Single-atom palladium anchored N-doped carbon towards oxygen electrocatalysis for rechargeable Zn-air batteries

Article Chemistry, Multidisciplinary

Coupling the Atomically Dispersed Fe-N3 Sites with Sub-5 nm Pd Nanocrystals Confined in N-Doped Carbon Nanobelts to Boost the Oxygen Reduction for Microbial Fuel Cells

Zinan Lin et al.

Summary: This study combines Fe and Pd together through a designed pyrolysis mechanism, forming FeN3-Pd@NC NBs, which exhibit outstanding activity and durability in the oxygen reduction reaction.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Physical

Enhanced bifunctional catalytic performance of nitrogen-doped carbon composite to oxygen reduction and evolution reactions with the regulation of graphene for rechargeable Zn-air batteries

Yang Xiang et al.

Summary: The strategy of synthesizing a nitrogen-doped carbon catalyst (NiFe-Mi-C-Gr) with graphene coating demonstrates enhanced gas separation and catalytic activity, showing superior bifunctional catalytic performance. The Zn-air battery assembled with this catalyst exhibits higher performance, surpassing other benchmark catalysts.

APPLIED SURFACE SCIENCE (2022)

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Article Chemistry, Physical

Inlaying metal-organic framework derived pancake-like TiO2 into three-dimensional BiOI for visible-light-driven generation of vanillin from sodium lignosulfonate

Jianhao Qiu et al.

Summary: Pancake-like TiO2 (M-TiO2) was embedded into three-dimensional flower-like BiOI to form M-TiO2/BiOI composites, which showed enhanced photocatalytic performance for generating vanillin from sodium lignosulfonate. The key role of h(+) and O-center dot(2)- in vanillin generation was identified during the study.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Multidisciplinary

In Situ Grown Co-Based Interstitial Compounds: Non-3d Metal and Non-Metal Dual Modulation Boosts Alkaline and Acidic Hydrogen Electrocatalysis

Tuzhi Xiong et al.

Summary: By combining interfacial engineering and elemental doping, a unique structure with high-valence non-3d metal and non-metal integration was achieved on stainless steel mesh for efficient hydrogen evolution reaction (HER) in both alkaline and acidic media, showing superior performance to commercial Pt/C catalysts.

SMALL (2022)

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Article Chemistry, Applied

Enhanced confinement synthesis of atomically dispersed Fe-N-C catalyst from resin polymer for oxygen reduction

Ailing Song et al.

Summary: An enhanced confinement strategy was utilized to synthesize a catalyst comprised of atomically dispersed Fe supported on porous nitrogen-doped graphitic carbon, resulting in enhanced catalytic activity towards the oxygen reduction reaction. The catalyst's improved activity originates from its highly active surface with atomically dispersed iron sites and multi-level three-dimensional structure, showing great commercialization potential in the future.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Green & Sustainable Science & Technology

Oxygen vacancy-based metal oxides photoanodes in photoelectrochemical water splitting

Yingying Wang et al.

Summary: This article discusses the strategies for introducing oxygen vacancies into nanomaterials, which is of great significance in improving the efficiency of photoelectrochemical water splitting. The effects of oxygen vacancies on improving light absorption efficiency, charge transfer efficiency, and charge injection efficiency are summarized. Several challenges that need to be addressed in the future are also proposed.

MATERIALS TODAY SUSTAINABILITY (2022)

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Article Engineering, Environmental

Non-oxygen anion-regulated in situ cobalt based heterojunctions for active alkaline hydrogen evolution catalysis

Qirong Tan et al.

Summary: This study reports a general strategy to enhance the HER properties of Co-based heterojunction catalysts by regulating the catalytic activity through anionic regulation and constructing dual nanostructures on a stainless steel mesh. The optimized SSM/CoOP catalyst exhibits similar HER performance to Pt-C catalysts and shows promising OER performance when used in an overall water splitting device.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Applied

One-pot synthesis of FeNxC as efficient catalyst for high-performance zinc-air battery

Yang Li et al.

Summary: Rechargeable zinc-air batteries have high theoretical energy density but suffer from high polarization and low energy efficiency. A noble-metal-free FeNxC electrocatalyst was developed to enhance oxygen reduction reaction kinetics, leading to improved performance in charge-discharge voltage gap, peak power density, and long-term durability. This work provides significant support for the practical application of zinc-air batteries in the future.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Applied

Unveiling the promotion of accelerated water dissociation kinetics on the hydrogen evolution catalysis of NiMoO4 nanorods

Tuzhi Xiong et al.

Summary: The water dissociation kinetics of nickel molybdate were successfully accelerated through in situ interfacial engineering and phosphorus doping, resulting in outstanding hydrogen evolution catalytic properties.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

PdAg/Ag(111) Surface Alloys: A Highly Efficient Catalyst of Oxygen Reduction Reaction

Minghao Hua et al.

Summary: In this article, the behavior of various Pd ensembles on the PdAg(111) surfaces for oxygen reduction reaction (ORR) intermediates was systematically investigated using density functional theory (DFT) simulation. The findings showed that Pd monomer with a Pd subsurface layer exhibited the best predicted performance. The subsurface coordination was able to explain this phenomenon, which was further supported by the analysis of electronic properties. Another advantage of PdAg SAA was the atomic-dispersed Pd as adsorption sites, which significantly improved the resistance to CO poisoning. By adjusting the Pd ensembles on the catalyst surface, an ORR catalyst combination with both predicted activity and high tolerance to CO poisoning could be designed.

NANOMATERIALS (2022)

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Review Chemistry, Inorganic & Nuclear

Recent advances in fuel cell reaction electrocatalysis based on porous noble metal nanocatalysts

Wenjing Cheng et al.

Summary: This article reviews the recent research advances in porous noble metal nanocatalysts for fuel cell-related reactions. It provides valuable insights into the inherent structural features of porous noble metal nanostructures, advanced synthetic strategies for their fabrication, and the structure-performance relationships, which are essential for the development of advanced electrocatalysts with high activity and stability.

DALTON TRANSACTIONS (2022)

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Article Chemistry, Inorganic & Nuclear

Highly graphited carbon-coated FeTiO3 nanosheets in situ derived from MXene: an efficient bifunctional catalyst for Zn-air batteries

Yingxinjie Wang et al.

Summary: This study demonstrates the efficient bifunctional activity of graphited carbon-coated FeTiO3 (FeTiO3@C) as a catalyst for rechargeable Zn-air batteries, achieved through in situ annealing Ti3C2Tx nanosheets in a rusted-reactor. The FeTiO3@C catalyst exhibits excellent oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) activities.

DALTON TRANSACTIONS (2022)

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Article Multidisciplinary Sciences

Spiny Pd/PtFe core/shell nanotubes with rich high-index facets for efficient electrocatalysis

Lu Tao et al.

Summary: The performance of fuel-cell related electrocatalysis heavily depends on the morphology, size and composition of the catalyst. The synthesis of Pt-based catalyst with high-index facets and hollow interiors can significantly enhance catalysis efficiency. The new catalyst, spiny Pd/PtFe core/shell nanotubes, demonstrates remarkable activity and stability in fuel-cell and alcohol oxidation reactions.

SCIENCE BULLETIN (2021)

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Article Chemistry, Physical

Modulation of Single Atomic Co and Fe Sites on Hollow Carbon Nanospheres as Oxygen Electrodes for Rechargeable Zn-Air Batteries

Vishal Jose et al.

Summary: This study presents a facile method for preparing bimetallic Fe and Co sites entrapped in nitrogen-doped hollow carbon nanospheres (Fe,Co-SA/CS), demonstrating promising activity for both oxygen reduction reaction (ORR) and oxygen evolution reaction (OER).

SMALL METHODS (2021)

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Article Chemistry, Multidisciplinary

MIL-101-Derived Mesoporous Carbon Supporting Highly Exposed Fe Single-Atom Sites as Efficient Oxygen Reduction Reaction Catalysts

Xiaoying Xie et al.

Summary: Fe single-atom catalysts with atomic FeNx active sites show great promise as alternatives to platinum-based catalysts for the oxygen reduction reaction. This study utilized a mesoporous MOF NH2-MIL-101(Al) as a precursor to prepare a series of N-doped carbon supports with well-defined mesoporous structure at different pyrolysis temperatures. The resulting Fe SAC-MIL101-T catalysts showed outstanding ORR activity in alkaline media and excellent performance in zinc-air batteries.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Defect engineering on three-dimensionally ordered macroporous phosphorus doped Co3O4-δ microspheres as an efficient bifunctional electrocatalyst for Zn-air batteries

Daorui Wang et al.

Summary: The three-dimensionally ordered macroporous (3DOM) Co3O4 electrocatalyst with phosphorization treatment demonstrates high bifunctionality for oxygen reduction and evolution reactions, showing promising potential for practical application.

ENERGY STORAGE MATERIALS (2021)

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Article Multidisciplinary Sciences

Regulating Fe-spin state by atomically dispersed Mn-N in Fe-N-C catalysts with high oxygen reduction activity

Gege Yang et al.

Summary: The research uncovered the mechanism of the oxygen reduction reaction on dual-metal atomically dispersed Fe,Mn/N-C catalyst, demonstrating its excellent performance and durability in fuel cells and metal-air batteries.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Electrochemical ammonia synthesis via nitrate reduction on Fe single atom catalyst

Zhen-Yu Wu et al.

Summary: The study reports a method for selectively converting nitrate to ammonia using an Fe single atom catalyst, which effectively prevents the formation of N-N coupling products while increasing the production rate of ammonia.

NATURE COMMUNICATIONS (2021)

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Article Nanoscience & Nanotechnology

Engineering Two-Phase Bifunctional Oxygen Electrocatalysts with Tunable and Synergetic Components for Flexible Zn-Air Batteries

Yanli Niu et al.

Summary: A novel bimetallic Co/CoFe nanomaterial supported on nanoflower-like N-doped graphitic carbon was prepared as an efficient bifunctional oxygen electrocatalyst. The material exhibited high activities for oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) with optimized adsorption energies. Experimental characterizations and density functional theory calculations revealed the formation of a Co/CoFe heterostructure and synergistic effects between the metal layer and NC support, enhancing electric conductivity and reaction kinetics.

NANO-MICRO LETTERS (2021)

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Article Chemistry, Physical

Electronic tuning of confined sub-nanometer cobalt oxide clusters boosting oxygen catalysis and rechargeable Zn-air batteries

Yangyang Tan et al.

Summary: This study predicted the electronic structure regulation of cobalt oxide nanoclusters using DFT simulation, and experimentally verified the enhancement of bifunctional oxygen performance through microporous MOFs confinement strategy. The optimized catalyst demonstrated outstanding performance in rechargeable Zn-air batteries, outperforming benchmark electrodes. DFT calculations showed that reducing particle size and coupling with Co-N can effectively regulate the charge distribution of CoOx nanoclusters and accelerate the overall ORR/OER kinetic process.

NANO ENERGY (2021)

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Article Chemistry, Multidisciplinary

Co/MoC Nanoparticles Embedded in Carbon Nanoboxes as Robust Trifunctional Electrocatalysts for a Zn-Air Battery and Water Electrocatalysis

Lei Zhang et al.

Summary: A concept of trifunctional catalyst design was proposed in this study, which fabricated high-efficiency N-doping carbon nanoboxes through interface engineering and nanoscale hollowing design. The catalyst not only showed outstanding performance in regenerative Zn-air battery, but also demonstrated good properties in overall water splitting, with both theoretical and experimental results confirming its role in facilitating charge transfer.

ACS NANO (2021)

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Article Chemistry, Physical

An efficient dual-metal single-atom catalyst for bifunctional catalysis in zinc-air batteries

Yiou Ma et al.

Summary: By using graphene oxide to anchor metal ions in nitrogen-doped graphene, a dual-metal-site bifunctional catalyst with atomically dispersed FeN4 and NiN4 has been developed, showing highly efficient bifunctional catalytic activity.

CARBON (2021)

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Article Engineering, Environmental

Hemin-assisted synthesis of peroxidase-like Fe-N-C nanozymes for detection of ascorbic acid-generating bio-enzymes

Wendong Liu et al.

Summary: The Fe-N co-doped porous carbon nanozymes exhibited high enzyme-like activities and were successfully applied in the detection of bioenzyme ALP. The nanozymes showed low detection limit and a wider linear activity range in the presence of AA inhibition, providing a promising strategy for bio-enzyme detection.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Multidisciplinary Sciences

Platinum single-atom catalyst coupled with transition metal/metal oxide heterostructure for accelerating alkaline hydrogen evolution reaction

Kai Ling Zhou et al.

Summary: Single-atom platinum immobilized NiO/Ni heterostructure acts as a highly efficient alkaline hydrogen evolution catalyst by enabling tunable binding abilities and enhancing water dissociation energy. Constructing hierarchical three-dimensional morphology further enhances the catalytic performance.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

Surface Phosphorus-Induced CoO Coupling to Monolithic Carbon for Efficient Air Electrode of Quasi-Solid-State Zn-Air Batteries

Huan Liu et al.

Summary: The study introduces a surface phosphorization-monolithic strategy to embed CoO nanoparticles into paulownia carbon plate as monolithic electrodes for Zn-air batteries. The resulting electrode shows remarkable catalytic activity and long-term cycling stability in quasi-solid-state or aqueous ZABs.

ADVANCED SCIENCE (2021)

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Article Chemistry, Inorganic & Nuclear

Enhanced activity towards oxygen electrocatalysis for rechargeable Zn-air batteries by alloying Fe and Co in N-doped carbon

Fengjiao Yu et al.

Summary: FeCo/N-C catalyst exhibits excellent activities in both the oxygen reduction and oxygen evolution reactions, surpassing commercial Pt/C and RuO2. In a rechargeable Zn-air battery, the FeCo/N-C based battery shows better durability and lower round-trip overpotential after 800 cycles compared to a battery using expensive Pt/C + RuO2 mixture catalyst.

DALTON TRANSACTIONS (2021)

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Article Chemistry, Physical

A dual-template strategy to engineer hierarchically porous Fe-N-C electrocatalysts for the high-performance cathodes of Zn-air batteries†

Dan Wang et al.

Summary: A dual-template strategy has been proposed for constructing hierarchically porous Fe-N-C catalysts, leading to improved active site accessibility and mass transfer, thereby enhancing ORR activity in Zn-air batteries. The experimental results showed significant improvements in both active site accessibility and mass transfer, resulting in enhanced ORR activity in conventional three-electrode cells and a high performance in a real-world liquid Zn-air battery.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Inorganic & Nuclear

MOF-derived Co/Cu-embedded N-doped carbon for trifunctional ORR/OER/HER catalysis in alkaline media†

Angela Macedo Andrade et al.

Summary: This report demonstrates a bimetallic Co/Cu-embedded N-doped carbon structure for trifunctional catalysis of oxygen reduction, oxygen evolution and hydrogen evolution reactions in alkaline media. The hybrid catalyst, synthesized through a metal-organic framework-based process, enables an active trifunctional catalysis with multiple favorable characteristics, including a high-surface-area morphology with a high concentration of sp(2) bonding for facilitated electron conduction.

DALTON TRANSACTIONS (2021)

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Article Chemistry, Physical

3D self-supported porous vanadium-doped nickel nitride nanosheet arrays as efficient bifunctional electrocatalysts for urea electrolysis

Rui-Qing Li et al.

Summary: In this study, V-doped Ni3N nanosheets arrays grown on nickel foam were developed as a bifunctional electrocatalyst for hydrogen evolution reaction (HER) and urea oxidation reaction (UOR). The catalyst exhibited excellent catalytic performances with low energy consumption and remarkable stability, making it promising for applications in energy-saving H-2 production and urea-related waste water treatment.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Co0.7Fe0.3 NPs confined in yolk-shell N-doped carbon: engineering multi-beaded fibers as an efficient bifunctional electrocatalyst for Zn-air batteries

Ling Long et al.

Summary: This study developed a bifunctional electrocatalyst consisting of Co0.7Fe0.3 alloy nanoparticles confined in N-doped carbon with a yolk-shell structure in multi-beaded fibers, exhibiting excellent OER and ORR performance. The hierarchical structure with abundant mesopores, high BET surface area, good electronic conductivity, and uniformly distributed active sites showed superior electrochemical performance compared to commercial catalysts. The Co0.7Fe0.3@NC2:1-800 Zn-air battery displayed higher open circuit voltage, larger power density, and better cycling stability, suggesting potential applications in energy conversion systems.

NANOSCALE (2021)

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Article Chemistry, Multidisciplinary

2D Nitrogen-Doped Carbon Nanotubes/Graphene Hybrid as Bifunctional Oxygen Electrocatalyst for Long-Life Rechargeable Zn-Air Batteries

Yangyang Xu et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Engineering, Environmental

New Insights into the Generation of Singlet Oxygen in the Metal-Free Peroxymonosulfate Activation Process: Important Role of Electron-Deficient Carbon Atoms

Yaowen Gao et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2020)

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Article Chemistry, Multidisciplinary

Atomically Dispersed Mn within Carbon Frameworks as High-Performance Oxygen Reduction Electrocatalysts for Zinc-Air Battery

Zhiyu Lin et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Review Chemistry, Multidisciplinary

Single-Atom Catalysts for Electrocatalytic Applications

Qiaoqiao Zhang et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Physical

Influence of pyrrolic and pyridinic-N in the size and distribution behaviour of Pd nanoparticles and ORR mechanism

Nipa Roy et al.

APPLIED SURFACE SCIENCE (2020)

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Article Multidisciplinary Sciences

Synthesis of lignin-derived nitrogen-doped carbon as a novel catalyst for 4-NP reduction evaluation

Yun Liu et al.

SCIENTIFIC REPORTS (2020)

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Article Chemistry, Physical

Performance enhancement and degradation mechanism identification of a single-atom Co-N-C catalyst for proton exchange membrane fuel cells

Xiaohong Xie et al.

NATURE CATALYSIS (2020)

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Article Chemistry, Inorganic & Nuclear

NiMOF-derived oxygen vacancy rich NiO with excellent capacitance and ORR/OER activities as a cathode material for Zn-based hybrid batteries

Dandan Xu et al.

DALTON TRANSACTIONS (2020)

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Article Chemistry, Physical

Hierarchical nickel cobalt sulfide nanosheet arrays supported on CuO/Cu hybrid foams as a rationally designed core-shell dendrite electrocatalyst for an efficient oxygen evolution reaction

Mengjie Lu et al.

SUSTAINABLE ENERGY & FUELS (2020)

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Article Chemistry, Physical

Anchoring Mo single atoms/clusters and N on edge-rich nanoporous holey graphene as bifunctional air electrode in Zn - air batteries

Peng Du et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

Tuning d-band centers by coupling PdO nanoclusters to WO3nanosheets to promote the oxygen reduction reaction

Jun-Hyeong Lee et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Tubular assemblies of N-doped carbon nanotubes loaded with NiFe alloy nanoparticles as efficient bifunctional catalysts for rechargeable zinc-air batteries

Xiaoying Xie et al.

NANOSCALE (2020)

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Article Chemistry, Physical

Non-covalent pre-organization of molecular precursors: A facile approach for engineering structures and activities of pyrolyzed Co-N-C electrocatalysts

Hao Mei et al.

CARBON (2019)

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Article Electrochemistry

Significant enhancement of the oxygen reduction activity of self-heteroatom doped coal derived carbon through oxidative pretreatment

Huimin Liu et al.

ELECTROCHIMICA ACTA (2019)

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Fe-N-C Single-Atom Nanozymes for the Intracellular Hydrogen Peroxide Detection

Lei Jiao et al.

ANALYTICAL CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Exceptional Performance of Hierarchical Ni-Fe (hydr)oxide@NiCu Electrocatalysts for Water Splitting

Yongfang Zhou et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Physical

All-solid-state sponge-like squeezable zinc-air battery

Zhenghui Pan et al.

ENERGY STORAGE MATERIALS (2019)

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Article Chemistry, Multidisciplinary

3D Carbon Electrocatalysts In Situ Constructed by Defect-Rich Nanosheets and Polyhedrons from NaCl-Sealed Zeolitic Imidazolate Frameworks

Yuqing Wang et al.

ADVANCED FUNCTIONAL MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Efficient Oxygen Reduction Reaction (ORR) Catalysts Based on Single Iron Atoms Dispersed on a Hierarchically Structured Porous Carbon Framework

Zhengping Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

Recent Advances toward the Rational Design of Efficient Bifunctional Air Electrodes for Rechargeable Zn-Air Batteries

Fan-Lu Meng et al.

SMALL (2018)

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Article Chemistry, Physical

Anchoring Mn3O4 Nanoparticles on Oxygen Functionalized Carbon Nanotubes as Bifunctional Catalyst for Rechargeable Zinc-Air Battery

Laiquan Li et al.

ACS APPLIED ENERGY MATERIALS (2018)

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Review Chemistry, Physical

Single-Atom Catalysts: Synthetic Strategies and Electrochemical Applications

Yuanjun Chen et al.

JOULE (2018)

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Fe-N Decorated Hybrids of CNTs Grown on Hierarchically Porous Carbon for High-Performance Oxygen Reduction

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ADVANCED MATERIALS (2014)

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Enhancing Electrocatalytic Oxygen Reduction on Nitrogen-Doped Graphene by Active Sites Implantation

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SCIENTIFIC REPORTS (2013)

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Synthesis of Monolayer-Patched Graphene from Glucose

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2012)

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Electrocatalytic oxidation and detection of hydrazine at carbon nanotube-supported palladium nanoparticles in strong acidic solution conditions

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ELECTROCHIMICA ACTA (2011)

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Single-atom palladium anchored N-doped carbon towards oxygen electrocatalysis for rechargeable Zn-air batteries

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