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Thermo-electrochemical cells for heat to electricity conversion: from mechanisms, materials, strategies to applications

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Improved Thermoelectric Performance of P-type SnTe through Synergistic Engineering of Electronic and Phonon Transports

Mengrong Li et al.

Summary: By alloying with Ag0.5Bi0.5Se and ZnO sequentially, both the electronic and phonon transports of SnTe were engineered to increase the Seebeck coefficient and reduce thermal conductivity. This synergistic engineering led to a significant improvement in TE performance with a peak ZT value of about 1.2 at around 870 K for the sample.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Initiating a Stretchable, Compressible, and Wearable Thermoelectric Generator by a Spiral Architecture with Ternary Nanocomposites for Efficient Heat Harvesting

Lirong Liang et al.

Summary: The study synthesized flexible PEDOT-Tos/Te/SWCNTs nanocomposite films and assembled them into 3D TEGs for efficient thermoelectric conversion. Through a spiral structure, device-level flexibility and compressibility were achieved, with stable energy output.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Flexible and Robust Bacterial Cellulose-Based Ionogels with High Thermoelectric Properties for Low-Grade Heat Harvesting

Kuankuan Liu et al.

Summary: Researchers successfully combined natural polymer and green solvent to prepare an ionogel with high tensile strength, skin-like mechanical stretchability, and adhesivity, demonstrating its potential in the field of thermoelectrics.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Significant Enhancement in the Thermoelectric Properties of Ionogels through the Solid Network Engineering

Zhuo Liu et al.

Summary: Ionic thermoelectric (TE) materials have attracted attention for their high thermovoltage but low conductivity. By engineering the solid networks in ionogels, the ionic conductivity and overall TE properties have been significantly improved, leading to the highest recorded ZT(i) value for ionic conductors.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Multidisciplinary Sciences

Zinc ion thermal charging cell for low-grade heat conversion and energy storage

Zhiwei Li et al.

Nature Communications (2022)

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Article Chemistry, Physical

Self-Healable Organic-Inorganic Hybrid Thermoelectric Materials with Excellent Ionic Thermoelectric Properties

Yoga Trianzar Malik et al.

Summary: By incorporating SiO2 nanoparticles into organic-inorganic ionic TE composites, a new material with high ionic TE figure of merit and self-healing/stretching properties has been developed. This material maintains its TE properties under severe external stresses and demonstrates a high energy density under temperature difference.

ADVANCED ENERGY MATERIALS (2022)

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Review Materials Science, Multidisciplinary

Ionic thermoelectrics: principles, materials and applications

Hanlin Cheng et al.

Summary: Waste heat harvesting is crucial for sustainable development, with thermoelectric generators (TEGs) being the only feasible technology for recovering low-grade heat. Ionic conductors, with their high thermopower, have emerged as the next-generation TE materials.

JOURNAL OF MATERIALS CHEMISTRY C (2022)

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Article Chemistry, Physical

Ion regulation in double-network hydrogel module with ultrahigh thermopower for low-grade heat harvesting

Chang Liu et al.

Summary: The research frontier of harvesting low-grade heat as a source of electrical power for self-powered wearable devices has shown promise, but current attainable thermopowers and constraints of rigid or complicated thermoelectric systems have hindered progress. By assembling porous electrodes and hybrid hydrogel, an ultrahigh thermopower of 19.32 mV K-1 was achieved on a stretchable thermoelectric module. This design provides an effective strategy to increase thermopower by regulating ion transport, resulting in high output power density, tailorable architecture, and excellent stretchability showcased in a thermoelectric wristband for body heat recovery.

NANO ENERGY (2022)

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Article Nanoscience & Nanotechnology

High-Precision Ionic Thermocouples Fabricated Using Potassium Ferri/Ferrocyanide and Iron Perchlorate

Jei Gyeong Jeon et al.

Summary: The ionic thermocouple is a new type of electronic component for temperature measurement, which offers higher accuracy and sensitivity. By using ionic conductors instead of traditional electrical conductors, the ionic thermocouple generates higher voltage output, providing more precise temperature measurements. Additionally, it can be easily miniaturized and has flexible and stretchable properties.

ADVANCED ELECTRONIC MATERIALS (2022)

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Article Multidisciplinary Sciences

Giant and bidirectionally tunable thermopower in nonaqueous ionogels enabled by selective ion doping

Sijing Liu et al.

Summary: Ionic thermoelectric materials have great potential in thermal sensing, but the lack of effective n-type materials hinders their applications. A thermopower regulation strategy through ion doping has been proposed to modulate the sign and magnitude of the thermopower in ionogels. A prototype wearable device with high thermopower has been demonstrated, showing promise for ultrasensitive thermal detection.

SCIENCE ADVANCES (2022)

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Article Engineering, Environmental

Bacterial cellulose-based hydrogel thermocells for low-grade heat harvesting

Yudong Zong et al.

Summary: This study focuses on the development of hydrogel thermoelectrochemical cells using bacterial cellulose, which exhibits high mechanical properties and simple production processes. The cells demonstrate high efficiency in harvesting low-grade heat and have potential applications in various fields.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Nanoscience & Nanotechnology

Regulating Thermogalvanic Effect and Mechanical Robustness via Redox Ions for Flexible Quasi-Solid-State Thermocells

Peng Peng et al.

Summary: This study proposed a flexible quasi-solid-state TEC based on a rational design of a hydrogel electrolyte, in which the thermogalvanic effect and mechanical robustness are simultaneously regulated via multivalent ions. The introduced redox ions endow the hydrogel with excellent heat-to-electricity conversion capability and act as ionic crosslinks for effective energy dissipation. The optimized TEC exhibits a high Seebeck coefficient and significantly improved fracture toughness, demonstrating its potential as a flexible and durable energy supply system for wearable applications.

NANO-MICRO LETTERS (2022)

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Article Chemistry, Physical

Cost-effective n-type thermocells enabled by thermosensitive crystallizations and 3D multi-structured electrodes

Boyang Yu et al.

Summary: The study developed a novel Cu-based thermosensitive crystallization approach and 3D multi-structured electrodes to improve the performance of n-type thermocells. The optimized Cu/Cu2+ system exhibited high values for Seebeck coefficient and power density, with a competitive cost-performance metric, outperforming the p-type benchmark. Additionally, a high-performance p-n junction of thermocells was demonstrated, showing a significant enhancement in output, paving the way for advancing integrated devices.

NANO ENERGY (2022)

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Article Chemistry, Multidisciplinary

Thermosensitive-CsI3-crystal-driven high-power I-/I3- thermocells

Hui Wang et al.

Summary: This paper presents a thermosensitive crystallization strategy to increase the Seebeck coefficient (Se) and power density of I-/I-3(-) thermocells. By adding Cs+ ions, a thermosensitive crystal CsI3 is formed, which improves the concentration gradient of free I-3(-) and enhances Se. This strategy provides a new way to build high-power thermocells for low-grade heat harvesting.

CELL REPORTS PHYSICAL SCIENCE (2022)

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Article Chemistry, Multidisciplinary

A Wavy-Structured Highly Stretchable Thermoelectric Generator with Stable Energy Output and Self-Rescuing Capability

Zhuoxin Liu et al.

Summary: This study proposes a wavy architecture and stretchable self-healable hydrogel to create a TEG with good wearability and high energy output, providing constant energy supply upon injuries or damages.

CCS CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Antifreezing Zwitterionic Hydrogel Electrolyte with High Conductivity of 12.6 mS cm-1 at-40 °C through Hydrated Lithium Ion Hopping Migration

Jianbo Yang et al.

Summary: The new zwitterionic polymer hydrogel electrolytes address the challenge of achieving high conductivity and flexibility at subzero temperatures, making them suitable for use in energy storage devices. The antifreezing electrolyte exhibits outstanding conductivity and mechanical properties, leading to high specific capacitance in supercapacitors.

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Article Chemistry, Multidisciplinary

High-Efficiency Perovskite Solar Cells with Imidazolium-Based Ionic Liquid for Surface Passivation and Charge Transport

Xuejie Zhu et al.

Summary: In this study, DMIMPF6 ionic liquid was used to passivate surface defects of perovskite, resulting in increased solar cell efficiency and enhanced long-term stability of the device.

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Review Chemistry, Multidisciplinary

Thermoelectric Converters Based on Ionic Conductors

Xun Wu et al.

Summary: Ionic thermoelectric materials represent a new paradigm for harvesting low-grade heat with higher Seebeck coefficient and lower thermal conductivity, and possess advantages of high flexibility, low cost, limited environmental pollution, and self-healing capability. They have been applied in supercapacitors, wearable devices, and fire warning systems, showing great potential for future development.

CHEMISTRY-AN ASIAN JOURNAL (2021)

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Hybrid thermoelectrochemical and concentration cells for harvesting low-grade waste heat

Kyunggu Kim et al.

Summary: The hybrid thermoelectrochemical and concentration cell (i-TCC) based on carbonate solvents outperforms current n-type TECs, showing high Seebeck coefficient, figure of merit, and Carnot efficiency at temperatures above 40 degrees Celsius. It provides a new perspective in harvesting low-grade waste heat.

CHEMICAL ENGINEERING JOURNAL (2021)

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Thermopower and harvesting heat

Xun Shi et al.

SCIENCE (2021)

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Article Chemistry, Physical

Insights into the Thermopower of Thermally Regenerative Electrochemical Cycle for Low Grade Heat Harvesting

Chun Cheng et al.

Summary: Thermally regenerative electrochemical cycle (TREC) technology converts low-grade heat into electrical power using NiHCF cathode and Zn anode. By introducing mixed membranes and mixed pH electrolytes, the thermopower of the system was effectively improved. This work advances the understanding and design of TREC systems.

ACS ENERGY LETTERS (2021)

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Article Engineering, Chemical

Ionic thermoelectric materials and devices

Dan Zhao et al.

Journal of Energy Chemistry (2021)

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Article Chemistry, Physical

All-Soft and Stretchable Thermogalvanic Gel Fabric for Antideformity Body Heat Harvesting Wearable

Tianpeng Ding et al.

Summary: A soft and stretchable thermogalvanic fabric woven from hydrogel fibers is proposed, with ideal mechanical properties for adapting to irregular and continuously deformed skin and achieving efficient body heat harvesting.

ADVANCED ENERGY MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Highly Stretchable PU Ionogels with Self-Healing Capability for a Flexible Thermoelectric Generator

Junhuai Xu et al.

Summary: The study developed a self-healable and stretchable PU ionogel with high mechanical stretchability and excellent ionic figure of merit. The PU ionogels showed stable thermoelectric capability under severe conditions and rapid self-healing abilities, making them promising for applications in wearable thermoelectric devices.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

An Electricity-Generating Window Made of a Transparent Energy Harvester of Thermocells

Ju Hwan Lee et al.

Summary: These windows can generate electricity while retaining their traditional functions and enhance energy efficiency in residential environments by capturing low-grade heat.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Embedding Aligned Graphene Oxides in Polyelectrolytes to Facilitate Thermo-Diffusion of Protons for High Ionic Thermoelectric Figure-of-Merit

Myunghwan Jeong et al.

Summary: The recently emerged ionic thermoelectric conversion with the Soret effect provides large thermopower, and by optimizing key parameters, outstanding thermoelectric responses can be achieved. The study reveals that the thermo-diffusion of water boosts proton transport, and when graphene oxide is embedded in the base material, it promotes ion transport and results in significantly improved ionic power factors and figure-of-merits.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

A flexible spring-shaped architecture with optimized thermal design for wearable thermoelectric energy harvesting

Haicai Lv et al.

Summary: A novel three-dimensional spring-like thermoelectric device (S-TED) is proposed, which inherits excellent flexibility, compressibility, and the ability to utilize waste heat under vertical temperature gradient. Compared to conventional TEDs, this device is optimized in contact enhancement, thermal insulation design, and heat dissipation efficiency, achieving high output power.

NANO ENERGY (2021)

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Article Chemistry, Physical

Elastic aerogel thermoelectric generator with vertical temperature-difference architecture and compression-induced power enhancement

Xiaodong Wang et al.

Summary: An elastic poly(3,4-ethylenedioxytiophene)-tosylate(PEDOT-Tos)/single-walled carbon nanotube (SWCNT) TE aerogel was fabricated for the first time, leading to the development of elastic TEGs with vertical-type aerogel legs displaying high TE performance and adjustable output power. Furthermore, the ultralight and compressible TEG showed excellent capability of harvesting heat under vertical temperature difference and mechanical deformation.

NANO ENERGY (2021)

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Article Chemistry, Physical

Wearable self-powered human motion sensors based on highly stretchable quasi-solid state hydrogel

Jianhao Chen et al.

Summary: Self-powered flexible sensors using hydrogel technology can detect human motion and sound, driven by harvested body heat. With impressive elongation and strain sensitivity, these sensors offer potential for various applications ranging from wearable electronics to health monitoring. The combination of flexibility, environmentally friendliness, sensitivity and thermoelectric performance makes them a promising choice in the field of self-powered sensors.

NANO ENERGY (2021)

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Article Multidisciplinary Sciences

Giant negative thermopower of ionic hydrogel by synergistic coordination and hydration interactions

Bin Chen et al.

Summary: By synergistic coordination and hydration interactions, we have successfully prepared an ionic hydrogel thermoelectric material with giant negative thermopower, exhibiting extremely high absolute thermopower. This ionic hydrogel shows promise for the design of high-thermopower ionic thermoelectric materials and low-grade heat energy harvesting.

SCIENCE ADVANCES (2021)

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Article Chemistry, Physical

Flexible and anti-freezing zinc-ion batteries using a guar-gum/sodium-alginate/ethylene-glycol hydrogel electrolyte

Jiawei Wang et al.

Summary: This study presents a new approach for developing natural polymer-based hydrogel electrolytes with high ionic conductivity and good antifreeze capability, achieved through blending guar gum and sodium alginate. The composite hydrogels demonstrated superior electrochemical performance in zinc-ion batteries, with excellent low-temperature discharge performance below -20 degrees C.

ENERGY STORAGE MATERIALS (2021)

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Flexible thermoelectric materials and devices: From materials to applications

Li Zhang et al.

Summary: This review summarizes the recent progress of flexible thermoelectric materials, including conducting polymers, organic/inorganic hybrid composites, and fully inorganic materials. The strategies and approaches for enhancing the thermoelectric properties of different flexible materials are detailed overviewed.

MATERIALS TODAY (2021)

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Review Chemistry, Multidisciplinary

Potentially Wearable Thermo-Electrochemical Cells for Body Heat Harvesting: From Mechanism, Materials, Strategies to Applications

Yuqing Liu et al.

Summary: This review summarizes the recent developments of potentially wearable thermo-electrochemical cells for body-heat harvesting, with a focus on flexible electrode materials, solid-state electrolytes, device fabrication, and strategies towards applications. It clarifies the challenges and provides future directions to enhance investigations on high-performance wearable TECs for practical and self-powered wearable devices.

ADVANCED SCIENCE (2021)

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Review Chemistry, Physical

Liquid-state thermocells: Opportunities and challenges for low-grade heat harvesting

Jiangjiang Duan et al.

Summary: Thermocells offer advantages such as low cost, scalability, and high thermopower, but face challenges such as low conversion efficiency, low power density, and stability issues. Future research directions aim to develop more cost-effective, robust, and simpler thermocells, and expand their applications in low-grade heat harvesting, temperature detection, cooling, and beyond.

JOULE (2021)

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Article Materials Science, Multidisciplinary

Ionic transport properties and their empirical correlations for thermal-to-electrical energy conversion

Ahrum Sohn et al.

Summary: Thermal-to-electrical energy conversion through thermo-diffusion of ions is a new and promising field with large thermopower and unique humidity dependency. Unlike conventional electronic thermoelectric materials, both ionic electrical conductivity and ionic thermopower improve simultaneously with increasing relative humidity, offering potential breakthroughs in performance enhancement. This work focuses on the Soret effect in solid-state polyelectrolytes, highlighting the potential for outstanding properties and new strategies in thermal-to-electrical energy conversion.

MATERIALS TODAY PHYSICS (2021)

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Article Nanoscience & Nanotechnology

Rational Design of Thermocells Driven by the Volume Phase Transition of Hydrogel Nanoparticles

Benshuai Guo et al.

Summary: Research has shown that liquid-state thermocells can achieve efficient thermoelectric conversion around physiological temperatures. By optimizing the choice and amount of redox chemical species, as well as selecting appropriate electrolyte salts, the performance of thermocells can be significantly improved. Additionally, a high correlation between the pH shift generated by the phase transition of nanoparticles and the Seebeck coefficient was discovered during nanoparticle screening.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Wearable Electronics Based on the Gel Thermogalvanic Electrolyte for Self-Powered Human Health Monitoring

Chenhui Bai et al.

Summary: This research focuses on converting body heat into electricity by fabricating a flexible thermogalvanic generator with Fe3+/Fe2+ as a redox pair. By incorporating a polyvinylidene fluoride diaphragm in the gel electrolyte, the Seebeck coefficient was effectively improved, leading to the establishment of a self-powered body temperature monitoring system.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Zn-Induced Defect Complexity for the High Thermoelectric Performance of n-Type PbTe Compounds

Yu Cao et al.

Summary: This study demonstrates the achievement of high ZT values in Zn-containing PbTe by designing complex defects, where Zn atoms occupy both Pb sites and interstitial sites, and couple with each other.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Stretchable and Freeze-Tolerant Organohydrogel Thermocells with Enhanced Thermoelectric Performance Continually Working at Subzero Temperatures

Wei Gao et al.

Summary: This study introduces a new method for addressing the challenges of low working temperatures, mechanical fragility, and poor thermoelectric performance of traditional aqueous thermocells by introducing a synergistic chaotropic effect. The organohydrogel thermocell designed in this work can still operate stably in extremely cold environments and has a high power density. This research provides new insights for providing reliable power sources for flexible electronic devices in extremely cold environments.

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Article Chemistry, Multidisciplinary

Mechanically Robust and Flexible Films of Ionic Liquid-Modulated Polymer Thermoelectric Composites

Zhipeng Li et al.

Summary: A new type of high-performance polymer thermoelectric composite with high thermoelectric performance and mechanical toughness has been reported, showing potential application prospects in addressing the issue of poor mechanical performance of TE composites.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Wearable Thermoelectric Materials and Devices for Self-Powered Electronic Systems

Yanhua Jia et al.

Summary: The emergence of artificial intelligence and the Internet of Things has led to a growing demand for wearable and maintenance-free power sources. Development of devices powered by body heat is now feasible, and thermoelectric materials have emerged as promising candidates for effective conversion of body heat into electricity. Wearable thermoelectric generators have become more flexible and stretchable, and various functional materials, processing techniques, and device design strategies are discussed in this review. Challenges in organic TE materials, interfacial engineering, and assessments of device performance are also addressed, with suggestions provided for future developments in the area of wearable TE materials and devices.

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Double-network thermocells with extraordinary toughness and boosted power density for continuous heat harvesting

Zhouyue Lei et al.

Summary: This study introduces double chemically crosslinked networks to address the mechanical challenges of thermocells while also improving power density. The newly designed thermocell shows large stretchability, impressive strength, extraordinary toughness, and a boosted output power density.

JOULE (2021)

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Article Chemistry, Physical

Heat-triggered high-performance thermocells enable a self-powered forest fire alarm

Boyang Yu et al.

Summary: By optimizing the structure of the thermocell and enhancing the thermogalvanic effect, a new technology has been successfully developed to power wireless sensor networks using heat from fire and effectively detect and alarm forest fires. This technology enables hibernation during peace time and rapid awakening when fire occurs, offering hope in combating the globally increasing forest fires.

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Thermogalvanic energy harvesting from forced convection cooling of 100-200 °C surfaces generating high power density

Yutaka Ikeda et al.

Summary: This study achieved a high power generation density of up to 10 W m(-2) during liquid forced convection cooling of a 170 degrees C surface, demonstrating the feasibility of thermogalvanic conversion. By utilizing a microchannel concept, high heat transfer coefficients and large interelectrode temperature differences were achieved, enabling effective power recovery based on liquid cooling.

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Thermogalvanic cells demonstrate inherent physiochemical limitations in redox-active electrolytes at water-in-salt concentrations

Mark A. Buckingham et al.

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High-efficiency thermocells driven by thermo-electrochemical processes

Meng Li et al.

Summary: Thermocells, a promising technology for converting low-grade heat into electricity, have recently seen breakthroughs in efficiency and power output. However, challenges such as volatility and degradation of redox couples continue to exist in the application of thermocells.

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Thermally regenerative electrochemical cycle for low-grade heat harnessing

Hang Zhang et al.

Summary: The review discusses the potential of converting low-grade heat into electricity using thermally regenerative electrochemical cycles. It highlights the challenges faced in current systems, such as low efficiency and high cost. Suggestions for material and system optimizations are provided to enhance the thermoelectric performance for practical applications.

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Md Al Mahadi Hasan et al.

Summary: This review provides a concise overview of the latest evolution in redox-based energy generation and the integration of redox-induced electricity generators with sensor devices, while focusing on current trends for energy solutions and performance enhancement techniques currently being investigated.

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Passive, high-efficiency thermally-localized solar desalination

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Summary: Solar desalination technologies show great potential for addressing the water-energy nexus, but bridging the gap between laboratory scale innovations and commercial applications is crucial. Key factors such as water production, reliability, and cost balance need to be systematically addressed to enable high-performance solar desalination systems.

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