☆ 4.8 Review

Single-molecule magnets beyond a single lanthanide ion: the art of coupling

CHEMICAL SCIENCE (2022)

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Summary: Mixed-valence dilanthanide complexes with a singly occupied lanthanide-lanthanide sigma-bonding orbital were reported, showing outstanding magnetic properties due to the strong alignment of the sigma-bonding and f electrons on both lanthanides. The combination of a well-isolated high-spin ground state and large magnetic anisotropy in (Cp-iPr5)(2)Dy2I3 results in an enormous coercive magnetic field at high temperatures.

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