A microporous dysprosium-based MOF for selective CO2 capture at ambient temperature

Article Chemistry, Multidisciplinary

A Highly Stable Yttrium Organic Framework as a Host for Optical Thermometry and D2O Detection

Thomas W. Chamberlain et al.

Summary: The yttrium organic framework is stable under hydrothermal and air conditions, and can be used as a ratiometric luminescent thermometer and a D2O sensor with high sensitivity.

CHEMISTRY-A EUROPEAN JOURNAL (2022)

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Article Chemistry, Multidisciplinary

Binary Solvent System Composed of Polar Protic and Polar Aprotic Solvents for Controlling the Dimensionality of MOFs in the Solvothermal Synthesis

Rajib Moi et al.

Summary: The nature of solvent, pH, temperature, reactant stoichiometry, concentration of precursors, and counterions are crucial factors that influence the synthesis of MOFs. These parameters play a role in determining the formation of crystalline product and dictate the overall network dimension or topology.

CRYSTAL GROWTH & DESIGN (2022)

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Article Chemistry, Multidisciplinary

Temperature-Induced Structural Transformations of Lanthanide Coordination Polymers Based on a Semirigid Tricarboxylic Acid Ligand: Crystal Structures and Luminescence Properties

Mei-Yu Xu et al.

Summary: Three novel types of lanthanide coordination polymers were successfully synthesized via a hydrothermal method. The 1D chain and 3D Ln-MOFs can transform into a more stable 0D cage structure through temperature-induced ligand's configuration transformation. The materials were characterized using various analytical techniques, and it was found that the 3D Eu-MOFs exhibit good sensitivity and selectivity towards Fe3+ ions in methanol solutions.

CRYSTAL GROWTH & DESIGN (2022)

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Article Chemistry, Multidisciplinary

Robust and Radiation-Resistant Hofmann-Type Metal-Organic Frameworks for Record Xenon/Krypton Separation

Jiyan Pei et al.

Summary: This paper reports on the discovery of two robust and radiation-resistant MOFs with adjacent metal sites and perfect pore sizes that can efficiently separate xenon from krypton. These materials exhibit record-high xenon uptake capacities and selectivities, and the locations of xenon molecules within one of the MOFs were visualized using single-crystal X-ray diffraction.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Review Chemistry, Physical

Research progress in metal-organic frameworks (MOFs) in CO2 capture from post-combustion coal-fired flue gas: characteristics, preparation, modification and applications

Zhiqiang Sun et al.

Summary: In this review, the characteristics, preparation methods, modification methods, and applications of metal-organic frameworks (MOFs) for CO2 capture in post-combustion coal-fired flue gas are discussed. The use of machine learning in the development and screening of MOFs is also explored. The review aims to provide technical and theoretical guidance for the development and industrial application of high-performance MOF materials for CO2 capture in the post-combustion coal-fired flue gas.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Nanoscience & Nanotechnology

Mixed-Ligand Metal-Organic Frameworks for All-in-One Theranostics with Controlled Drug Delivery and Enhanced Photodynamic Therapy

Hui Zhang et al.

Summary: This study reports a versatile mixed-porphyrin ligand MOF as a multifunctional matrix for multimodality-guided synergistic therapy. The MOFs exhibit excellent fluorescence, MR, and photothermal trimodality imaging, redox-responsive drug release, and enhanced PDT/PTT.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Physical

Pore-Nanospace Engineering of Mixed-Ligand Metal-Organic Frameworks for High Adsorption of Hydrofluorocarbons and Hydrochlorofluorocarbons

Yang-Yang Xiong et al.

Summary: The isostructural mixed-ligand metal-organic frameworks (MOFs) have been developed for efficient adsorption of hydrofluorocarbon (HFC) and hydrochlorotluorocarbon (HCFC). The introduction of methyl groups in the MOFs enables fine regulation of greenhouse gas adsorption performance.

CHEMISTRY OF MATERIALS (2022)

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Article Chemistry, Inorganic & Nuclear

The Chemistry of Zirconium/Carboxylate Clustering Process: Acidic Conditions to Promote Carboxylate-Unsaturated Octahedral Hexamers and Pentanuclear Species

Jon Pascual-Colino et al.

Summary: This study investigates the initial stages of zirconium-carboxylate clustering process in alcohol/water mixtures. By controlling the chemistry, six new compounds have been isolated, providing a new building block for the design of metal-organic materials.

INORGANIC CHEMISTRY (2022)

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Article Chemistry, Inorganic & Nuclear

Two Multiresponsive Luminescent Zn-MOFs for the Detection ofDifferent Chemicals in Simulated Urine and Antibiotics/Cations/Anions in Aqueous Media

Guoxuan Xian et al.

Summary: Two Zn-MOFs with high water stability and luminescence sensing performance were synthesized and found to be able to detect organic solvents, ions, antibiotics, and chemicals in simulated urine with excellent anti-interference ability and recyclability.

INORGANIC CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

Electrostatic Secondary-Sphere Interactions That Facilitate Rapid and Selective Electrocatalytic CO2 Reduction in a Fe-Porphyrin-Based Metal-Organic Framework

Ran Shimoni et al.

Summary: This study demonstrates the significant enhancement of CO2 reduction activity and selectivity by electrostatic secondary-sphere functionalities in MOF materials. In situ Raman analysis reveals that immobilizing pendent positively-charged groups adjacent to MOF-residing Fe-porphyrin catalysts stabilizes weakly-bound CO intermediates and allows for control of the catalytic reaction by varying the ionic strength of the electrolyte.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Inorganic & Nuclear

Two Robust Isoreticular Metal-Organic Frameworks with Different Interpenetration Degrees Exhibiting Disparate Breathing Behaviors

Yueying Zhu et al.

Summary: This paper reports two stable metal-organic frameworks (MOFs) with different interpenetration degrees. These frameworks were constructed using the hard-soft acid-base (HSAB) theory and structural regulation strategy, and their potential applications in gas separation were demonstrated.

INORGANIC CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

Radicals Scavenging MOFs Enabling Targeting Delivery of siRNA for Rheumatoid Arthritis Therapy

Lina Guo et al.

Summary: A targeted nanomedicine based on metal-organic frameworks (MOFs) is developed to re-educate diseased macrophages for rheumatoid arthritis (RA) therapy. The nanomedicine effectively down-regulates cytokines and eliminates reactive oxygen and nitrogen species, repolarizing macrophages and achieving excellent anti-RA efficacy in a mice model.

SMALL (2022)

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Article Chemistry, Physical

A Binuclear Cerium-Based Metal-Organic Framework as an Artificial Monooxygenase for the Saturated Hydrocarbon Aerobic Oxidation with High Efficiency and High Selectivity

Guanfeng Ji et al.

Summary: An artificial binuclear cerium monooxygenase catalyst with high selectivity and activity for oxidation of inert C-H bonds was obtained by constructing a metal-organic framework (MOF) with active sites similar to natural enzymes. The MOF exhibited a unique catalytic performance and could be recycled without loss of selectivity and activity, providing a blueprint for designing new artificial monooxygenase for inert alkane oxidation.

ACS CATALYSIS (2022)

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Article Chemistry, Multidisciplinary

VOC Mixture Sensing with a MOF Film Sensor Array: Detection and Discrimination of Xylene Isomers and Their Ternary Blends

Peng Qin et al.

Summary: In this study, an array of sensors coated with metal-organic frameworks (MOFs) is used to detect and identify ternary xylene isomer mixtures. Molecular simulations provide insights into the sensing mechanism, and guidelines for detecting complex mixtures of volatile molecules are provided.

ACS SENSORS (2022)

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Review Chemistry, Inorganic & Nuclear

Regeneration strategies for metal-organic frameworks post acidic gas capture

Nishesh Kumar Gupta et al.

Summary: This article provides a comprehensive review of various methods for the regeneration of MOFs after capturing H2S, SO2, and NO2. Pressure and temperature swing methods can reactivate MOFs after physical adsorption of gases. Although regenerating MOFs with chemisorbed sulfurous gases poses more difficulties, reactivation strategies such as solvent and ultraviolet irradiation-based treatments can be recommended.

COORDINATION CHEMISTRY REVIEWS (2022)

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Article Chemistry, Multidisciplinary

Next steps for solvent-based CO2 capture; integration of capture, conversion, and mineralisation

David J. Heldebrant et al.

Summary: This article details how solvent-based carbon capture integrated with conversion can play a crucial role in achieving a net-zero emission economy. By integrating solvent-based CO2 capture and conversion, it is possible to produce CO2-derived fuels, chemicals, and materials more efficiently and at a lower cost, while also providing new reactive pathways for the production of products that cannot be made today. The article also discusses the key role of solvents in integration and emphasizes their adaptability to different needs in capture, conversion, and mineralization.

CHEMICAL SCIENCE (2022)

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Article Chemistry, Physical

Devising ultra-robust mixed-matrix membrane separators using functionalized MOF-poly(phenylene oxide) for high-performance vanadium redox flow batteries

Prerana Sharma et al.

Summary: A novel hybrid polymer membrane based on an ionic metal-organic framework (IMOF) has been synthesized and shown outstanding performance in vanadium redox flow batteries (VRFBs), making it a promising candidate for the storage of renewable energy.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Physical

Solvent dependent Zinc(II) coordination polymers with 1,3,5-benzenetricarboxylic acid and the selective photocatalytic degradation for organic dyes

Fang-Kuo Wang et al.

Summary: Three zinc coordination polymers with different structures were synthesized, using different solvents to construct lattice networks of different dimensions. One of the compounds was found to exhibit selective photocatalytic degradation for organic dyes.

JOURNAL OF MOLECULAR STRUCTURE (2021)

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Article Chemistry, Physical

Synthesis and spectroscopic properties of two different structural Schiffbase Zn(II) complexes constructed with/without auxiliary ligands

Shu-Zhen Zhang et al.

Summary: Two Schiffbase binuclear Zn(II) complexes with different crystal structures were synthesized, with the introduction of auxiliary ligand 4,4'-bpy leading to significant changes in the structure and fluorescence properties of the complexes.

JOURNAL OF MOLECULAR STRUCTURE (2021)

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Article Chemistry, Multidisciplinary

Charge Transportation in Zn(II)/Cd(II)-Based 2D MOFs of 5-Nitro-isophthalate with Isonicotinic Hydrazide

Kaushik Naskar et al.

Summary: Two new families of electro-conductive 2D metal organic frameworks (MOFs) of Zn(II)/Cd(II) with different structural topologies and electron transport capabilities have been isolated and characterized. The larger Cd(II) cation size and stronger pi-pi stacking in sample 2 may contribute to its higher charge mobility compared to sample 1.

CRYSTAL GROWTH & DESIGN (2021)

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Review Chemistry, Multidisciplinary

MOF-Based Membranes for Gas Separations

Qihui Qian et al.

CHEMICAL REVIEWS (2020)

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Review Chemistry, Inorganic & Nuclear

A practical guide to calculate the isosteric heat/enthalpy of adsorptionviaadsorption isotherms in metal-organic frameworks, MOFs

Alexander Nuhnen et al.

DALTON TRANSACTIONS (2020)

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Article Environmental Sciences

Outlook of carbon capture technology and challenges

Tabbi Wilberforce et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2019)

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Review Nanoscience & Nanotechnology

Trends in Solid Adsorbent Materials Development for CO2 Capture

Maryam Pardakhti et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Physical

被撤回的出版物: Temperature induced two new trinuclear Co(II) cluster-based compounds: Luminescent, photocatalytic and anti-breast cancer properties (Retracted article. See vol. 1275, 2023)

Yong Hong et al.

JOURNAL OF MOLECULAR STRUCTURE (2019)

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Article Engineering, Chemical

Liquid-Assisted Mechanochemical Synthesis of Copper Based MOF-505 for the Separation of CO2 over CH4 or N2

Yongwei Chen et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2018)

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Article Chemistry, Physical

Syntheses, structures and properties of four Cd(II) coordination polymers induced by the pH regulator

Yun Xu et al.

JOURNAL OF MOLECULAR STRUCTURE (2018)

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Article Chemistry, Multidisciplinary

Fabrication of a microporous Dy(III)-organic framework with polar channels for 5-Fu (fluorouracil) delivery and inhibiting human brain tumor cells

Lei Chen et al.

STRUCTURAL CHEMISTRY (2018)

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Article Chemistry, Multidisciplinary

Applied Topological Analysis of Crystal Structures with the Program Package ToposPro

Vladislav A. Blatov et al.

CRYSTAL GROWTH & DESIGN (2014)

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Article Chemistry, Multidisciplinary

Reversible switching of slow magnetic relaxation in a classic lanthanide metal-organic framework system

Qi Zhou et al.

CHEMICAL COMMUNICATIONS (2013)

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Article Multidisciplinary Sciences

Porous materials with pre-designed single-molecule traps for CO2 selective adsorption

Jian-Rong Li et al.

NATURE COMMUNICATIONS (2013)

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Article Chemistry, Multidisciplinary

Modifying Cage Structures in Metal-Organic Polyhedral Frameworks for H2 Storage

Yong Yan et al.

CHEMISTRY-A EUROPEAN JOURNAL (2011)

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Review Chemistry, Multidisciplinary

Synthesis, Structure, and Carbon Dioxide Capture Properties of Zeolitic Imidazolate Frameworks

Anh Phan et al.

ACCOUNTS OF CHEMICAL RESEARCH (2010)

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Article Chemistry, Inorganic & Nuclear

A Series of (6,6)-Connected Porous Lanthanide Organic Framework Enantiomers with High Thermostability and Exposed Metal Sites: Scalable Syntheses, Structures, and Sorption Properties

Hai-Long Jiang et al.

INORGANIC CHEMISTRY (2010)

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Article Chemistry, Multidisciplinary

Tuning MOF CO2 Adsorption Properties via Cation Exchange

Jihyun An et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2010)

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Article Chemistry, Multidisciplinary

Strong CO2 Binding in a Water-Stable, Triazolate-Bridged Metal-Organic Framework Functionalized with Ethylenediamine

Aude Demessence et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2009)

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Article Chemistry, Multidisciplinary

A short history of SHELX

George M. Sheldrick

ACTA CRYSTALLOGRAPHICA A-FOUNDATION AND ADVANCES (2008)

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Article Chemistry, Inorganic & Nuclear

Synthesis, structure, and luminescent and magnetic properties of novel lanthanide metal-organic frameworks with zeolite-like topology

Zhongyue Li et al.

INORGANIC CHEMISTRY (2007)

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Review Chemistry, Inorganic & Nuclear

Coordination polymer networks with O- and N-donors: What they are, why and how they are made

Adeline Y. Robin et al.

COORDINATION CHEMISTRY REVIEWS (2006)

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Article Multidisciplinary Sciences

Exceptional chemical and thermal stability of zeolitic imidazolate frameworks

Kyo Sung Park et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2006)

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Article Chemistry, Multidisciplinary

Effects of functionalization, catenation, and variation of the metal oxide and organic linking units on the low-pressure hydrogen adsorption properties of metal-organic frameworks

JLC Rowsell et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2006)

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Article Chemistry, Multidisciplinary

A lanthanide metal-organic framework with high thermal stability and available Lewis-acid metal sites

Xiaodan Guo et al.

CHEMICAL COMMUNICATIONS (2006)

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Article Chemistry, Multidisciplinary

Hydrogen sorption in functionalized metal-organic frameworks

JLC Rowsell et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2004)

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Article Chemistry, Multidisciplinary

Single-crystal structure validation with the program PLATON

AL Spek

JOURNAL OF APPLIED CRYSTALLOGRAPHY (2003)

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A microporous dysprosium-based MOF for selective CO2 capture at ambient temperature

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