期刊
JOURNAL OF ENERGY CHEMISTRY
卷 25, 期 4, 页码 566-570出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jechem.2016.02.012
关键词
Mesoporous ordered carbon; Oxygen reduction reaction; Electrocatalyst; Heteroatom doping; In-situ synthesis
资金
- University of Electronic Science and Technology of China [Y02002010301080]
- National Science Foundation of China [51502032]
- Natural Science Foundation of Zhejiang Province [LQ14E020003]
Metal-free, heteroatom functionalized carbon-based catalysts have made remarkable progress in recent years in a wide range of applications related to energy storage and energy generation. In this study, high surface area mesoporous ordered sulphur doped carbon materials are obtained via one-pot hydrothermal synthesis of carbon/SBA-15 composite after removal of in-situ synthesized hard template SiO2. 2-thiophenecarboxy acid as sulphur source gives rise to sulphur doping level of 5.5 wt%. Comparing with pristine carbon, the sulphur doped mesoporous ordered carbon demonstrates improved electro-catalytic activity in the oxygen reduction reaction in alkaline solution. (C) 2016 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
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