☆ 4.6 Review

Switching gas permeation through smart membranes by external stimuli: a review

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Transition Metal Dichalcogenide-based Membranes for Water Desalination, Gas Separation, and Energy Storage

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Summary: This comprehensive review summarizes the different fabrication methods of TMDC-based membranes and introduces recent modification strategies to improve their microstructural properties. The applications of TMDCs-based membranes in wastewater treatment, desalination, proton exchange, gas separation, and energy devices are extensively discussed. The current engineering hurdles and research directions for improving the separation efficiency, stability, and permeability of these membranes are highlighted.

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Januar Widakdo et al.

Summary: In this study, smart membrane materials composed of ionic liquid (IL), PVDF, and graphene were demonstrated, aiming for fast response and adjustable selectivity. The infusion of IL increased the beta crystal phase of PVDF, which was further assisted by the presence of graphene. The optimized membrane exhibited excellent CO2/N-2 selectivity and CO2 permeability, surpassing the theoretical upper bound. The mechanism of selective transportation of CO2 gas through the membrane was explored both theoretically and experimentally using PALS and DFT simulations.

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Review Green & Sustainable Science & Technology

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Article Engineering, Chemical

Pebax-based membrane filled with photo-responsive Azo@NH2-MIL-53 nanoparticles for efficient SO2/N2 separation

Qingping Xin et al.

Summary: The preparation of mixed matrix membranes (MMMs) using metal-organic framework (MOF) as fillers is an effective way to enhance the gas permeability and selectivity of membranes. In this study, NH2-MIL-53 nanoparticles were synthesized and modified with aminoazobenzene (Azo) to fabricate multifunctional Azo@NH2-MIL-53 nanoparticles. These nanoparticles were incorporated into the Pebax matrix to form MMMs for efficient and controllable SO2 separation. The incorporation of Azo@NH2-MIL-53 not only increased the specific surface area and pore size of NH2-MIL-53, but also enhanced the affinity and solubility selectivity of SO2. Moreover, the light-responsive characteristics of Azo allowed the conformation and adsorption capacity of NH2-MIL-53 to be controlled dynamically under different light conditions. Therefore, the mixed matrix membrane coupled with photo-responsive MOF holds great promise for achieving more efficient and energy-saving gas separation processes.

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Article Engineering, Chemical

Smart light-responsive hierarchical metal organic frameworks constructed mixed matrix membranes for efficient gas separation

Qingping Xin et al.

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Article Engineering, Environmental

A robust calcium-based microporous metal-organic framework for efficient CH4/N2 separation

Miao Chang et al.

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Xinyi Wan et al.

Summary: A novel BN nanosheets supported magnetic ionic liquid membrane (BN-SMILM) with nanoconfined magnetic ionic liquid (MIL) in 2D nanochannels of BN membrane is developed for efficient CO2 separation. The nanoconfinement effect enhances CO2 transport, resulting in high selectivity and permeability above the Robeson upper-bound, and promising applications in CO2 separation with excellent long-term stability. This work provides a new strategy for preparing high-performance supported liquid membrane materials for practical environmental and energy applications.

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Hongwei Fan et al.

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NATURE COMMUNICATIONS (2021)

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Omid T. Qazvini et al.

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NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

Pressure-Responsive Two-Dimensional Metal-Organic Framework Composite Membranes for CO2 Separation

Yunpan Ying et al.

Summary: The study demonstrates the use of pressure-responsive ultrathin membranes for CO2 separation, by controlling gas permeation direction to achieve CO2-induced gate opening and closing behaviors, resulting in significantly increased CO2 permeance and selectivity.

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Article Chemistry, Multidisciplinary

Multivariate Polycrystalline Metal-Organic Framework Membranes for CO2/CH4 Separation

Weidong Fan et al.

Summary: Membrane technology shows great potential in natural gas separation, with the polycrystalline MIL-160 membrane demonstrating enhanced molecular sieving effect. By controlling the pore size and environment of the MIL-160 membrane, improved gas separation efficiency can be achieved. The fluorine-functionalized multivariate MIL-160/CAU-10-F membrane exhibits significant advantages in CO2/CH4 separation performance.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Light-responsive metal-organic framework sheets constructed smart membranes with tunable transport channels for efficient gas separation

Qingping Xin et al.

Summary: This study introduces a new type of light-responsive metal-organic framework [Co(azpy)] sheets for smart mixed matrix membranes (MMMs), which exhibit significantly improved selectivity for SO2(CO2)/N-2 gases. The permeability and selectivity of the Co(azpy) sheets-loaded smart MMMs can respond to external light stimuli and achieve high levels of performance. Additionally, in a humidified state, the CO2 permeability and CO2/N-2 selectivity of MMMs surpass the upper bound reported by Robeson in 2019.

RSC ADVANCES (2021)

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Article Chemistry, Multidisciplinary

Disclosing the Role of Defect-Engineered Metal-Organic Frameworks in Mixed Matrix Membranes for Efficient CO2 Separation: A Joint Experimental-Computational Exploration

Tae Hoon Lee et al.

Summary: Incorporating defects in metal-organic frameworks (MOFs) offers opportunities to manipulate microporosity and functionalities, particularly in CO2 separation applications. This study demonstrates that defect-engineered UiO-66/PEGDA MMMs exhibit similar filler-matrix interfacial properties regardless of the defect concentrations, showing potential for ultrafast gas transport pathways. MMMs containing the most defective UiO-66 show enhanced CO2/N-2 separation performance, overcoming limitations in pure polymers.

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Article Chemistry, Physical

Tailoring of graphene-organic frameworks membrane to enable reversed electrical-switchable permselectivity in CO2 separation

Januar Widakdo et al.

Summary: This research presents a smart membrane for CO2 separation by adding polydopamine to PVDF/G membranes to enhance permeability and permselectivity, achieving selective gas separation. The membrane exhibits high piezoelectric properties and switchability, with unique pore characteristics transitioning from bimodal to single pore distribution.

CARBON (2021)

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Effect of composition of few-layered transition metal dichalcogenide nanosheets on separation mechanism of hydrogen selective membranes

Degu Lere Keshebo et al.

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MgAl-CO3 layered double hydroxide as potential filler in substrate layer of composite membrane for enhanced carbon dioxide separation

N. Fajrina et al.

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Review Chemistry, Physical

A review on the recent advancements in graphene-based membranes and their applications as stimuli-responsive separation materials

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Summary: Graphene and its derivatives have exceptional physicochemical properties that make them excellent candidates for membranes used in separation technology, especially for environmental applications like wastewater treatment and gas purification. By utilizing smart membranes constructed with graphene and polymeric materials, the issues of fouling and decline in performance seen in conventional membranes can be overcome, leading to a more reliable and efficient separation process.

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MXene-Based Membranes for Separation Applications

Lingzhi Huang et al.

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Chenyu Zhu et al.

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GREEN CHEMICAL ENGINEERING (2021)

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Pushing Rubbery Polymer Membranes To Be Economic for CO2 Separation: Embedment with Ti3C2Tx MXene Nanosheets

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Change of gas permeation by photoinduced switching of zeolite-azobenzene membranes of type MFI and FAU

K Weh et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2002)

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