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Polysaccharides-Based Injectable Hydrogels: Preparation, Characteristics, and Biomedical Applications

COLLOIDS AND INTERFACES (2022)

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Review Chemistry, Multidisciplinary

Self-Healing Injectable Hydrogels for Tissue Regeneration

Pascal Bertsch et al.

Summary: Biomaterials that can self-heal and maintain their structural integrity have significant advantages in biomedicine. Self-healing injectable hydrogels, a new type of biomaterial, have emerged in the past decade. These hydrogels can temporarily fluidize and then recover their mechanical properties under shear stress. They can be administered locally and minimally invasively, and have moldable properties for personalized medicine. Additionally, they facilitate tissue regeneration through their viscoelastic and diffusive nature. However, challenges remain in balancing self-healing and injectability with physical stability, establishing consensus on rheological characterization, and translating them into therapeutically effective formulations for specific tissues.

CHEMICAL REVIEWS (2023)

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Review Chemistry, Multidisciplinary

Copper-Free Click Chemistry: Applications in Drug Delivery, Cell Tracking, and Tissue Engineering

Hong Yeol Yoon et al.

Summary: Traditional organic chemical reactions often require organic solvents, toxic catalysts, heat, or high pressure. However, copper-free click chemistry offers a more favorable alternative with its fast reaction rates and orthogonality in water, buffer solutions, and physiological conditions without the need for toxic catalysts. This has led to its growing interest in biomedical research, where it has been used in various applications such as molecular imaging and therapy.

ADVANCED MATERIALS (2022)

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Article Chemistry, Applied

Injectable thiol-ene hydrogel of galactoglucomannan and cellulose nanocrystals in delivery of therapeutic inorganic ions with embedded bioactive glass nanoparticles

Qingbo Wang et al.

Summary: The study introduces an injectable nanocomposite hydrogel cured by light-induced thiol-ene addition, with features of faster crosslinking, more stable mechanics, and higher bioactivity, suitable for fabrication of digitally designed hydrogel constructs.

CARBOHYDRATE POLYMERS (2022)

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Article Chemistry, Applied

Preparation and characterization of Gum Arabic Schiff's bases based on 9-aminoacridine with in vitro evaluation of their antimicrobial and antitumor potentiality

Naglaa Salem El-Sayed et al.

Summary: This study successfully prepared conjugates of 9-aminoacridine (9-AA) and Gum Arabic (GA) through a Schiff's base pH-responsive bond, which exhibited broad-spectrum antimicrobial and antitumor activities. The incorporation of 9-AA into GA significantly enhanced the in vitro activities against various bacteria and fungi, showing potential for further development as therapeutic agents.

CARBOHYDRATE POLYMERS (2022)

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Article Multidisciplinary Sciences

Injectable amnion hydrogel-mediated delivery of adipose-derived stem cells for osteoarthritis treatment

Maumita Bhattacharjee et al.

Summary: Current treatment strategies for osteoarthritis (OA) mainly focus on symptom management and have limited disease-modifying effects. However, there is growing interest in using adipose-derived stem cells (ADSCs) and biomimetic injectable hydrogels as cell delivery systems for OA treatment. In this study, an amnion membrane (AM) hydrogel was developed as a biomimetic injectable hydrogel that can self-assemble and retain stem cells at the target site. The study demonstrated that both the AM hydrogel and ADSCs possess anti-inflammatory and chondroprotective properties, and their combined use can promote cartilage tissue regeneration in a rat OA model.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2022)

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Article Materials Science, Multidisciplinary

Functionalization of an Injectable Self-Healing pH-Responsive Hydrogel by Incorporating a Curcumin/Polymerized β-Cyclodextrin Inclusion Complex for Selective Toxicity to Osteosarcoma

Lun Yuan et al.

Summary: An injectable self-healing hydrogel carrying curcumin with pH-responsive drug release and selective toxicity for osteosarcoma therapy was developed, showing potential for long-term drug delivery and targeted treatment.

ACS APPLIED POLYMER MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Bioactive Injectable Hydrogel Dressings for Bacteria-Infected Diabetic Wound Healing: A Pull-Push Approach

Kunbao Zhang et al.

Summary: This study introduces a bioactive hydrogel, named OCMC-Tob/PEI hydrogel, for the treatment of infected wounds in patients with chronic diabetes. The hydrogel achieves dual effects of anti-inflammation and anti-infection by scavenging danger molecules and releasing antibiotics.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Visible-Light-Mediated Nano-biomineralization of Customizable Tough Hydrogels for Biomimetic Tissue Engineering

Hongqiu Wei et al.

Summary: A straightforward and low-cost visible-lightmediated nano-biomineralization strategy was developed for rapid preparation of Biomineralized tough hydrogels (BTHs). This strategy allows for the improvement of mechanical and biological properties of BTHs, making them suitable for applications such as skin repair and bone regeneration.

ACS NANO (2022)

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Article Materials Science, Multidisciplinary

A spray-filming, tissue-adhesive, and bioactive polysaccharide self-healing hydrogel for skin regeneration

Shuyuan Wu et al.

Summary: This study developed a multifunctional self-healing hydrogel as a wound dressing, which demonstrated strong tissue adhesion, spray film-forming ability, and excellent bioactivity. The hydrogel exhibited rapid self-healing performance, robust mechanical strength, and strong adhesion, as well as spray film-forming ability, hemostatic property, antibacterial property, and good biocompatibility. It is a promising candidate for full-thickness skin wound healing.

MATERIALS & DESIGN (2022)

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Article Chemistry, Multidisciplinary

Skin-Inspired Packaging of Injectable Hydrogel Sensors Enabled by Photopolymerizable and Swellable Hydrogels toward Sustainable Electronics

Meijin Zhao et al.

Summary: Inspired by the delamination structures of skin, researchers have developed a packaged hydrogel strain sensor (PHSS) that combines high sensitivity, linear sensing, good transparency, and conformal adhesion. The PHSS is able to accurately detect human motion and electrophysiological signals. Through the packaging strategy, the sensor's lifespan is increased, and the external hydrogel film allows for reusability.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Article Pharmacology & Pharmacy

Polymerized β-Cyclodextrin-Based Injectable Hydrogel for Sustained Release of 5-Fluorouracil/Methotrexate Mixture in Breast Cancer Management: In Vitro and In Vivo Analytical Validations

Saud Almawash et al.

Summary: An inclusion complexation of polymerized beta-cyclodextrin and cholesterol end-capping branched polyethylene glycol was used to construct a self-assembled hydrogel. The hydrogel exhibited white color, rubbery texture, and homogeneity. In vitro release studies showed sustained release of anticancer drugs for 14 days and the hydrogel demonstrated significant anti-tumor effects in vivo.

PHARMACEUTICS (2022)

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Article Pharmacology & Pharmacy

Oleyl Conjugated Histidine-Arginine Cell-Penetrating Peptides as Promising Agents for siRNA Delivery

Muhammad Imran Sajid et al.

Summary: Recent approvals of siRNA-based products have led to exploration of siRNA as a potential treatment option for cancer and other diseases. This study introduces a series of oleyl-conjugated histidine-arginine peptides as a promising nonviral siRNA delivery tool.

PHARMACEUTICS (2022)

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Article Materials Science, Multidisciplinary

Harnessing a biopolymer hydrogel reinforced by copper/tannic acid nanosheets for treating bacteria-infected diabetic wounds

Shengye You et al.

Summary: This study developed a multifunctional hydrogel wound dressing with antibacterial and ROS scavenging abilities, which can promote diabetic wound healing and restore skin physiological functions.

MATERIALS TODAY ADVANCES (2022)

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Article Biochemistry & Molecular Biology

High performance hydrogel electrodes based on sodium alginate-g-poly (AM-c o-ECA-co-AMPS for supercapacitor application

Naglaa Salem El-Sayed et al.

Summary: This study describes the rational design of a new polyanionic electrically conductive hydrogel based on sodium alginate-g-poly(AM-co-ECA-co-AMPS) and investigates the impact of rGO on the performance of the hydrogels. The chemical composition, crystalline, and morphological structure of the synthesized hydrogels were characterized using various techniques, and their electrochemical performance was evaluated through different tests. The ECH2.5 composite hydrogel exhibited promising capacitance, rate capability, and cycling stability, making it a good candidate for electrode material in supercapacitor applications.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2022)

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Article Chemistry, Physical

Coupling of 3-Aminopropyl Sulfonic Acid to Cellulose Nanofibers for Efficient Removal of Cationic Dyes

Naglaa Salem El-Sayed et al.

Summary: A novel anionic nanostructured cellulose derivate was prepared by coupling TEMPO-oxidized cellulose nanofibers with 3-aminopropyl sulfonic acid (3-APSA). The surface morphology of the cellulose nanofibers was improved after the 3-APSA coupling, resulting in enhanced adsorption capacity for methylene blue. The study suggests that chemical grafting via 3-APSA is a reliable method to design high-performance adsorbent materials for water pollutant remediation.

MATERIALS (2022)

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Review Engineering, Biomedical

Recent Advances in Injectable Hydrogels for Controlled and Local Drug Delivery

Fabio Rizzo et al.

Summary: Injectable hydrogels are of great interest in the biomedical field for their potential in controlled and localized drug delivery while limiting nonspecific drug distribution in healthy tissues. Stimuli-responsive injectable hydrogels have been designed to change shape or volume in response to environmental stimuli, ensuring optimal drug delivery to target sites.

ADVANCED HEALTHCARE MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Injectable, Intrinsically Antibacterial Conductive Hydrogels with Self-Healing and pH Stimulus Responsiveness for Epidermal Sensors and Wound Healing

Ling Fan et al.

Summary: This study developed a chitosan-based hydrogel with self-healing, conductive, and antibacterial properties, which can be used as a sensor to monitor human health in real-time and promote wound healing. The injectable hydrogel, fabricated via Schiff base linkage and hydrogen bond, shows pH responsiveness and broad-spectrum antibacterial properties.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Biochemistry & Molecular Biology

In Situ Forming Cellulose Nanofibril-Reinforced Hyaluronic Acid Hydrogel for Cartilage Regeneration

Hongbo Zhao et al.

Summary: The study demonstrates the development of a strategy integrating nanomaterials to prepare hyaluronic acid (HA) hydrogels with sufficient mechanical loading for cartilage tissue production and repair, offering a promising solution to the current challenge in cartilage tissue engineering.

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Article Chemistry, Applied

Bioactive chitosan biguanidine-based injectable hydrogels as a novel BMP-2 and VEGF carrier for osteogenesis of dental pulp stem cells

Baharak Divband et al.

Summary: Injectable hydrogels loaded with VEGF and BMP-2 promote proliferation and osteogenic differentiation of DPSCs, showing potential for bone defect treatment.

CARBOHYDRATE POLYMERS (2021)

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Article Biochemistry & Molecular Biology

Synthesis, characterization, and cytotoxicity evaluation of dextran-myristoyl-ECGKRK peptide conjugate

Naglaa Salem El-Sayed et al.

Summary: A novel drug delivery system based on myristoylated ECGKRK peptide-decorated dextran was successfully synthesized in this study, showing the ability to self-assemble into nanoparticles and potential non-toxicity in various cancer cell lines.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2021)

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Review Chemistry, Multidisciplinary

Thiolated polymeric hydrogels for biomedical application: Cross-linking mechanisms

Simona Summonte et al.

Summary: Thiomers, such as thiolated hyaluronic acid and chitosan, are widely studied for their high reactivity in hydrogel synthesis. They exhibit in situ gelling properties and can undergo various click reactions, making them versatile materials for tissue engineering, regenerative medicine, and drug delivery.

JOURNAL OF CONTROLLED RELEASE (2021)

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Review Engineering, Environmental

Polysaccharides; Classification, Chemical Properties, and Future Perspective Applications in Fields of Pharmacology and Biological Medicine (A Review of Current Applications and Upcoming Potentialities)

Aiman Saleh A. Mohammed et al.

Summary: Polysaccharides, essential macromolecules with important biological functions, have drawn increasing attention due to their wide range of biological and pharmacological activities. They can be obtained from various sources and modified to enhance their properties, making them promising candidates in biomedical and pharmaceutical fields. Challenges and limitations in their pharmaceutical utilities are also discussed.

JOURNAL OF POLYMERS AND THE ENVIRONMENT (2021)

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Article Materials Science, Biomaterials

Injectable thioketal-containing hydrogel dressing accelerates skin wound healing with the incorporation of reactive oxygen species scavenging and growth factor release

Zhen An et al.

Summary: This study developed a ROS-responsive injectable polyethylene glycol hydrogel containing thioketal bonds to deliver epidermal growth factor (EGF), effectively scavenging excessive ROS and controlling EGF release for wound regeneration. The EGF@PEG-TK hydrogel treatment showed benefits in protecting cells from oxidative stress, accelerating wound closure, and reducing scar formation in full-thickness skin defects, providing a promising strategy for antioxidant hydrogel dressing to facilitate wound repair.

BIOMATERIALS SCIENCE (2021)

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Review Biochemistry & Molecular Biology

Recent Advances in Injectable Dual Crosslinking Hydrogels for Biomedical Applications

Wenlin Chu et al.

Summary: Injectable dual crosslinking hydrogels show great promise in improving therapeutic efficacy in minimally invasive surgery, with accurate implantation into deeply enclosed sites and repair of irregular lesions. Current fabrication considerations and application progress are important for their further development and transformation in the biomedical field.

MACROMOLECULAR BIOSCIENCE (2021)

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Article Materials Science, Biomaterials

Guest-Host Supramolecular Assembly of Injectable Hydrogel Nanofibers for Cell Encapsulation

Beverly Miller et al.

Summary: This study developed a mechanically robust fibrous hydrogel with shear-thinning behavior, rapid self-healing, and cytocompatibility, suitable for minimally invasive delivery. Human mesenchymal stromal cells encapsulated in this fibrous hydrogel showed high viability and enhanced cell spreading and alignment, demonstrating its potential for cell and tissue engineering applications.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2021)

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Article Nanoscience & Nanotechnology

Mussel-Inspired Bisphosphonated Injectable Nanocomposite Hydrogels with Adhesive, Self-Healing, and Osteogenic Properties for Bone Regeneration

Bo Wang et al.

Summary: Injectable hydrogels mimicking the natural extracellular matrix have advantages such as microinvasive implantation and complex defect repair, but current options for bone repair lack tissue adhesion, self-healing, and osteogenic activity. A new strategy involving mussel-inspired bisphosphonated injectable nanocomposite hydrogels with adhesive, self-healing, and osteogenic properties has been developed, showing excellent biocompatibility and promoting cell viability, proliferation, migration, and osteogenesis differentiation. The hydrogels, dually cross-linked, also demonstrate potential for bone regeneration with the successful healing of a rat cranial defect.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Engineering, Biomedical

A supramolecular host-guest interaction-mediated injectable hydrogel system with enhanced stability and sustained protein release

Seung Yong Lee et al.

Summary: The F127-Ad/CDP hydrogel, developed through host-guest interactions, serves as a versatile protein delivery system with controllable durability and drug release characteristics. By adjusting the number of adamantane molecules in the system, the stability and injectability of the hydrogel can be modulated.

ACTA BIOMATERIALIA (2021)

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Article Engineering, Biomedical

Injectable adaptive self-healing hyaluronic acid/poly (γ-glutamic acid) hydrogel for cutaneous wound healing

Rong Yang et al.

Summary: The bionic extracellular matrix hydrogels developed in this study possess dynamic covalent network and self-healing capability, showing typical viscoelastic characteristics, degradation property, and free radical scavenging capability. The properties of the hydrogels can be tuned by adjusting polymer content, and they significantly enhance wound healing process by promoting angiogenesis and collagen deposition, demonstrating great application potential in biomedical areas.

ACTA BIOMATERIALIA (2021)

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Article Biology

Fabrication of alginate-based hydrogel cross-linked via horseradish peroxidase for articular cartilage engineering

Sepideh Saghati et al.

Summary: The study found that Alg, HRP, and H2O2 concentrations affect the gelation time of Alg-based hydrogels, and proper ratios can result in appropriate biomaterials.

BMC RESEARCH NOTES (2021)

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Article Biochemical Research Methods

Targeted Delivery of Cabazitaxel Using Cyclic Cell-Penetrating Peptide and Biomarkers of Extracellular Matrix for Prostate and Breast Cancer Therapy

Shang Eun Park et al.

Summary: Targeted drug delivery for cancer therapy is being explored using cyclic cell-penetrating peptides conjugated with chemotherapeutic agents. The conjugates demonstrated reduced proliferation of cancer cells overexpressing specific biomarkers, while being less toxic to normal cells. This strategy shows potential in enhancing the efficacy and specificity of chemotherapeutic agents.

BIOCONJUGATE CHEMISTRY (2021)

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Article Chemistry, Applied

Fabrication of self-healing pectin/chitosan hybrid hydrogel via Diels-Alder reactions for drug delivery with high swelling property, pH-responsiveness, and cytocompatibility

De-qiang Li et al.

Summary: A self-healing pectin/chitosan hydrogel with pH-responsiveness was prepared in this study, greatly improving its performance through the Diels-Alder reaction and showing excellent self-healing capability and cytocompatibility.

CARBOHYDRATE POLYMERS (2021)

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Article Biochemistry & Molecular Biology

Preparation and characterization of a dual cross-linking injectable hydrogel based on sodium alginate and chitosan quaternary ammonium salt

Zhijie Geng et al.

Summary: The dual crosslinking hydrogel prepared using chitosan quaternary ammonium salt and sodium alginate demonstrated continuous injectability, a homogeneous 3D network structure, and good mechanical properties. It also showed excellent biocompatibility with non-toxicity towards NIH-3T3 cells, making it an ideal biomaterial for further applications in the field of biomedical engineering.

CARBOHYDRATE RESEARCH (2021)

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Article Biochemistry & Molecular Biology

Dual-enzymatically cross-linked gelatin hydrogel promotes neural differentiation and neurotrophin secretion of bone marrow-derived mesenchymal stem cells for treatment of moderate traumatic brain injury

Jinrui Li et al.

Summary: A novel injectable gelatin hydrogel scaffold enhances neural regeneration for TBI treatment. Low-crosslinked gelatin hydrogel promotes cell survival and neural differentiation, enhances neurotrophins secretion from BMSC. BMSC-laden gelatin hydrogel implants significantly reduce damaged area, improve inflammation, attenuate neuronal apoptosis, promote endogenous neural cell survival and proliferation, and enhance neurological function recovery in TBI mice.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2021)

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Article Materials Science, Biomaterials

Injectable nanofiber-polysaccharide self-healing hydrogels for wound healing

Hongyun Xuan et al.

Summary: A novel hydrogel based on carboxymethyl chitosan and aldehyde functionalized sodium alginate was developed with the addition of carboxymethyl-functionalized polymethyl methacrylate short nanofibers. The hydrogel demonstrated excellent injectability and self-healing abilities, as well as significantly promoting wound healing in rats according to in vivo experiments.

MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS (2021)

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Article Materials Science, Biomaterials

Synergy coordination of cellulose-based dialdehyde and carboxyl with Fe3+ recoverable conductive self-healing hydrogel for sensor

Ying Wang et al.

Summary: A novel dual ionic network cellulose-based composite conductive self-healing hydrogel was developed with high elongation, rapid recoverability, high conductive sensitivity, and good biocompatibility. The addition of DACNFs in the hydrogel increased the self-healing efficiency and stretching sensitivity.

MATERIALS SCIENCE AND ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS (2021)

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Article Materials Science, Biomaterials

Tannic acid-inspired, self-healing, and dual stimuli responsive dynamic hydrogel with potent antibacterial and anti-oxidative properties

Wen Shi et al.

Summary: Dynamic hydrogels based on boronic ester dynamic covalent bonds exhibit good self-healing and shear-thinning capabilities, and the utilization of TA for the green synthesis of silver nanoparticles resulted in a hybrid dynamic hydrogel with potent antibacterial activities. Moreover, these hydrogels can release loaded proteins in response to pH and ROS, while also showing high free radical and ROS scavenging capacities for anti-oxidative properties.

JOURNAL OF MATERIALS CHEMISTRY B (2021)

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Review Materials Science, Biomaterials

Advances in multifunctional chitosan-based self-healing hydrogels for biomedical applications

Yi Ou et al.

Summary: Chitosan, a natural polycationic polysaccharide, plays a vital role in the formation of self-healing hydrogels with multiple functionalities. The self-healing mechanisms involve various physical and chemical interactions, providing strategies for multifunctionalization. Additionally, chitosan-based self-healing hydrogels find wide applications in wound dressings, delivery vehicles, scaffolds, and biological sensors.

JOURNAL OF MATERIALS CHEMISTRY B (2021)

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Carboxymethyl Cellulose-Based Hydrogel: Dielectric Study, Antimicrobial Activity and Biocompatibility

Gamal Turky et al.

Summary: This study investigated the antimicrobial activity, biocompatibility, and electrical conductivity of polypyrrole on conducting hydrogels. The results showed that the addition of polypyrrole improved the conductivity and permittivity of the hydrogels, reduced energy loss, and maintained good compatibility with cells. The prepared hydrogels also demonstrated strong potential for energy storage systems and displayed excellent antimicrobial activity against various pathogens.

ARABIAN JOURNAL FOR SCIENCE AND ENGINEERING (2021)

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Synergistic enhancement of tendon-to-bone healing via anti-inflammatory and pro-differentiation effects caused by sustained release of Mg2+/curcumin from injectable self-healing hydrogels

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Summary: A composite hydrogel was developed for promoting rotator cuff tendon-to-bone healing through sustained release of curcumin and Mg2+, demonstrating significant anti-inflammatory and pro-differentiation effects. The hydrogel exhibited excellent biocompatibility and injectability, and enhanced tendon-to-bone healing in a rat model of rotator cuff tear at 8 weeks post-surgery.

THERANOSTICS (2021)

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A Novel Double-Crosslinking-Double-Network Design for Injectable Hydrogels with Enhanced Tissue Adhesion and Antibacterial Capability for Wound Treatment

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POLYMER (2020)

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An injectable click-crosslinked hyaluronic acid hydrogel modified with a BMP-2 mimetic peptide as a bone tissue engineering scaffold

Seung Hun Park et al.

ACTA BIOMATERIALIA (2020)

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Redox and pH dual-responsive injectable hyaluronan hydrogels with shape-recovery and self-healing properties for protein and cell delivery

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Adhesive, Self-Healing, and Antibacterial Chitosan Hydrogels with Tunable Two-Layer Structures

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Carrageenan-based physically crosslinked injectable hydrogel for wound healing and tissue repairing applications

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Calogero Fiorica et al.

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JOURNAL OF MATERIALS CHEMISTRY B (2020)

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Luyu Wang et al.

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A novel injectable in situ forming gel based on carboxymethyl hexanoyl chitosan/hyaluronic acid polymer blending for sustained release of berberine

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Yujie Zhong et al.

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Injectable hydrogels from enzyme-catalyzed crosslinking as BMSCs-laden scaffold for bone repair and regeneration

Yajie Zhang et al.

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Recent Progress of Polysaccharide-Based Hydrogel Interfaces for Wound Healing and Tissue Engineering

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ADVANCED MATERIALS INTERFACES (2019)

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Review Biochemistry & Molecular Biology

Hydrogels Based on Schiff Base Linkages for Biomedical Applications

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Injectable Hydrogels for Cancer Therapy over the Last Decade

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PHARMACEUTICS (2019)

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Chemical gelling of hydrogels-based biological macromolecules for tissue engineering: Photo- and enzymatic-crosslinking methods

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INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2019)

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Design of injectable hydrogels of gelatin and alginate with ferric ions for cell transplantation

Mina Anamizu et al.

ACTA BIOMATERIALIA (2019)

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Cellulose-based injectable hydrogel composite for pH-responsive and controllable drug delivery

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Click Chemistry as a Tool for Cell Engineering and Drug Delivery

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MOLECULES (2019)

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An in vitro and in vivo comparison of cartilage growth in chondrocyte-laden matrix metalloproteinase-sensitive poly(ethylene glycol) hydrogels with localized transforming growth factor β3

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ACTA BIOMATERIALIA (2019)

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Article Chemistry, Multidisciplinary

Supramolecular nanofibrillar hydrogels as highly stretchable, elastic and sensitive ionic sensors

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Polysaccharide-Based Hybrid Self-Healing Hydrogel Supports the Paracrine Response of Mesenchymal Stem Cells

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Self-assembled supramolecular thermoreversible beta-cyclodextrin/ethylene glycol injectable hydrogels with difunctional Pluronic (R) 127 as controlled delivery depot of curcumin. Development, characterization and in vitro evaluation

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Strengthening injectable thermo-sensitive NIPAAm-g-chitosan hydrogels using chemical cross-linking of disulfide bonds as scaffolds for tissue engineering

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CARBOHYDRATE POLYMERS (2018)

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Injectable hydrogels based on the hyaluronic acid and poly (γ-glutamic acid) for controlled protein delivery

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New approach for immobilization of 3-aminopropyltrimethoxysilane and TiO2 nanoparticles into cellulose for BJ1 skin cells proliferation

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CARBOHYDRATE POLYMERS (2018)

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Biological activities and pharmaceutical applications of polysaccharide from natural resources: A review

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Rational design of novel water-soluble ampholytic cellulose derivatives

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Synthesis, characterization, and in vitro cytotoxicity of fatty acyl-CGKRK-chitosan oligosaccharides conjugates for siRNA delivery

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Injectable hydrogels for delivering biotherapeutic molecules

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Schiff base-containing dextran nanogel as pH-sensitive drug delivery system of doxorubicin: Synthesis and characterization

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Injectable in situ cross-linking hyaluronic acid/carboxymethyl cellulose based hydrogels for drug release

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High encapsulation and localized delivery of curcumin from an injectable hydrogel

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Cyclodextrin-based host-guest supramolecular hydrogel and its application in biomedical fields

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Flexible, Stretchable Sensors for Wearable Health Monitoring: Sensing Mechanisms, Materials, Fabrication Strategies and Features

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High performance strain sensors based on chitosan/carbon black composite sponges

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An injectable self-healing hydrogel with adhesive and antibacterial properties effectively promotes wound healing

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Tannic Acid Physically Cross-Linked Responsive Hydrogel

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Injectable Hydrogels for Regenerative Medicine

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TISSUE ENGINEERING AND REGENERATIVE MEDICINE (2018)

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Dual Function Injectable Hydrogel for Controlled Release of Antibiotic and Local Antibacterial Therapy

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The production of injectable hydrazone crosslinked gellan gum-hyaluronan-hydrogels with tunable mechanical and physical properties

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Schiff base bond-linked polysaccharide-doxorubicin conjugate for upregulated cancer therapy

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Wearable, Healable, and Adhesive Epidermal Sensors Assembled from Mussel-Inspired Conductive Hybrid Hydrogel Framework

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Polysaccharides based injectable hydrogel compositing bio-glass for cranial bone repair

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Nature-Inspired Structural Materials for Flexible Electronic Devices

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Syntheses of New Antimicrobial Cellulose Materials Based 2-((2-aminoethyl)amino)-4-aryl-6-indolylnicotinonitriles

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EGYPTIAN JOURNAL OF CHEMISTRY (2017)

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pH-responsive self-healing injectable hydrogel based on N-carboxyethyl chitosan for hepatocellular carcinoma therapy

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ACTA BIOMATERIALIA (2017)

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Pullulan microbeads/Si-HPMC hydrogel injectable system for the sustained delivery of GDF-5 and TGF-β1: new insight into intervertebral disc regenerative medicine

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Antibacterial anti-oxidant electroactive injectable hydrogel as self-healing wound dressing with hemostasis and adhesiveness for cutaneous wound healing

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Hydrogels for Biomedical Applications: Their Characteristics and the Mechanisms behind Them

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GELS (2017)

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Redox-Sensitive Hydroxyethyl Starch-Doxorubicin Conjugate for Tumor Targeted Drug Delivery

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High-Performance Strain Sensors with Fish-Scale-Like Graphene-Sensing Layers for Full-Range Detection of Human Motions

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Article Engineering, Biomedical

The functional response of alginate-gelatin-nanocrystalline cellulose injectable hydrogels toward delivery of cells and bioactive molecules

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ACTA BIOMATERIALIA (2016)

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Article Biochemistry & Molecular Biology

Improved Mechanical Properties and Sustained Release Behavior of Cationic Cellulose Nanocrystals Reinforeced Cationic Cellulose Injectable Hydrogels

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Click Chemistry in Biomaterials, Nanomedicine, and Drug Delivery

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Design, synthesis, and evaluation of chitosan conjugated GGRGDSK peptides as a cancer cell-targeting molecular transporter

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INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2016)

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pH and Redox Dual Stimuli-Responsive Injectable Hydrogels Based on Carboxymethyl Cellulose Derivatives

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MACROMOLECULAR RESEARCH (2016)

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Review Materials Science, Biomaterials

Polysaccharide based nanogels in the drug delivery system: Application as the carrier of pharmaceutical agents

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MATERIALS SCIENCE AND ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS (2016)

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Cyclic Peptide Containing Hydrophobic and Positively Charged Residues as a Drug Delivery System for Curcumin

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CURRENT DRUG DELIVERY (2016)

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Visible-light-initiated hydrogels preserving cartilage extracellular signaling for inducing chondrogenesis of mesenchymal stem cells

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A nucleoside responsive diaminotriazine-based hydrogen bonding strengthened hydrogel

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Crosslinking biopolymers for biomedical applications

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TRENDS IN BIOTECHNOLOGY (2015)

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Engineered Microtissues Formed by Schiff Base Crosslinking Restore the Chondrogenic Potential of Aged Mesenchymal Stem Cells

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ADVANCED HEALTHCARE MATERIALS (2015)

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Article Cell & Tissue Engineering

A Hyaluronan-Based Injectable Hydrogel Improves the Survival and Integration of Stem Cell Progeny following Transplantation

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STEM CELL REPORTS (2015)

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Hydrogel: Preparation, characterization, and applications: A review

Enas M. Ahmed

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Biomedical Applications of Supramolecular Systems Based on Host-Guest Interactions

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CHEMICAL REVIEWS (2015)

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Supramolecular Polymers Constructed from Macrocycle-Based Host-Guest Molecular Recognition Motifs

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ACCOUNTS OF CHEMICAL RESEARCH (2014)

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Review Chemistry, Multidisciplinary

Cyclodextrin-Based Host-Guest Supramolecular Nanoparticles for Delivery: From Design to Applications

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ACCOUNTS OF CHEMICAL RESEARCH (2014)

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In vivo assessment of guided neural stem cell differentiation in growth factor immobilized chitosan-based hydrogel scaffolds

Hang Li et al.

BIOMATERIALS (2014)

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A novel thermo-sensitive hydrogel based on thiolated chitosan/hydroxyapatite/beta-glycerophosphate

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CARBOHYDRATE POLYMERS (2014)

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Editorial Material Polymer Science

In situ-forming injectable hydrogels for regenerative medicine

Jeong-A. Yang et al.

PROGRESS IN POLYMER SCIENCE (2014)

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Flexible Carbon Nanotube Films for High Performance Strain Sensors

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SENSORS (2014)

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Smart hydrogels as functional biomimetic systems

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BIOMATERIALS SCIENCE (2014)

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Supramolecular host-guest polymeric materials for biomedical applications

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Injectable Nano-Network for Glucose-Mediated Insulin Delivery

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ACS NANO (2013)

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Review Pharmacology & Pharmacy

Novel crosslinking methods to design hydrogels

W. E. Hennink et al.

ADVANCED DRUG DELIVERY REVIEWS (2012)

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Enzyme-catalyzed crosslinkable hydrogels: Emerging strategies for tissue engineering

Liliana S. Moreira Teixeira et al.

BIOMATERIALS (2012)

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Stimuli-responsive supramolecular polymeric materials

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CHEMICAL SOCIETY REVIEWS (2012)

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Design and characterization of a novel amphiphilic chitosan nanocapsule-based thermo-gelling biogel with sustained in vivo release of the hydrophilic anti-epilepsy drug ethosuximide

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JOURNAL OF CONTROLLED RELEASE (2012)

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Review Polymer Science

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JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS (2012)

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Tunable Growth Factor Delivery from Injectable Hydrogels for Tissue Engineering

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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In-situ forming biodegradable glycol chitosan-based hydrogels: Synthesis, characterization, and chondrocyte culture

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MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS (2012)

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Click Chemistry with Polymers, Dendrimers, and Hydrogels for Drug Delivery

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PHARMACEUTICAL RESEARCH (2012)

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Article Engineering, Biomedical

Enzyme-mediated cross-linking of Pluronic copolymer micelles for injectable and in situ forming hydrogels

Soo Hyeon Lee et al.

ACTA BIOMATERIALIA (2011)

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Article Biochemistry & Molecular Biology

Synthesis of Multiresponsive and Dynamic Chitosan-Based Hydrogels for Controlled Release of Bioactive Molecules

Yaling Zhang et al.

BIOMACROMOLECULES (2011)

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Cellulose nanowhisker aerogels

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GREEN CHEMISTRY (2010)

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Article Chemistry, Physical

Injectable solid hydrogel: mechanism of shear-thinning and immediate recovery of injectable beta-hairpin peptide hydrogels

Congqi Yan et al.

SOFT MATTER (2010)

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Article Engineering, Biomedical

Injectable in situ forming biodegradable chitosan-hyaluronic acid based hydrogels for cartilage tissue engineering

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BIOMATERIALS (2009)

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Synthesis of thermosensitive P(NIPAAm-co-HEMA)/cellulose hydrogels via click chemistry

Jing Zhang et al.

CARBOHYDRATE POLYMERS (2009)

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Review Pharmacology & Pharmacy

Polysaccharides-based nanoparticles as drug delivery systems

Zonghua Liu et al.

ADVANCED DRUG DELIVERY REVIEWS (2008)

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Review Multidisciplinary Sciences

Wound repair and regeneration

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NATURE (2008)

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Article Biochemistry & Molecular Biology

Glutaraldehyde and glyoxal cross-linked chitosan microspheres for controlled delivery of centchroman

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CARBOHYDRATE RESEARCH (2006)

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