☆ 4.7 Review

Bio-inspired nanostructured g-C3N4-based photocatalysts: A comprehensive review

CHINESE JOURNAL OF CATALYSIS (2022)

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Metal-free four-in-one modification of g-C3N4 for superior photocatalytic CO2 reduction and H2 evolution

Mahmoud Kamal Hussien et al.

Summary: This study presents a green method for synthesizing a metal free modified g-C3N4 photocatalyst, achieving high efficiency in gas-phase CO2 reduction and hydrogen generation without the need for any cocatalyst. This work provides a new avenue for exploring rational modifications of g-C3N4 nanosheets for efficient clean energy production.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Multidisciplinary

Unraveling the dual defect sites in graphite carbon nitride for ultra-high photocatalytic H2O2 evolution

Xu Zhang et al.

Summary: Defect engineering modified graphite carbon nitride (g-C3N4) with dual defect sites, -C N groups and N vacancies, has been found to significantly enhance the photocatalytic production of H2O2. The dual defect sites form an electron-rich structure and lead to a more localized charge density distribution, which improves light absorption, carrier separation, selectivity, and activity of H2O2 generation. The N vacancies effectively adsorb and activate O-2, while the -C N groups facilitate the adsorption of H+, synergistically promoting H2O2 generation. The modified g-C3N4 achieved a high H2O2 generation rate and apparent quantum efficiency, surpassing previously reported g-C3N4-based photocatalysts.

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Article Chemistry, Multidisciplinary

ortho-Terphenylene Viologens with Through-Space Conjugation for Enhanced Photocatalytic Oxidative Coupling and Hydrogen Evolution

Ben He et al.

Summary: A series of novel ortho-terphenylene viologen derivatives with through-space conjugation were reported. These derivatives showed strong photoluminescence and special redox characteristics, making them suitable for photocatalytic reactions and hydrogen production.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Multidisciplinary Sciences

Single-atom Cu anchored catalysts for photocatalytic renewable H2 production with a quantum efficiency of 56%

Yumin Zhang et al.

Summary: In this work, highly dispersed and large loading amount of copper single-atoms were successfully achieved on TiO2, exhibiting excellent photocatalytic hydrogen evolution performance and stability. Furthermore, it demonstrated an apparent quantum efficiency of 56% at 365 nm, representing a significant breakthrough in this field.

NATURE COMMUNICATIONS (2022)

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Review Chemistry, Applied

Role of transition metal oxides in g-C3N4-based heterojunctions for photocatalysis and supercapacitors

Liqi Bai et al.

Summary: g-C3N4 has emerged as a promising 2D photocatalyst due to its unique structure and low cost, but faces limitations. Designing heterojunctions based on g-C3N4 is a promising approach to improving photocatalytic activity and showing potential in electrochemical energy storage.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

Sea-urchin-like ReS2 nanosheets with charge edge-collection effect as a novel cocatalyst for high-efficiency photocatalytic H2 evolution

Bo Lin et al.

Summary: The recombination of charge carriers in semiconductor photocatalysts limits the practical application of solar-driven H-2 evolution. In this study, sea-urchin-like ReS2 nanosheet/TiO2 nanoparticle heterojunctions (SURTHs) were constructed to achieve high charge separation efficiency. The unique sea-urchin-like structure of SURTHs enables an unusual charge edge-collection effect, leading to accelerated charge separation and transfer. As a result, the photocatalytic H-2 evolution rate of SURTHs is significantly improved compared to P25 TiO2.

CHINESE CHEMICAL LETTERS (2022)

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Article Chemistry, Multidisciplinary

Two-Dimensional Defective Boron-Doped Niobic Acid Nanosheets for Robust Nitrogen Photofixation

Yanting Zhang et al.

Summary: This study reports the efficient nitrogen photofixation using two-dimensional boron-doped niobic acid nanosheets with oxygen vacancies, achieving enhanced ammonia evolution rates under visible-light irradiation in pure water. The synergy of boron dopant and oxygen vacancy plays a crucial role in regulating the band structure of niobic acid, facilitating charge transfer, reducing energy barriers, and promoting high rates of ammonia evolution, providing a general strategy for designing active photocatalysts for solar nitrogen conversion.

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Article Chemistry, Physical

Enhancing electron density of bulk g-C3N4 through phosphorus doping for promoting photocatalytic hydrogen evolution reaction

Bo Yan et al.

Summary: The use of polyphosphate cyanogen as a phosphorus source to prepare phosphorus-doped bulk g-C3N4 with a coral-like hierarchical structure is beneficial for the photocatalytic hydrogen evolution reaction (HER), by increasing electron density and accelerating the separation and transfer of photoexcited electron-hole pairs. This study opens up possibilities for further development of phosphorus-doped g-C3N4 for solar energy conversion to hydrogen energy.

APPLIED SURFACE SCIENCE (2021)

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Article Nanoscience & Nanotechnology

Photocatalytic CO2 Reduction Enabled by Interfacial S-Scheme Heterojunction between Ultrasmall Copper Phosphosulfide and g-C3N4

Xiandi Zhang et al.

Summary: The study focuses on enhancing photocatalytic CO2 reduction by anchoring ultrasmall copper phosphosulfide nanocrystals on 2D g-C3N4 nanosheets, forming an S-scheme heterojunction for efficient separation and migration of charge carriers, leading to significantly increased generation rate of CO and paving the way for the application of TMPSs in photocatalytic processes.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Anodic TiO2 Nanotubes on 3D-Printed Titanium Meshes for Photocatalytic Applications

Hanna Sopha et al.

Summary: In this study, large 3D Ti meshes were fabricated by direct ink writing and wirelessly anodized for the first time to prepare highly photocatalytically active TiO2 nanotube layers. The TNT layers with nanotube diameters of up to 110 nm and thicknesses of up to 3.3 μm showed superior performance for the photocatalytic degradation of methylene blue.

NANO LETTERS (2021)

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Article Chemistry, Physical

Composition-dependent micro-structure and photocatalytic performance of g-C3N4 quantum dots@SnS2 heterojunction

Sheng-Qi Guo et al.

Summary: The study investigates the effect of composition ratio on the micro-structure and photocatalytic activity of semiconductor combinations using CNQD(n)@SnS2 heterojunction. Optimal composition results in efficient pollutant degradation, while excess composition hinders the separation of photo-induced charge carriers, reducing overall activity. This research provides insights for the rational design of highly active photocatalysts.

NANO RESEARCH (2021)

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Article Chemistry, Physical

Facet-Regulating Local Coordination of Dual-Atom Cocatalyzed TiO2 for Photocatalytic Water Splitting

Tingcha Wei et al.

Summary: By engineering the exposed facets of TiO2 supports, the coordination environment of PtAu dual atoms can be regulated, leading to a significant increase in the H-2 evolution rate. The PtAu dual-atom cocatalyzed PtAu/{001}-TiO2 showed a 1000-fold increase compared to blank {001}-TiO2, with 4 times higher production rate than PtAu/{101}-TiO2.

ACS CATALYSIS (2021)

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Article Engineering, Chemical

Improved visible-light driven photocatalysis by loading Au onto C3N4 nanorods for degradation of RhB and reduction of CO2

Dandan Wang et al.

Summary: A series of plasmonic photocatalysts were prepared using a solution-assembly technique, exhibiting high photocatalytic activity under visible light. The improved performance was mainly attributed to the strong localized surface plasmon resonance effect.

ADVANCED POWDER TECHNOLOGY (2021)

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Article Chemistry, Physical

Nitrogen doping-mediated oxygen vacancies enhancing co-catalyst-free solar photocatalytic H2 production activity in anatase TiO2 nanosheet assembly

Mohamed Esmat et al.

Summary: Introducing oxygen vacancies (Vo) into TiO2 photocatalyst along with N doping is proposed as an alternative strategy for achieving efficient co-catalyst-free solar photocatalytic activity under less extreme conditions. The synthesized material exhibits good co-catalyst-free solar photocatalytic activity for hydrogen evolution via water splitting under irradiation with simulated solar light, showing higher efficiency compared to typical co-catalyst-free defective TiO2 materials. The introduced Vo is believed to play a role in facilitating charge separation and improving photocatalytic efficiency.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Single ruthenium atom supported on g-C3N4 as an efficient photocatalyst for nitrogen fixation in ultra-pure water

Li Li et al.

Summary: In this study, ruthenium (Ru) single atoms were successfully decorated on the surface of graphitic carbon nitride (g-C3N4), leading to improved efficiency in photocatalytic nitrogen fixation.

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2D/2D atomic double-layer WS2/Nb2O5 shell/core nanosheets with ultrafast interfacial charge transfer for boosting photocatalytic H2 evolution

Bo Lin et al.

Summary: A new DLWS/Nb2O5 photocatalyst with a unique 2D/2D shell/core interface has been designed for achieving high-efficiency charge transfer, leading to a significantly increased photocatalytic H2 evolution rate.

CHINESE CHEMICAL LETTERS (2021)

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Article Chemistry, Physical

In situ preparation of g-C3N4 nanosheet/FeOCl: Achievement and promoted photocatalytic nitrogen fixation activity (Publication with Expression of Concern. See vol. 616, 2022)

Van-Huy Nguyen et al.

Summary: Climate change, global warming, and population growth have prompted researchers to use eco-friendly methods for the N-2 reduction reaction. A new visible-light-driven photocatalyst consisting of FeOCl particles adhered to NS-CN showed remarkable photoactivity in NH4+ production reaction. Various factors such as electron quenchers, pH, and solvent were studied to understand the mechanism behind the improved N-2 fixation efficiency.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Experimental Strategy and Mechanistic View to Boost the Photocatalytic Activity of Cs3Bi2Br9 Lead-Free Perovskite Derivative by g-C3N4 Composite Engineering

Lidia Romani et al.

Summary: The rational design of heterojunctions based on metal halide perovskites is effective for creating novel photocatalysts for relevant solar-driven reactions. This study demonstrates a significant increase in hydrogen photogeneration and effective catalytic activity in degrading organic pollutants through the synergistic coupling of a lead-free Cs3Bi2Br9 perovskite derivative with g-C3N4. The research provides solid evidence and rationale for the possible application of metal halide perovskites in photocatalysis.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Understanding the synergistic effect of Co-loading and B-doping in g-C3N4 for enhanced photocatalytic activity for overall solar water splitting

B. R. Bhagat et al.

Summary: The effective approach of loading metal (Co) and doping non-metal (B) together enhances the photocatalytic activity of g-C3N4, forming p-type and n-type semiconductors with lower overpotential values for oxygen and hydrogen evolution reactions, making it a potential candidate for overall photocatalytic water splitting.

CARBON (2021)

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Article Engineering, Environmental

Hierarchical defect-rich flower-like BiOBr/Ag nanoparticles/ultrathin g-C3N4 with transfer channels plasmonic Z-scheme heterojunction photocatalyst for accelerated visible-light-driven photothermal-photocatalytic oxytetracycline degradation

Jiaxin Ni et al.

Summary: A defect-rich flower-like BiOBr combined with Ag nanoparticles and ultrathin g-C3N4 was prepared to construct a plasmonic Z-scheme heterojunction for efficient degradation of oxytetracycline. The results demonstrated the generation of a hierarchical plasmonic Z-scheme which led to the remarkable removal and mineralization of oxytetracycline. The catalyst showed excellent reusability and stability, with a unique spatial hierarchical framework contributing to its extraordinary performance.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Direct Attack and Indirect Transfer Mechanisms Dominated by Reactive Oxygen Species for Photocatalytic H2O2 Production on g-C3N4 Possessing Nitrogen Vacancies

Jun Luo et al.

Summary: This study uses nitrogen deficiency carbon nitride as a model catalyst and proposes multiple reaction mechanisms for photocatalytic H2O2 production based on experiment and simulation results. It demonstrates that H2O2 can be generated through multiple pathways.

ACS CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

The bionic sunflower: a bio-inspired autonomous light tracking photocatalytic system

Jingjing Qin et al.

Summary: This work proposes a novel photocatalytic concept to boost any traditional photocatalytic reaction by optimally using the solar energy from the sun's passage.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Physical

Recent advances in g-C3N4-based photocatalysts incorporated by MXenes and their derivatives

Huilin Hou et al.

Summary: This article explores the incorporation of 2D MXenes and their derivatives into g-C3N4 to enhance their performance as advanced photocatalysts. The discussion includes fundamental photocatalytic mechanisms, strategies for constructing hybrid photocatalysts with a solid 2D/2D interfacial contact, and typical applications in environmental and energy fields. Additionally, concluding remarks and future perspectives in this area are proposed.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Review Chemistry, Physical

A review on g-C3N4 incorporated with organics for enhanced photocatalytic water splitting

Jinnan Liang et al.

Summary: The review systematically studies the latest developments in morphology control of g-C3N4 as a photocatalyst, including nanorods, nanotubes, nanosheets, nanospheres, porous structures, and other different tunable nanostructures; discusses the incorporation strategies of g-C3N4 with various organic compounds, aiming to improve the overall photocatalytic performance; theoretically presents applications in water splitting, CO2 reduction, pollutant degradation, and environmental disinfection; and proposes research challenges and prospects of organic compound composited g-C3N4 towards hydrogen evolution through water splitting.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Applied

Novel S-scheme 2D/2D BiOBr/g-C3N4 heterojunctions with enhanced photocatalytic activity

Bin Zhang et al.

Summary: The design and construction of heterojunction photocatalysts with staggered energy band structure and appropriate interfacial contact is an effective way to achieve outstanding photocatalytic performance. A novel 2D/2D BiOBr/g-C3N4 heterojunction was successfully obtained by a convenient in situ self-assembly route, showing superior degradation and hydrogen production activity under simulated sunlight irradiation.

CHINESE JOURNAL OF CATALYSIS (2021)

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Fine tuning of phosphorus active sites on g-C3N4 nanosheets for enhanced photocatalytic decontamination

Lian-Lian Liu et al.

Summary: This study successfully synthesized post-P-doped gCN nanosheets with highly active P sites introduced by C/P substitution, leading to increased specific surface area and exposed active sites for optimized photocatalytic reactions. The nanosheets exhibited excellent visible light photoactivity towards bisphenol A degradation, demonstrating promising potential for efficient water and wastewater treatment with rationally designed visible-light-responsive photocatalysts.

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Integrating active C3N4 moieties in hydrogen-bonded organic frameworks for efficient photocatalysis

Tao Li et al.

Summary: HOFs provide a platform for self-assembling functional species into ordered structures, with PFC-42-Pt demonstrating outstanding photocatalytic activity in the production of hydrogen under visible light irradiation. The ordered arrangement of PFC-42-Pt significantly enhances its photocatalytic activity, as further evidenced by recrystallization experiments.

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2D PtS nanorectangles/g-C3N4 nanosheets with a metal sulfide-support interaction effect for high-efficiency photocatalytic H2 evolution

Bo Lin et al.

Summary: A new in situ vapor-phase growth method was developed to construct 2D PtS nanorectangles as cocatalysts on g-C3N4 nanosheets, achieving optimized hydrogen evolution rates through unusual metal sulfide-support interactions.

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Beyond C3N4 pi-conjugated metal-free polymeric semiconductors for photocatalytic chemical transformations

Long Yang et al.

Summary: This review article introduces the development of metal-free polymeric photocatalysts with large pi-conjugated units for various chemical transformations. The focus is on the rational manipulation of pi-conjugation enlargement, charge separation, electronic structures, and band structures in the design of these catalysts. The strategies provide potential avenues to address challenges in catalyst activity, selectivity, and stability for further development in this field.

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Fabrication and photocatalytic activity of graphitic-C3N4 quantum dots-decorated basic zinc carbonate prepared by a co-precipitation method

Ping Zhao et al.

Summary: The research synthesized graphitic carbon nitride quantum dots (CNQDs) with a high quantum yield by incorporating barbituric acid into the structure. They then introduced the CNQDs onto the surface of basic zinc carbonate (BZC) to enhance the degradation efficiency of tetracycline. The Z-scheme mechanism proposed for the enhanced photocatalytic degradation rate is attributed to the major roles played by O-2(-) and OH radicals due to the suitable bandgap. Finally, the formation and possible photocatalytic mechanisms of the CNQDs/BZC composite are proposed.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Mu Xiao et al.

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Inter-plane heterojunctions within 2D/2D FeSe2/g-C3N4 nanosheet semiconductors for photocatalytic hydrogen generation

Jia Jia et al.

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The nonmetal modulation of composition and morphology of g-C3N4-based photocatalysts

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Dual cocatalysts decorated three dimensionally ordered mesoporous g-C3N4 with homogeneous wall thickness for enhanced photocatalytic performance

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Chloroplast-granum-inspired porous nanorods composed of g-C3N4 ultrathin nanosheets as visible light photocatalysts for highly enhanced hydrogen production

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2020)

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Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance

Qijun Tang et al.

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Three-dimensional flower heterojunction g-C3N4/Ag/ZnO composed of ultrathin nanosheets with enhanced photocatalytic performance

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One-step synthesis of iodine-doped g-C3N4 with enhanced photocatalytic nitrogen fixation performance

Xiuli Hu et al.

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Bio-inspired honeycomb-like graphitic carbon nitride for enhanced visible light photocatalytic CO2 reduction activity

Maxwell Selase Akple et al.

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Hybridization of g-C3N4 quantum dots with 1D branched TiO2 fiber for efficient visible light-driven photocatalytic hydrogen generation

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Honeycomb-like g-C3N4/CeO2-x nanosheets obtained via one step hydrothermal-roasting for efficient and stable Cr(VI) photo-reduction

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Tin diselinide a stable co-catalyst coupled with branched TiO2 fiber and g-C3N4 quantum dots for photocatalytic hydrogen evolution

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Fabrication of alveolate g-C3N4 with nitrogen vacancies via cobalt introduction for efficient photocatalytic hydrogen evolution

Zhen Tian et al.

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Embedding few-layer Ti3C2Tx into alkalized g-C3N4 nanosheets for efficient photocatalytic degradation

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Atypical Oxygen-Bearing Copper Boosts Ethylene Selectivity toward Electrocatalytic CO2 Reduction

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Prominent co -catalytic e ffect of CoP nanoparticles anchored on high-crystalline g-C 3 N 4 nanosheets for enhanced visible -light photocatalytic degradation of tetracycline in wastewater

Feng Guo et al.

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2D g-C3N4 for advancement of photo-generated carrier dynamics: Status and challenges

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Operando Spectroscopic Investigation of a Boron-Doped CuO Catalyst and Its Role in Selective Electrochemical C-C Coupling

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Facile synthesis and photoelectrochemical properties of novel TiN/C3N4/CdS nanotube core/shell arrays

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C3N4 modified with single layer ZIF67 nanoparticles for efficient photocatalytic degradation of organic pollutants under visible light

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A facile sulfur-assisted method to synthesize porous alveolate Fe/g-C3N4 catalysts with ultra-small cluster and atomically dispersed Fe sites

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Step-scheme porous g-C3N4/Zn0.2Cd0.8S-DETA composites for efficient and stable photocatalytic H2 production

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Recent progress in g-C3N4 quantum dots: synthesis, properties and applications in photocatalytic degradation of organic pollutants

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Synergy between van der waals heterojunction and vacancy in ZnIn2S4/g-C3N4 2D/2D photocatalysts for enhanced photocatalytic hydrogen evolution

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Directed holey and ordered g-C3N4.5nanosheets by a hard template nanocasting approach for sustainable visible-light hydrogen evolution with prominent quantum efficiency

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Construction of a push-pull system in g-C3N4for efficient photocatalytic hydrogen evolution under visible light

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The effect of n-π* electronic transitions on the N2 photofixation ability of carbon self-doped honeycomb-like g-C3N4 prepared via microwave treatment

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Spatial positioning effect of dual cocatalysts accelerating charge transfer in three dimensionally ordered macroporous g-C3N4 for photocatalytic hydrogen evolution

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Controllable synthesis of nanotube-type graphitic C3N4 and their visible-light photocatalytic and fluorescent properties

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Efficient Visible-Light Photocatalytic Hydrogen Evolution and Enhanced Photostability of Core/Shell CdS/g-C3N4 Nanowires

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Synthesis of porous Fe3O4/g-C3N4 nanospheres as highly efficient and recyclable photocatalysts

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