly observes and evaluates the phase transition of particles under different relative humidity and temperature conditions, based on the aspect ratio of the particles. The results show that solid organic particles transition to semi-solid and liquid states at specific relative humidity levels.

RSC ADVANCES (2021)

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Article Chemistry, Physical

Molecular dynamics simulations demonstrate that non-ideal mixing dominates subsaturation organic aerosol hygroscopicity

Daniel Roston

Summary: The study reveals that current force fields may not be suitable for simulating extreme environments of aerosol particles, highlighting some shortcomings in current understanding of hygroscopic growth and cloud nucleation. The widely used model of hygroscopicity breaks down in cases of deviations from ideal solution behavior, but a revised model incorporating non-ideal mixing rescues the general framework and helps understand simulation results and atmospheric aerosol behaviors over a full range of humidity.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Article Environmental Sciences

A two-component parameterization of marine ice-nucleating particles based on seawater biology and sea spray aerosol measurements in the Mediterranean Sea

Jonathan Trueblood et al.

Summary: INPs have a significant impact on cloud properties over oceans. Recent studies show that marine INPs come from two classes of organic matter in SSAs, yet current parameterizations may mask specific trends. This paper proposes a new parameterization based on field study results to better understand the connection between ocean biology and marine INP abundance.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Compositions and mixing states of aerosol particles by aircraft observations in the Arctic springtime, 2018

Kouji Adachi et al.

Summary: Aerosol particles collected in the Arctic at different altitudes showed variations in composition, size, and sources. Mineral-dust and sea-salt particles decreased in number fraction with increasing altitude, while K-bearing particles increased within a biomass burning plume originating from Siberia. Chlorine in sea-salt particles was replaced with sulfate at high altitudes.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency

Duseong S. Jo et al.

Summary: Secondary organic aerosol (SOA) is a significant contributor to fine particulate matter in the atmosphere, with volatility-based SOA parameterizations showing reasonable performance but potential errors when applied to future climatic conditions. Explicit mechanism predictions suggest variability in isoprene epoxydiols (IEPOX SOA) concentrations across different scenarios, highlighting the importance of capturing key physicochemical drivers for accurate SOA concentration predictions in climate studies.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Ozonolysis of fatty acid monolayers at the air-water interface: organic films may persist at the surface of atmospheric aerosols

Benjamin Woden et al.

Summary: The study focused on the ozonolysis of fatty acid monolayers to understand the behavior of organic-coated aerosols under realistic atmospheric conditions. Residual surface films, suspected to be formed of nonanoic acid and a mixture of compounds, were found to be retained at the interface after ozonolysis at near-zero temperatures, with potential implications for cloud formation. The presence of stable reaction products also indicates the possibility of inert monolayer build-up during the aerosol life cycle.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Effects of liquid-liquid phase separation and relative humidity on the heterogeneous OH oxidation of inorganic-organic aerosols: insights from methylglutaric acid and ammonium sulfate particles

Hoi Ki Lam et al.

Summary: This study investigated how phase separation in model aqueous droplets containing an inorganic salt and an organic acid alters the heterogeneous OH reactivity. It was found that the reactivity is slightly higher in phase-separated droplets due to the higher surface concentrations of organic molecules when the relative humidity decreases. Understanding aerosol phase state is crucial for probing heterogeneous reactivity under different environmental conditions.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Environmental Sciences

Mass accommodation and gas-particle partitioning in secondary organic aerosols: dependence on diffusivity, volatility, particle-phase reactions, and penetration depth

Manabu Shiraiwa et al.

Summary: The study introduces an effective mass accommodation coefficient that considers the penetration depth into the particle phase, addressing key issues in the gas-particle partitioning of organic compounds in secondary organic aerosols (SOA).

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

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Article Chemistry, Multidisciplinary

Aerosol Optical Tweezers Constrain the Morphology Evolution of Liquid-Liquid Phase-Separated Atmospheric Particles

Kyle Gorkowski et al.

CHEM (2020)

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Article Chemistry, Analytical

Dual-Balance Electrodynamic Trap as a Microanalytical Tool for Identifying Gel Transitions and Viscous Properties of Levitated Aerosol Particles

David S. Richards et al.

ANALYTICAL CHEMISTRY (2020)

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Article Chemistry, Physical

Mass Accommodation Coefficients of Water on Organics from Complementary Photoacoustic and Light Scattering Measurements on Laser-Trapped Droplets

Sandra Roy et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2020)

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Article Chemistry, Physical

Interfacial Water Mediates Oligomerization Pathways of Monoterpene Carbocations

Shinnosuke Ishizuka et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

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Article Multidisciplinary Sciences

Radiative absorption enhancements by black carbon controlled by particle-to-particle heterogeneity in composition

Laura Fierce et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2020)

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Article Multidisciplinary Sciences

Surface reservoirs dominate dynamic gas-surface partitioning of many indoor air constituents

Chen Wang et al.

SCIENCE ADVANCES (2020)

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Article Chemistry, Multidisciplinary

Environmental Processing of Short-Chain Fatty Alcohols Induced by Photosensitized Chemistry of Brown Carbons

Bo You et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Organic Enrichment, Physical Phase State, and Surface Tension Depression of Nascent Core-Shell Sea Spray Aerosols during Two Phytoplankton Blooms

Hansol D. Lee et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Reactive VOC Production from Photochemical and Heterogeneous Reactions Occurring at the Air-Ocean Interface

Gordon A. Novak et al.

ACCOUNTS OF CHEMICAL RESEARCH (2020)

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Review Chemistry, Multidisciplinary

Liquid-Liquid Phase Separation in Supermicrometer and Submicrometer Aerosol Particles

Miriam Arak Freedman

ACCOUNTS OF CHEMICAL RESEARCH (2020)

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Review Environmental Sciences

Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review

Kirill Semeniuk et al.

ATMOSPHERE (2020)

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Review Engineering, Environmental

Organosulfates in Ambient Aerosol: State of Knowledge and Future Research Directions on Formation, Abundance, Fate, and Importance

Martin Brueggemann et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2020)

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Article Multidisciplinary Sciences

The surface tension of surfactant-containing, finite volume droplets

Bryan R. Bzdek et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2020)

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Article Chemistry, Physical

Anomalous pH-Dependent Enhancement of p-Methyl Benzoic Acid Sum-Frequency Intensities: Cooperative Surface Adsorption Effects

Richard S. Andino et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2020)

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Article Chemistry, Physical

Free Energy and Dynamics of Organic-Coated Water Droplet Coalescence

Chi Yuen Pak et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2020)

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Article Chemistry, Multidisciplinary

Spectroscopic and Photochemical Properties of Secondary Brown Carbon from Aqueous Reactions of Methylglyoxal

Aaron W. Harrison et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Real-Time Measurements of pH Changes in Single, Acoustically Levitated Droplets Due to Atmospheric Multiphase Chemistry

Liron Cohen et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Article Environmental Sciences

Characterization of organic aerosol at a rural site influenced by olive waste biomass burning

Rosa Perez Pastor et al.

CHEMOSPHERE (2020)

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Article Environmental Sciences

Light absorption of black carbon aerosols strongly influenced by particle morphology distribution

Yu Wu et al.

ENVIRONMENTAL RESEARCH LETTERS (2020)

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Review Chemistry, Physical

Particle formation and surface processes on atmospheric aerosols: A review of applied quantum chemical calculations

Angelina Leonardi et al.

INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Physicochemical Mixing State of Sea Spray Aerosols: Morphologies Exhibit Size Dependence

Hansol D. Lee et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Production of Peroxy Radicals from the Photochemical Reaction of Fatty Acids at the Air-Water Interface

Nathalie Hayeck et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Hourly Measurements of Organic Molecular Markers in Urban Shanghai, China: Primary Organic Aerosol Source Identification and Observation of Cooking Aerosol Aging

Qiongqiong Wang et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Molecular reactions at aqueous interfaces

Manuel F. Ruiz-Lopez et al.

NATURE REVIEWS CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Mulitphase Atmospheric Chemistry in Liquid Water: Impacts and Controllability of Organic Aerosol

Annmarie G. Carlton et al.

ACCOUNTS OF CHEMICAL RESEARCH (2020)

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Review Chemistry, Multidisciplinary

Aerosol Optical Tweezers Elucidate the Chemistry, Acidity, Phase Separations, and Morphology of Atmospheric Microdroplets

Ryan C. Sullivan et al.

ACCOUNTS OF CHEMICAL RESEARCH (2020)

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Review Chemistry, Multidisciplinary

CAICE Studies: Insights from a Decade of Ocean-Atmosphere Experiments in the Laboratory

Kathryn J. Mayer et al.

ACCOUNTS OF CHEMICAL RESEARCH (2020)

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Article Chemistry, Physical

Surface pKa of Saturated Carboxylic Acids at the Air/Water Interface: A Quantum Chemical Approach

Yuri B. Vysotsky et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2020)

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Article Chemistry, Physical

In Situ Spectroscopic Probing of Polarity and Molecular Configuration at Aerosol Particle Surfaces

Yuqin Qian et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

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Review Environmental Sciences

Chemical identity and cardiovascular toxicity of hydrophobic organic components in PM2.5

Zenghua Qi et al.

ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY (2020)

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Article Engineering, Environmental

Enhanced Photochemical Volatile Organic Compounds Release from Fatty Acids by Surface-Enriched Fe(III)

Di Huang et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2020)

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Article Chemistry, Physical

Diol it up: The influence of NaCl on methylglyoxal surface adsorption and hydration state at the air-water interface

Brittany P. Gordon et al.

JOURNAL OF CHEMICAL PHYSICS (2020)

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Article Chemistry, Physical

Relating Structure and Ice Nucleation of Mixed Surfactant Systems Relevant to Sea Spray Aerosol

Russell J. Perkins et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2020)

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Review Chemistry, Multidisciplinary

Photoinduced Oxidation Reactions at the Air-Water Interface

Josep M. Anglada et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Quantifying the Counterion-Specific Effect on Surfactant Adsorption Using Modeling, Simulation, and Experiments

Mengsu Peng et al.

LANGMUIR (2020)

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Article Multidisciplinary Sciences

Predicting the influence of particle size on the glass transition temperature and viscosity of secondary organic material

Markus Petters et al.

SCIENTIFIC REPORTS (2020)

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Review Chemistry, Multidisciplinary

Indoor Surface Chemistry: Developing a Molecular Picture of Reactions on Indoor Interfaces

Andrew P. Ault et al.

CHEM (2020)

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Article Chemistry, Multidisciplinary

Marine Bacteria Affect Saccharide Enrichment in Sea Spray Aerosol during a Phytoplankton Bloom

Elias S. Hasenecz et al.

ACS EARTH AND SPACE CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Relationship between the Bulk and Surface Basicity of Aliphatic Amines: A Quantum Chemical Approach

Elena S. Kartashynska et al.

ACS OMEGA (2020)

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Article Environmental Sciences

Model for estimating activity coefficients in binary and ternary ionic surfactant solutions The CMC based ionic surfactant activity (CISA) model for atmospheric applications

Silvia M. Calderon et al.

JOURNAL OF ATMOSPHERIC CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Insights into the behavior of nonanoic acid and its conjugate base at the air/water interface through a combined experimental and theoretical approach

Man Luo et al.

CHEMICAL SCIENCE (2020)

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Review Chemistry, Multidisciplinary

Radical chemistry in oxidation flow reactors for atmospheric chemistry research

Zhe Peng et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Environmental Sciences

Predicting secondary organic aerosol phase state and viscosity and its effect on multiphase chemistry in a regional-scale air quality model

Ryan Schmedding et al.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2020)

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Article Chemistry, Physical

Role of the Counterions in the Surface Tension of Aqueous Surfactant Solutions. A Computer Simulation Study of Alkali Dodecyl Sulfate Systems

Gyorgy Hantal et al.

COLLOIDS AND INTERFACES (2020)

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Article Environmental Sciences

Sea spray aerosol organic enrichment, water uptake and surface tension effects

Luke T. Cravigan et al.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2020)

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Article Environmental Sciences

Global inorganic nitrate production mechanisms: comparison of a global model with nitrate isotope observations

Becky Alexander et al.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2020)

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Article Chemistry, Physical

From atoms to aerosols: probing clusters and nanoparticles with synchrotron based mass spectrometry and X-ray spectroscopy

Musahid Ahmed et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2020)

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Article Environmental Sciences

Biomass-burning-derived particles from a wide variety of fuels - Part 1: Properties of primary particles

Crystal D. McClure et al.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2020)

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Article Environmental Sciences

Establishing a model organic film of low volatile compound mixture on aqueous aerosol surface

Siyang Li et al.

ATMOSPHERIC ENVIRONMENT (2019)

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Article Chemistry, Physical

Organic Surfactants Protect Dissolved Aerosol Components against Heterogeneous Oxidation

Jennifer A. Faust et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2019)

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Article Chemistry, Physical

Surface Tensions of Picoliter Droplets with Sub-Millisecond Surface Age

Rachael E. H. Miles et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2019)

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Review Geochemistry & Geophysics

Aerosol Mixing State: Measurements, Modeling, and Impacts

N. Riemer et al.

REVIEWS OF GEOPHYSICS (2019)

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Article Environmental Sciences

Alterations in the surface properties of sea spray aerosols introduced by the presence of sterols

Shumin Cheng et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2019)

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Article Chemistry, Multidisciplinary

Insights into the Headgroup and Chain Length Dependence of Surface Characteristics of Organic-Coated Sea Spray Aerosols

Shumin Cheng et al.

ACS EARTH AND SPACE CHEMISTRY (2019)

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Article Multidisciplinary Sciences

Multiphase reactivity of polycyclic aromatic hydrocarbons is driven by phase separation and diffusion limitations

Shouming Zhou et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2019)

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Article Engineering, Environmental

Organosulfur Compounds Formed from Heterogeneous Reaction between SO2 and Particulate-Bound Unsaturated Fatty Acids in Ambient Air

Ming Zhu et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS (2019)

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Article Chemistry, Multidisciplinary

In Situ Surface Tension Measurements of Hanging Droplet Methylglyoxal/Ammonium Sulfate Aerosol Mimics under Photooxidative Conditions

Thomas Beier et al.

ACS EARTH AND SPACE CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Shedding Light on Photosensitized Reactions within Marine-Relevant Organic Thin Films

Jonathan Trueblood et al.

ACS EARTH AND SPACE CHEMISTRY (2019)

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Article Chemistry, Analytical

Correlating 3D Morphology, Phase State, and Viscoelastic Properties of Individual Substrate-Deposited Particles

Kamal K. Ray et al.

ANALYTICAL CHEMISTRY (2019)

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A short overview of the microbial population in clouds: Potential roles in atmospheric chemistry and nucleation processes

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Review Engineering, Environmental

Adsorption and Reaction of Trace Gas-Phase Organic Compounds on Atmospheric Water Film Surfaces: A Critical Review

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Heterogeneous oxidation of atmospheric aerosol particles by gas-phase radicals

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NATURE CHEMISTRY (2010)

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Reactive intermediates revealed in secondary organic aerosol formation from isoprene

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An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds

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Surfactant Control of Gas Transport and Reactions at the Surface of Sulfuric Acid

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ACCOUNTS OF CHEMICAL RESEARCH (2009)

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Atmospheric composition change: Climate-Chemistry interactions

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Composition Domains in Monoterpene Secondary Organic Aerosol

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ENVIRONMENTAL SCIENCE & TECHNOLOGY (2009)

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Beyond single particle mass spectrometry: multidimensional characterisation of individual aerosol particles

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INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY (2009)

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Relative importance of organic coatings for the heterogeneous hydrolysis of N2O5 during summer in Europe

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Oxidation of oleic acid at the air-water interface and its potential effects on cloud critical supersaturations

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Chemistry and Microphysics of Atmospheric Aerosol Surfaces: Laboratory Techniques and Applications

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ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS (2009)

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The formation, properties and impact of secondary organic aerosol: current and emerging issues

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ATMOSPHERIC CHEMISTRY AND PHYSICS (2009)

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Review Meteorology & Atmospheric Sciences

On the formation and growth of atmospheric nanoparticles

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ATMOSPHERIC RESEARCH (2008)

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Primary submicron marine aerosol dominated by insoluble organic colloids and aggregates

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GEOPHYSICAL RESEARCH LETTERS (2008)

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A thermodynamic model of mixed organic-inorganic aerosols to predict activity coefficients

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ATMOSPHERIC CHEMISTRY AND PHYSICS (2008)

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Mass transfer effects on the hygroscopic growth of ammonium sulfate particles with a water-insoluble coating

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Heterogeneous ice nucleation rate coefficient of water droplets coated by a nonadecanol monolayer

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A single parameter representation of hygroscopic growth and cloud condensation nucleus activity

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ATMOSPHERIC CHEMISTRY AND PHYSICS (2007)

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Chemical and microphysical characterization of ambient aerosols with the aerodyne aerosol mass spectrometer

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Molecular size evolution of oligomers in organic aerosols collected in urban atmospheres and generated in a smog chamber

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Review Environmental Sciences

Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature)

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ATMOSPHERIC CHEMISTRY AND PHYSICS (2006)

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The effect of physical and chemical aerosol properties on warm cloud droplet activation

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ATMOSPHERIC CHEMISTRY AND PHYSICS (2006)

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Thermodynamic models of aqueous solutions containing inorganic electrolytes and dicarboxylic acids at 298.15 K. 1. The acids as nondissociating components

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JOURNAL OF PHYSICAL CHEMISTRY A (2006)

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Article Chemistry, Physical

Thermodynamic models of aqueous solutions containing inorganic electrolytes and dicarboxylic acids at 298.15 K. 2. Systems including dissociation equilibria

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Photoemission from liquid aqueous solutions

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CHEMICAL REVIEWS (2006)

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The influence of organic films at the air-aqueous boundary on atmospheric processes

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Towards understanding ice nucleation by long chain alcohols

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Critical appraisal of salting-out and its implications for chemical and biological sciences

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CHEMICAL REVIEWS (2005)

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ENVIRONMENTAL SCIENCE & TECHNOLOGY (2004)

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A review of surface ozone background levels and trends

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ATMOSPHERIC ENVIRONMENT (2004)

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Measurement of OH and HO2 in the troposphere

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CHEMICAL REVIEWS (2003)

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Dimeric and oligomeric surfactants. Behavior at interfaces and in aqueous solution: a review

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ADVANCES IN COLLOID AND INTERFACE SCIENCE (2002)

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Molecular dynamics simulations of template-assisted nucleation: Alcohol monolayers at the air-water interface and ice formation

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Preactivation in the nucleation of ice by Langmuir films of aliphatic alcohols

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Thermodynamic modelling of aqueous aerosols containing electrolytes and dissolved organic compounds

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Adsorption and surface tension of ionic surfactants at the air-water interface: review and evaluation of equilibrium models

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COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS (2001)

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Review Chemistry, Physical

Dynamic surface tension and adsorption mechanisms of surfactants at the air-water interface

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ADVANCES IN COLLOID AND INTERFACE SCIENCE (2000)

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