期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 4, 期 41, 页码 9687-9696出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6tc02629j
关键词
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资金
- National Natural Science Foundation [51373013, 50903004]
- Beijing Young Talents Plan [YETP0489]
- BUCT Fund for Disciplines Construction and Development [XK1509]
We have developed a cellulose nanocrystal-based nanocomposite photonic film with a sandwich structure to mimic the shell structure of the Chrysina genus of beetles. The nanocomposite film was fabricated by embedding a uniaxially oriented polyamide-6 (PA-6) layer as a half-wave retarder layer between two cellulose nanocrystals (CNCs)/polyethylene glycol diacrylate (PEGDA) layers with a left-handed chiral nematic photonic structure. As a result, the reflectance intensity of the obtained nanocomposite film exceeds 50% (hyper-reflection) at a certain wavelength. More interestingly, asymmetric expansion/shrinkage of the CNCs/PEGDA layer in the nanocomposite film allows for simultaneous and reversible three-dimensional deformation behavior as well as the shift of the Bragg reflection when exposed to a humid environment. The proposed self-assembled photonic material will be attractive to be used as an optical anti-counterfeiting film, a tunable bandpass filter, a reflector or polarizer and a humidity-responsive actuator.
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