4.6 Article

Curing and self-healing of enzymatic construction materials using nanoparticles

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CELL REPORTS PHYSICAL SCIENCE
卷 3, 期 9, 页码 -

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CELL PRESS
DOI: 10.1016/j.xcrp.2022.101039

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  1. National Science Foundation [2223664]

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The article describes a method that allows for the rapid curing of enzymatic construction materials under ambient conditions using low-power lasers and the incorporation of nanoparticles, supporting on-site manufacturing capability for construction materials.
Preparation of construction materials on site may offer advantages in transportation and storage. However, a major limitation of on-site preparation of some materials is the need for heat and oven desic-cation for adequate curing. Here, we describe a method that allows rapid curing under ambient conditions through the addition of 0.1% iron oxide nanoparticles to a carbon-negative enzymatic construc-tion material (ECM) to make ECM-n. Specifically, we show that a low-power laser (3W at 808 nm) can cure ECM-n to an optimal me-chanical strength in 12 h, which can be compared to the 14-day period needed for in situ air drying. In addition, the incorporation of nanoparticles allows rapid self-healing of large-scale flaws and that incandescent light can be used if lasers are not available. This method establishes an on-site manufacturing capability for ECM-n and other construction materials and supports thermal controlla-bility of the local structure in low-temperature regions.

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