Application of MOFs and COFs for photocatalysis in CO2 reduction, H2 generation, and environmental treatment

Article Nanoscience & Nanotechnology

The Fabrication of Pd Single Atoms/Clusters on COF Layers as Co-catalysts for Photocatalytic H2 Evolution

Xiaomin Ren et al.

Summary: The optimization of the particle size of co-catalysts is crucial for enhancing the photocatalytic activity of semiconductors.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Engineering, Environmental

Molybdenum phosphide coupled with highly dispersed nickel confined in porous carbon nanofibers for enhanced photocatalytic CO2 reduction

Shuaiqi Gong et al.

Summary: Photocatalytic CO2 reduction using renewable solar energy is a promising strategy for managing global carbon balance. However, the process of oriented photogenerated electron delivery is challenging. In this study, we developed a method to construct porous nitrogen-doped carbon nano-fibers loaded with highly dispersed nickel and molybdenum phosphide nanoparticles for efficient CO2 reduction. The porous carbon nanofibers improved charge/mass transfer and CO2 adsorption, while the highly dispersed nickel species stabilized by coordinating Ni-N bonds with N from the carbon nanofibers adjusted the material's band structure and altered the transfer route of the photogenerated carriers. The resulting Ni-MoP@NCPF exhibited high CO product selectivity and rate under visible light irradiation, outperforming the Ni-free MoP@NCPF. These findings provide new insights into cost-effective transition metal compounds for photocatalytic CO2 reduction through morphology, composition, and heterointerface engineering.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Facile fabrication of melamine sponge@covalent organic framework composite for enhanced degradation of tetracycline under visible light

Duoyu Lin et al.

Summary: In this study, a novel melamine sponge@COF composite sponge was successfully prepared using a reactive seeding strategy, enabling uniform and sturdy growth of small-sized COF-TpTt on the melamine sponge fibers. The composite sponge effectively overcomes the poor recyclability of general COFs, showing excellent photocatalytic activity towards the degradation of tetracycline antibiotics under visible light. This work provides a simple strategy for the preparation of COF-based composite materials with high degradation performance, easy circulation, and high stability for desired catalytic applications.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

A recyclable indoor air filter system based on a photocatalytic metal-organic framework for the removal of harmful volatile organic compounds

Junsuk Lee et al.

Summary: This study presents an indoor VOC filter system using a photocatalytic metalorganic framework (MOF) filter (PMF) based on MIL-100(Fe) with excellent adsorption and decomposition performance under UV light. The PMF showed high removal efficiency and stability in durability tests, making it suitable for various indoor applications.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Visible-light-driven photocatalytic degradation of ofloxacin by g-C3N4/NH2-MIL-88B(Fe) heterostructure: Mechanisms, DFT calculation, degradation pathway and toxicity evolution

Qi Su et al.

Summary: In this study, g-C3N4/NH2-MIL-88B(Fe) (MCN-x) heterostructures were successfully prepared and exhibited excellent degradation performance towards ofloxacin under visible light. The introduction of g-C3N4 in MCN-60 composite notably promoted the separation of photogenerated electron-hole pairs, leading to efficient photocatalytic activity.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Environmental Sciences

Design and construction strategies to improve covalent organic frameworks photocatalyst's performance for degradation of organic pollutants

Si-Yu Hu et al.

Summary: COFs are a class of crystalline porous organic polymers that have received extensive attention in the field of photocatalytic degradation. Strategies to improve the photocatalytic activity of COFs include design of ligands and structures, with a focus on COF composites. The photocatalytic mechanism and future prospects of COFs in photocatalytic degradation are discussed.

CHEMOSPHERE (2022)

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Article Chemistry, Physical

Hydrolytically stable citrate capped Fe3O4@UiO-66-NH2 MOF: A hetero-structure composite with enhanced activity towards Cr (VI) adsorption and photocatalytic H2 evolution

Suraj Prakash Tripathy et al.

Summary: A magnetically separable hetero-structure photocatalyst and adsorbent composite MU-2 with high adsorption capacity and photocatalytic H-2 evolution activity has been designed and prepared for efficient Cr (VI) remediation and clean energy conversion.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Physical

Self-assembly hybridization of COFs and g-C3N4: Decipher the charge transfer channel for enhanced photocatalytic activity

Han Wang et al.

Summary: Organic semiconductors are recognized as a new generation of photocatalysts for pollutants degradation and energy production. In this study, a TpMa/CN heterojunction was fabricated via a controllable self-assembly approach, showing enhanced visible-light absorption and improved photocatalytic activities.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Multidisciplinary Sciences

Selective ligand removal to improve accessibility of active sites in hierarchical MOFs for heterogeneous photocatalysis

Shaghayegh Naghdi et al.

Summary: In this study, the authors demonstrate that selective ligand removal in metal-organic frameworks (MOFs) can introduce new active sites and mesopores, leading to enhanced photocatalytic hydrogen evolution. This strategy allows for the purposeful engineering of hierarchical MOFs, advancing their applicability in environmental and energy technologies.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Applied

Construction of TiO2-covalent organic framework Z-Scheme hybrid through coordination bond for photocatalytic CO2 conversion

Lei Wang et al.

Summary: In this study, a covalent organic framework (COF) was constructed with CuTAPP and p-benzaldehyde, integrated with TiO2 to form a Z-scheme hybrid system. The framework showed enhanced photocatalytic performance in CO2 conversion, attributed to the photosensitizer effect of the porphyrin block and the establishment of a Z-scheme system for carrier separation.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

One-Step MOF-Templated Strategy to Fabrication of Ce-Doped ZnIn2S4 Tetrakaidecahedron Hollow Nanocages as an Efficient Photocatalyst for Hydrogen Evolution

Huitao Fan et al.

Summary: This study successfully synthesized Ce-doped ZnIn2S4 photocatalysts with hollow nanocages using a one-step hydrothermal method. Both experimental and theoretical results showed that the doping of Ce and the formation of hollow nanocages improved light capture and the separation of photogenerated charge carriers.

ADVANCED SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Enhanced Photocatalytic Activity of Porphyrin Nanodisks Prepared by Exfoliation of Metalloporphyrin-Based Covalent Organic Frameworks

Xinxi Li et al.

Summary: The synthesis of organic polymers from COFs by changing the unit molecule can enhance photocatalytic activity. In this study, the exfoliation of metalloporphyrin-based COFs and adjustment of the layer thickness were found to enhance photocatalytic activity.

ACS OMEGA (2022)

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Article Chemistry, Physical

Pd single-atom decorated CdS nanocatalyst for highly efficient overall water splitting under simulated solar light

Wei Li et al.

Summary: This study presents a CdS-Pd nanocatalyst with improved stability and activity for solar-induced overall water splitting. The CdS-Pd nanocatalyst showed 110-fold higher activity than pristine CdS. It also demonstrated high apparent quantum yields under broadband light illumination. The findings provide important insights for the development of stable and efficient CdS-based photocatalysts for hydrogen production.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Covalent organic framework based WO3@COF/rGO for efficient visible-light-driven H2 evolution by two-step separation mode

Han Yan et al.

Summary: A core-shell COF-based Z-scheme heterojunction was synthesized, and by constructing a Z-scheme charge transfer pathway and using rGO as a carrier, the photocatalytic activity of COF was enhanced.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Amino-functionalized Ti-metal-organic framework decorated BiOI sphere for simultaneous elimination of Cr(VI) and tetracycline

Dingliang Dai et al.

Summary: A flower-like MIL-125-NH2@BiOI composite was fabricated by a solvothermal method for the simultaneous elimination of Cr(VI)/tetracycline mixed pollutants under visible light. The strong interaction between amino in MIL-125-NH2 and Bi3+ of BiOI promotes the formation of the unique inlaid structure, leading to accelerated charge carrier transfer. The photocatalytic efficiency can be further boosted in the coexistence of Cr(VI) and tetracycline, showcasing a synergistic effect for improved removal efficiency.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Inorganic & Nuclear

In situ growth of UIO-66-NH2 on thermally stabilized electrospun polyacrylonitrile nanofibers for visible-light driven Cr (VI) photocatalytic reduction

Meimei Zhou et al.

Summary: UIO-66-NH2 was successfully deposited onto thermally stabilized electrospun polyacrylonitrile (PAN) nanofibers, providing ideal nucleation points for MOFs growth. The resulting UIO-66-NH2@TSPAN nanofibers showed enhanced visible light driven photocatalytic activity towards reduction of Cr(VI) due to improved light response and photothermal conversion ability. The mechanical flexibility and structural stability of the nanofibrous photocatalyst allowed for easy operation and outstanding reusable capability.

JOURNAL OF SOLID STATE CHEMISTRY (2022)

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Review Environmental Sciences

Recent advances in performance improvement of Metal-organic Frameworks to remove antibiotics: Mechanism and evaluation

Jingwen Zhang et al.

Summary: This review summarizes the effectiveness of Metal-Organic Frameworks (MOFs) based adsorption and photocatalysis strategies in addressing antibiotic pollution and environmental repair. Strategies to improve the properties of MOFs for removal and the removal mechanisms are discussed. Additionally, new evaluation methods for MOFs to remove antibiotics are presented.

SCIENCE OF THE TOTAL ENVIRONMENT (2022)

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Article Engineering, Chemical

Excellent photoreduction performance of U(VI) on metal organic framework/covalent organic framework heterojunction by solar-driven

Xin Zhong et al.

Summary: This study investigated the photocatalytic reduction of U(VI) using MOF photocatalysts. The results showed that the NH2--MIL-125(Ti)@TpPa-1 heterojunction had better photoreduction efficiency and could convert U(VI) into U(IV). Photogenerated electrons and superoxide radicals played important roles in the photoreduction process. The hybridization of MOF@COF acted synergistically in the adsorption-photocatalytic reduction of U(VI).

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Multidisciplinary Sciences

Pyridinium salt-based covalent organic framework with well-defined nanochannels for efficient and selective capture of aqueous 99TcO4-

Mengjie Hao et al.

Summary: A cationic pyridinium salt-based COF with high surface area and ordered pore structure was reported, showing exceptional adsorption properties towards radioactive ions and potential for nuclear waste management.

SCIENCE BULLETIN (2022)

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Article Chemistry, Multidisciplinary

Converging Cooperative Functions into the Nanospace of Covalent Organic Frameworks for Efficient Uranium Extraction from Seawater

Mengjie Hao et al.

Summary: This study presents a new strategy for efficient extraction of uranium from seawater by combining the functions of adsorption and photocatalysis in covalent organic frameworks (COFs). The developed COFs demonstrated exceptional performance in sequestering and reducing uranyl from natural seawater under visible light irradiation, offering promising candidates for efficient uranium extraction.

CCS CHEMISTRY (2022)

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Article Chemistry, Physical

Highly efficient uranium extraction by a piezo catalytic reduction-oxidation process

Yawen Cai et al.

Summary: This study reports a highly efficient uranium extraction method from water using a piezo-catalytic process. By utilizing a hollow cubic shaped Zn2SnO4/SnO2 as a piezo catalyst, the adsorbed U(VI) is reduced to UO2 and then oxidized to (UO(2)2)(2), which can be efficiently separated from the solution under ultrasonic irradiation.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

Synthesis of acidic MIL-125 from plastic waste: Significant contribution of N orbital for efficient photocatalytic degradation of chlorobenzene and toluene

Xiaodong Zhang et al.

Summary: In this study, we synthesized MIL-125 using plastic-based terephthalic acid and modified it with amino and nitro groups. The results showed that amino modification promoted the visible absorption range and acidity of MIL-125, leading to efficient catalytic degradation of chlorobenzene and toluene.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Multidisciplinary

Highly Efficient Electrocatalytic Uranium Extraction from Seawater over an Amidoxime-Functionalized In-N-C Catalyst

Xiaolu Liu et al.

Summary: Seawater contains uranium at a concentration of approximately 3.3 ppb, making it a valuable and sustainable nuclear fuel source. This study developed an adsorption-electrocatalytic platform for extracting uranium from seawater using atomically dispersed indium anchored on hollow nitrogen-doped carbon capsules functionalized with flexible amidoxime moieties. The platform showed excellent uranyl capture properties and high selectivity for uranium extraction over vanadium in seawater. X-ray absorption spectroscopy and in situ Raman results provided detailed insights into the molecular mechanism of uranium extraction. This work contributes to the growing suite of technologies for harvesting valuable metals from the earth's oceans.

ADVANCED SCIENCE (2022)

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Article Engineering, Environmental

Super-efficient extraction of U(VI) by the dual-functional sodium vanadate (Na2V6O16•2H2O) nanobelts

Yifeng Zhang et al.

Summary: This study demonstrates a super-efficient and high-selective method for extracting U(VI) from wastewater using dual-functional Na2V6O16 center dot 2H(2)O (NVO) nanobelts in a weak acid environment. The soluble U(VI) is immobilized by NVO nanobelts through a chemical reaction combined with complexations induced by electrostatic attraction. This method shows great potential in U(VI) extraction and environmental pollution control.

CHEMICAL ENGINEERING JOURNAL (2022)

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Review Chemistry, Inorganic & Nuclear

Advanced photocatalysts for uranium extraction: Elaborate design and future perspectives

Tao Chen et al.

Summary: Nuclear energy is a promising energy source to replace traditional fossil fuels due to its high energy density and carbon-free emission. However, the limited storage of uranium ore and uranium-containing wastewater pose challenges to the sustainable development of nuclear energy. Therefore, extracting and recycling uranium from seawater and wastewater is necessary for the sustainable development of nuclear energy and environmental protection.

COORDINATION CHEMISTRY REVIEWS (2022)

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Review Environmental Sciences

Recent developments of doped g-C3N4 photocatalysts for the degradation of organic pollutants

Xiaolu Liu et al.

Summary: Graphitic carbon nitride (g-C3N4) has high thermal stability and a moderate band gap, but its performance is limited by issues like insufficient absorption of visible light. Element doping is an effective strategy to enhance its photocatalytic properties and improve performance.

CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY (2021)

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Article Chemistry, Physical

Eosin Y bidentately bridged on UiO-66-NH2 by solvothermal treatment towards enhanced visible-light-driven photocatalytic H2 production

Jinwen Shi et al.

Summary: This study developed a solvothermal method to synthesize EY-sensitized UiO-66-NH2, enhancing the connection between EY and UiO-66-NH2, improving the transfer rate of photogenerated electrons, and significantly increasing the H-2 evolution rate and apparent quantum efficiency.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Review Chemistry, Multidisciplinary

Microwave-Assisted Synthesis of Covalent Organic Frameworks: A Review

Borja Diaz de Grenu et al.

Summary: This article presents a comprehensive compilation of research results on microwave-assisted synthesis of COFs, covering the synthesis, characteristics, and general issues related to COFs and microwaves. Current and future perspectives on this topic are also discussed.

CHEMSUSCHEM (2021)

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Article Chemistry, Physical

2D Covalent Organic Frameworks with an Incorporated Manganese Complex for Light Driven Carbon Dioxide Reduction

Denan Wang et al.

Summary: This study reports the direct incorporation of a manganese CO2 molecular catalyst (MC) into COFs (Mn-TTA-COF) and evaluates its capability as a photocatalyst for visible light driven CO2 reduction. The photocatalytic activity of Mn-TTA-COF is found to be low, mainly due to the elimination of the CO ligand in the Mn MC upon light illumination. However, the stability and efficiency of Mn MC are significantly enhanced after being incorporated into COFs, suggesting the potential of COFs as a platform for creating next-generation photocatalysts.

CHEMPHOTOCHEM (2021)

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Article Engineering, Environmental

Construction of NH2-MIL-125(Ti)/CdS Z-scheme heterojunction for efficient photocatalytic H2 evolution

Xiaohui Zhang et al.

Summary: The research team successfully designed a Z-scheme CdS/NH2-MIL-125(Ti) heterojunction photocatalyst, which can significantly enhance the hydrogen evolution rate and provide a new avenue for solar-driven energy conversion.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Nanoscience & Nanotechnology

In Situ Fabrication of Porous MOF/COF Hybrid Photocatalysts for Visible-Light-Driven Hydrogen Evolution

Ping Xue et al.

Summary: This study successfully prepared a series of Cu-3 (HHTP)(2)-MOF/Tp-Pa-1-COF hybrids and demonstrated superior photocatalytic performance, achieving efficient hydrogen evolution under visible light irradiation by promoting charge transfer effectively and inhibiting recombination of photogenerated electron-hole pairs.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Functionalized Iron-Nitrogen-Carbon Electrocatalyst Provides a Reversible Electron Transfer Platform for Efficient Uranium Extraction from Seawater

Hui Yang et al.

Summary: The study demonstrates an adsorption-electrocatalysis strategy using a functionalized iron-nitrogen-carbon catalyst for efficient uranium extraction from seawater, reducing uranium concentration to very low levels and providing technological innovation in this field.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Oil-Water-Oil Triphase Synthesis of Ionic Covalent Organic Framework Nanosheets

Zheyuan Guo et al.

Summary: This study introduces a triphase method for the synthesis of ionic covalent organic framework nanosheets, demonstrating the production of iCOFNs with excellent properties and their potential applications in the field of ultrathin COF membranes. The innovative approach of using the oil-water-oil system provides a new platform for the synthesis and application of iCOFNs.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Thiazolo[5,4-d]Thiazole-Based Donor-Acceptor Covalent Organic Framework for Sunlight-Driven Hydrogen Evolution

Wenqian Li et al.

Summary: The 2D covalent organic framework PyTz-COF shows exceptional optoelectronic properties, photocatalytic ability, and photoelectrochemical activity, making it suitable for solar energy harvesting and conversion.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Metal-free Fenton-like photocatalysts based on covalent organic frameworks

Qiaobo Liao et al.

Summary: This study presents a metal-free covalent organic framework (COF)-based standalone photocatalyst with superior reactivity for Fenton-like reactions, surpassing other well-known metal-free photocatalysts and comparable to metal-containing catalysts in terms of performance and generality. Large porosity, high density of photoactive triazine moiety, suitable bandgap, efficient charge separation and transfer, as well as abundant H2O2 binding sites and reaction centers contribute to its outstanding performance for water pollution remediation.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Multidisciplinary

Encapsulation of Cobalt Oxide into Metal-Organic Frameworks for an Improved Photocatalytic CO2 Reduction

Yiwen Ma et al.

Summary: In this study, CoOx nanoparticles were loaded in MIL-101(Cr) channels to create a novel CoOx/MIL-101(Cr) system for enhancing photocatalytic CO2 reduction. The optimized conditions led to significantly improved performance compared to bare CoOx and MIL-101(Cr), offering a new pathway for the rational design of efficient MOF systems for photocatalytic reduction of CO2.

CHEMSUSCHEM (2021)

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Article Engineering, Environmental

Highly sensitive SERS detection and photocatalytic degradation of 4-ami- nothiophenol by a cost-effective cobalt metal-organic framework-based sandwich-like sheet

Changli Shi et al.

Summary: An innovative composite sheet (Ag/ZIF-67/TiO2/Cu) with well-dispersed Ag nanoparticles was successfully developed for highly sensitive detection and efficient degradation of 4-aminothiophenol. This novel sheet exhibited outstanding SERS response to 4-ATP with only 0.5 wt% Ag, high photocatalytic degradation capability reaching 100% efficiency within 15 minutes, and excellent reusability.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Chemistry, Inorganic & Nuclear

Recent advances of Zr based metal organic frameworks photocatalysis: Energy production and environmental remediation

Xiansheng Zhang et al.

Summary: Zirconium (Zr) based metal organic frameworks (Zr-MOFs) materials have shown increasing interest in the field of photocatalysis due to their large surface area, ordered porous structure, and excellent water-tolerant properties. These materials have been reported to exhibit excellent photocatalytic performance and are applied in various areas such as water splitting, carbon dioxide reduction, organic pollutant removal, and Cr(VI) reduction, with detailed mechanisms of these processes being described. Future developments and challenges of Zr-MOFs photocatalyst are also discussed.

COORDINATION CHEMISTRY REVIEWS (2021)

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Review Chemistry, Inorganic & Nuclear

Metal-organic frameworks for photocatalytic detoxification of chromium and uranium in water

Vanish Kumar et al.

Summary: This review highlights the potential of metal-organic framework (MOF)-based materials for the photo-reductive demineralization of heavy and radioactive metal(loid) pollutants. It emphasizes on the recent progress in the development of MOF-based photocatalysts for the reduction of Cr(VI) and U(VI) metal(loid)s in water, focusing on key performance metrics and modification strategies. The optimal performers identified were Zn-MOF/BUC-21@titanate nanotube/Ag@Ag3PO4@MIL-125-NH2 and MOF-derived g-C3N4 nanosheets.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Chemistry, Multidisciplinary

Effect of Linker Distribution in the Photocatalytic Activity of Multivariate Mesoporous Crystals

Belen Lerma-Berlanga et al.

Summary: Metal-Organic Frameworks are used as crystalline matrices to synthesize multiple component or multivariate solids, allowing for property customization. By optimizing synthesis through high-throughput methods, it is possible to create multivariate frameworks with efficient light sensitization, chemical stability, and porosity for photocatalysis applications. Solvent-assisted linker exchange reactions can control the distribution of linkers in crystals, affecting their performance in photocatalytic activities.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Zirconium-Based Metal-Organic Framework Particle Films for Visible-Light-Driven Efficient Photoreduction of CO2

Pei-Xian Li et al.

Summary: This study successfully prepared MOF films for photocatalytic CO2 reduction, achieving good photocatalytic activity and reusability. By measuring photocurrent response and electrochemical impedance spectroscopy of the PET@NH2-UiO-66 film, it was confirmed that the electron-hole pairs in the film separate rapidly.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Article Engineering, Environmental

Construction of direct Z-scheme Bi5O7I/UiO-66-NH2 heterojunction photocatalysts for enhanced degradation of ciprofloxacin: Mechanism insight, pathway analysis and toxicity evaluation

Chen Zhao et al.

Summary: Z-scheme Bi5O7I/UiO-66-NH2 heterojunction photocatalysts were successfully constructed via ball-milling, showing superior CIP removal efficiency compared to pristine Bi5O7I and UiO-66-NH2. Among them, the heterojunction with 50 wt% UiO-66-NH2 content (BU-5) exhibited excellent structural stability and optimal CIP removal efficiency, achieving 96.1% removal within 120 minutes of illumination.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Physical

Design and fabrication of a perylene dimiide functionalized g-C3N4@UiO-66 supramolecular photocatalyst: Insight into enhancing the photocatalytic performance

Anasheh Mardiroosi et al.

Summary: A unique PCN@UiO-66 material with superior photocatalytic degradation efficiency was prepared, exhibiting higher degradation efficiency compared to other materials. The maximum photodegradation efficiency was achieved at pH 7. The enhanced efficiency can be attributed to improved visible light absorption and reduced charge recombination rate by perylene dimiide (PDI) photofunctional groups.

JOURNAL OF MOLECULAR STRUCTURE (2021)

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Article Chemistry, Physical

Effect of linkages on photocatalytic H2 evolution over covalent organic frameworks

Ruowei Lu et al.

Summary: In this study, three tunable COF platforms with different linkages were constructed to investigate their visible-light photocatalytic hydrogen production (PHP) performance. It was found that the dianhydride substituted imide-COF (PMDA-COF) showed a sustainable and stable PHP rate under visible light irradiation, along with excellent photo-generated charge separation capabilities. The D-A molecular heterojunction in PMDA-COF plays a crucial role in modifying the electronic band structure and separating the reduction and oxidation sites.

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Building a Pyrazole-Benzothiadiazole-Pyrazole Photosensitizer into Metal-Organic Frameworks for Photocatalytic Aerobic Oxidation

Ji-Kang Jin et al.

Summary: Charge separation is crucial in regulating photochemical properties in photocatalysts design. Metal-organic frameworks (MOFs) are promising candidates for heterogeneous photocatalysis due to their designability and photon absorption tunability. A pyrazole-benzothiadiazole-pyrazole organic molecule with a donor-acceptor-donor conjugated pi-system was designed for fast charge separation, resulting in a more effective heterogeneous photocatalyst JNU-204, which demonstrated stability and reusability in aerobic oxidation reactions under visible-light irradiation. JNU-204 also showed applications in the synthesis of marine natural product core skeletons.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Engineering, Environmental

Boosting photocatalytic CO2 reduction over a covalent organic framework decorated with ruthenium nanoparticles

Ke Guo et al.

Summary: The study developed Ru/TpPa-1 catalysts for photocatalytic reduction of CO2 under visible light irradiation, showing significantly enhanced activity compared to TpPa-1. The interactions between Ru NPs and TpPa-1 were found to enhance visible-light harvesting and extend the service life of photo-generated charge carriers.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Chemical

A direct Z-scheme BiOBr/TzDa COF heterojunction photocatalyst with enhanced performance on visible-light driven removal of organic dye and Cr(VI)

Yan Zhang et al.

Summary: Efficient Z-scheme heterojunction photocatalyst BTDC was successfully synthesized by modifying 2D BiOBr with 2D TzDa COF, showing excellent performance in degrading RhB and reducing Cr(VI) under visible light. The enhanced efficiency of BTDC was attributed to accelerated charge carriers separation and transport, enhanced visible light absorption, and increased specific surface area.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

In Situ Porphyrin Substitution in a Zr(IV)-MOF for Stability Enhancement and Photocatalytic CO2 Reduction

Xiang-Jing Kong et al.

Summary: In this study, a strategy for enhancing stability and functionality in labile Zr(IV)-MOFs through in situ porphyrin substitution has been proposed. The introduction of a robust linear porphyrin ligand significantly improved the chemical stability of the resulting MOFs. The modified MOFs exhibited high catalytic activity in CO2 photoreduction, showing promise for converting unstable MOFs into robust functional materials.

SMALL (2021)

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Review Chemistry, Physical

Pickering emulsions stabilized by metal-organic frameworks, graphitic carbon nitride and graphene oxide

Fanyu Zhang et al.

Summary: Pickering emulsions, stabilized by solid particles, are a heterogeneous system with micrometre-sized droplets dispersed in another phase, which can have their properties adjusted by using different types of solid particles, and have been widely applied in areas such as material science and catalysis.

SOFT MATTER (2021)

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Article Multidisciplinary Sciences

Rational design of isostructural 2D porphyrin-based covalent organic frameworks for tunable photocatalytic hydrogen evolution

Rufan Chen et al.

Summary: Covalent organic frameworks show promise in photocatalytic hydrogen generation from water, with the incorporation of different transition metals allowing for tuning of the hydrogen evolution rate.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Recent advances in photocatalytic multivariate metal organic frameworks-based nanostructures toward renewable energy and the removal of environmental pollutants

S. Patial et al.

Summary: Water pollution and energy crises are major challenges for sustainability in the modern world. Solar energy-driven photocatalysis using multi-variate metal-organic frameworks (MTV-MOFs) shows promise in environmental remediation, with their flexible tunability and enhanced surface area for diverse applications.

MATERIALS TODAY ENERGY (2021)

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Article Chemistry, Multidisciplinary

Interfacial Microenvironment Modulation Boosting Electron Transfer between Metal Nanoparticles and MOFs for Enhanced Photocatalysis

Mingliang Xu et al.

Summary: The presence of surfactants on the surface of metal cocatalysts can significantly affect the electron transfer rate between the metal and MOF, and removing these surfactants can improve the efficiency of photocatalytic hydrogen production.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Synthesis of a Boron-Imidazolate Framework Nanosheet with Dimer Copper Units for CO2 Electroreduction to Ethylene

Ping Shao et al.

Summary: Understanding the relationship between structure and composition and the catalytic activity in the electrochemical CO2 reduction reaction is crucial for the design of efficient electrocatalysts. Catalysts featuring Cl-bridged Cu-2 units have been shown to enhance selectivity and activity for C2H4, with neighboring Cu monomers acting as regulators and providing different reaction paths.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Engineering, Environmental

In-situ growth of Ti3C2@MIL-NH2 composite for highly enhanced photocatalytic H2 evolution

Yujie Li et al.

Summary: Efficient metal-organic frameworks (MOFs) for photocatalytic H-2 production from water have gained significant attention, but their poor conductivity limits their activity. A Ti-based MOF composite (Ti3C2@MIL-NH2) was developed, showing superior H-2 evolution performance with a high rate. Intimate interfacial contact between Ti3C2 and MIL-NH2 accelerates electron transfer and improves photo-generated charge separation efficiency.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

IL-assisted synthesis of defect-rich polyaniline/NH2-MIL-125 nanohybrids with strengthened interfacial contact for ultra-fast photocatalytic degradation of acetaldehyde under high humidity

Syed Jalil Shah et al.

Summary: The novel IL-PANI/NMIL(Ti) nanohybrids exhibit superior photodegradation performance for CH3CHO with abundant defects and enhanced catalytic activity. Smart grafting increases the adsorption rate of CH3CHO and expands the light absorption range. Furthermore, the degradation rate of CH3CHO is further enhanced at higher humidity levels.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Chemistry, Multidisciplinary

Metal-Organic Frameworks With Variable Valence Metal-Photoactive Components: Emerging Platform for Volatile Organic Compounds Photocatalytic Degradation

Yuhang Qian et al.

Summary: Newly emerging metal-organic frameworks (MOFs) materials are highly diverse in structures and performances, making them promising artificial catalysts for addressing multiple challenges in the fields of energy and environment. MOFs have been successfully synthesized as powerful photocatalysts for important redox reactions, but face limitations in their application for indoor-air VOC pollutants cleaning due to restricted diffusion of pollutant molecules and active species within their porous structures.

FRONTIERS IN CHEMISTRY (2021)

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Article Chemistry, Physical

Imide modification coupling with NH2-MIL-53(Fe) boosts the photocatalytic performance of graphitic carbon nitride for efficient water remediation

Xiaosi Wang et al.

Summary: Perylene diimide (PDI) was introduced into the framework of g-C3N4 to build a polymer with a donor-acceptor structure, optimizing the energy band structure and increasing visible light responsiveness. This modification also led to an increased exposure of reactive sites, resulting in superior performance in the photodegradation of organic pollutants in wastewater treatment.

JOURNAL OF CATALYSIS (2021)

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Review Green & Sustainable Science & Technology

Recent developments in the photocatalytic applications of covalent organic frameworks: A review

Junhua You et al.

Summary: Covalent Organic Frameworks (COFs) are crystalline covalent polymers with high surface area and stable porosity, showing great potential for functionalization. Researchers are highly interested in novel and advanced COF materials for their wide range of useful applications. The use of COFs in photocatalytic applications is rapidly developing, offering an exciting avenue for scientific contributions in the field.

JOURNAL OF CLEANER PRODUCTION (2021)

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Article Multidisciplinary Sciences

Extremely stable amidoxime functionalized covalent organic frameworks for uranium extraction from seawater with high efficiency and selectivity

Gong Cheng et al.

Summary: A polyarylether-based covalent organic framework functionalized with open-chain amidoxime was synthesized for efficient uranium extraction from seawater. The adsorbent demonstrated high selectivity for uranium over vanadium, with significantly enhanced adsorption capacity, and high stability, making it a promising material for uranium extraction from natural seawater.

SCIENCE BULLETIN (2021)

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Article Nanoscience & Nanotechnology

NH2-UiO-66 Coated with Two-Dimensional Covalent Organic Frameworks: High Stability and Photocatalytic Activity

Yongchao Wang et al.

Summary: The coupling of NH2-UiO-66 with COFs can improve its photocatalytic performance and stability, with high stability in alkaline environment and good photocatalytic H-2 evolution rate.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Multidisciplinary

A Review of MOFs and Their Composites-Based Photocatalysts: Synthesis and Applications

Yongteng Qian et al.

Summary: MOFs-based photocatalysts have unique morphology, high performance, stability, easy synthesis, and low cost. This review introduces synthetic strategies, summarizes various types of MOFs composite photocatalysts, and highlights different applications of MOFs-based photocatalysts.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

N-Heterocyclic Carbene-Stabilized Ultrasmall Gold Nanoclusters in a Metal-Organic Framework for Photocatalytic CO2 Reduction

Yilin Jiang et al.

Summary: Ultrafine gold nanoclusters (Au-NCs) can be stabilized in a heterogeneous nucleation approach within an NHC-functionalized porous matrix, with tunable sizes based on MOF topology for superior photocatalytic CO2 reduction activity. Control experiments using different functionalized MOFs resulted in Au species aggregation. The synergistic catalytic effect of MOFs and Au-NCs through covalent bonding bridges was revealed in mechanistic studies, contributing to the excellent performance of the Au-NC@MOF composite.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Photocatalysis-activated SR-AOP over PDINH/MIL-88A(Fe) composites for boosted chloroquine phosphate degradation: Performance, mechanism, pathway and DFT calculations

Xiao-Hong Yi et al.

Summary: PDINH/MIL-88A(Fe) composites were fabricated using a facile ball-milling strategy, showing outstanding degradation performance towards CQ under low power LED visible light. The activation of PDS over P25M175 and pristine MIL-88A contributed to boosted CQ degradation efficiency through direct and indirect electron transfer. Active radicals and singlet oxygen were found to participate in the CQ decomposition, with proposed degradation pathways and toxicity evaluations of intermediates.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Environmental

NH2-MIL-125(Ti) encapsulated with in situ-formed carbon nanodots with up-conversion effect for improving photocatalytic NO removal and H2 evolution

Youzhou He et al.

Summary: The bifunctional photocatalyst CDs@NH2-MIL-125(Ti) exhibits great NO removal and H2 evolution capabilities under visible light irradiation, showing higher efficiency compared to pristine NH2MIL-125(Ti). Characterization using various techniques suggests that the encapsulated CDs enhance visible light utilization and serve as electron receivers to improve photocatalytic performance. Fabricating CDs with metal-organic frameworks (MOFs) proves to be an effective strategy for enhancing simultaneous NO elimination and H2 evolution in photocatalysis.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

MIL-88B(Fe)-coated photocatalytic membrane reactor with highly stable flux and phenol removal efficiency

Chechia Hu et al.

Summary: In this study, two photocatalytic membrane reactors (PMRs) were successfully developed for phenol degradation, with the PHMR system showing significantly enhanced phenol removal efficiency and stable flux, while the PFMR system had lower flux but demonstrated good recyclability and stability. Both systems exhibited promising potential as effective, feasible, and sustainable wastewater treatment systems.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

In-situ synthesis of Z-Scheme MIL-100(Fe)/α-Fe2O3 heterojunction for enhanced adsorption and Visible-light photocatalytic oxidation of O-xylene

Lu Chen et al.

Summary: The MIL-100(Fe)/?-Fe2O3 photocatalysts showed high efficiency in the PCO of VOCs, with a remarkable o-xylene removal rate reaching 100% under 250W xenon lamp irradiation. The hybrid material exhibited a large specific surface area and evenly distributed active sites for effective adsorption of target molecules, suggesting potential for air purification applications. Additionally, the reversible conversion of Fe(III) and Fe(II) under light irradiation plays a key role in the oxidation of o-xylene and generation of reactive radicals in the Z-scheme structure.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Vinylene-linked covalent organic frameworks with enhanced uranium adsorption through three synergistic mechanisms

Rui-Han Xu et al.

Summary: The study presents a vinylene-linked covalent organic framework (Tp-TMT) as a uranium adsorbent, which enhances uranium adsorption through selective ligand binding, chemical reduction, and photocatalytic reduction mechanisms. Tp-TMT exhibits outstanding uranium adsorption capacity under light irradiation through synergistic effects of its unique structure and excellent photocatalytic activity.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Chemical

Coupling Covalent Organic Frameworks and Carbon Nanotube Membranes to Design Easily Reusable Photocatalysts for Dye Degradation

Hongbo Xue et al.

Summary: COF/CNT membranes with enhanced photocatalytic activity and superior degradation capacity were prepared by utilizing carbon nanotube membranes as substrates, resulting in significant improvement in degradation efficiency and reusability.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2021)

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Article Chemistry, Inorganic & Nuclear

High Proton Conductivity in Nafion/Ni-MOF Composite Membranes Promoted by Ligand Exchange under Ambient Conditions

Hongfei Wang et al.

Summary: Metal-organic frameworks (MOFs) show promise as crystalline porous materials for proton conduction. Exploration of preparation methods and proton transfer mechanisms, combined with ligand exchange strategy, can enhance the proton conductivity of MOFs for potential future applications.

INORGANIC CHEMISTRY (2021)

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Article Chemistry, Inorganic & Nuclear

Bandgap Modulation in Zr-Based Metal-Organic Frameworks by Mixed-Linker Approach

Rushie Mae Cedeno et al.

Summary: This study investigated the effect of mixed organic linkers on the bandgap modulation of Zirconium-based MOFs UiO-66 and MIL-140A using density functional theory. It was found that mixed-linker systems exhibit unique electronic properties and bandgap reduction due to the formation of mid-gap states. Pi-pi stacking interactions were identified as a significant factor in bandgap modulation, demonstrating the potential to engineer the electronic properties of MOFs through a mixed-linker approach.

INORGANIC CHEMISTRY (2021)

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Article Chemistry, Inorganic & Nuclear

Zn(II)-MOF with flexible dicarboxylate ligand with different N-donor linkage as photocatalyst for aromatic dye degradation

Wuxin Hu et al.

Summary: A new Zn(II)-based metal-organic framework (MOF) has been synthesized and found to exhibit efficient photocatalytic performance in degrading methyl violet under UV light. Experimental and theoretical calculations were used to investigate and explain the degradation mechanism.

INORGANIC CHEMISTRY COMMUNICATIONS (2021)

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Article Chemistry, Physical

Electrospun graphene oxide/MIL-101(Fe)/poly(acrylonitrile-co-maleic acid) nanofiber: A high-efficient and reusable integrated photocatalytic adsorbents for removal of dye pollutant from water samples

Zhujun Huang et al.

Summary: The electrospun graphene oxide/MIL-101(Fe)/poly(acrylonitrile-co-maleic acid) nanofibers exhibit excellent adsorption ability and photocatalytic activity, making them effective in removing dye pollutants from water.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Engineering, Environmental

Degradation of diclofenac in water under LED irradiation using combined g-C3N4/NH2-MIL-125 photocatalysts

V. Muelas-Ramos et al.

Summary: This study investigates the photocatalytic degradation of diclofenac using hybrid materials composed of graphitic carbon nitride (g-C3N4) and titanium-metal organic framework (NH2-MIL-125) in various mass proportions. The hybrid materials exhibited higher photocatalytic activity than the individual components, with a 50:50 MOF:g-C3N4 ratio yielding the highest conversion rate, completely eliminating diclofenac in 2 hours. Identification of by-products species allowed for proposing a degradation pathway under the experimental conditions.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Materials Science, Multidisciplinary

Facile construction of highly efficient MOF-based Pd@UiO-66-NH2@ZnIn2S4 flower-like nanocomposites for visible-light-driven photocatalytic hydrogen production

Mengting Cao et al.

Summary: Metal-organic-frameworks-based composite photocatalysts, including the novel Pd@UiO-66-NH2@ZnIn2S4 nanocomposites, show significantly improved photocatalytic activity compared to individual components. The enhanced performance is mainly attributed to the matched band gap of ZnIn2S4 and UiO-66-NH2, as well as the introduction of Pd NPs for broadening spectral response range and promoting charge carrier separation.

JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Tunable Band Gaps in MUV-10(M): A Family of Photoredox-Active MOFs with Earth-Abundant Open Metal Sites

Kevin Fabrizio et al.

Summary: This research focuses on the role of titanium-based metal-organic frameworks in photocatalytic reactions, finding that Ti-MOFs can be modified synthetically to include ions that control the energy levels of photoactive orbitals, thereby regulating the electronic structure and band gaps of MOFs. By measuring the Fermi levels of photoexcited MOFs, the mechanism of charge storage in Ti-MOFs is revealed.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Perovskite Quantum Dots Encapsulated in a Mesoporous Metal-Organic Framework as Synergistic Photocathode Materials

Guan-Yu Qiao et al.

Summary: Encapsulating CsPbBr3 nanocrystals into a stable metal-organic framework greatly enhances their photocatalytic performance, with significant charge transfer observed at the interface between the quantum dots and the MOF. This composite material shows excellent catalytic activity in oxygen reduction and evolution reactions, as well as serving as a synergistic photocathode in Li-O-2 batteries, highlighting the cooperative effect between CsPbBr3 and PCN-333(Fe).

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Engineering, Chemical

Integration of mixed ligand into a multivariate metal-organic framework for enhanced UV-light photocatalytic degradation of Rhodamine B

Jun-Cheng Jin et al.

Summary: The photocatalytic activity of a series of UIO-66 modified MOFs materials was evaluated for the degradation of Rhodamine B dye, with UiO-66-NO2/UiO-66-NH2 showing the best performance under UV light irradiation. The main reactive oxygen species generated during photocatalysis was found to be O-2(center dot-) radical anion. LC-MS experiments and band gap calculations confirmed the effectiveness of the strategy in enhancing photocatalytic efficiency for the degradation process.

JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS (2021)

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Article Engineering, Chemical

Construction of UiO-66@MoS2 flower-like hybrids through electrostatically induced self-assembly with enhanced photodegradation activity towards lomefloxacin

Di Gao et al.

Summary: A novel heterojunction photocatalyst, fabricated via a simple method, exhibited remarkable performance for the degradation of lomefloxacin hydrochloride under visible-light irradiation. Characterizations and photoelectrochemical property analysis confirmed its effective photocatalytic activity.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Chemical

Facile sonochemical synthesis of CdS/COF heterostructured nanocomposites and their enhanced photocatalytic degradation of Bisphenol-A

Chen Sun et al.

Summary: In this study, new CdS/COF heterostructured nanocomposites were synthesized using a facile sonochemical irradiation method and were found to have enhanced photocatalytic degradation performance towards BPA with the addition of COF. Among the prepared materials, 0.5 wt% CdS/COF exhibited the highest photocatalytic activity, with h(+) and center dot O-2(-) identified as the main active radicals in the photocatalytic reaction for BPA degradation. Additionally, 0.5 wt% CdS/COF showed photocatalytic stability and reusability in degrading BPA.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Biomedical

Acridine-Based Covalent Organic Framework Photosensitizer with Broad-Spectrum Light Absorption for Antibacterial Photocatalytic Therapy

Cuiping Zhang et al.

Summary: TPDA, an acridine-based COF photosensitizer, has been synthesized with multiple active sites and shows high antibacterial activities, wide optical absorption spectrum, and efficient protection against skin infections in fish within a short time.

ADVANCED HEALTHCARE MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Construction of Core-Shell MOF@COF Hybrids with Controllable Morphology Adjustment of COF Shell as a Novel Platform for Photocatalytic Cascade Reactions

Meng-Yao Zhang et al.

Summary: A successful strategy was proposed to enhance the photocatalytic performance by synthesizing Ti-MOF@TpTt hybrids, which demonstrated the potential in improving the photocatalytic ability of MOF@COF hybrid materials.

ADVANCED SCIENCE (2021)

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Article Multidisciplinary Sciences

On-Surface Bottom-Up Construction of COF Nanoshells towards Photocatalytic H2 Production

Yao Chen et al.

Summary: The rational design of an outer shell is crucial for enhancing the photocatalytic efficiency of core-shell structured photocatalysts. In this study, a covalent organic framework (COF) nanoshell was synthesized and deposited on the cadmium sulfide (CdS) core to improve light-harvesting and charge separation efficiency, leading to superior photocatalytic H-2 evolution compared to other COF-based photocatalysts. This framework nanoshell provides insights into advanced shell architecture design for coordinated charge and molecule transport in core-shell structured photocatalysts.

RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Surface-coordinated metal-organic framework thin films (SURMOFs): From fabrication to energy applications

Yi-Hong Xiao et al.

Summary: Metal-organic frameworks (MOFs) with liquid-phase epitaxial (LBL) growth on substrates surfaces, known as SURMOFs, offer controlled thickness, homogeneous film and preferred growth orientation, making them ideal candidates for energy storage and conversion. Different methods like layer by layer dipping, pump, spray, spin-coating and flowing techniques are used for SURMOFs fabrication, which find applications in electrocatalysis, photocatalysis and solar cells.

ENERGYCHEM (2021)

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Article Chemistry, Physical

A new strategy for constructing covalently connected MOF@COF core-shell heterostructures for enhanced photocatalytic hydrogen evolution

Hong-Yu Zhang et al.

Summary: A new strategy for constructing covalently linked MOF-COF hybrid materials by post-synthetic modification of metal nodes has been developed in this work, leading to enhanced efficiency of photocatalytic hydrogen evolution.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Environmental Sciences

High-Efficiency Photoenhanced Extraction of Uranium from Natural Seawater by Olefin-Linked Covalent Organic Frameworks

Wei-Rong Cui et al.

Summary: This study introduces a method of extracting uranium from seawater using COFs and proposes a novel COF (PT-BN-AO) with antibiofouling activity and enhanced uranium extraction capacity. The new COF demonstrates superior photocatalytic and photoelectric properties, increasing the uranium extraction capacity.

ACS ES&T WATER (2021)

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Review Chemistry, Multidisciplinary

Cobalt-based metal-organic frameworks for the photocatalytic reduction of carbon dioxide

Wanxia Zhang et al.

Summary: Metal-organic frameworks (MOFs) are porous materials with a large specific surface area and adjustable pore size. Cobalt-based MOFs face challenges in photocatalytic reduction of CO2, and current research focuses on methods to enhance catalytic performance and address associated challenges.

NANOSCALE (2021)

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Article Chemistry, Physical

Highly dispersed Ru nanoparticles on a bipyridine-linked covalent organic framework for efficient photocatalytic CO2 reduction

Ziling Liu et al.

Summary: The study successfully confines highly dispersed Ru nanoparticles in a photosensitizing COF, constructing composites with significantly enhanced activity for converting CO2 into valuable hydrocarbons efficiently.

SUSTAINABLE ENERGY & FUELS (2021)

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Article Chemistry, Physical

Interfacially synthesized 2D COF thin film photocatalyst: efficient photocatalyst for solar formic acid production from CO2 and fine chemical synthesis

Dolly Yadav et al.

Summary: The study successfully synthesized an efficient, recyclable covalent organic framework thin film photocatalyst with substantial stability and flexibility, and capable of multi-faceted photocatalysis under visible light.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Review Chemistry, Multidisciplinary

Amorphous inorganic semiconductors for the development of solar cell, photoelectrocatalytic and photocatalytic applications

Bing Wang et al.

Summary: Amorphous inorganic semiconductors have been increasingly studied for their unique properties in various applications such as solar cells and photocatalysis. While their success has been demonstrated, the underlying mechanisms remain unclear. There are promising prospects for further developments in the applications of amorphous inorganic semiconductors.

CHEMICAL SOCIETY REVIEWS (2021)

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Review Chemistry, Multidisciplinary

A review of the research status of CO2 photocatalytic conversion technology based on bibliometrics

Xiaopeng Li et al.

Summary: The bibliometric analysis reveals China's leading position in the field of carbon dioxide conversion, with a focus on the research status and challenges in photocatalytic CO2 conversion. Future development will be guided by the analysis results and existing issues.

NEW JOURNAL OF CHEMISTRY (2021)

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Review Multidisciplinary Sciences

Orderly Porous Covalent Organic Frameworks-based Materials: Superior Adsorbents for Pollutants Removal from Aqueous Solutions

Xiaolu Liu et al.

Summary: COFs are crystalline porous polymers known for their chemical stability and porosity, making them promising materials for removing toxic heavy metal ions, radionuclides, and organic pollutants efficiently. Various interaction mechanisms between pollutants and COF materials, as well as the adsorption properties of COF-based materials compared to other adsorbents, have been studied and summarized.

INNOVATION (2021)

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Review Chemistry, Physical

Recent advances on TiO2-based photocatalysts toward the degradation of pesticides and major organic pollutants from water bodies

Sofian Kanan et al.

CATALYSIS REVIEWS-SCIENCE AND ENGINEERING (2020)

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Article Chemistry, Multidisciplinary

Highly Stable Phosphonate-Based MOFs with Engineered Bandgaps for Efficient Photocatalytic Hydrogen Production

Zhu Yun-Pei et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Synthesis of bipyridine-based covalent organic frameworks for visible-light-driven photocatalytic water oxidation

Jian Chen et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Engineering, Environmental

Boosting visible-light hydrogen evolution of covalent-organic frameworks by introducing Ni-based noble metal-free co-catalyst

Hong Dong et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Review Chemistry, Multidisciplinary

Covalent Organic Frameworks: Design, Synthesis, and Functions

Keyu Geng et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Improved Photoreduction of CO2 with Water by Tuning the Valence Band of Covalent Organic Frameworks

Lu-jie Wang et al.

CHEMSUSCHEM (2020)

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Article Chemistry, Multidisciplinary

A Metal-Free Donor-Acceptor Covalent Organic Framework Photocatalyst for Visible-Light-Driven Reduction of CO2 with H2O

Kai Lei et al.

CHEMSUSCHEM (2020)

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Article Chemistry, Physical

Building Block Design for Minimizing Defects in the Construction of Two-Dimensional Covalent Organic Frameworks

You-Liang Zhu et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

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Article Chemistry, Physical

Insight into the Activity and Stability of RhXP Nano-Species Supported on g-C3N4 for Photocatalytic H2 Production

Hongjun Dong et al.

ACS CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

2D sp2 Carbon-Conjugated Porphyrin Covalent Organic Framework for Cooperative Photocatalysis with TEMPO

Ji-Long Shi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Physical

Covalent organic frameworks for photocatalytic applications

Qing Yang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Engineering, Environmental

Enhanced moisture-resistance and excellent photocatalytic performance of synchronous N/Zn-decorated MIL-125(Ti) for vaporous acetaldehyde degradation

Zhu Gao et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Engineering, Environmental

TiO2-UiO-66-NH2 nanocomposites as efficient photocatalysts for the oxidation of VOCs

Jinhui Zhang et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Engineering, Chemical

Photocatalytic Reduction and Recognition of Cr(VI): New Zn(II)-Based Metal-Organic Framework as Catalytic Surface

Harpreet Kaur et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Article Chemistry, Multidisciplinary

Donor-acceptor type [4+3] covalent organic frameworks: sub-stoichiometric synthesis and photocatalytic application

Qiaobo Liao et al.

SCIENCE CHINA-CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

New Core-Shell Hybrid Material IR-MOF3@COF-LZU1 for Highly Efficient Visible-Light Photocatalyst Degrading Nitroaromatic Explosives

Jun Zhao et al.

LANGMUIR (2020)

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Article Chemistry, Multidisciplinary

Covalent Organic Framework Hosting Metalloporphyrin-Based Carbon Dots for Visible-Light-Driven Selective CO2Reduction

Hong Zhong et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Ru Species Supported on MOF-Derived N-Doped TiO2/C Hybrids as Efficient Electrocatalytic/Photocatalytic Hydrogen Evolution Reaction Catalysts

Baolin Yan et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Modulating Benzothiadiazole-Based Covalent Organic Frameworks via Halogenation for Enhanced Photocatalytic Water Splitting

Weiben Chen et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Ionothermal Synthesis of Imide-Linked Covalent Organic Frameworks

Johannes Maschita et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Regenerable Covalent Organic Frameworks for Photo-enhanced Uranium Adsorption from Seawater

Wei-Rong Cui et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Solar-Driven Nitrogen Fixation Catalyzed by Stable Radical-Containing MOFs: Improved Efficiency Induced by a Structural Transformation

Kong-Qiu Hu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Energy & Fuels

Recent Progress on Exploring Stable Metal–Organic Frameworks for Photocatalytic Solar Fuel Production

Xu‐Sheng Wang et al.

Solar RRL (2020)

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Article Chemistry, Multidisciplinary

Rational Design of Covalent Cobaloxime-Covalent Organic Framework Hybrids for Enhanced Photocatalytic Hydrogen Evolution

Kerstin Gottschling et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Physical

Constructing electron delocalization channels in covalent organic frameworks powering CO2 photoreduction in water

Yonggang Xiang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Applied

De novo synthesis and particle size control of iron metal organic framework for diclofenac drug delivery

Pamela Berilyn So et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2020)

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Review Chemistry, Inorganic & Nuclear

Exchange reactions in metal-organic frameworks: New advances

Ming-Ming Xu et al.

COORDINATION CHEMISTRY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Metalloporphyrin-based covalent organic frameworks composed of the electron donor-acceptor dyads for visible-light-driven selective CO2reduction

Haowei Lv et al.

SCIENCE CHINA-CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

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