期刊
ORGANIC CHEMISTRY FRONTIERS
卷 9, 期 23, 页码 6708-6716出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2qo01410f
关键词
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资金
- National Natural Science Foundation of China [21971104, 22271136]
- Shenzhen Bay Laboratory [SZBL2019062801006]
- Guangdong Innovative Program [2019BT02Y335]
- Guangdong Provincial Key Laboratory of Catalysis [2020B121201002]
- Shenzhen Key Laboratory of Small Molecule Drug Discovery and Synthesis [ZDSYS20190902093215877]
- Shenzhen Nobel Prize Scientists Laboratory Project [C17783101]
As the key structural unit, five-membered carbocycles are commonly found in natural products. Daphniphyllum alkaloids, with their complex structures and interesting bioactivity, have attracted synthetic chemists' attention. This review focuses on the novel or relatively rarely used strategies and methods for constructing the five-membered carbocycle in recent Daphniphyllum alkaloid synthesis, covering from January 2017 to August 2022.
As the key structural unit, five-membered carbocycles are widely found in the framework of natural products. Among these molecules, Daphniphyllum alkaloids are particularly intriguing targets for synthetic chemists owing to their complex structures and interesting bioactivity. Within extensive synthetic studies of these alkaloids, various strategies and methods have been utilized for the construction of all carbon five-membered rings. Besides the classics, in this review we would like to focus on the novel or relatively rarely used strategies and methods for the five-membered carbocycle construction in recent Daphniphyllum alkaloid synthesis, covering from January 2017 to August 2022.
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