期刊
CHEMICAL COMMUNICATIONS
卷 58, 期 77, 页码 10861-10864出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc04199e
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资金
- Italian Association for Cancer Research (AIRC) [IG 25003]
- 'Departments of Excellence' program of the Italian Ministry for Education, University and Research (MIUR)
This study presents a novel strategy for NMR chemosensors by utilizing self-assembled cavity structures on silica nanoparticles. These nanohybrids demonstrate selective detection of physiologically relevant compounds through STD-based NMR experiments.
We report a strategy for the realization of NMR chemosensors based on the spontaneous self-assembly of lower rim pyridinium-functionalized tetraphopshonate cavitands on commercial silica nanoparticles. These nanohybrids enable the selective detection of physiologically relevant N-methylated amines, with a limit of detection of 31 mu M, via STD-based NMR experiments, achieving for the first time fine structural selectivity in nanoparticle-assisted NMR chemosensing.
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