期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 24, 期 47, 页码 28994-29003出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cp04426a
关键词
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资金
- CALIPSOplus [730872]
- COST Action [CA18212]
- COST (European Cooperation in Science and Technology)
- MICINN (Spanish Ministry of Science and Innovation) [PID2019-110091GB-I00, MCIN/AEI/10.13039/501100011033]
- Program for Centers of Excellence in RD [CEX2018-000805-M]
We investigated the fragmentation dynamics of adamantane dications generated through core-ionization at the carbon edge and subsequent Auger decay. By employing high-resolution electron spectroscopy, energy-resolved electron-ion multi-coincidence spectroscopy, and various theoretical models, we were able to fully characterize the processes involved after ionization. Our findings demonstrate the observation of energy- and site-sensitivity even in a highly-symmetric molecule lacking any unique atomic site.
We investigate the fragmentation dynamics of adamantane dications produced after core-ionization at the carbon edge followed by Auger decay. The combination of high-resolution electron spectroscopy, energy-resolved electron-ion multi-coincidence spectroscopy and different theoretical models allows us to give a complete characterization of the processes involved after ionization. We show that energy- and site-sensitivity is observed even for a highly-symmetric molecule that lacks any unique atomic site.
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