期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 4, 期 42, 页码 16454-16461出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ta06285g
关键词
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资金
- China Scholarship Council [201506165038]
- Natural Science Foundation of Hubei Province [ZRZ2015000203]
- Technology Creative Project of Excellent Middle & Young Team of Hubei Province [T201511]
- Director Fund of the WNLO
In this study, we report hierarchical TiO2 sphere-sulfur frameworks assisted with graphene as a cathode material for high performance lithium-sulfur batteries. With this strategy, the volume expansion and aggregation of sulfur nanoparticles can be effectively mitigated, thus enabling high sulfur utilization and improving the specific capacity and cycling stability of the electrode. Modification of the TiO2-S nanocomposites with graphene can trap the polysulfides via chemisorption and increase the electronic connection among various components. The graphene-assisted TiO2-S composite electrodes exhibit high specific capacity of 660 mA h g(-1) at 5C with a capacity loss of only 0.04% per cycle in the prolonged charge-discharge processes at 1C.
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