期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 4, 期 18, 页码 7020-7026出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ta10550a
关键词
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资金
- Human Resources Development program of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korean Ministry of Trade, Industry, and Energy [20154010200840]
- National Research Foundation of Korea (NRF) - Ministry of Science, ICT, and Future Planning [NRF-2014R1A2A1A11049801]
Despite the extremely high theoretical specific capacity of lithium oxygen (Li-O-2) electrochemistry, low energy efficiency resulting from the large potential gap between the discharge and charge makes this system impractical. In this report, an iron cobalt bimetal decorated carbon nanotube (FeCo-CNT) composite was synthesized as a catalytic air cathode material for Li-O-2 batteries. An Li-O-2 battery using FeCo-CNT air electrodes exhibited higher efficiency (72.15%) than that of pristine CNTs (62.57%) as well as higher capacity (3600 mA h g(-1) vs. 1276 mA h g(-1)). Spectroscopic and electron microscopy analyses showed that the improved cell performances can be attributed to the catalytic effect of FeCo. As cost-effective non-noble metal catalysts, FeCo-CNTs demonstrated performance comparable to noble metal catalysts in Li-O-2 systems.
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