期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 4, 期 35, 页码 13582-13588出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ta04432h
关键词
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资金
- Repsol, S. A.
- European Regional Development Funds (ERDF)
- European Regional Development Funds (FEDER)
- MINECO [ENE2012-3651, MAT2014-59961-C2-1-R]
- AGAUR [FI-2013-B-00769]
Tin electrodeposition on carbon fibers have been implemented for gas diffusion electrodes for the electroreduction of CO2 to formate in a electrochemical flow cell design. Unlike other approaches, this method does not incorporate any additive or binder in the electrode, thus improving their catalytic performances. Once optimized, the system shows an improved dependence of the effective production of formate yield by surface and time units, mol m(-2) s(-1), on the consumed energy by mol, W h mol(-1). It reduces the formic acid production energy cost, requiring less than 250 W h mol(-1), with formate faradaic efficiency as high as 71% and is fully stable for at least 6 hours.
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