期刊
CHEMICAL COMMUNICATIONS
卷 58, 期 82, 页码 11583-11586出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc04032h
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资金
- Core Research for Evolutional Science and Technology of the Japan Science and Technology Agency [JPMJCR16P3, JP21H05011, JP21K14449]
- Japan Society for the Promotion of Science
High-silica CHA-type aluminosilicates were synthesized hydrothermally in the absence of fluoride media, with the seed-assisted aging treatment playing a crucial role in the crystallization. These aluminosilicates exhibited a long catalytic lifetime and high selectivity towards lower olefins in the methanol-to-olefins reaction.
High-silica CHA-type aluminosilicates (Si/Al molar ratio >100) were synthesized hydrothermally in the absence of fluoride media, where the seed-assisted aging treatment played an important role on the crystallization. These aluminosilicates showed a long catalytic lifetime with high selectivity toward lower olefins in the methanol-to-olefins reaction.
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