4.7 Article

Electro-coagulation coupled with solid carrier enhanced GDCMBR as pretreatment for NF dual membrane system during surface brackish water treatment

期刊

JOURNAL OF CLEANER PRODUCTION
卷 380, 期 -, 页码 -

出版社

ELSEVIER SCI LTD
DOI: 10.1016/j.jelepro.2022.135021

关键词

Gravity-driven membrane filtration; Biofilm; Ceramic membrane; Electro-coagulation; Solid carriers

资金

  1. National Natural Science Foundation of China
  2. Natural Science Foundation of Guangdong Province, China
  3. [52170070]
  4. [2021A1515012275]

向作者/读者索取更多资源

The novel EC-GDCMBR-NF dual membrane system was tested for long-term treatment of surface brackish water. The system showed high flux and effective removal of organic substances, particulate matters, NH3-N, and micropollutants. This study demonstrates the potential of the system for brackish water purification.
The novel electmcoagulation (EC) coupled with solid carriers enhanced gravity-driven ceramic membrane bioreactor (GDCMBR) as pretreatment for nanofiltration (NF) dual membrane system was conducted to surface brackish water treatment for long-term (85 days) operation, at a current density of 2 mA/cm(2) and hydraulic retention time of 9 min, 172 min for EC cell, GDCMBR with solid carriers respectively. Warm operation condition was beneficial to improve permeate flux, and it can reach up to 33.0 L/m(2)/h at similar to 25 degrees C. In particular, the addition of solid carriers endowed the EC-GDCMBR system with a higher stable flux, due to the mitigation of fouling layer. The biofilms on the filler and membrane enabled to completely remove NH3-N via biological nitrification and denitrification, verifying by the progressive growth of Nitrospira, Bacteroide and Helicobacter in high-throughput sequencing. In EC-GDCMBR pretreatment, the organic substances and particulate matters could be effectively eliminated. Owing to the hypersaline property of surface brackish water, the electric flocculation effect was obviously enhanced, especially for UV254 removal. Moreover, the subsequent NF unit played a major role in dislodging the hardness and salinity from the final effluent. In addition, EC-GDCMBR-NF dual membrane system also enabled to remove micmpollutants (i.e. antibiotics), in which the purification mechanism could be ascribed to the biofilm adsorption and NF membrane rejection. Overall, the results of this study suggest the potential for long-term operation during brackish water purification.

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