☆ 4.8 Review

Electrocatalytic Reduction of Carbon Dioxide to High-Value Multicarbon Products with Metal-Organic Frameworks and Their Derived Materials

ACS MATERIALS LETTERS (2022)

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Article Chemistry, Multidisciplinary

Highly Ethylene-Selective Electrocatalytic CO2 Reduction Enabled by Isolated Cu-S Motifs in Metal-Organic Framework Based Precatalysts

Chun Fang Wen et al.

Summary: Stable Cu-S motifs dispersed in a Cu-based metal-organic framework precatalyst can enhance the efficiency of converting CO2 to C2+ products. The presence of partially oxidized Cu delta+ species stabilized by the Cu-S motif during CO2RR leads to high ethylene selectivity and current density.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Dynamic Restructuring of Coordinatively Unsaturated Copper Paddle Wheel Clusters to Boost Electrochemical CO2 Reduction to Hydrocarbons**

Wei Zhang et al.

Summary: The study demonstrates that the defect-containing metal-organic framework can accelerate the electrochemical CO2 reduction reaction. By investigating the dynamic behavior of Cu-CPW, it is found to act as an active site in the deep CO2 reduction reaction.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Imparting CO2 Electroreduction Auxiliary for Integrated Morphology Tuning and Performance Boosting in a Porphyrin-based Covalent Organic Framework

Yi-Rong Wang et al.

Summary: This study has successfully prepared COF nanosheets with superior performance using a functionalizing exfoliation agent, providing a new possibility for the development of efficient CO2 electroreduction catalysts.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Review Chemistry, Multidisciplinary

MOF-enabled confinement and related effects for chemical catalyst presentation and utilization

Jian Liu et al.

Summary: This review focuses on how porous, catalyst-containing MOFs utilize molecular-scale confinement to regulate reactant and product transport, catalyst activity, and stability, to achieve desired chemical transformations with superior selectivity or efficacy compared to catalysts in homogeneous solution environments.

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Review Chemistry, Inorganic & Nuclear

Mixed component metal-organic frameworks: Heterogeneity and complexity at the service of application performances

Marta Viciano-Chumillas et al.

Summary: The synthesis of mixed-component metal-organic frameworks (MOFs) is a rapidly growing research field, offering unique possibilities to incorporate multiple functionalities and properties that are not simply the sum of each component. Despite challenges, promising ways to utilize the intrinsic properties of mixed-components MOFs for breakthroughs in catalysis and nanotechnology are presented through exemplary cases.

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Article Chemistry, Multidisciplinary

Preparation of Au@Pd Core-Shell Nanorods with fcc-2H-fcc Heterophase for Highly Efficient Electrocatalytic Alcohol Oxidation

Xichen Zhou et al.

Summary: The Au@Pd core-shell nanorods with a unique fcc-2H-fcc heterophase exhibit superior electrocatalytic ethanol oxidation performance, contributing to insights into the catalytic mechanism. The exceptional performance of the heterophase Au@Pd nanorods is attributed to the unconventional 2H phase, the 2H/fcc phase boundary, and the lattice expansion of the Pd shell.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Multidisciplinary

Surface Molecular Functionalization of Unusual Phase Metal Nanomaterials for Highly Efficient Electrochemical Carbon Dioxide Reduction under Industry-Relevant Current Density

Juan Wang et al.

Summary: The surface molecular functionalization of metal nanorods has been shown to improve the performance of electrochemical CO2 reduction reaction by enhancing selectivity and current density. This method can be extended to other nanomaterials and derivatives to boost performance.

SMALL (2022)

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Article Multidisciplinary Sciences

Au-activated N motifs in non-coherent cupric porphyrin metal organic frameworks for promoting and stabilizing ethylene production

Xulan Xie et al.

Summary: This study demonstrates the successful insertion of Au nanoneedles into a metalloporphyrin framework, resulting in activated C-C coupling and enhanced ethylene production. The modulation of the metalloporphyrin structure by metal impregnation allows for control of the CO2 reduction reaction pathway.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Multidisciplinary

Decreasing the Overpotential of Aprotic Li-CO2 Batteries with the In-Plane Alloy Structure in Ultrathin 2D Ru-Based Nanosheets

Yunhao Wang et al.

Summary: This work presents a facile one-pot solvothermal method for the synthesis of ultrathin 2D Ru-M (M = Co, Ni, and Cu) nanosheets, which can be used as cathode catalysts for Li-CO2 batteries. The RuCo nanosheets demonstrate excellent catalytic performance with low charge voltage, small overpotential, and high energy efficiency. The study indicates the feasibility of improving the electrochemical performance of Li-CO2 batteries through the in-plane metal alloy sites of ultrathin 2D alloy nanomaterials.

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Article Chemistry, Multidisciplinary

Confined Growth of Silver-Copper Janus Nanostructures with {100} Facets for Highly Selective Tandem Electrocatalytic Carbon Dioxide Reduction

Yangbo Ma et al.

Summary: This study reports the synthesis of highly selective Ag-Cu Janus nanostructures for the electrocatalytic reduction of CO2 to multicarbon products. The Ag-Cu Janus nanostructures demonstrated superior selectivity and performance compared to Cu nanocubes. The study provides an effective strategy for designing advanced catalysts for the extensive application of CO2RR.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Flexible Cuprous Triazolate Frameworks as Highly Stable and Efficient Electrocatalysts for CO2 Reduction with Tunable C2H4/CH4 Selectivity

Lin-Ling Zhuo et al.

Summary: Flexible Cu(I) triazolate frameworks have been developed as efficient and stable electrocatalysts for CO2 reduction. By changing the size of the ligand side groups, the selectivity ratio of C2H4/CH4 can be tuned and inverted, leading to high selectivities of C2H4, CH4, and hydrocarbons. Computational simulations revealed the structural changes and cooperative interactions of Cu(I) during the reaction, and the ligand side groups played a critical role in controlling catalyst flexibility and selectivity.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Review Chemistry, Physical

Design concept for electrocatalysts

Yao Wang et al.

Summary: Metal-based electrocatalysts with different sizes have shown different catalytic behaviors, and regulating the coordination environment of active sites is crucial for designing efficient electrocatalysts. This review summarizes the recent progress in heterogeneous supported single atoms, nanoclusters, and nanoparticles catalysts, proposing key factors for enhancing electrocatalytic performance and discussing current challenges and future opportunities in this field.

NANO RESEARCH (2022)

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Article Chemistry, Multidisciplinary

Transient Solid-State Laser Activation of Indium for High-Performance Reduction of CO2 to Formate

Weihua Guo et al.

Summary: The limited understanding of the local environment of active sites and synthetic skills hinder the delivery of industrially-relevant current densities with low overpotentials and high selectivity for CO2 reduction. This study presents a method using transient laser induction of metal salts to produce defect-rich indium nanoparticles (L-In) with extreme conditions and rapid kinetics. These L-In nanoparticles exhibit a small onset overpotential and high current density in a flow cell, with a formate Faradaic efficiency of 98%. The formation rate of formate is significantly higher than previous results, outperforming commercial indium. This study suggests that transient solid-state laser induction provides a facile and cost-effective approach to tailor the activity of ligand-free and defect-rich materials.

SMALL (2022)

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Article Chemistry, Physical

PtCu@Ir-PCN-222: Synergistic Catalysis of Bimetallic PtCu Nanowires in Hydrosilane-Concentrated Interspaces of an Iridium(III)-Porphyrin-Based Metal-Organic Framework

Chunying Chen et al.

Summary: In this study, a series of porphyrinic metal-organic framework composites encapsulated with bimetallic PtCu nanowires were synthesized and investigated for their catalytic performance in Si-H bond functionalization. The results showed that PtCu@Ir-PCN-222 exhibited efficient catalytic activity for the hydrolytic oxidation of hydrosilane and CO2 hydrosilylation. Theoretical studies revealed the interaction between Ir(III) porphyrin and hydrosilane, as well as the high Si-H activation ability of PtCu alloys.

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Article Chemistry, Multidisciplinary

A Porous p-p Stacking Framework with Dicopper(I) Sites and Adjacent Proton Relays for Electroreduction of CO2 to C2+ Products

Hao-Lin Zhu et al.

Summary: In this study, a stable pi-pi stacking framework was reported for electrochemical CO2 reduction, showing impressive performance with high Faradaic efficiency for C2+ products. In-situ infrared spectroscopy, density functional theory calculations, and control experiments revealed the mechanism of hydrogenation and C-C coupling in this framework.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Efficient Electrocatalytic Reduction of CO2 to Ethane over Nitrogen-Doped Fe2O3

Peng Chen et al.

Summary: This study reports a novel nitrogen-doped gamma-Fe2O3 electrocatalyst that can efficiently generate ethane in electrochemical reactions. The results showed that the enrichment of oxygen vacancies in the FeO1.5-nNn sites of the catalyst stabilized reaction intermediates and facilitated the generation of ethane by lowering the reaction energy barrier. This work provides a strategy for the design of efficient CO2 reduction catalysts.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Understanding the structure-performance relationship of active sites at atomic scale

Runze Li et al.

Summary: This article discusses the key factors affecting the catalytic performance of metal-based atomically dispersed catalysts and their relationship with the active sites. It first introduces the effectiveness of active site design through coordination effects, then discusses the role of chemical bonds in the active sites and the influence of the spacing of active atoms in intermetallic compounds on catalytic behavior. Additionally, the importance of synergistic effects in catalyst design is emphasized, and the key parameters affecting catalytic performance at the atomic scale are summarized.

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Article Chemistry, Multidisciplinary

Freestanding 2D NiFe Metal-Organic Framework Nanosheets: Facilitating Proton Transfer via Organic Ligands for Efficient Oxygen Evolution Reaction

Yizhe Liu et al.

Summary: A novel LDHs-assisted approach is developed to synthesize freestanding bimetallic 2D metal-organic framework nanosheets (2D MOF NSs) with outstanding activities and proton transfer ability in the oxygen evolution reaction (OER).

SMALL (2022)

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Article Chemistry, Physical

A Stable and Low-Cost Metal-Azolate Framework with Cyclic Tricopper Active Sites for Highly Selective CO2 Electroreduction to C2+ Products

Da-Shuai Huang et al.

Summary: This study demonstrates a stable and low-cost metal-azolate framework as an efficient and selective electrocatalyst for the reduction of CO2 into multicarbon (C-2(+)) products. The catalyst exhibits remarkable performance and can be synthesized on a large scale under environmentally benign conditions.

ACS CATALYSIS (2022)

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Review Chemistry, Multidisciplinary

2D π-conjugated metal organic frameworks for CO2 electroreduction

Deren Yang et al.

Summary: Electrochemical conversion of CO2 into valuable chemicals and fuels is a promising route to utilize CO2 source. Nano-level or atomic-level catalyst design has been extensively researched to improve the efficiency and durability of CO2 conversion. Metal-organic frameworks (MOFs) offer new opportunities for CO2 reduction catalysts by integrating the advantages of traditional catalysts and single-atom catalysts. This review summarizes recent advances in 2D pi-conjugated MOF catalysts and their practical applications in CO2 reduction reactions.

SMARTMAT (2022)

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Article Chemistry, Physical

Metal-Organic Framework-Based Electrocatalysts for CO2 Reduction

Syed Shoaib Ahmad Shah et al.

Summary: Metal-organic frameworks (MOFs) are a promising class of electrocatalysts for CO2 reduction, characterized by high porosity and large surface area. By enhancing performance, exploring the structure-activity relationship, and employing specific structure tuning strategies, novel catalysts can be designed effectively.

SMALL STRUCTURES (2022)

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Article Chemistry, Multidisciplinary

Highly Ethylene-Selective Electrocatalytic CO2 Reduction Enabled by Isolated Cu-SMotifs in Metal-Organic Framework Based Precatalysts

Chun Fang Wen et al.

Summary: In this study, a strategy based on local sulfur doping of a Cu-based metal-organic framework precatalyst was developed for enhancing ethylene selectivity in the CO2 reduction reaction. Experimental and theoretical studies showed that the Cu-S motif played a key role in the catalytic process of the precatalyst.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

A 3D Cu-Naphthalene-Phosphonate Metal-Organic Framework with Ultra-High Electrical Conductivity

Craig A. Peeples et al.

Summary: The conductive phosphonate metal-organic framework, TUB40, exhibits high electrical conductance and a unique structure, making it a promising electrode material for supercapacitors.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Inorganic & Nuclear

A historical perspective on porphyrin-based metal-organic frameworks and their applications

Xuan Zhang et al.

Summary: Porphyrins are important molecules widely found in nature, and recent interest in using them as building blocks for metal-organic frameworks has increased rapidly. Porphyrin-based MOFs with atomically precise structures provide an ideal platform for studying structure-function relationships in the solid state without compromising the inherent properties of the porphyrin building blocks.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Multidisciplinary Sciences

Precise fabrication of single-atom alloy co-catalyst with optimal charge state for enhanced photocatalysis

Yating Pan et al.

Summary: Metal-organic framework (MOF) stabilized bimetallic Pd@Pt nanoparticles with adjustable Pt coordination environment and controlled structure from core-shell to single-atom alloy (SAA) have been fabricated. It was found that Pt surface charge regulation can be achieved by changing its coordination environment and the structure of the Pd@Pt co-catalyst, redistributing the charge between Pd and Pt. The optimized Pd-10@Pt-1/MOF composite, featuring an unprecedented SAA co-catalyst, exhibits exceptionally high photocatalytic hydrogen production activity surpassing its corresponding counterparts.

NATIONAL SCIENCE REVIEW (2021)

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Review Nanoscience & Nanotechnology

Generating Catalytic Sites in UiO-66 through Defect Engineering

Xiao Feng et al.

Summary: UiO-66 is considered as an epitome of metal-organic frameworks (MOFs) due to its stability and capability to withstand high numbers of defects without structural collapse. Numerous studies have focused on constructing catalytic sites in UiO-66 through defect engineering to enhance performance.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Predesign of Catalytically Active Sites via Stable Coordination Cluster Model System for Electroreduction of CO2 to Ethylene

Yun-Feng Lu et al.

Summary: In this study, three crystalline trinuclear copper clusters were designed as catalysts for the selective electroreduction of CO2 to C2H4, showing high selectivity and adjustable efficiency by replacing counter anions. DFT calculations confirmed that the designed catalysts facilitate the C-C coupling of identical intermediates, leading to the formation of symmetrical C2H4 products in a sustainable way.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Synergetic Cobalt-Copper-Based Bimetal-Organic Framework Nanoboxes toward Efficient Electrochemical Oxygen Evolution

Weiren Cheng et al.

Summary: Novel CoCu-based bimetallic metal-organic framework nanoboxes (CoCu-MOF NBs) were reported as promising catalysts for efficient electrochemical oxygen evolution reaction (OER), showing excellent activity and stability. The high OER activity of CoCu-MOF NBs is believed to be attributed to the post-formed CoCu-based oxyhydroxide analogue during OER, which promotes fast OER kinetics through electronic synergy between Co and neighbouring Cu atoms.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Rational Fabrication of Low-Coordinate Single-Atom Ni Electrocatalysts by MOFs for Highly Selective CO2 Reduction

Yan Zhang et al.

Summary: A single-atom Ni catalyst with different N coordination numbers was fabricated using a post-synthetic metal substitution strategy. The Ni-N-3-C catalyst showed significantly enhanced COOH* formation leading to accelerated CO2 reduction, achieving high CO Faradaic efficiency and excellent performance in Zn-CO2 battery. This work provides a new approach for modulation of coordination microenvironment in single-atom catalysts for CO2 utilization.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Metal-Organic-Framework-Supported Molecular Electrocatalysis for the Oxygen Reduction Reaction

Zuozhong Liang et al.

Summary: Synthesizing metal-organic framework (MOF)-supported Co porphyrins for the oxygen reduction reaction (ORR) leads to improved activity and selectivity. The grafted Co porphyrins show boosted ORR activity and improved selectivity for the 4e ORR, demonstrating potential for application as air electrode catalysts in Zn-air batteries.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Multidisciplinary Sciences

Insights on forming N,O-coordinated Cu single-atom catalysts for electrochemical reduction CO2 to methane

Yanming Cai et al.

Summary: Single-atom catalysts are promising for catalyzing CO2 reduction to produce high value hydrocarbons, but most reactions yield CO. In this study, a low-temperature calcining process was used to fabricate a carbon-dots-based SAC which efficiently converts CO2 to methane.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

2D Copper Tetrahydroxyquinone Conductive Metal-Organic Framework for Selective CO2 Electrocatalysis at Low Overpotentials

Leily Majidi et al.

Summary: A 2D copper-based conductive MOF, Cu-THQ, exhibits excellent catalytic activity for aqueous CO2 reduction reaction (CO2RR) with low overpotentials. The material shows high CO production rate and current density at low overpotentials, making it a promising candidate for practical applications in CO2RR.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Pristine Hollow Metal-Organic Frameworks: Design, Synthesis and Application

Tianjie Qiu et al.

Summary: Metal-organic frameworks (MOFs), with their versatile and highly tunable compositions and structures, show promise in constructing complex hollow nanocomposites with enhanced properties and designability. They are considered as promising building units for fabricating materials with faster mass transport, multiple active components, more exposed active sites, and better compatibility compared to bulk MOFs.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Multidisciplinary

Two-Dimensional Metal-Organic Framework Materials: Synthesis, Structures, Properties and Applications

Gouri Chakraborty et al.

Summary: Porous layered coordination polymers (CPs) in the field of metal-organic frameworks (MOFs) have gained attention for their modular nature and tunable structures, enabling various applications such as gas adsorption, storage, and catalysis. 2D MOFs are known for their ultrathin nanosheets similar to graphene, making them useful for technological applications.

CHEMICAL REVIEWS (2021)

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Article Chemistry, Multidisciplinary

Enhanced Cuprophilic Interactions in Crystalline Catalysts Facilitate the Highly Selective Electroreduction of CO2 to CH4

Lei Zhang et al.

Summary: Cu(I)-based catalysts are essential for the electrocatalytic CO2 reduction, and in this study, two stable copper(I)-based catalysts with inherent cuprophilic interactions were synthesized for highly selective CO2-to-CH4 conversion. The substitution of sulfate radicals with hydroxyl radicals led to a dynamic crystal structure transition, enhancing the cuprophilic interactions inside the catalyst structure. The enhanced cuprophilic interactions in NNU-33(H) showed outstanding CH4 selectivity, representing the best crystalline catalyst for electrocatalytic CO2-to-CH4 conversion.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Review Chemistry, Multidisciplinary

Metal-Organic Frameworks Derived Functional Materials for Electrochemical Energy Storage and Conversion: A Mini Review

Xue Feng Lu et al.

Summary: Metal-organic frameworks (MOFs) have been recognized as versatile precursors or templates for preparing high-performance electrodes or catalysts in electrochemical energy storage and conversion (EESC), due to their high surface area, tunable pore sizes, and diverse chemical compositions and physical structures. Research focuses on the composition/structure/performance relationship and practical applications in various EESC systems, providing insights into the future development of MOF-derived functional materials.

NANO LETTERS (2021)

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Article Chemistry, Physical

Interface-Enhanced Catalytic Selectivity on the C2 Products of CO2 Electroreduction

Zhen Li et al.

Summary: By using a nitrogen-doped carbon overlayer on the Cu surface, the selectivity and efficiency of the CO2 reduction reaction can be significantly improved, directing towards valuable products such as ethylene and ethanol. Additionally, the overlayer also protects the stability of the copper substrate.

ACS CATALYSIS (2021)

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Article Multidisciplinary Sciences

Promoting ethylene production over a wide potential window on Cu crystallites induced and stabilized via current shock and charge delocalization

Hao Sun et al.

Summary: The substrate-catalyst interaction plays a critical role in steering the pathway of electrochemical CO2 reduction. Here the authors show the crystalline states of copper in reconstructed metal-organic frameworks were induced and stabilized by Ketjen Black conducting support, promoting C2H4 production.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4

Yu Zhang et al.

Summary: The study demonstrates that the ECR selectivity depends strongly on the Cu site coordination environment in crystalline porous catalysts, with Cu-DBC showing higher selectivity and activity due to the lower energy barriers of Cu-O-4 sites during the ECR process. This provides a platform for constructing highly selective ECR catalysts with potential applications in the energy conversion field.

NATURE COMMUNICATIONS (2021)

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Efficient propyne/propadiene separation by microporous crystalline physiadsorbents

Yun-Lei Peng et al.

Summary: This study introduces a physisorptive approach using microporous metal-organic frameworks for the selective separation of propyne/propadiene mixtures. Experimental results demonstrate that MOFs with open metal sites and cage-based molecule traps exhibit high performance for propyne/propadiene separation.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Cu-MOFs Derived Porous Cu Nanoribbons with Strengthened Electric Filed for Selective CO2 Electroreduction to C2+ Fuels

Hang Huo et al.

Summary: Constructing mesoporous Cu nanoribbons through in-situ electrochemical reduction of Cu-based metal organic frameworks allows for achieving a high C2+ Faradaic efficiency of 82.3% in a flow-cell electrolyzer, demonstrating excellent selectivity for synthesizing C2+ chemicals.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Design Strategies for Enhanced Conductivity in Metal-Organic Frameworks

Eric M. Johnson et al.

Summary: Metal-organic frameworks (MOFs) are a class of materials with permanent porosity, high surface area, and crystallinity, offering potential for a wide range of applications, particularly in conductive materials. The continued development of conductive MOFs has led to a growing library of materials with conductivity, while factors affecting conductivity in MOFs have become more apparent. Pathways to enhance conductivity across a variety of MOF structures are being explored in fundamental studies derived from proposed methods.

ACS CENTRAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Integration of Pd nanoparticles with engineered pore walls in MOFs for enhanced catalysis

Luyan Li et al.

Summary: The study encapsulated naked Pd nanoparticles in a metal-organic framework (MOF) to regulate Pd microenvironment and interactions with substrates, resulting in significantly improved activity and selectivity in organic silane dehydrogenation coupling and hydrogenation of halogenated nitrobenzenes. This approach surpasses traditional methods, indicating the potential of metal NPs@MOF composites for efficiently integrating well-accessible metal sites with engineered microenvironments.

CHEM (2021)

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Article Chemistry, Multidisciplinary

Designing MOF Nanoarchitectures for Electrochemical Water Splitting

Ben Zhang et al.

Summary: This paper presents the most pivotal advances in engineering MOF nanoarchitectures for efficient electrochemical water splitting. It summarizes the design of catalytic centers for MOF-based/derived electrocatalysts and discusses breakthroughs in catalytic activities, identification of highly active sites, and fundamental mechanisms. Additionally, it provides comprehensive commentary on current primary challenges and future perspectives in water splitting and its commercialization for hydrogen production.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

The Current Status of MOF and COF Applications

Ralph Freund et al.

Summary: The amalgamation of different disciplines at the heart of reticular chemistry has broadened the boundaries of chemistry. Reticular design enables precise prediction of crystalline framework structures, tunability of chemical composition, and fine-tuning of material properties in metal-organic frameworks and covalent organic frameworks. Leveraging the unique properties of reticular materials has led to significant advances in both fundamental and applied research.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Zwitterionic ultrathin covalent organic polymers for high-performance electrocatalytic carbon dioxide reduction

Yun Song et al.

Summary: Covalent organic polymers are emerging as electrode materials for CO2 reduction reactions, with a new ultrathin COP material reported here showing high CO conversion efficiency and excellent stability due to its unique structure and electronic effects.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Multidisciplinary

Highly Selective CO2 Electroreduction to C2H4 Using a Metal-Organic Framework with Dual Active Sites

Xiao-Feng Qiu et al.

Summary: In this study, a metal-organic framework (PcCu-Cu-O) was reported as an electrocatalyst for converting CO2 to C2H4, showing higher efficiency compared to discrete molecular copper-phthalocyanine. In-situ infrared spectroscopy and control experiments indicated that the synergistic effect between the CuPc unit and the CuO4 unit contributes to lowering the energy barrier for C-C dimerization.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Review Chemistry, Physical

Tandem catalysis in electrochemical CO2 reduction reaction

Yating Zhu et al.

Summary: Electrochemical CO2 reduction through tandem catalysis has shown promise in enhancing efficiency, with limitations primarily due to high overpotential and poor selectivity in producing highly reduced carbon compounds. Recent advances in tandem catalysis for CO2RR have provided effective methods to improve performance, indicating potential for further research and development.

NANO RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Cu/Cu2O Interconnected Porous Aerogel Catalyst for Highly Productive Electrosynthesis of Ethanol from CO2

Chansol Kim et al.

Summary: The study introduced a novel porous Cu/Cu2O aerogel network to achieve high ethanol productivity by electrocatalytic CO2RR, showing promising potential for ethanol production. Experimental results demonstrated that the aerogel produced ethanol as the major product and exhibited excellent electrosynthesis performance.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Recent Progresses in Electrochemical Carbon Dioxide Reduction on Copper-Based Catalysts toward Multicarbon Products

Jinli Yu et al.

Summary: Electrochemical carbon dioxide reduction reaction offers a promising way of converting CO2 to value-added chemicals, but the conversion to more valuable multicarbon products remains challenging. Recent progress in using copper-based catalysts for electrochemical CO2 reduction to multicarbon products is reviewed, with a focus on catalyst engineering and cell engineering approaches.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Conductive Two-Dimensional Phthalocyanine-based Metal-Organic Framework Nanosheets for Efficient Electroreduction of CO2

Jun-Dong Yi et al.

Summary: Metal-organic frameworks (MOFs) are promising alternatives for CO2RR due to their periodic arrangement of isolated metal active sites, but traditional MOFs have poor conductivity. Researchers have prepared conductive 2D phthalocyanine-based MOF nanosheets, which exhibit a high efficiency and selectivity for CO production.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Phosphorus Induced Electron Localization of Single Iron Sites for Boosted CO2 Electroreduction Reaction

Xiaohui Sun et al.

Summary: In this study, the introduction of single P atoms was found to enhance the performance of a single Fe atom catalyst in the electrochemical reduction of CO2. Experimental and computational analysis revealed that the presence of single P atoms improved the electronic localization of Fe center, leading to the stabilization of the key *COOH intermediate and enhanced CO2 electrochemical reduction performance.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Partial Coordination-Perturbed Bi-Copper Sites for Selective Electroreduction of CO2 to Hydrocarbons

Rui Wang et al.

Summary: This study developed a stable crystalline single-chain catalyst model system for systematically investigating the influence of synergistic effects on the selective generation of products in the electrochemical CO2RR.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Implanting Numerous Hydrogen-Bonding Networks in a Cu-Porphyrin-Based Nanosheet to Boost CH4 Selectivity in Neutral-Media CO2 Electroreduction

Yi-Rong Wang et al.

Summary: This study successfully utilized a Cu-porphyrin-based large-scale and ultrathin nanosheet as an electrocatalyst for CO2RR, achieving high CO2 conversion efficiency under neutral conditions. By constructing hydrogen-bonding networks, proton migration and intermediate stabilization were facilitated, providing a new pathway for efficient CO2RR catalyst development.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

A Facile Strategy for Constructing a Carbon-Particle-Modified Metal-Organic Framework for Enhancing the Efficiency of CO2 Electroreduction into Formate

Zi-Hao Zhu et al.

Summary: A stable porous 3D In-MOF V11 was constructed with two types of channels, exhibiting moderate catalytic activity in CO2 electroreduction. By introducing suitable molecules transformed into carbon particles, the efficiency of electroreduction was significantly improved, demonstrating the universality of this method in enhancing CO2 conversion.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Inorganic & Nuclear

Recent advances in the development of electronically and ionically conductive metal-organic frameworks

Guangxun Zhang et al.

Summary: Metal-organic frameworks (MOFs) have gained increasing attention as porous materials and are widely applied in various fields, but their low conductivity hinders their development. Strategic modulation of the conductive properties of MOFs is needed to achieve optimal performance and broad applications.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Chemistry, Multidisciplinary

A New Hexagonal Cobalt Nanosheet Catalyst for Selective CO2 Conversion to Ethanal

Jie Yin et al.

Summary: A new form of catalyst using ferromagnetic hexagonal-close-packed (hcp) Co nanosheets has been developed for selective reduction of CO2 to ethanal. Through experimental testing and density functional theory (DFT) calculations, it was found that the unique intralayer electron transfer on the hcp Co surface promotes selective formation of ethanal by suppressing complete hydrogenation of intermediate products.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Physical

Highly Efficient Electroconversion of CO2 into CH4 by a Metal-Organic Framework with Trigonal Pyramidal Cu(I)N3 Active Sites

Hao-Lin Zhu et al.

Summary: In this study, a Cu-based metal-organic framework was introduced as a catalyst for the efficient and selective reduction of CO2 to CH4. The in situ-generated trigonal pyramidal Cu(I)N-3 was identified as the electrochemical active site, while the hydrogen-bonding interactions of adjacent aromatic hydrogen atoms played a key role in stabilizing key intermediates of carbon dioxide reduction and inhibiting the hydrogen evolution reaction, demonstrating a high performance in electroreduction of CO2 to CH4.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Metal-Organic Frameworks for Electrocatalysis: Catalyst or Precatalyst?

Weiran Zheng et al.

ACS ENERGY LETTERS (2021)

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Review Chemistry, Physical

Recent Progress on Two-Dimensional Materials

Cheng Chang et al.

Summary: Research on two-dimensional materials has been rapidly increasing in the past seventeen years, starting from graphene and expanding into a diverse family with unique structures and properties, making them attractive candidates for various applications. Major breakthroughs have been made in the last five years in developing synthetic methods, exploring new properties, identifying innovative applications, and pushing for commercialization in the field of 2D materials.

ACTA PHYSICO-CHIMICA SINICA (2021)

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Review Chemistry, Multidisciplinary

Recent advances in electrocatalysis with phthalocyanines

Shaoxuan Yang et al.

Summary: The applications of phthalocyanines (Pcs) in electrocatalysis have attracted attention due to their advantages of low cost, facile synthesis, and good chemical stability. Pcs offer high tailorability and structural diversity, making them promising for optimization in electrochemical devices and for various electrochemical reactions. Further research is needed to explore the structure-composition catalytic activity relationships of different Pc materials for future practical applications.

CHEMICAL SOCIETY REVIEWS (2021)

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Article Chemistry, Physical

Establishing spatially elastic hydrogen-bonding interaction in electrochemical process for selective CO2-to-CH4 conversion

Sheng-Nan Sun et al.

Summary: This study investigates the effects of spatially elastic hydrogen-bonding microenvironment on improving the CO2-to-CH4 electroreduction performance by designing a Cu-based supramolecular structure model system. Experimental and theoretical results show that subtle changes in hydrogen-bonding interaction can significantly improve the faradic efficiency for CH4.

CHEM CATALYSIS (2021)

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Review Materials Science, Multidisciplinary

Surface modification of metal materials for high-performance electrocatalytic carbon dioxide reduction

Yangbo Ma et al.

Summary: The study highlights recent advances in surface modification of metal materials for electrocatalytic CO2 reduction reaction (CO2RR) and their impact on the performance along with the underlying mechanisms.

MATTER (2021)

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Review Chemistry, Multidisciplinary

Hard-templated metal-organic frameworks for advanced applications

Esmail Doustkhah et al.

Summary: Template-directing strategies have opened new frontiers in synthesising metal-organic frameworks, particularly in catalysis, batteries, supercapacitance, drug delivery, and sieving; a variety of hard templates are discussed for directing MOF growth, classified into three categories, with detailed explanations on rationale and enhanced functionalities.

CHEMICAL SOCIETY REVIEWS (2021)

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Article Chemistry, Multidisciplinary

Building a stable cationic molecule/electrode interface for highly efficient and durable CO2 reduction at an industrially relevant current

Jianjun Su et al.

Summary: Methylation of CoTAPc improves current density for CO2 reduction, but severe leaching of catalysts leads to rapid decay in current density. A new in situ functionalization strategy with covalent grafting onto carbon nanotubes shows a 700% increase in CO partial current density and high stability.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

State of the Art and Prospects in Metal-Organic Framework (MOF)-Based and MOF-Derived Nanocatalysis

Qi Wang et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Potential Link between Cu Surface and Selective CO2 Electroreduction: Perspective on Future Electrocatalyst Designs

Gracita M. Tomboc et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Supramolecular Tuning Enables Selective Oxygen Reduction Catalyzed by Cobalt Porphyrins for Direct Electrosynthesis of Hydrogen Peroxide

Peter T. Smith et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Highly Efficient Porous Carbon Electrocatalyst with Controllable N-Species Content for Selective CO2 Reduction

Lin Ye et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Multidisciplinary

Recent Advances in Carbon Dioxide Hydrogenation to Methanol via Heterogeneous Catalysis

Xiao Jiang et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Investigating the Origin of Enhanced C2+ Selectivity in Oxide-/Hydroxide-Derived Copper Electrodes during CO2 Electroreduction

Qiong Lei et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Physical

Molecular enhancement of heterogeneous CO2 reduction

Dae-Hyun Nam et al.

NATURE MATERIALS (2020)

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Article Multidisciplinary Sciences

Efficient electron transmission in covalent organic framework nanosheets for highly active electrocatalytic carbon dioxide reduction

Hong-Jing Zhu et al.

NATURE COMMUNICATIONS (2020)

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Review Chemistry, Physical

Mechanistic Understanding of CO2 Reduction Reaction (CO2RR) Toward Multicarbon Products by Heterogeneous Copper-Based Catalysts

Tanya K. Todorova et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

Substantial Turnover Frequency Enhancement of MOF Catalysts by Crystallite Downsizing Combined with Surface Anchoring

A. Lisa Semrau et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

Tuning Zr12O22 Node Defects as Catalytic Sites in the Metal-Organic Framework hcp UiO-66

Xi Chen et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

Engineering Local Coordination Environments of Atomically Dispersed and Heteroatom-Coordinated Single Metal Site Electrocatalysts for Clean Energy-Conversion

Yuanzhi Zhu et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Physical

Metal-Organic Framework-Based Materials for Energy Conversion and Storage

Tianjie Qiu et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Physical

Boosting CO2 Electroreduction to CH4 via Tuning Neighboring Single-Copper Sites

Anxiang Guan et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Physical

Integration of Strong Electron Transporter Tetrathiafulvalene into Metalloporphyrin-Based Covalent Organic Framework for Highly Efficient Electroreduction of CO2

Qiao Wu et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Multidisciplinary

Metal-Organic Layers Leading to Atomically Thin Bismuthene for Efficient Carbon Dioxide Electroreduction to Liquid Fuel

Changsheng Cao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Single-Atom Iron Catalysts on Overhang-Eave Carbon Cages for High-Performance Oxygen Reduction Reaction

Chun-Chao Hou et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Metal-Organic Framework-Derived Carbon Nanorods Encapsulating Bismuth Oxides for Rapid and Selective CO2 Electroreduction to Formate

Peilin Deng et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Water-Soluble Polymers with Appending Porphyrins as Bioinspired Catalysts for the Hydrogen Evolution Reaction

Lisi Xie et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Multidisciplinary Sciences

Synergistic electroreduction of carbon dioxide to carbon monoxide on bimetallic layered conjugated metal-organic frameworks

Haixia Zhong et al.

NATURE COMMUNICATIONS (2020)

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Article Multidisciplinary Sciences

Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon

Kun Zhao et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Physical

Facet-Dependent Selectivity of Cu Catalysts in Electrochemical CO2 Reduction at Commercially Viable Current Densities

Gian Luca De Gregorio et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

Heterogeneous Catalysts with Well-Defined Active Metal Sites toward CO2 Electrocatalytic Reduction

Deren Yang et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Protecting Copper Oxidation State via Intermediate Confinement for Selective CO2 Electroreduction to C2+ Fuels

Peng-Peng Yang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Co-immobilization of a Rh Catalyst and a Keggin Polyoxometalate in the UiO-67 Zr-Based Metal-Organic Framework: In Depth Structural Characterization and Photocatalytic Properties for CO2 Reduction

Youven Benseghir et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Multidisciplinary Sciences

Accelerated discovery of CO2 electrocatalysts using active machine learning

Miao Zhong et al.

NATURE (2020)

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Review Chemistry, Multidisciplinary

Phase engineering of nanomaterials

Ye Chen et al.

NATURE REVIEWS CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Freestanding Millimeter-Scale Porphyrin-Based Monoatomic Layers with 0.28 nm Thickness for CO2Electrocatalysis

Deren Yang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Electrochemical Reduction of Carbon Dioxide to 1-Butanol on Oxide-Derived Copper

Louisa Rui Lin Ting et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Energy & Fuels

Molecular engineering of dispersed nickel phthalocyanines on carbon nanotubes for selective CO2 reduction

Xiao Zhang et al.

NATURE ENERGY (2020)

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Review Chemistry, Physical

Conductive Metal-Organic Frameworks: Design, Synthesis, and Applications

Haibing Meng et al.

SMALL METHODS (2020)

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Article Chemistry, Multidisciplinary

Highly Selective CO2 Electroreduction to CH4 by In Situ Generated Cu2O Single-Type Sites on a Conductive MOF: Stabilizing Key Intermediates with Hydrogen Bonding

Jun-Dong Yi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Enhancing CO2Electroreduction to Methane with a Cobalt Phthalocyanine and Zinc-Nitrogen-Carbon Tandem Catalyst

Long Lin et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Ethylene Selectivity in Electrocatalytic CO2 Reduction on Cu Nanomaterials: A Crystal Phase-Dependent Study

Ye Chen et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Stable and Efficient Single-Atom Zn Catalyst for CO2 Reduction to CH4

Lili Han et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Highly Electrocatalytic Ethylene Production from CO2 on Nanodefective Cu Nanosheets

Bingxing Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Multidisciplinary Sciences

A scalable method for preparing Cu electrocatalysts that convert CO2 into C2+ products

Taehee Kim et al.

NATURE COMMUNICATIONS (2020)

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Article Multidisciplinary Sciences

Heterophase fcc-2H-fcc gold nanorods

Zhanxi Fan et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Physical

Bi-Based Metal-Organic Framework Derived Leafy Bismuth Nanosheets for Carbon Dioxide Electroreduction

Jian Yang et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Physical

Recent Advances in MOF-Derived Single Atom Catalysts for Electrochemical Applications

Zhongxin Song et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Phase-Selective Epitaxial Growth of Heterophase Nanostructures on Unconventional 2H-Pd Nanoparticles

Yiyao Ge et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Undercoordinated Active Sites on 4H Gold Nanostructures for CO2 Reduction

Yuxuan Wang et al.

NANO LETTERS (2020)

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Article Chemistry, Physical

Phase Engineering of Nanomaterials for Clean Energy and Catalytic Applications

Huangxu Li et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

Anchoring Zn-phthalocyanines in the pore matrices of UiO-67 to improve highly the photocatalytic oxidation efficiency

Cai-Xia Lu et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Multidisciplinary

Hierarchical Tuning of the Performance of Electrochemical Carbon Dioxide Reduction Using Conductive Two-Dimensional Metallophthalocyanine Based Metal-Organic Frameworks

Zheng Meng et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Metal-Organic Layers for Electrocatalysis and Photocatalysis

Lingyun Cao et al.

ACS CENTRAL SCIENCE (2020)

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Article Chemistry, Multidisciplinary

Axial Cl/Br atom-mediated CO2 electroreduction performance in a stable porphyrin-based metal-organic framework

Qing Huang et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Physical

Highly stable two-dimensional bismuth metal-organic frameworks for efficient electrochemical reduction of CO2

Fang Li et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Review Chemistry, Inorganic & Nuclear

Transition metal macrocycles for heterogeneous electrochemical CO2 reduction

Fang Lv et al.

COORDINATION CHEMISTRY REVIEWS (2020)

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Review Chemistry, Inorganic & Nuclear

MOF-based atomically dispersed metal catalysts: Recent progress towards novel atomic configurations and electrocatalytic applications

Dong-Dong Ma et al.

COORDINATION CHEMISTRY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Spatial Confinement in Copper-Porphyrin Frameworks Enhances Carbon Dioxide Reduction to Hydrocarbons

Yinzheng Zhou et al.

CELL REPORTS PHYSICAL SCIENCE (2020)

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Article Materials Science, Multidisciplinary

Ultrasensitive Detection of Electrolyte Leakage from Lithium-Ion Batteries by Ionically Conductive Metal-Organic Frameworks

Yang Lu et al.

MATTER (2020)

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Review Chemistry, Inorganic & Nuclear

Rational design and synthesis of ultramicroporous metal-organic frameworks for gas separation

Ting Wang et al.

COORDINATION CHEMISTRY REVIEWS (2020)

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Review Materials Science, Multidisciplinary

Rational Design of Metal-Organic Frameworks towards Efficient Electrocatalysis

Shuo Dou et al.

ACS MATERIALS LETTERS (2020)

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Article Chemistry, Multidisciplinary

Bimetallic metal-organic frameworks and their derivatives

Liyu Chen et al.

CHEMICAL SCIENCE (2020)

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Review Chemistry, Physical

Carbon-based single-atom catalysts for CO2 electroreduction: progress and optimization strategies

Xiu-Li Lu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Review Chemistry, Multidisciplinary

From metal-organic frameworks to single/dual-atom and cluster metal catalysts for energy applications

Chun-Chao Hou et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Article Chemistry, Multidisciplinary

A planar binuclear cobalt(ii) phthalocyanine as a highly efficient catalyst for the oxidation of a mercaptan

Sergey G. Makarov et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Physical

Metal-organic framework-derived cupric oxide polycrystalline nanowires for selective carbon dioxide electroreduction to C2 valuables

Fan Yang et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Physical

Metal-organic framework derived copper catalysts for CO2 to ethylene conversion

Kaili Yao et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Review Chemistry, Multidisciplinary

MOF-derived electrocatalysts for oxygen reduction, oxygen evolution and hydrogen evolution reactions

Hao-Fan Wang et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

A Semiconducting Polymer Nano-prodrug for Hypoxia-Activated Photodynamic Cancer Therapy

Dong Cui et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

DNAzyme-Loaded Metal-Organic Frameworks (MOFs) for Self-Sufficient Gene Therapy

Huimin Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

One-Pot Synthesis of Framework Porphyrin Materials and Their Applications in Bifunctional Oxygen Electrocatalysis

Bo-Quan Li et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Review Chemistry, Multidisciplinary

Electrochemical CO2 Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design

Md Golam Kibria et al.

ADVANCED MATERIALS (2019)

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Review Chemistry, Multidisciplinary

Understanding the Roadmap for Electrochemical Reduction of CO2 to Multi-Carbon Oxygenates and Hydrocarbons on Copper-Based Catalysts

Yao Zheng et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Physical

Enhanced N-doping in mesoporous carbon for efficient electrocatalytic CO2 conversion

Min Kuang et al.

NANO RESEARCH (2019)

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Review Multidisciplinary Sciences

What would it take for renewably powered electrosynthesis to displace petrochemical processes?

Phil De Luna et al.

SCIENCE (2019)

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Review Chemistry, Physical

Recent Trends, Benchmarking, and Challenges of Electrochemical Reduction of CO2 by Molecular Catalysts

Kamal Elouarzaki et al.

ADVANCED ENERGY MATERIALS (2019)

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Review Chemistry, Multidisciplinary

Progress and Perspectives of Electrochemical CO2 Reduction on Copper in Aqueous Electrolyte

Stephanie Nitopi et al.

CHEMICAL REVIEWS (2019)

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Review Chemistry, Inorganic & Nuclear

Synthesis of MOF-derived nanostructures and their applications as anodes in lithium and sodium ion batteries

Ming Zhong et al.

COORDINATION CHEMISTRY REVIEWS (2019)

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Article Multidisciplinary Sciences

Integration of a (-Cu-S-)n plane in a metal-organic framework affords high electrical conductivity

Abhishek Pathak et al.

NATURE COMMUNICATIONS (2019)

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Review Chemistry, Physical

Designing materials for electrochemical carbon dioxide recycling

Michael B. Ross et al.

NATURE CATALYSIS (2019)

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Article Chemistry, Physical

Cooperative copper centres in a metal-organic framework for selective conversion of CO2 to ethanol

Bing An et al.

NATURE CATALYSIS (2019)

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Article Chemistry, Multidisciplinary

Scalable Production of Efficient Single-Atom Copper Decorated Carbon Membranes for CO2 Electroreduction to Methanol

Hengpan Yang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Review Energy & Fuels

Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels

Yuvraj Y. Birdja et al.

NATURE ENERGY (2019)

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Article Chemistry, Multidisciplinary

Bismuth Single Atoms Resulting from Transformation of Metal-Organic Frameworks and Their Use as Electrocatalysts for CO2 Reduction

Erhuan Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Three-Dimensional Phthalocyanine Metal-Catecholates for High Electrochemical Carbon Dioxide Reduction

Roc Matheu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Multidisciplinary Sciences

Domino electroreduction of CO2 to methanol on a molecular catalyst

Yueshen Wu et al.

NATURE (2019)

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Article Multidisciplinary Sciences

Carbon dioxide electroreduction to C2 products over copper-cuprous oxide derived from electrosynthesized copper complex

Qinggong Zhu et al.

NATURE COMMUNICATIONS (2019)

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Article Chemistry, Multidisciplinary

A Noble-Metal-Free Metal-Organic Framework (MOF) Catalyst for the Highly Efficient Conversion of CO2 with Propargylic Alcohols

Sheng-Li Hou et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

In Situ Generation of an N-Heterocyclic Carbene Functionalized Metal-Organic Framework by Postsynthetic Ligand Exchange: Efficient and Selective Hydrosilylation of CO2

Xu Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Cu/Bi metal-organic framework-based systems for an enhanced electrochemical transformation of CO2 to alcohols

Jonathan Albo et al.

JOURNAL OF CO2 UTILIZATION (2019)

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Article Chemistry, Physical

Catalysis by Metal Organic Frameworks: Perspective and Suggestions for Future Research

Dong Yang et al.

ACS CATALYSIS (2019)

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Article Chemistry, Physical

A Water-Soluble Cu Complex as Molecular Catalyst for Electrocatalytic CO2 Reduction on Graphene-Based Electrodes

Jiong Wang et al.

ADVANCED ENERGY MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Biomimetic Metal-Organic Framework Nanoparticles for Cooperative Combination of Antiangiogenesis and Photodynamic Therapy for Enhanced Efficacy

Huan Min et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Cathodized copper porphyrin metal-organic framework nanosheets for selective formate and acetate production from CO2 electroreduction

Jian-Xiang Wu et al.

CHEMICAL SCIENCE (2019)

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Article Chemistry, Multidisciplinary

Metal-organic framework-derived indium-copper bimetallic oxide catalysts for selective aqueous electroreduction of CO2

Weiwei Guo et al.

GREEN CHEMISTRY (2019)

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Article Materials Science, Multidisciplinary

Disclosing CO2 Activation Mechanism by Hydroxyl-Induced Crystalline Structure Transformation in Electrocatalytic Process

Qing Huang et al.

MATTER (2019)

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Article Chemistry, Multidisciplinary

Size dependent selectivity of Cu nano-octahedra catalysts for the electrochemical reduction of CO2 to CH4

Pranit Lyengar et al.

CHEMICAL COMMUNICATIONS (2019)

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Article Chemistry, Multidisciplinary

MOF-derived nitrogen-doped nanoporous carbon for electroreduction of CO2 to CO: the calcining temperature effect and the mechanism

Yonglong Zheng et al.

NANOSCALE (2019)

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Article Chemistry, Multidisciplinary

A cobalt arylphosphonate MOF - superior stability, sorption and magnetism

Yunus Zorlu et al.

CHEMICAL COMMUNICATIONS (2019)

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Review Nanoscience & Nanotechnology

Nanomaterials derived from metal-organic frameworks

Song Dang et al.

NATURE REVIEWS MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Amorphizing of Cu Nanoparticles toward Highly Efficient and Robust Electrocatalyst for CO2 Reduction to Liquid Fuels with High Faradaic Efficiencies

Yan-Xin Duan et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Multidisciplinary

A Cooperative Pillar-Template Strategy as a Generalized Synthetic Method for Flexible Homochiral Porous Frameworks

Jing Jin et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Review Chemistry, Multidisciplinary

Atomically Dispersed Metal Sites in MOF-Based Materials for Electrocatalytic and Photocatalytic Energy Conversion

Zibin Liang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

Iron Porphyrins Embedded into a Supramolecular Porous Organic Cage for Electrochemical CO2 Reduction in Water

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