☆ 4.8 Review

How membrane characteristics influence the performance of CO2 and CO electrolysis

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Review Chemistry, Multidisciplinary

Electrocatalysis in Alkaline Media and Alkaline Membrane-Based Energy Technologies

Yao Yang et al.

Summary: This article provides a comprehensive review of the fundamentals of electrocatalysis in alkaline media and its applications in alkaline-based energy technologies. Nonprecious anion exchange membrane fuel cells offer a promising alternative to proton exchange membrane fuel cells for sluggish oxygen reduction reaction. The understanding of proton-coupled electron transfer and active sites has contributed to the development of high-performance and durable alkaline fuel cells.

CHEMICAL REVIEWS (2022)

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Article Engineering, Chemical

Impact of side-chains in poly(dibenzyl-co-terphenyl piperidinium) copolymers for anion exchange membrane fuel cells

Hae Min Kim et al.

Summary: This study reports the use of side-chain-type s-PDTP copolymers as ionomers and membranes for anion exchange membrane fuel cells (AEMFCs). These copolymers exhibit high alkaline stability, excellent micromorphology, and high OH- conductivity. The ionomers with moderate ion-exchange-capacity and rational water uptake show optimal AEMFC performance.

JOURNAL OF MEMBRANE SCIENCE (2022)

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Review Energy & Fuels

Gas diffusion electrodes, reactor designs and key metrics of low-temperature CO2 electrolysers

David Wakerley et al.

Summary: Chemicals and fuels can be generated from CO2 via electrolysers that employ gas diffusion electrodes. This review discusses the key advances and remaining shortfalls of GDE-based CO2 electrolysers, as well as provides an overview of partial current densities, efficiencies, and stabilities achieved.

NATURE ENERGY (2022)

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Article Nanoscience & Nanotechnology

Three-Electrode Study of Electrochemical Ionomer Degradation Relevant to Anion-Exchange-Membrane Water Electrolyzers

Raina A. Krivina et al.

Summary: Anion-exchange-membrane water electrolyzers show promise for low-cost operation, but more research is needed to understand degradation and failure modes. Supporting electrolytes can improve performance and durability, but the interactions between anions and the ionomer membrane remain poorly understood.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Analytical

Measuring the alkaline stability of anion-exchange membranes

Saja Haj-Bsoul et al.

Summary: One significant barrier in developing durable anion-exchange membranes for fuel cells and water electrolyzers is their limited chemical stability to alkali. The commonly used ex-situ tests do not adequately simulate the actual operando conditions, yielding misleading degradation rates. The study introduces a unique ex-situ method for determining the alkaline stability of AEMs under in-situ operating environments and provides stability trends for various AEM compositions.

JOURNAL OF ELECTROANALYTICAL CHEMISTRY (2022)

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Article Engineering, Chemical

Evaluation of water states in thin proton exchange membrane manufacturing using terahertz time-domain spectroscopy

D. F. Alves-Lima et al.

Summary: Perfluorinated sulfonic-acid ionomers are commonly used proton exchange membrane materials, and understanding their structure is crucial for optimizing membrane performance. Terahertz time-domain spectroscopy can analyze water states and retention properties in membranes, and can be applied to thin ionomers. This technique enables rapid parameter space investigation for membrane optimization.

JOURNAL OF MEMBRANE SCIENCE (2022)

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Review Nanoscience & Nanotechnology

Gas diffusion electrodes and membranes for CO2 reduction electrolysers

Eric W. Lees et al.

Summary: This review explores material design strategies for controlling the transport of products and reactants in electrochemical reactors that convert CO2 emissions into chemicals and fuels, focusing on the design and development of gas diffusion electrodes (GDEs) and polymer electrolyte membranes tailored for the CO2 reduction reaction (CO2RR).

NATURE REVIEWS MATERIALS (2022)

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Article Chemistry, Physical

A microchanneled solid electrolyte for carbon-efficient CO2 electrolysis

Yi Xu et al.

Summary: The electrochemical reduction of CO2 has the potential to convert carbon emissions into valuable chemicals and fuels, but it currently suffers from low carbon efficiency. This study presents a microchanneled solid electrolyte that can capture and recycle carbonate ions before reaching the anode, resulting in a CO2 loss reduction of approximately 3%. By incorporating fixed quaternary ammonium cations, the selectivity for multi-carbon products reaches 77%.

JOULE (2022)

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Article Nanoscience & Nanotechnology

Urea-Functionalized Silver Catalyst toward Efficient and Robust CO2 Electrolysis with Relieved Reliance on Alkali Cations

Sahil Garg et al.

Summary: We have developed a new strategy to improve the reactivity and durability of a membrane electrode assembly (MEA)-type electrolyzer for CO2 electrolysis to CO. By modifying the silver catalyst layer with urea, we have successfully promoted electrochemical CO2 reduction (CO2R), relieved limitations of alkali cation transport, and mitigated salt precipitation in the gas diffusion electrode. The urea-modified Ag catalyst exhibited significantly better CO selectivity and energy efficiency than the untreated Ag catalyst, and maintained stable performance over 200 hours. Our work provides an alternative approach to fabricating catalyst interfaces in MEAs, with important implications for CO2 electrolysis and fuel cells.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Physical

Rigorous Evaluation of Liquid Products in High-Rate CO2/CO Electrolysis

Ming Ma et al.

Summary: In this work, the water crossover phenomenon in CO2 electrolysis is analyzed and its impact on the catalytic selectivity of liquid products is demonstrated. A reliable method for quantifying liquid products in high-rate CO2/CO electrolysis is proposed.

ACS ENERGY LETTERS (2022)

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Article Chemistry, Multidisciplinary

Local reaction environment for selective electroreduction of carbon monoxide

Ming Ma et al.

Summary: This study presents a simple experimental method to determine the local pH value in high-rate CO electroreduction by measuring the CO2 capture rate. It is found that an increased OH- concentration near the cathodic GDE surface can promote acetate formation and inhibit the formation of other C2+ products. High CO coverage is also found to be necessary for C2+ formation.

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Article Electrochemistry

Overview: State-of-the Art Commercial Membranes for Anion Exchange Membrane Water Electrolysis

Dirk Henkensmeier et al.

Summary: Water electrolysis is considered a promising method for storing and distributing large amounts of renewable energy, but current technologies face challenges such as high costs and scarce catalysts. Anion exchange membrane (AEM) water electrolysis is seen as a potential solution, with advantages including low cost, high operational capacity, and fast response times.

JOURNAL OF ELECTROCHEMICAL ENERGY CONVERSION AND STORAGE (2021)

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Review Engineering, Chemical

Bipolar membranes: A review on principles, latest developments, and applications

R. Parnamae et al.

Summary: Bipolar membranes (BPMs) are a special class of ion-exchange membranes that generate protons and hydroxide ions via water dissociation mechanism, finding applications in various sectors. Research and development in BPMs over the past two decades have led to a growing market and attention due to technical, environmental, and economic advancements. This review article provides an overview of BPM technology, discussing the current state of the art, properties, theoretical models, applications, optimization, fabrication advances, and potential novel applications.

JOURNAL OF MEMBRANE SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Monoclinic Scheelite Bismuth Vanadate Derived Bismuthene Nanosheets with Rapid Kinetics for Electrochemically Reducing Carbon Dioxide to Formate

Wenxiu Ma et al.

Summary: The study demonstrates the fabrication of bismuthene nanosheets as efficient electrocatalysts for CO(2) reduction to formate. The bismuthene nanosheets exhibit high formate Faradaic efficiency over a wide potential window, outperforming state-of-the-art electrocatalysts. Both experimental and theoretical investigations suggest that bismuthene nanosheets promote fast reaction kinetics towards formate production.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Next-generation anion exchange membrane water electrolyzers operating for commercially relevant lifetimes

Behrooz Motealleh et al.

Summary: The use of Sustainion (R) anion exchange membranes in alkaline anion exchange membrane water electrolysis has shown good performance relative to industrial parameters, with stability and longer lifetime. Accelerated voltage shock tests were used to simulate daily cycling performance over 30 years, showing that performance can be improved by adding zirconia to the polymer matrix and mechanically reinforcing the membrane.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Chemistry, Multidisciplinary

Improving the efficiency of CO2 electrolysis by using a bipolar membrane with a weak-acid cation exchange layer

Zhifei Yan et al.

Summary: This study investigates the effects of local environments on ionic flows in membrane electrolysers, and demonstrates the measurement and manipulation of local pH to improve CO₂ reduction efficiency.

NATURE CHEMISTRY (2021)

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Article Engineering, Chemical

Amphiphilic cone-shaped cationic calix[4]arene composite anion exchange membranes with continuous ionic channels

Wanting Chen et al.

Summary: The novel amphiphilic cone-shaped inducer TQCX is proposed to create continuous ionic channels in AEM, which improves hydroxide conductivity of the composite membrane. Molecular dynamics simulation reveals the mechanism of inducing ionic clusters and constructing continuous channels by TQCX, achieving a 70% improvement in hydroxide conductivity at 3 wt% TQCX.

JOURNAL OF MEMBRANE SCIENCE (2021)

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Article Chemistry, Physical

Carbonate Ion Crossover in Zero-Gap, KOH Anolyte CO2 Electrolysis

Peter Mardle et al.

Summary: The study demonstrates the importance of anolyte concentration and volume in determining the energetic conversion efficiency of a room-temperature zero-gap, KOH anolyte CO2 electrolyzer. Carbonate ion crossover is shown to significantly impact the ECell during continuous operation. Thicker and/or lower ion-exchange capacity variant membranes can reduce carbonate ion crossover by approximately 20%, which is crucial for the economic viability of direct CO2 electrolysis systems. Future membrane designs should focus on reducing carbonate crossover without compromising electrolyzer efficiency and stability.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Review Energy & Fuels

Designing anion exchange membranes for CO2 electrolysers

Danielle A. Salvatore et al.

Summary: New technologies are needed to efficiently convert carbon dioxide into fuels and chemicals at near-ambient temperatures and pressures. Anion exchange membranes in zero-gap reactors show promise for mediating the electrochemical CO2 reduction reaction, but challenges remain in tailoring these membranes to meet the requirements of CO2RR systems.

NATURE ENERGY (2021)

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Article Chemistry, Physical

Local Chemical Environment Governs Anode Processes in CO2 Electrolyzers

Adam Vass et al.

Summary: The electrolysis community aims to replace the commonly used Ir anode catalyst with a more abundant and stable material like Ni. However, despite Ni being considered a potential replacement, long-term operation reveals that Ni leads to rapid cell failure compared to Ir. This is due to a decrease in anolyte pH and the development of a detrimental chemical environment at the anode.

ACS ENERGY LETTERS (2021)

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Article Engineering, Chemical

Comb-shaped anion exchange membranes: Hydrophobic side chains grafted onto backbones or linked to cations?

Juanjuan Han et al.

Summary: The study found that the topology of comb-shaped anion exchange membranes has a significant impact on membrane properties, with membranes where side chains are grafted onto backbones showing better ion conduction and chemical stability compared to those with side chains tethered to cations. Increasing side chain length enhances the chemical stability of the membranes.

JOURNAL OF MEMBRANE SCIENCE (2021)

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Article Energy & Fuels

Operando cathode activation with alkali metal cations for high current density operation of water-fed zero-gap carbon dioxide electrolysers

B. Endrodi et al.

Summary: Precipitates that form in the cathode of continuous-flow CO2 electrolysers hinder their long-term operation, but the alkali metals they are formed from actually boost activity. Researchers address this dichotomy by periodically infusing the cathode with alkaline cations, enabling the electrolyser to operate stably and efficiently for extended periods.

NATURE ENERGY (2021)

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Article Thermodynamics

Temperature enhances the ohmic and mass transport behaviour in membrane electrode assembly carbon dioxide electrolyzers

Hisan W. Shafaque et al.

Summary: Increasing the operating temperature of a carbon dioxide electrolyzer can significantly reduce ohmic resistances and improve mass transport limitations, leading to higher performance. However, challenges such as the impact of liquid water in the electrode and product gas saturation at high temperatures should be considered.

ENERGY CONVERSION AND MANAGEMENT (2021)

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Article Multidisciplinary Sciences

CO2 electrolysis to multicarbon products in strong acid

Jianan Erick Huang et al.

Summary: Carbon dioxide electroreduction (CO2R) is being actively studied as a promising route to convert carbon emissions to valuable chemicals and fuels. A study found that concentrating potassium cations in the vicinity of electrochemically active sites accelerates CO2 activation to enable efficient CO2R in acid. The research achieved a high CO2R efficiency on copper at pH <1 with a single-pass CO2 utilization of 77%.

SCIENCE (2021)

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Article Multidisciplinary Sciences

Efficiency and selectivity of CO2 reduction to CO on gold gas diffusion electrodes in acidic media

Mariana C. O. Monteiro et al.

Summary: Large scale CO2 electrolysis to produce CO has traditionally been done in neutral and alkaline media, but recent research shows that it can also be achieved in acidic media with higher efficiency. Operating at current densities up to 200 mA cm(-2), CO faradaic efficiencies between 80-90% were obtained in sulfate electrolyte, representing a step towards the application of acidic electrolyzers for CO2 electroreduction.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Fast Bulky Anion Conduction Enabled by Free Shuttling Phosphonium Cations

Xiaolin Ge et al.

Summary: This study introduces an alternative polyrotaxane AEM with a non-tethered and free-shuttling phosphonium cation, which accelerates the diffusion conduction of bulky anions. The highly conductive nature of this membrane was achieved at a relatively lower ion-exchange capacity, showcasing its potential for new applications in ion conduction processes.

RESEARCH (2021)

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Editorial Material Chemistry, Physical

Cations play an essential role in CO2 reduction

Leanne D. Chen

Summary: Computational studies have hypothesized a vital role of cations in electrocatalysis, which is now supported by experimental evidence showing that CO2 reduction does not occur without cations.

NATURE CATALYSIS (2021)

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Article Chemistry, Physical

Absence of CO2 electroreduction on copper, gold and silver electrodes without metal cations in solution

Mariana C. O. Monteiro et al.

Summary: The study found that metal cations play a crucial role in stabilizing the CO2 intermediate during the reduction process on gold electrodes. Density functional theory simulations confirmed that partially desolvated metal cations enable the reduction by stabilizing the CO2- intermediate through short-range electrostatic interactions. In conclusion, the positively charged species from the electrolyte are key to stabilizing the crucial reaction intermediate.

NATURE CATALYSIS (2021)

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Article Chemistry, Physical

Electroosmotic flow steers neutral products and enables concentrated ethanol electroproduction from CO2

Rui Kai Miao et al.

Summary: By reversing the direction of ion and electroosmotic transport with a porous proton exchange layer, both convective and diffusive routes of ethanol loss are blocked, resulting in less than 1% ethanol crossover to the anode and achieving an ethanol concentration of 13.1 wt % directly from the cathode outlet.

JOULE (2021)

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Article Green & Sustainable Science & Technology

Techno-economic assessment of low-temperature carbon dioxide electrolysis

Haeun Shin et al.

Summary: This work provides a comprehensive techno-economic assessment of four major products of low-temperature CO2 electrolysis and prioritizes technological development with systematic guidelines to facilitate market deployment.

NATURE SUSTAINABILITY (2021)

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Article Materials Science, Multidisciplinary

Chemical upgrade of carbon monoxide to acetate on an atomically dispersed copper catalyst via CO-insertion

X. Fu et al.

Summary: This study reports a new synthetic strategy for atomically dispersing copper atoms on nitrogen-rich porous carbon, achieving high catalytic efficiency in electrochemical CO reduction. Different from the C-C coupling mechanism on metallic copper, a CO insertion mechanism is proposed for acetate production on the single site copper catalyst.

MATERIALS TODAY PHYSICS (2021)

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Review Chemistry, Multidisciplinary

Recent advances in innovative strategies for the CO2 electroreduction reaction

Xinyi Tan et al.

Summary: The CO2RR system faces limitations in practical applications due to low current density, poor CO2 utilization, and energy efficiency. To improve its performance, systematic consideration and optimization of each component are necessary. This review focuses on innovative design strategies for tandem catalysts, electrolytes, electrodes, and devices, as well as discussions on opportunities and challenges for future advancements in the CO2RR system.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Reducing the crossover of carbonate and liquid products during carbon dioxide electroreduction

Christopher McCallum et al.

Summary: A new numerical model combined with machine learning analysis was proposed to optimize MEA electrolyzers, achieving significant improvements in CO2 utilization and energy efficiency. Future research directions were also suggested based on the results.

CELL REPORTS PHYSICAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Rigorous assessment of CO2 electroreduction products in a flow cell

Zhuang-Zhuang Niu et al.

Summary: The study highlights the potential of flow-cell reactors in enhancing the efficiency of CO2 reduction reaction, but emphasizes the need for a standard testing methodology to ensure accurate product detection and fair performance comparisons. Through systematic experiments, the study identifies commonly overlooked factors in product measurements and proposes a modified testing system for accurate assessment of CO2RR products in flow cells.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Physical

The role of electrode wettability in electrochemical reduction of carbon dioxide

Mengran Li et al.

Summary: The wettability of the electrode plays a crucial role in CO2RR by affecting the reactivity, selectivity, and stability of the electrode. Improving cathode performance by altering the wettability of the catalyst layer in gas-diffusion electrodes can lead to more efficient CO2RR. Current challenges and opportunities lie in developing efficient and selective cathodes for CO2RR at industrially relevant rates.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Performance and stability comparison of Aemion™ and Aemion plus ™ membranes for vanadium redox flow batteries

Brian Shanahan et al.

Summary: This study evaluates the properties of two commercial AEMs, Aemion and Aemion+, and finds that Aemion+ features the best performance for vanadium redox-flow battery operation.

RSC ADVANCES (2021)

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Review Chemistry, Multidisciplinary

Regulating the oxidation state of nanomaterials for electrocatalytic CO2 reduction

Zhi-Zheng Wu et al.

Summary: Electrochemical carbon dioxide reduction reaction (CO2RR) converts CO2 into value-added chemicals and fuels, addressing renewable energy shortage and environmental pollution. Regulating the oxidation state of catalysts has been identified as an effective method for designing high-performing CO2RR catalysts that can influence catalyst activity and selectivity.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Orientation of a bipolar membrane determines the dominant ion and carbonic species transport in membrane electrode assemblies for CO2 reduction

Marijn A. Blommaert et al.

Summary: A bipolar membrane can be used in reverse bias and forward bias in an electrochemical cell. The orientation of the BPM affects the environment of the CO2 reduction catalyst and ion transport mechanism. Reverse bias reduces CO2 crossover and cathodic potential, while forward bias shows lower CO selectivity and higher salt concentration.

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Masa Hren et al.

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Comparative study of anion exchange membranes for low-cost water electrolysis

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Structure-transport relationships of poly(aryl piperidinium) anion-exchange membranes: Eeffect of anions and hydration

Xiaoyan Luo et al.

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High-performance alkaline water electrolysis using Aemion™ anion exchange membranes

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CO2 electrolysis to multicarbon products at activities greater than 1 A cm-2

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Managing Hydration at the Cathode Enables Efficient CO2 Electrolysis at Commercially Relevant Current Densities

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Accelerated discovery of CO2 electrocatalysts using active machine learning

Miao Zhong et al.

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Electrocatalytic reduction of CO2 to ethylene and ethanol through hydrogen-assisted C-C coupling over fluorine-modified copper

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Quantifying the critical effect of water diffusivity in anion exchange membranes for fuel cell applications

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Predicting the solvation structure and vehicular diffusion of hydroxide ion in an anion exchange membrane using nonreactive molecular dynamics simulation

Vikas Dubey et al.

CHEMICAL PHYSICS LETTERS (2020)

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Enhanced multi-carbon alcohol electroproduction from CO via modulated hydrogen adsorption

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The future of low-temperature carbon dioxide electrolysis depends on solving one basic problem

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Achieving High-Performance and 2000 h Stability in Anion Exchange Membrane Fuel Cells by Manipulating Ionomer Properties and Electrode Optimization

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Quantification of water transport in a CO2 electrolyzer

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ENERGY & ENVIRONMENTAL SCIENCE (2020)

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High carbonate ion conductance of a robust PiperION membrane allows industrial current density and conversion in a zero-gap carbon dioxide electrolyzer cell

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Understanding cation effects in electrochemical CO2 reduction (vol 12, pg 3001, 2019)

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Electrochemical CO2 reduction using alkaline membrane electrode assembly on various metal electrodes

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Hydroxide Ion Diffusion in Anion-Exchange Membranes at Low Hydration: Insights from Ab Initio Molecular Dynamics

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Molecular electrocatalysts can mediate fast, selective CO2 reduction in a flow cell

Shaoxuan Ren et al.

SCIENCE (2019)

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Multilayer Electrolyzer Stack Converts Carbon Dioxide to Gas Products at High Pressure with High Efficiency

B. Endrodi et al.

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Electrolyte Effects on the Electrochemical Reduction of CO2

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Alkaline polymer electrolyte fuel cells stably working at 80 °C

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Nanoporous Copper Silver Alloys by Additive-Controlled Electrodeposition for the Selective Electroreduction of CO2 to Ethylene and Ethanol

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Anion conducting multiblock copolymers with multiple head-groups

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High efficiency electrochemical reduction of CO2 beyond the two-electron transfer pathway on grain boundary rich ultra-small SnO2 nanoparticles

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The Alkaline Stability of Anion Exchange Membrane for Fuel Cell Applications: The Effects of Alkaline Media

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Quaternized aryl ether-free polyaromatics for alkaline membrane fuel cells: synthesis, properties, and performance - a topical review

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High Rate, Selective, and Stable Electroreduction of CO2 to CO in Basic and Neutral Media

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Bipolar Membranes Inhibit Product Crossover in CO2 Electrolysis Cells

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Anion Exchange Membranes' Evolution toward High Hydroxide Ion Conductivity and Alkaline Resiliency

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Understanding how high-performance anion exchange membrane fuel cells were achieved: Component, interfacial, and cell-level factors

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Technical photosynthesis involving CO2 electrolysis and fermentation

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High-rate electroreduction of carbon monoxide to multi-carbon products

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Synthesis and characterization of anion exchange multi-block copolymer membranes with a fluorine moiety as alkaline membrane fuel cells

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N-Spirocyclic Quaternary Ammonium lonenes for Anion-Exchange Membranes

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Poly(terphenylene) Anion Exchange Membranes: The Effect of Backbone Structure on Morphology and Membrane Property

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Cationic Side-Chain Attachment to Poly(Phenylene Oxide) Backbones for Chemically Stable and Conductive Anion Exchange Membranes

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Effect of Water on the Stability of Quaternary Ammonium Groups for Anion Exchange Membrane Fuel Cell Applications

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Hydrocarbon-Based Polymer Electrolyte Membranes: Importance of Morphology on Ion Transport and Membrane Stability

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N-Alkyl Interstitial Spacers and Terminal Pendants Influence the Alkaline Stability of Tetraalkylammonium Cations for Anion Exchange Membrane Fuel Cells

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One-step electrosynthesis of ethylene and ethanol from CO2 in an alkaline electrolyzer

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Anion-exchange membranes with polycationic alkyl side chains attached via spacer units

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Side-chain-type anion exchange membranes bearing pendant quaternary ammonium groups via flexible spacers for fuel cells

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Electrochemical generation of syngas from water and carbon dioxide at industrially important rates

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Electrolysis of CO2 to Syngas in Bipolar Membrane-Based Electrochemical Cells

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Synergistic Electrochemical CO2 Reduction and Water Oxidation with a Bipolar Membrane

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ACS ENERGY LETTERS (2016)

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Mechanically Tough and Chemically Stable Anion Exchange Membranes from Rigid-Flexible Semi-Interpenetrating Networks

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Structure-Property Relationships in Hydroxide-Exchange Membranes with Cation Strings and High Ion-Exchange Capacity

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Review Electrochemistry

The cathodic reduction of carbon dioxide-What can it realistically achieve? A mini review

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ELECTROCHEMISTRY COMMUNICATIONS (2015)

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Studies on Degradation of Copper Nano Particles in Cathode for CO2 Electrolysis to Organic Compounds

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A review of radiation-grafted polymer electrolyte membranes for alkaline polymer electrolyte membrane fuel cells

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Characterization and Chemical Stability of Anion Exchange Membranes Cross-Linked with Polar Electron-Donating Linkers

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A durable anion conducting membrane with packed anion-exchange sites and an aromatic backbone for solid-state alkaline fuel cells

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Fluorene-Based Hydroxide Ion Conducting Polymers for Chemically Stable Anion Exchange Membrane Fuel Cells

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A strategy to construct alkali-stable anion exchange membranes bearing ammonium groups via flexible spacers

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Alkaline Stability of Quaternary Ammonium Cations for Alkaline Fuel Cell Membranes and Ionic Liquids

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Use of Bipolar Membranes for Maintaining Steady-State pH Gradients in Membrane-Supported, Solar-Driven Water Splitting Michael

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Anion-exchange membranes in electrochemical energy systems

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Quaternized polybenzimidazoles with imidazolium cation moieties for anion exchange membrane fuel cells

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Hydroxide, halide and water transport in a model anion exchange membrane

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Absence of Schroeder's Paradox in a Nanostructured Block Copolymer Electrolyte Membrane

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Assessing the Effects of Crowding, Pore Size, and Interactions on Electro-Osmotic Drag Coefficients

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Base Stable Pyrrolidinium Cations for Alkaline Anion Exchange Membrane Applications

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Mechanistic analysis of ammonium cation stability for alkaline exchange membrane fuel cells

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Towards High Conductivity in Anion-Exchange Membranes for Alkaline Fuel Cells

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CHEMSUSCHEM (2013)

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A strategy for disentangling the conductivity-stability dilemma in alkaline polymer electrolytes

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Study on hydrophobicity degradation of gas diffusion layer in proton exchange membrane fuel cells

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ENERGY CONVERSION AND MANAGEMENT (2013)

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Water uptake, ionic conductivity and swelling properties of anion-exchange membrane

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JOURNAL OF POWER SOURCES (2013)

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Two-dimensional NMR spectroscopy reveals cation-triggered backbone degradation in polysulfone-based anion exchange membranes

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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2013)

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Electrodialytic Transport Properties of Anion-Exchange Membranes Prepared from Poly(vinyl alcohol) and Poly(vinyl alcohol-co-methacryloyl aminopropyl trimethyl ammonium chloride)

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MEMBRANES (2013)

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Transport properties of proton- and hydroxide-exchange membranes for fuel cells

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ELECTROCHIMICA ACTA (2012)

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Assessing the influence of different cation chemistries on ionic conductivity and alkaline stability of anion exchange membranes

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JOURNAL OF MATERIALS CHEMISTRY (2012)

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Sodium chloride sorption in sulfonated polymers for membrane applications

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JOURNAL OF MEMBRANE SCIENCE (2012)

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Hydroxide Degradation Pathways for Substituted Trimethylammonium Cations: A DFT Study

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JOURNAL OF PHYSICAL CHEMISTRY C (2012)

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Article Polymer Science

Subsecond Morphological Changes in Nafion during Water Uptake Detected by Small-Angle X-ray Scattering

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ACS MACRO LETTERS (2012)

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Hydration of NaHCO3, KHCO3, (HCO3-)2, HCO3- and CO32- from molecular dynamics simulation and speed of sound measurements

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CHEMICAL PHYSICS LETTERS (2011)

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Review Engineering, Chemical

Anion exchange membranes for alkaline fuel cells: A review

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JOURNAL OF MEMBRANE SCIENCE (2011)

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Calculation of Water Diffusion Coefficients in an Anion Exchange Membrane Using a Water Permeation Technique

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JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2011)

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Article Electrochemistry

Electrochemical Conversion of Carbon Dioxide to Formate in Alkaline Polymer Electrolyte Membrane Cells

S. R. Narayanan et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2011)

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Article Engineering, Chemical

Thickness dependence of water permeation through proton exchange membranes

Makoto Adachi et al.

JOURNAL OF MEMBRANE SCIENCE (2010)

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Article Engineering, Chemical

On the resistances of membrane, diffusion boundary layer and double layer in ion exchange membrane transport

Piotr Dlugolecki et al.

JOURNAL OF MEMBRANE SCIENCE (2010)

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Article Chemistry, Multidisciplinary

Tunable High Performance Cross-Linked Alkaline Anion Exchange Membranes for Fuel Cell Applications

Nicholas J. Robertson et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2010)

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Article Electrochemistry

Anion Exchange Membrane Fuel Cells: Experimental Comparison of Hydroxide and Carbonate Conductive Ions

Murat Unlu et al.

ELECTROCHEMICAL AND SOLID STATE LETTERS (2009)

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Article Electrochemistry

Evolution of Permanent Deformations (or Memory) in Nafion 117 Membranes with Changes in Temperature, Relative Humidity and Time, and Its Importance in the Development of Medium Temperature PEMFCs

G. Alberti et al.

FUEL CELLS (2009)

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Article Chemistry, Physical

Hydration of Ionomers and Schroeder's Paradox in Nafion

Viatcheslav Freger

JOURNAL OF PHYSICAL CHEMISTRY B (2009)

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Article Electrochemistry

Correlation of In Situ and Ex Situ Measurements of Water Permeation Through Nafion NRE211 Proton Exchange Membranes

Makoto Adachi et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2009)

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Review Electrochemistry

Chlor-alkali electrolysis with oxygen depolarized cathodes:: history, present status and future prospects

Imad Moussallem et al.

JOURNAL OF APPLIED ELECTROCHEMISTRY (2008)

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Article Engineering, Chemical

Current status of ion exchange membranes for power generation from salinity gradients

Piotr Dlugolecki et al.

JOURNAL OF MEMBRANE SCIENCE (2008)

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Article Electrochemistry

State of water in perfluorosulfonic ionomer (Nafion 117) proton exchange membranes

Zijie Lu et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2008)

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Article Electrochemistry

Design of an electrochemical cell making syngas (CO+H-2) from CO2 and H2O reduction at room temperature

Charles Delacourt et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2008)

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Article Chemistry, Multidisciplinary

Proton activity in Nafion films: Probing exchangeable protons with methylene blue

Brian Seger et al.

LANGMUIR (2007)

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Article Chemistry, Physical

Ab Initio molecular dynamics study of carbon dioxide and bicarbonate hydration and the nucleophilic attack of hydroxide on CO2

Kevin Leung et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2007)

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Article Engineering, Chemical

An experimental study of Schroeder's paradox in Nafion and Dowex polymer electrolytes

Maria Bass et al.

DESALINATION (2006)

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Article Physics, Condensed Matter

Neutron diffraction study on the hydration structure of carbonate ion by means of 12C/13C isotopic substitution method

Yasuo Kameda et al.

PHYSICA B-CONDENSED MATTER (2006)

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Article Chemistry, Multidisciplinary

Determination of the rate constants for the carbon dioxide to bicarbonate inter-conversion in pH-buffered seawater systems

KG Schulz et al.

MARINE CHEMISTRY (2006)

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Article Electrochemistry

Transport in polymer-electrolyte membranes - I. Physical model

AZ Weber et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2003)

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Article Multidisciplinary Sciences

The nature and transport mechanism of hydrated hydroxide ions in aqueous solution

ME Tuckerman et al.

NATURE (2002)

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Article Energy & Fuels

An overview of Biomass pyrolysis

A Demirbas et al.

ENERGY SOURCES (2002)

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