期刊
ORGANIC CHEMISTRY FRONTIERS
卷 3, 期 3, 页码 349-353出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5qo00387c
关键词
-
资金
- Chinese NSF [81430080, 81125021]
- Major State Basic Research Development Program [2015CB910603]
- SIMM [CASIMM0120154002/2002]
A rhodium-catalyzed oxidative annulation of N-acyl anilines with alkynes was developed by using the acylamino group as a traceless directing group for the first time. Various N-acyl anilines and para-or meta-substituted diphenylacetylenes were well tolerated, and a series of 1,2,3,4-tetrasubstituted naphthalenes were readily synthesized in good to excellent yields. Meanwhile, this method also provides a new strategy for the N-dearylation of N-phenylamides.
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