4.6 Article

Superconductivity in TlBi2 with a large Kadowaki-Woods ratio

期刊

PHYSICAL REVIEW B
卷 106, 期 22, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.106.224501

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资金

  1. Ministry of Science and Technology of China
  2. National Natural Science Foundation of China (NSFC)
  3. Fundamen- tal Research Funds for the Central Universities
  4. [2022YFA1403202]
  5. [11974095]
  6. [12074335]

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This paper investigates the superconducting and normal state properties of TlBi2 with the AlB2-type structure. It is found that TlBi2 exhibits bulk superconductivity and is a phonon-mediated s-wave superconductor. Furthermore, the study reveals that the temperature dependence of the resistivity, p(T), shows a linear relationship at high temperatures and can be described by the Fermi-liquid theory at low temperatures. Interestingly, the Kadowaki-Woods ratio of TlBi2 is unexpectedly large compared to many heavy fermion compounds.
In this paper, the superconducting and normal state properties of TlBi2 with the AlB2-type structure were studied by resistivity, magnetization, and specific heat measurements. It was found that bulk superconductivity with Tc = 6.2 K emerges in TlBi2, which is a phonon-mediated s-wave superconductor with a strong electron-phonon coupling (lambda ep = 1.38) and a large superconducting gap (A0/kBTc = 2.25). We found that the p(T) exhibits an unusual T-linear dependence above 50 K, and can be well described by the Fermi-liquid theory below 20 K. Interestingly, its Kadowaki-Woods ratio A/gamma 2 [9.2 x 10-5 mu Q cm(mol K2/mJ)2] is unexpectedly one order of magnitude larger than that obtained in many heavy fermion compounds, although the electronic correlation is not so strong.

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