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Article
Chemistry, Physical
Yingfei Hu et al.
Summary: Efficient and low-cost electrocatalysts for hydrogen evolution reaction (HER) are synthesized by synthesizing two different types of CoS2 under low sulfur and high sulfur concentration conditions. The study shows that CoS impurity phase is easily formed when the sulfur concentration is low, while at high sulfur concentration, the growth of CoS impurity phase is inhibited and leads to phase-pure CoS2. The electrochemical investigation reveals that the CoS2 (HS) electrode has a higher onset potential and a lower required overpotential compared to the CoS2 (LS) electrode.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2023)
Article
Materials Science, Multidisciplinary
Xuan-Pu Wang et al.
Summary: Loading monoclinic beta-AgVO3 on hexagonal CdS nanorods to construct a one-dimensional (1D)/1D p-n heterojunction accelerated the separation of photogenerated electrons and holes, improving the photocatalytic hydrogen production activity.
Article
Chemistry, Physical
Juan Shao et al.
Summary: Tuning surface termination can enhance the carrier dynamics and photoredox performance of photocatalysts by modifying their physicochemical properties. In this study, a Si photocatalyst was prepared by magnesium-thermal reduction and treated with trifluoroacetic acid (TFA). The TFA-terminated Si photocatalyst (TFA-Si) showed improved capacitance, surface area, wettability, charge carrier density, photocurrent, and reduced impedance and overpotential, resulting in enhanced water adsorption/reduction and photoexcited-carrier dynamics. TFA-Si exhibited high photocatalytic H2 evolution activity and oxidation capacity for water oxidation. This work expands the applications of Si-based materials in photocatalysis.
ACS APPLIED ENERGY MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Jiafeng Zhu et al.
Summary: Design and synthesis of a multifunctional Mo-modified ZIS wrapped NTO microrods photocatalyst with enhanced interfacial electric field (IEF) effect and typical S-scheme heterojunction is reported. The catalyst exhibits wide-spectrum light absorption properties, excellent visible light-to-thermal energy effect, electron mobility, charges transfer, and strong IEF, resulting in efficient visible-light-driven photocatalytic hydrogen evolution. The Mo-1.4-ZIS@NTO catalyst shows superior performance with a high H2 evolution rate and apparent quantum efficiency.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Physical
Zhiliang Jin et al.
Summary: As a new two-dimensional carbon hybrid material, graphdiyne has attracted much attention due to its good electrical conductivity, tunable electronic structure, and special electron transfer enhancement properties. It has great potential in the field of hydrogen evolution for photocatalytic water decomposition.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Engineering, Environmental
Huabin Chen et al.
Summary: By tracking the flow direction of electrons, the significantly improved photocatalytic performance of 2D/2D g-C3N4/In2S3 heterostructures for H2O2 production in organic electron donor-free condition is revealed. The experiments confirm that in the g-C3N4/In2S3 heterostructures, photoexcited electrons move from g-C3N4 to In2S3, while holes remain in g-C3N4, effectively separating the charges. Radical trapping experiments confirm that the photoexcited electrons accumulated on the conduction band of In2S3 in g-C3N4/In2S3 heterostructures generate H2O2 through a two-step one-electron reduction reaction of O2.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Environmental
Yuxing Shi et al.
Summary: The development of photocatalysts that maximize the use of solar spectra for efficient photocatalysis is urgently needed. In this study, a core-shell Co3O4@ZnIn2S4 heterojunction was synthesized for high-efficient photothermal-assisted photocatalytic hydrogen production. The results showed that the optimized Co3O4@ZnIn2S4 sample exhibited impressive hydrogen production rates under both AM 1.5G and real sunlight irradiation. Furthermore, the study investigated the influence of reaction solution temperature on the photocatalytic activity induced by the photothermal effect.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Physical
Shan Yang et al.
Summary: The researchers aim to find inexpensive cocatalysts that can enhance the photocatalytic activity of catalysts. In this study, a series of CoS2/g-C3N4 composite photocatalysts were synthesized by depositing CoS2 on the surface of g-C3N4. The size of CoS2 species was adjustable and affected the photocatalysis. The 5CoS2/CN sample with an appropriate nano size of CoS2 cocatalyst exhibited the best photocatalytic performance in producing H2 under visible light irradiation. Its photocatalytic activity was significantly higher than pure g-C3N4 and comparable to Pt/CN catalyst.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2023)
Article
Chemistry, Physical
Bo Su et al.
Summary: Hierarchical Co9S8@Cd0.8Zn0.2S-DETA nanocages with an S-scheme interface were fabricated as a photocatalyst for CO2 reduction, achieving high rates of CO and H2 production. The amine groups enhanced CO2 adsorption and activation, while the hierarchical hollow heterostructure promoted charge separation and transfer. The use of a cocatalyst resulted in a high apparent quantum efficiency of 9.45% at 420 nm.
ADVANCED ENERGY MATERIALS
(2023)
Article
Engineering, Chemical
Xiaohong Li et al.
Summary: In this study, the hydrogen evolution performance of CdS nanorods is improved by using ZnCo2O4. ZnCo2O4 nanospheres are synthesized using hydrothermal and calcination methods, and CdS nanorods are synthesized using the solvothermal method. The introduction of ZnCo2O4 expands the adsorption range of light and improves the performance of photocatalytic hydrogen evolution, providing reference for developing high-efficiency photocatalysts.
FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING
(2023)
Article
Materials Science, Multidisciplinary
Tian Wang et al.
Summary: The photocatalytic performance can be significantly improved by constructing suitable heterojunction photocatalysts. In this study, a unique new double S-scheme heterojunction photocatalyst was constructed by self-assembly of GDY and ZnAl-LDH. The formation of an internal electric field between CuI-GDY and ZnAl-LDH interface broadened the light absorption range and improved the redox ability of the photocatalytic system.
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
(2023)
Article
Chemistry, Physical
Qi Li et al.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Chemistry, Physical
Shiwen Du et al.
Summary: Having an insight into the optimizations of intrinsic properties of cocatalysts via doping foreign atoms to promote solar-driven water splitting is important. Zero-dimensional/one-dimensional structured TMCoSe/CdS0.95Se0.05 was successfully synthesized, and the FeCoSe/CdS0.95Se0.05 photocatalyst showed the most excellent H2 evolution performance. The activity can be attributed to the Schottky-type heterojunction formed between FeCoSe cocatalyst and CdS0.95Se0.05, enhancing charge carrier separation and utilization.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Chemistry, Physical
Guping Zhang et al.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Chemistry, Multidisciplinary
Jiaqiang Li et al.
Summary: In this study, a GDY/Gr/GDY sandwiched architecture was designed to improve the K-ion storage performance. Experimental results showed that the GDY/Gr/GDY electrode exhibited better capacity output and cyclic stability. In situ testing revealed the reversibility of the GDY/Gr/GDY electrode. A full-cell device demonstrated the potential of the GDY/Gr/GDY anode for K-ion batteries.
Article
Chemistry, Multidisciplinary
Mengxi Tan et al.
Summary: The construction of an ultrathin 2D ZnIn2S4/g-C3N4 Z-scheme heterojunction through in-situ growth of ZnIn2S4 on g-C3N4 allows for greatly improved hydrogen evolution performance by carefully regulating the interface structure. The optimized photocatalyst demonstrates significant photocatalytic activity without Pt, attributing to the synergistic effect of abundant active sites, enhanced photoresponse, and valid interfacial charge transfer channels. Spectroscopic analyses and density functional theory (DFT) calculations confirm that the enhanced photocatalytic performance is also due to promoted interfacial charge separation in the 2D Z-scheme heterojunction.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Physical
Youlin Wu et al.
Summary: Surface modification of photocatalytic materials is an effective way to enhance their semiconductor activity. By utilizing a simple surface modification strategy and constructing abundant active sites, the photocatalytic activity can be improved. The introduction of NiAl-LDH-P can enhance the utilization of Zn0.5Cd0.5S on solar energy and promote the transfer rate of photogenerated carriers. The construction of the Zn0.5Cd0.5S/NiAl-LDH-P S-scheme heterojunction can change the hydrogen evolution site and improve the activity and stability of hydrogen production.
Article
Chemistry, Multidisciplinary
Haiming Gong et al.
Summary: An S-scheme heterojunction was constructed by modifying the surface of Ni-based metal-organic framework (Ni-MOF) through different in situ treatment strategies. The in situ formation of NiS2, NiO, and Ni2P on the Ni-MOF surface improved the hydrogen production activity by accepting electrons from the conduction band of Ni-MOF. Coupling 2D CeO2 with Ni-MOF/P successfully built the S-scheme heterojunction, leading to a significantly higher hydrogen production rate.
Article
Chemistry, Multidisciplinary
Xiaoyu Luan et al.
Summary: Directly extracting hydrogen energy from water to achieve sustainable hydrogen energy generation is a major step towards a zero-pollution hydrogen-fueled economy. The new concept of hydrogen energy conversion allows for the efficient generation of electric energy by reducing nitrate to ammonia. The hydrogen conversion device demonstrates high capacity and efficiency, surpassing lithium and battery solutions.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Physical
Hongying Li et al.
Summary: This research successfully prepared a composite catalyst Ni-MOF-74/BiVO4/P with excellent performance by modification, achieving the directional migration of photo-generated carriers and increasing the hydrogen production.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2022)
Article
Chemistry, Physical
Fangshu Xing et al.
Summary: Efficient aromatic alcohol oxidation with simultaneous H-2 evolution under aqueous conditions was achieved using a polyoxometalate (POM)-incorporated ZnIn2S4 dual-functional photocatalytic system. The synergy between HPM and ZIS contributed to the formation of a Z-type heterojunction structure, enhancing redox capacity. The sub-nanometer size of POM clusters ensured faster interfacial charge transfer kinetics.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2022)
Article
Engineering, Multidisciplinary
Yi Cai et al.
Summary: Converting solar energy into hydrogen production is a promising solution to address the energy crisis, but developing photocatalytic materials with positive visible light response, high efficiency, and photostability remains a challenge. In this study, a one-photon excitation path system was developed by combining 3D ZnIn2S4 micro-flowers with 0D CoS2 nanoparticles for hydrogen evolution, achieving an optimal hydrogen evolution rate of 22.24 mmol h-1 g-1. This work sheds light on the design of 0D/3D photocatalysts with high hydrogen evolution performance through a one-photon excitation pathway.
COMPOSITES PART B-ENGINEERING
(2022)
Article
Engineering, Chemical
Junke Li et al.
Summary: The exploration of multiple composite materials with heterojunction structures is important for high-yield hydrogen photocatalytic evolution. In this study, a Mo2S3/Bi2O2CO3 composite with a unique n-n heterojunction and 2D spatial structure was successfully prepared. The composite material with 3% Bi2O2CO3 exhibited the highest photocatalytic effect.
SEPARATION AND PURIFICATION TECHNOLOGY
(2022)
Article
Chemistry, Physical
Kai Wang et al.
Summary: This study presents a novel zinc cadmium sulfide/nickel cobalt phosphide heterojunction for highly efficient photocatalytic hydrogen generation. The zinc cadmium sulfide/nickel cobalt phosphide-3% composite exhibits the highest photocatalytic hydrogen generation performance in a lactic acid aqueous solution at 450 nm, and demonstrates excellent photostability. This research provides a new perspective for solar energy conversion.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Zhiliang Jin et al.
Summary: Graphdiyne was successfully synthesized and used to prepare the GDY/CuI/MIL-53(Al) S-scheme heterojunction for photocatalytic hydrogen production from water. The final hydrogen evolution rate was significantly higher than that of MIL-53(Al) after optimization of experimental conditions. The mechanism of charge transfer was also demonstrated.
Article
Green & Sustainable Science & Technology
Zhiliang Jin et al.
Summary: Graphdiyne (g-CnH2n-2), a novel two-dimensional carbon allotrope material composed of sp-and sp2-hybrid carbon network, has great potential in photocatalysis. In this study, the researchers successfully prepared a high-performance graphdiyne/NiS composite photocatalyst by using Cu+ contained material as a catalyst.
Article
Chemistry, Inorganic & Nuclear
Teng Li et al.
Summary: This study developed a new strategy for catalyst synthesis by forming a stable bonding state on the catalyst surface through a one-step oxidation-phosphorus doping strategy. This bonding state effectively inhibits the recombination of photogenerated carriers and enhances the migration rate of photogenerated electrons, accelerating the process of photocatalytic hydrogen evolution. The research provides new insights and effective strategies for catalyst surface design and the development of photocatalytic hydrogen evolution.
INORGANIC CHEMISTRY
(2022)
Article
Chemistry, Physical
Xiangyi Wang et al.
Summary: In this study, Ag/Ag2O was grown in situ on a CeO2 substrate by a one-step method to form a Ag/Ag2O/CeO2 photocatalyst. The composite catalyst showed low overpotential, small electrochemical impedance, and wide light absorption wavelength, which are favorable for the development of a photocatalytic system. The combination of CeO2 and Eosin Y provided photogenerated electrons, while the heterostructure of the Ag/Ag2O/CeO2 system facilitated the separation of electrons on the conduction band of CeO2. The Ag/Ag2O/CeO2 catalyst exhibited excellent photocatalytic performance for hydrogen production, especially Ag/Ag2O/CeO2-30, which had the highest hydrogen production efficiency compared to Ag/Ag2O and CeO2. Therefore, Ag/Ag2O/CeO2 can be considered as a promising photocatalyst worth developing.
JOURNAL OF PHYSICAL CHEMISTRY C
(2022)
Article
Chemistry, Physical
Renyou Zeng et al.
Summary: The prepared NiSeS/ZnSe photocatalyst exhibits high hydrogen evolution rate and apparent quantum yield, outperforming most ZnSe-based photocatalysts. Ni-Se dual vacancies introduce a local polarization electric field, accelerating surface charge transfer and reducing reaction barriers.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2022)
Article
Materials Science, Multidisciplinary
Guorong Wang et al.
Summary: This study successfully improved the efficiency of solar photocatalytic water decomposition for hydrogen production by constructing a 2%Cu2S/CZS step-scheme heterojunction. The introduction of Cu2S has advantages of reducing particle agglomeration, broadening the light response range, and accelerating charge separation and transfer.
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
(2022)
Article
Engineering, Chemical
Kaicheng Yang et al.
Summary: In this research, a nano hybrid material was developed for efficient photocatalytic hydrogen evolution. The material has a unique structure and porous framework that allows for multivariate collaborative catalysis. Additionally, it exhibits excellent charge transfer rate and lower carrier recombination rate, resulting in smaller hydrogen evolution overpotential.
SEPARATION AND PURIFICATION TECHNOLOGY
(2022)
Article
Chemistry, Physical
Hongying Li et al.
Summary: By regulating the morphology and constructing heterojunction, a three-dimensional nanoflower morphology MoSx/In2O3 composite catalyst was prepared, which significantly improved the hydrogen evolution activity and solved the light absorption issue of In2O3.
ACTA PHYSICO-CHIMICA SINICA
(2022)
Article
Chemistry, Applied
Zizhan Liang et al.
Summary: Conjugated covalent organic frameworks (COFs) hold great promise in photocatalytic hydrogen evolution due to their high crystallinity, large surface area, and distinct structure. However, COFs exhibit poor charge separation, making it crucial to investigate highly effective COF-based photocatalysts. In this study, a conjugated COF/perylene diimide urea polymer (PUP) hetero-structure with S-scheme interfacial charge-transfer channels was successfully developed and manufactured. The optimized photocatalytic hydrogen-evolution rate of TATF-COF/PUP was 3.5 times that of pure TATF-COF and comparable to or even higher than that of previously reported COF-based photocatalysts, resulting in an apparent quantum efficiency of up to 19.7% at 420 nm.
CHINESE JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Applied
Zhaobo Fan et al.
Summary: Graphdiyne (GDY) is a promising two-dimensional carbon hybrid material with good conductivity and adjustable electronic structure. In this study, GDY was successfully prepared and characterized. By utilizing GDY's unique properties, GDY/CdSe heterojunctions were established and applied to photocatalytic hydrogen evolution, showing significantly enhanced activity compared to GDY and CdSe alone. The study provides a feasible approach for large-scale GDY preparation and demonstrates its potential in photocatalysis.
CHINESE JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Physical
Xiangyi Wang et al.
Summary: In this study, a new carbon material GDY was prepared and introduced into metal oxide Co3O4, constructing a highly efficient photocatalyst Co3O4/GDY composite. The migration of photoelectrons was effectively regulated, resulting in high hydrogen production. The introduction of carbon materials into metal oxides has great potential in the field of photocatalysis.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Chemistry, Applied
Junxian Bai et al.
Summary: A 2D/2D/2D layered heterojunction photocatalyst with cascaded 2D coupling interfaces was designed and constructed, which effectively promoted spatially directional charge separation and transport between CdS and WO3 nanosheets, resulting in an increased visible-light hydrogen evolution rate.
CHINESE JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Applied
Zhiliang Jin et al.
Summary: Graphdiyne (GDY), a novel two-dimensional carbon hybrid material, has attracted significant attention due to its unique and excellent properties. This study reports new progress in the preparation of a composite material, Co9S8-GDY-CuI, using CuI powder as a catalytic material and a facile hydrothermal method. The Co9S8-GDY-CuI exhibited hydrogen production activity 10.29 times higher than that of pure GDY in the sensitization system. Characterization techniques provided evidence for the successful preparation of the material and its superior photocatalytic activity. A possible reaction mechanism and the effects of Co9S8 nanoparticles were also discussed.
CHINESE JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Applied
Wangjing Xie et al.
Summary: In this study, planar unsaturated sulfurs in CoS2 nanowires have been activated through constructing Graphdiyne-CoS2 heterojunction nanocomposites, leading to enhanced electron transfer energy barriers and improved catalytic performance for hydrogen evolution reaction. The heterojunction exhibits superior HER catalytic performance and stability, paving the way for further efficient transition metal disulfides catalyst manufacture.
JOURNAL OF ENERGY CHEMISTRY
(2021)
Article
Engineering, Environmental
Xiangyu Meng et al.
Summary: Molybdenum based compounds, such as MoCx, MoSe2, MoS2 MoPx, MoOx and their derivatives, have been considered as alternative catalysts to platinum in hydrogen evolution reactions. Mo2Bx (x = 1 or 4) has been investigated for the first time as active components in a visible-light driven photocatalytic hydrogen production system, showing excellent hydrogen evolution activities. The electron deficient atom boron (B) content in Mo2Bx samples affects their photocatalytic activities, with Mo B-2(4) exhibiting better activity than Mo2B due to differences in electron transfer rates.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Physical
Yanhua Song et al.
Summary: In this study, CoS nanoflower as a cocatalyst was loaded onto two-dimension carbon nitride (2D CN) to enhance the photocatalytic performance for the degradation of Rhodamine B. The CoS nanoflower demonstrated the capability of extracting photogenerated electrons rapidly from 2D CN to promote efficient charge separation. The CoS/2D CN showed improved degradation activity compared to 2D CN, as well as superior photostability after four cycles, and was also effective for photocatalytic H2 evolution reaction.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2021)
Article
Chemistry, Physical
Qiaoqiao Mu et al.
Summary: The study successfully utilized MOF of Co(BDC) as a bridge to connect the heterogeneous CdS photosensitizer and molecular co-catalyst, promoting photocatalytic CO2 reduction reactions with high CO yield rate and selectivity. The improved photocatalytic performance was attributed to efficient charge transfer at interfaces and the MOF layer expediting mass kinetics of the triphasic solid-liquid-gas reaction.
JOURNAL OF CATALYSIS
(2021)
Article
Chemistry, Physical
Kangwei Ma et al.
Summary: In this study, a noble-metal-free polyoxometalate Cu3POM was successfully coupled with mesoporous, multiphase TiO2 to create a highly efficient photocatalytic system for hydrogen production. The composite system exhibited excellent photocatalytic activity by increasing active sites, enhancing stability, and narrowing band gap. This innovative combination provides new insights into the design of efficient photocatalytic materials for H₂ production.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Nanoscience & Nanotechnology
Teng Yan et al.
Summary: This study successfully constructed the NiTiO3-CuI-GD ternary system to improve hydrogen production activity through morphology modulation and energy band structure design, proposing an S-scheme heterojunction photocatalytic reaction mechanism.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Zhi-liang Jin et al.
Summary: This study reports an innovative progress in preparing graphdiyne using Cu+ catalyst and coupling it with NiAl-LDH for photocatalytic hydrogen production, resulting in significantly enhanced activity. The successful synthesis of graphdiyne nanosheets by a cross-coupling method is confirmed, leading to improved photocatalytic hydrogen evolution performance.
CHEMISTRY-A EUROPEAN JOURNAL
(2021)
Article
Chemistry, Multidisciplinary
Libo Wang et al.
Summary: Efficient hierarchical photocatalysts, such as the S-scheme core-shell TiO2@ZnIn2S4 heterojunction, have gained attention for photocatalytic CO2 reduction. The improved performance is attributed to the inhibited recombination of photogenerated charge carriers induced by the S-scheme heterojunction, as well as the large specific surface areas and abundant active sites. In situ irradiated X-ray photoelectron spectroscopy, work function calculation, and electron paramagnetic resonance measurements confirm the S-scheme photogenerated charge transfer mechanism.
Article
Chemistry, Applied
Rongchen Shen et al.
Summary: This study combines low-cost metallic Ni3C cocatalysts with twin nanocrystal Zn0.5Cd0.5S (ZCS) solid solution homojunctions to achieve efficient visible-light-driven H-2 evolution. The ZCS-1 heterojunction/homojunction nanohybrid shows the highest photocatalytic H-2-evolution rate, indicating a more efficient photocatalytic H-2 evolution compared to other noble metal photocatalytic systems. The unique strategy of constructing heterojunction/homojunction hybrid nanostructures demonstrates improved catalytic activity for H-2 evolution under visible light.
CHINESE JOURNAL OF CATALYSIS
(2021)
Article
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Weixiang Zhou et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
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(2019)
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(2019)
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(2019)
Article
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ACS ENERGY LETTERS
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Review
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ACTA PHYSICO-CHIMICA SINICA
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JOURNAL OF PHYSICAL CHEMISTRY C
(2017)
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