期刊
CHEMICAL COMMUNICATIONS
卷 58, 期 57, 页码 7944-7947出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc02314h
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资金
- National Key RD Program [2021YFC3001103]
- National Natural Science Foundation [22178165, 21921006]
- Natural Science Foundation of Jiangsu Province [BK20211262]
- priority academic program development of Jiangsu higher education institutions (PAPD)
- State Key Laboratory of MaterialsOriented Chemical Engineering of China [ZK201902]
A novel method for synthesizing hollow MOFs using the self-deliquescence of hydration water in metallic precursors and low water solubility solvents at the two-phase interface is proposed. The resulting hierarchically porous hollow MOFs exhibit significant enhancements in CO2 separation and catalysis.
A novel single-solvent-interfacial strategy is proposed to synthesize hollow MOFs, fabricated at the two-phase interface originated from the self-deliquescence of hydration water in the metallic precursors and the solvents with low water solubility. The as-fabricated HMOFs with hierarchically porous structures exhibit significant enhancement in CO2 separation and catalysis.
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