☆ 4.8 Review

Membranes prepared from graphene-based nanomaterials for water purification: a mini-review

NANOSCALE (2022)

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Reshapable MXene/Graphene Oxide/Polyaniline Plastic Hybrids with Patternable Surfaces for Highly Efficient Solar-Driven Water Purification

Xiao-Peng Li et al.

Summary: The study developed reshappable Ti3C2Tx MXene/graphene oxide (GO)/polyaniline (PANI) hybrids with variable shapes and patternable surfaces for efficient solar-driven purification of seawater and wastewater. The hybrids exhibit high water evaporation rates and outstanding evaporation efficiency under 1-sun irradiation, making them highly efficient in generating clean water with satisfactory ion rejection rates.

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Summary: The study introduces a solar-driven water evaporator based on a porous hydrogel sponge, which is realized by in-situ growth of hydrogel on polyurethane sponge for durability and efficiency. The hydrogel evaporator shows high water evaporation rate, long-term stability, and cost-effectiveness.

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Review Chemistry, Multidisciplinary

Tailored design of nanofiltration membranes for water treatment based on synthesis-property-performance relationships

Kunpeng Wang et al.

Summary: Progress has been made in tailored design of NF membranes by optimizing interfacial polymerization techniques, adopting new manufacturing processes and materials. The property-performance relationships based on solvent/solute mass transfer theories and mathematical models have been discussed, along with conclusions on membrane structural and physicochemical parameter regulation to improve membrane separation performance, as well as existing and potential applications of NF membranes in water treatment processes. Challenges and prospects of tailored design of NF membranes for water treatment applications are also highlighted.

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Article Biophysics

Graphene oxide enriched with oxygen-containing groups: on the way to an increase of antioxidant activity and biocompatibility

Abdelsattar O. E. Abdelhalim et al.

Summary: This article investigates the comprehensive biocompatibility of synthesised graphene oxide enriched with oxygen-containing functional groups. The study includes tests on haemocompatibility, antioxidant activity, genotoxicity, and metabolic activity of cells.

COLLOIDS AND SURFACES B-BIOINTERFACES (2022)

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Advances in preparation, mechanism and applications of graphene quantum dots/semiconductor composite photocatalysts: A review

Chunyu Cheng et al.

Summary: Graphene quantum dots (GQDs) are efficient photocatalytic materials that combine the advantages of quantum dots and carbon materials, showing potential in various applications. This study comprehensively discusses the preparation, mechanisms, and applications of GQDs composite semiconductor materials in photocatalysis, offering guidance for future research.

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Article Engineering, Chemical

Graphene oxide/silica composite nanofiltration membrane: Adjustment of the channel of water permeation

Huihui Deng et al.

Summary: The use of composite membranes with GO and SiO2 nanoparticles can effectively adjust the channel microstructure for water treatment, greatly enhancing water flux and rejection rate by controlling the size of nanosheets and nanoparticles.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Engineering, Chemical

Interfacial polymerization of a covalent organic framework layer on titanium dioxide@graphene oxide/polyacrylonitrile mixed-matrix membranes for high-performance dye separation

Qiao Liu et al.

Summary: The influences of the pore structure, microtopography, and chemical structure of support membranes on the structure and performance of the COF composite membranes were studied. The TiO2@GO/PAN support membranes with hydrophilic and smooth top surface, homogenous pore distribution, and large pore size enabled easy infiltration of aqueous-phase solutions and the formation of a stable interface. The COF composite membranes exhibited excellent filtration performance with a thin crystalline layer on the support membrane.

JOURNAL OF MEMBRANE SCIENCE (2022)

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Article Engineering, Chemical

Separation of mono-/di-valent ions via charged interlayer channels of graphene oxide membranes

Qingbo Huang et al.

Summary: In this study, a graphene oxide (GO) membrane with charged interlayer channels was developed for the separation of mono-/di-valent ions. The membrane achieved selective transport of monovalent ions by utilizing size-sieving and electrostatic repulsion. The introduction of polyethyleneimine (PEI) into the interlayer channels not only controlled the charge property but also increased the hydrophilicity of the membrane surface. The optimal GO-PEI membrane exhibited high permeation rates and selectivity for monovalent ions.

JOURNAL OF MEMBRANE SCIENCE (2022)

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Review Nanoscience & Nanotechnology

Recent Advances in Graphene Oxide Membranes for Nanofiltration

Liu Yang et al.

Summary: This article reviews the research advances on high-performance nanofiltration membranes based on two-dimensional graphene oxide (GO), including preparation methods, chemical modification and physical manipulation of transport channels, theoretical calculation, molecular dynamics simulation, and the superior nanofiltration performance of GO-based membranes. The challenges and prospects for future development in membrane technology are also discussed.

ACS APPLIED NANO MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Graphene Oxide Nanofiltration Membrane Based on Three-Dimensional Size-Controllable Metal-Organic Frameworks for Water Treatment

Huaijiao Qu et al.

Summary: This paper reports the development of composite nanofiltration membranes by embedding zeolite imidazole framework-8 (ZIF-8) nanoporous material in a graphene oxide (GO) membrane. The composite membrane shows improved separation and permeability compared to the pure GO membrane, and remains stable during long-term permeation process. The study also investigates the effects of different ZIF-8 particle sizes on the water permeability of the composite membrane.

ACS APPLIED NANO MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Lamellar MXene Nanofiltration Membranes for Electrostatic Modulation of Molecular Permeation: Implications for Fine Separation

Jing Li et al.

Summary: This study demonstrates that the separation performance of Ti3C2Tx-MXene lamellar nanofiltration membranes can be modulated by applying external electrostatic fields. The filtration performance of the membranes on cationic and anionic dyes can be improved or declined depending on the polarity of the electric field. The regulation mechanisms are discussed, which are likely attributed to the changes in electrostatic interactions induced by the external electric field.

ACS APPLIED NANO MATERIALS (2022)

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Article Chemistry, Physical

Sustainable development of graphitic carbon nanosheets from plastic wastes with efficient photothermal energy conversion for enhanced solar evaporation

Marliyana Aizudin et al.

Summary: By solvothermal treatment and carbonization, plastic waste can be transformed into graphitic carbon nanosheets, exhibiting excellent photothermal conversion efficiency and high evaporation rate in a solar evaporator.

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Review Chemistry, Multidisciplinary

Recent Progress in Graphene/Polymer Nanocomposites

Xianxian Sun et al.

Summary: Nanocomposites with graphene as filler have attracted increasing attention due to their unique properties. This review summarizes recent progress on graphene/polymer nanocomposites, focusing on strengthening/toughening, electrical conduction, thermal transportation, and photothermal energy conversion. The influence of graphene configuration on properties and the role of interfacial interaction between graphene and polymer are analyzed, providing insights for preparing high-performance nanocomposites in the future.

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Article Biophysics

Long period grating in double cladding fiber coated with graphene oxide as high-performance optical platform for biosensing

Flavio Esposito et al.

Summary: In this study, a novel fiber-optic biosensor was developed and tested for label-free detection of C-reactive protein in serum. The device showed enhanced sensitivity and visibility of grating resonances by tuning the working point to the mode transition region through etching of the outer fiber cladding. Coating the fiber transducer with graphene oxide enabled covalent immobilization of the biological recognition element, resulting in a low detection limit and a wide working range of clinical relevance.

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Tunable Graphene Oxide Nanofiltration Membrane for Effective Dye/Salt Separation and Desalination

Chao Xing et al.

Summary: In this study, a graphene oxide membrane with tunable interlayer distance was fabricated for effective dye separation and desalination in saline textile wastewater treatment. The membrane achieved high dye rejection rates (>99%) and low salt rejection rates (<6.5%) in the first filtration stage, while demonstrating a desalination rate of up to 51.8% in the second stage. The membrane also showed excellent practical advantages such as high permeability, antifouling performance, and stability, with the potential for regenerating dye and producing clean water through multistage filtration systems.

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Intensifying Heat Using MOF-Isolated Graphene for Solar-Driven Seawater Desalination at 98% Solar-to-Thermal Efficiency

Xuemei Han et al.

Summary: The study presents a novel photothermal material G@ZIF, which demonstrates high energy conversion efficiency under artificial sunlight and is applicable for various practical applications, such as steam generators and water treatment systems.

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Mutually Reinforced Polymer-Graphene Bilayer Membranes for Energy-Efficient Acoustic Transduction

Assad U. Khan et al.

Summary: A new bilayer composite material made of polyetherimide and single-layer graphene was prepared, exhibiting high aspect ratio suspension and ultrastrong support. The membrane generates high-quality sound under electromechanical actuation, with high energy efficiency.

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Design, Fabrication, and Mechanism of Nitrogen-Doped Graphene-Based Photocatalyst

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Summary: Nitrogen-doped graphene (NG) as a derivative of graphene, with the ability to break the undifferentiated structure, open the bandgap, and provide an uneven electron density distribution, retains the advantages of graphene while offering novel properties for photocatalysis. With wide applications in hydrogen production, CO2 reduction, pollutant degradation, and other directions, NG-based photocatalysis shows great potential for addressing energy and environmental challenges.

ADVANCED MATERIALS (2021)

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Nitrogen-doped graphene quantum dots hydrogels for highly efficient solar steam generation

Ahmad Allahbakhsh

Summary: Solar evaporation using nitrogen-doped graphene quantum dots hydrogels shows high efficiency, with the smallest lateral size range N-GQDs precursor achieving the highest solar steam generation efficiency. The performance of these hydrogels is attributed to their colloidal morphology, high hydrophilicity, hierarchical pore structure, and low thermal conductivity.

DESALINATION (2021)

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Interfacial Solar Evaporation by a 3D Graphene Oxide Stalk for Highly Concentrated Brine Treatment

Casey T. K. Finnerty et al.

Summary: In this work, a 3D graphene oxide stalk with near capillary wicking limit is demonstrated to achieve high evaporation efficiency, ultrahigh evaporative surface area index (EAI), omnidirectional sunlight utilization, and high evaporation flux under dark conditions.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Nanoscience & Nanotechnology

Graphene oxide membranes with stable porous structure for ultrafast water transport

Wen-Hai Zhang et al.

Summary: The study presents a highly stable and ultrapermeable zeolitic imidazolate framework-8 (ZIF-8)-nanocrystal-hybridized graphene oxide membrane prepared using ice templating and in situ crystallization of ZIF-8. The selective growth of ZIF-8 in microporous defects enhances water permeability and mechanical integrity, leading to a 30-fold increase in permeability compared to graphene oxide membranes (GOms). The technique also improves permselectivity and offers potential for developing next-generation nanofiltration membranes.

NATURE NANOTECHNOLOGY (2021)

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Review Green & Sustainable Science & Technology

Application of graphene in energy storage device - A review

A. G. Olabi et al.

Summary: The study explored the application of graphene in energy storage devices, absorbers, and electrochemical sensors, recognizing the need to address current limitations to improve performance. The advantages of graphene have widened its application in electroanalytical and electrochemical sensors, but further refinement is necessary for broader application.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2021)

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Review Chemistry, Physical

Graphene/MoS2 Nanohybrid for Biosensors

Jinho Yoon et al.

Summary: Researchers have focused on the application of graphene and MoS2 in the field of biosensors, conducting extensive studies in this area. By developing nanohybrid materials consisting of graphene and MoS2, various types of biosensors can be developed.

MATERIALS (2021)

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Fabrication of PEI modified GO/MXene composite membrane and its application in removing metal cations from water

Xin Zhao et al.

Summary: In this study, PEI modified GO/MXene composite membranes were fabricated and tested, showing a synergistic effect in water permeability and rejection of metal cations, especially with improved rejection of Ca2+ and Mg2+. The removal mechanism of metal ions mainly involved steric effect and electrostatic effect, which indicates great potential for water softening in practical applications.

JOURNAL OF MEMBRANE SCIENCE (2021)

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Decimeter-Scale Atomically Thin Graphene Membranes for Gas-Liquid Separation

Dandan Hou et al.

Summary: This study presents a facile method for fabricating nanoporous atomically thin membranes (NATMs) by directly casting a porous polymer substrate onto graphene. The resulting flexible nanoporous polymer substrate provides sufficient mechanical support without compromising the permeance of the NATMs. The NATMs, with proper pore size and a uniform spongelike structure, demonstrate salt resistance and 3-5 times higher gas permeance than commercial polymeric membranes, bridging the gap between laboratory-scale proof-of-concept and practical applications in the industry.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Physical

Poly(p-phenylene benzobisoxazole) nanofiber/reduced graphene oxide composite aerogels toward high-efficiency solar steam generation

Meiling Chen et al.

Summary: This study demonstrates an interfacial solar evaporator made from PBONF/RGO composite aerogels, which shows fast and durable solar-vapor conversion with a high efficiency of 98.4% under unconcentrated one sun irradiation. The PBONFs not only strengthen the mechanical properties of composite aerogels, but also offer great potential applications in wastewater purification in extreme environments, such as aerospace.

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS (2021)

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Article Chemistry, Multidisciplinary

Designing Carbonized Loofah Sponge Architectures with Plasmonic Cu Nanoparticles Encapsulated in Graphitic Layers for Highly Efficient Solar Vapor Generation

Liteng Ren et al.

Summary: A hybrid material of three-dimensional carbonized loofah sponges, graphene layers, and copper nanoparticles was successfully synthesized, showing improved light harvesting and high evaporation rates. The localized heating effect of stabilized copper nanoparticles led to a surface temperature of 72 degrees C and a high vapor generation rate of 1.54 kg m(-2) h(-1) with a solar thermal efficiency of 90.2% under 1 Sun illumination. These results suggest a promising perspective in practical applications in the purification of sewage and muddy water using this Cu-based photothermal material.

NANO LETTERS (2021)

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Article Engineering, Environmental

3D graphene-like zeolite-templated carbon with hierarchical structures as a high-performance adsorbent for volatile organic compounds

Nam Sun Kim et al.

Summary: The study compared the dynamic adsorption of benzene on different carbon materials and found that hierarchical mesoporous/microporous beta zeolite-templated carbon (HBTC) had higher adsorption capacity and breakthrough time for benzene compared to commercial activated carbon (AC) and solely microporous beta zeolite-templated carbon (BTC). Introducing mesoporosity into microporous BTC to form a hierarchically mesoporous/microporous structure solved the diffusion problem and improved benzene adsorption performance. The HBTC showed promising potential for volatile organic compound (VOC) adsorption with higher adsorption capacity and better performance at 10% breakthrough compared to other tested carbons.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Biotechnology & Applied Microbiology

Graphene-based membrane techniques for heavy metal removal: A critical review

Yasser Vasseghian et al.

Summary: Graphene-based membranes (GBMs) have unique physical and chemical properties that make them suitable for applications such as pollutant removal and water desalination, offering high potential. GBM techniques are capable of producing large, leak-free, and fouling-free membranes, showing promise for the removal of hazardous pollutants from water.

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Yadong Yu et al.

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TRENDS IN FOOD SCIENCE & TECHNOLOGY (2021)

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Preparation of Thin-Film Composite Nanofiltration Membranes Doped with N- and Cl-Functionalized Graphene Oxide for Water Desalination

Francisco J. Garcia-Picazo et al.

Summary: In this study, chemically modified graphene oxide was utilized as a crosslinking agent in thin-film composite nanofiltration membranes, leading to enhanced permeance and salt rejection. Functionalized graphene oxide showed improved dispersibility and membrane performance, providing a new approach for water desalination applications.

POLYMERS (2021)

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Article Chemistry, Physical

Ultrahigh-Energy-Density Sorption Thermal Battery Enabled by Graphene Aerogel-Based Composite Sorbents for Thermal Energy Harvesting from Air

Taisen Yan et al.

Summary: This paper introduces an ultrahigh-energy/power-density sorption thermal battery enabled by graphene aerogel-based composite sorbents for efficient thermal harvesting and storage. The STB achieves record energy density and power density for space heating through the multistep water desorption-sorption mechanism of CaCl2@GA sorbent. Overall, this work provides a promising low-carbon route for efficient thermal energy harvesting, storage, and utilization.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Multidisciplinary

A Facile and Scalable Method of Fabrication of Large-Area Ultrathin Graphene Oxide Nanofiltration Membrane

Zhiyu Liu et al.

Summary: The scalable ultrathin uniform GO membrane fabrication technique reported in this study utilizes Mayer rod-coating and short-time, high-power UV reduction to produce large area, thin GO membranes. The interlayer spacing of the membrane can be effectively reduced and regulated to improve salt rejection rate, while the fabricated membrane shows superior water permeability and high separation efficiency, along with excellent mechanical stability under harsh conditions. The developed fabrication method can be scaled up using a roll-to-roll industrial production process, solving the current bottleneck in GO membrane research and enabling industrial usage of GO membrane.

ACS NANO (2021)

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Correction Biophysics

Facile fabrication of a novel 3D rose like lanthanum doped zirconia decorated reduced graphene oxide nanosheets: An efficient electro-catalyst for electrochemical reduction of futuristic anti-cancer drug salinomycin during pharmacokinetic study (vol 150, 111849, 2020)

Saad A. Alkahtani et al.

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Article Chemistry, Physical

Intercalation of N-doped graphene into graphene oxide-based membranes to improve their overall nanofiltration performance

Ruitong Hou et al.

Summary: In this study, N-doped graphene was intercalated with graphene oxide membranes to form GNM, which significantly enhanced water flux and dye separation efficiency while maintaining stability in water purification processes.

CHEMICAL PHYSICS LETTERS (2021)

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Article Chemistry, Physical

A graphene assembled porous fiber-based Janus membrane for highly effective solar steam generation

Qingxin Zhou et al.

Summary: The study demonstrates that the graphene fiber-based Janus membrane evaporator shows superior performance in solar absorbance, photothermal property, and energy conversion efficiency, making it highly effective in seawater desalination and heavy metal wastewater purification.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Review Chemistry, Multidisciplinary

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Cosimo Anichini et al.

Summary: Graphene, a 2D material with outstanding physical properties, can be combined with other nanomaterials or molecules to form hybrid functional materials, showcasing new properties and enhanced characteristics. These hybrids exhibit superior performances compared to individual components in various technological applications, such as sensing, water purification, energy storage, biomedical applications, catalysis, and optoelectronics.

SMALL (2021)

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Swelling Pressures of Graphite Oxide and Graphene Oxide Membranes in Water and Ethanol

Artem Iakunkov et al.

Summary: The swelling of graphene oxide (GO) membranes and bulk graphite oxide under confinement conditions can produce high pressures, with differences observed in the pressure increase kinetics in water and ethanol. The swelling pressure is crucial for applications of GO membranes and can be used as an estimation for suction pressure in pervaporation or vapor permeation applications.

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Summary: A simple and cost-effective method was developed to prepare graphene/cellulose nanocrystals (CNCs) lamella network (GCLN) with melamine foam (MF) as the skeleton, achieving efficient evaporation under solar radiation and maintaining performance stability in harsh conditions and durability tests. With the excellent processability of MF, the 3D-shaped GCLN can be easily designed for enhanced evaporation rate.

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Wei Li et al.

Summary: The study developed a V-RGO foam with vertical channels as a solar-thermal energy converter for efficient solar steam generation, utilizing dynamic compression to adjust water's energy state. Optimal compression significantly decreased water vaporization enthalpy, resulting in a faster water evaporation rate under solar-light irradiation, offering a novel strategy for wastewater purification and seawater desalination.

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Three- dimensional nitrogen- doped holey graphene and transition metal oxide composites for sodium- ion batteries

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