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Synergistic strategies for the synthesis of Fe(ii)-based bifunctional fluorescent spin-crossover materials

DALTON TRANSACTIONS (2022)

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Summary: This study presents a mononuclear compound with aggregation-induced emission and thermally induced spin crossover (SCO) properties, showing effective control of luminescence intensity through spin transition. Unlike the traditional strategy, this research achieves effective coupling between SCO and luminescence by tuning intermolecular interactions through subtle structural changes. The results provide a rational strategy for constructing smart multifunctional materials with synergistic SCO and luminescence.

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Summary: A new spin crossover-fluorescent compound with a 2D structure and high sensitivity has been developed. Its magnetic and fluorescence properties can be simultaneously controlled by multiple external stimuli, including physical thermal treatment and chemical stimuli. The compound exhibits reversible variations and wide thermal hysteresis loops in its temperature-dependent magnetic susceptibility and fluorescence intensity.

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Summary: The passage discusses the growing interest in dual-emission materials for materials and life science applications, highlighting the lack of a systematic overview of the underlying processes. It classifies dual-emission phenomena and describes relevant mechanisms for materials science, while also providing references for further reading and inspiration for future designs of dual-emission materials.

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Summary: This study reports a bidirectional spin-state switch and fluorescence modulation of an Fe(II) complex based on a rhodamine B 2-pyridinecarbaldehyde hydrazone ligand, showing reversible spin-state changes at both room temperature and high temperature, as well as under acidification and alkalization treatment. The reversible spin-state switch was attributed to solvent loss and ligand tautomerization, leading to fluorescence enhancement in response to external stimuli.

CCS CHEMISTRY (2021)

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Summary: This study reported the fabrication of composites consisting of a fluorescent organic semiconductor polymer and a spin crossover compound, demonstrating a strong synergy between the spin transition of the Fe(II) compound and variations in the fluorescence of the organic polymer. The modulation of fluorescence was shown to be reversible, with an increase of <=20% compared to the original value.

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Construction of Magneto-Fluorescent Bifunctional Spin-Crossover Fe(II) Complex from Pyrene-Decorated Pybox Ligand

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Summary: The synthesis and properties studies of a mononuclear Fe(II) complex with a pyrene fluorophore-decorated ligand were reported. The complex showed incomplete spin-crossover in a certain temperature range and light-induced excited spin state trapping. Fluorescence was achieved in both solution and solid state, demonstrating the coexistence of spin-crossover and fluorescence in one compound.

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Summary: The study successfully obtained two Fe(ii) grid-like complexes using a coordination-driven supramolecular assembly strategy, demonstrating spin-crossover behavior in azido-bridged complexes. By substitution of the ligand, the complex showed a synergistic effect between spin-crossover behavior and luminescence.

DALTON TRANSACTIONS (2021)

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