☆ 3.8 Review

Recent progress in transition-metal-oxide-based electrocatalysts for the oxygen evolution reaction in natural seawater splitting: A critical review

ESCIENCE (2023)

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Article Electrochemistry

Ultrafast synthesis of Cu2O octahedrons inlaid in Ni foam for efficient alkaline water/seawater electrolysis

Huan Wang et al.

Summary: This study reports an ultrafast synthesis method for Cu2O octahedrons and their inlay in Ni foam, resulting in a self-supporting electrocatalyst. The electrocatalyst displays superior activity and stability in both oxygen and hydrogen evolution reactions, and exhibits low cell voltage and high current density when applied as bifunctional electrodes in alkaline seawater splitting.

ELECTROCHEMISTRY COMMUNICATIONS (2022)

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Article Chemistry, Inorganic & Nuclear

Strategies of designing electrocatalysts for seawater splitting

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Summary: This article systematically summarizes the electrochemical reactions mechanism involved in seawater splitting and discusses the strategies for preparing highly active and stable electrocatalysts, as well as pointing out the challenges in designing electrocatalysts for practical hydrogen production in seawater splitting.

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Review Chemistry, Multidisciplinary

Electrocatalytic Water Splitting: From Harsh and Mild Conditions to Natural Seawater

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Summary: Electrocatalytic water splitting is considered the most effective way to generate green energy-hydrogen and is seen as a promising solution to the world's energy crisis and climate change. While research has achieved high catalytic activities in harsh conditions, practical applications face challenges such as corrosion, catalyst stability, and technical difficulties. As a result, there is increasing focus on studying water splitting in mild conditions or even natural seawater to overcome these obstacles.

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Article Chemistry, Multidisciplinary

Strong Oxide-Support Interaction over IrO2/V2O5 for Efficient pH-Universal Water Splitting

Xiaozhong Zheng et al.

Summary: In this study, constructing strong oxide-support interaction (SOSI), ultrafine iridium oxide nanoclusters were anchored on a vanadium oxide support, leading to significant performance enhancement in the oxygen evolution reaction (OER). The distorted IrO2 active sites in the catalyst facilitate the O-O coupling process, resulting in low overpotentials and high-performance water electrolysis over a broad pH range. SOSI also ensures the stability of the catalyst.

ADVANCED SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Structural Buffer Engineering on Metal Oxide for Long-Term Stable Seawater Splitting

Linzhou Zhuang et al.

Summary: Seawater electrolysis is an attractive technique for mass production of green hydrogen. However, the presence of chloride ions in seawater can lead to deactivation of the oxygen evolution reaction (OER) catalysts. By utilizing a structural buffer engineering strategy, Co-2(OH)(3)Cl demonstrates long-term stability and a high OER selectivity in seawater electrolysis.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Physical

Constructing the Fe/Cr double (oxy)hydroxides on Fe3O4 for boosting the electrochemical oxygen evolution in alkaline seawater and domestic sewage

Lu Li et al.

Summary: Developing electrocatalysts that can be used directly in sewage and seawater is beneficial for turning waste into raw materials and producing H2. By constructing a heterointerface between Fe(Cr)OOH and Fe3O4, the overpotential of the oxygen evolution reaction (OER) was significantly reduced, promoting mass and electron transfer. The electrode showed efficient stability in alkaline seawater and domestic sewage, and the electrolyzer using it as an anode could deliver high current density at a small cell voltage.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Zn-VOx-Co nanosheets with amorphous/crystalline heterostructure for highly efficient hydrogen evolution reaction

Meng Chen et al.

Summary: Designing cost-effective catalysts with high-activity and ultra-stability is crucial for scaling-up the water electrolysis process for hydrogen production. This study successfully synthesized Zn-VOx-Co 2D nanosheets with a well-integrated heterostructure, which showed enhanced intrinsic electrocatalytic activity and long-term stability. The dual-doping of Zn and VOx optimized the d-band center of Co and improved the adsorption and desorption of H, opening a new avenue for designing electrocatalysts with unique crystalline-amorphous heterostructure.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Multidisciplinary

Large-Scale Synthesis of Spinel NixMn3-xO4 Solid Solution Immobilized with Iridium Single Atoms for Efficient Alkaline Seawater Electrolysis

Ning Wen et al.

Summary: This study developed a novel strategy for preparing a spinel NixMn3-xO4 solid solution immobilized with iridium single-atoms (Ir-SAs) for efficient oxygen evolution reaction (OER) performance in alkaline seawater. Experimental characterizations and theoretical calculations demonstrated the effect of Ir-SAs on improving the intrinsic OER activity and facilitating surface charge transfer kinetics.

ADVANCED SCIENCE (2022)

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Article Chemistry, Physical

Constructing high-activity Cobalt-based Perovskite hybrid by a top-down phase evolution method for the direct seawater electrolysis anode

Fuyue Liu et al.

Summary: A novel top-down phase evolution method was proposed to synthesize Co-based perovskite hybrid for enhanced OER catalytic activity in direct seawater electrolysis. The optimized perovskite hybrid showed further improved OER activity by active surface reconstruction, achieving stable electrolytic performance for 100 hours. The research provides new insights into designing high-performance perovskite hybrids for direct seawater electrolysis.

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Article Chemistry, Physical

Reversible vs Standard Hydrogen Electrode Scale in Interfacial Electrochemistry from a Theoretician's Atomistic Point of View

Axel Gross

Summary: In interfacial electrochemistry, it is commonly believed that the stability of adsorbate phases containing only hydrogen atoms is independent of the pH of the electrolyte, while the stability of adsorbate phases without hydrogen is independent of the pH on the scale of the standard hydrogen electrode. This Perspective argues that such Nernstian behavior can only occur if the free energy of the adsorbate phase is not affected by the electrochemical control parameters, which is generally not true. However, certain structural and chemical factors may lead to Nernstian behavior. The analysis also provides guidance for the validity of grand-canonical simulations using the computational hydrogen electrode concept.

JOURNAL OF PHYSICAL CHEMISTRY C (2022)

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Strategies of Anode Design for Seawater Electrolysis: Recent Development and Future Perspective

Tanveer ul Haq et al.

Summary: This review discusses the additional challenges of seawater electrolysis compared to freshwater splitting and summarizes the current effective strategies. It provides insights for the rational design of high-performance anodes and proposes a perspective on the fabrication of high-performance anodes for direct seawater electrolysis.

SMALL SCIENCE (2022)

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Review Chemistry, Physical

Recent Advances in Perovskite-Type Oxides for Energy Conversion and Storage Applications

Chunwen Sun et al.

Summary: This review discusses the research conducted by Professor John B. Goodenough on perovskite-type oxides more than 60 years ago, highlighting their crucial role in energy conversion and storage. It also emphasizes recent advances and novel design strategies for optimizing performance in various applications of perovskite oxides.

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Article Chemistry, Physical

Exceptional lattice-oxygen participation on artificially controllable electrochemistry-induced crystalline-amorphous phase to boost oxygen-evolving performance

Haijuan Zhang et al.

Summary: The study successfully constructed a crystalline-amorphous phase in La0.33SrCo0.5Fe0.5Ox (H-LSCF) nanofibers, which led to reduced overpotentials for oxygen-evolving reaction in potassium hydroxide solution. The enhanced stability and accelerated OER activity of this combination may be attributed to its favorable solid-liquid contact, high Co valence, and strong Co-O covalency.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Green & Sustainable Science & Technology

Perovskite and related oxide based electrodes for water splitting

Ning Han et al.

Summary: A scientometric analysis was conducted on the development of oxide-based catalysts for water splitting, revealing a significant increase in publications since 2012. China and the United States were identified as world leaders in scientific output regarding the use of oxide-based catalysts for water splitting.

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Article Chemistry, Multidisciplinary

Highly Effective Freshwater and Seawater Electrolysis Enabled by Atomic Rh-Modulated Co-CoO Lateral Heterostructures

Phan Khanh Linh Tran et al.

Summary: Atomic metal-modulated heterostructures, such as continuous cobalt-cobalt oxide lateral heterostructures implanted with well-dispersed rhodium atoms, have shown promise in developing high-performance multifunctional electrocatalysts for water splitting. The synergistic effects of uniform rhodium atoms and Co-CoO heterostructures provide rich multi-integrated active sites and excellent charge transfer, ultimately enhancing both hydrogen and oxygen evolution activities. In both freshwater and seawater conditions, the material displays superior overpotentials and cell voltages compared to earlier reported catalysts, making it a promising catalyst for green hydrogen generation via electrolysis applications.

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Redirecting dynamic surface restructuring of a layered transition metal oxide catalyst for superior water oxidation

Jian Wang et al.

Summary: A new method of modulating catalyst surface structure was proposed, showing significant performance and stability in the oxygen evolution reaction.

NATURE CATALYSIS (2021)

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Article Chemistry, Physical

Selective anodes for seawater splitting via functionalization of manganese oxides by a plasma-assisted process

Lorenzo Bigiani et al.

Summary: Through a specific material combination, selective triggering of oxygen generation and reduction of chlorine production in seawater has been achieved. The combination of MnO2 and Co3O4 performs the best in alkaline seawater splitting, showing significant results.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Dmitry Bokov et al.

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ADVANCES IN MATERIALS SCIENCE AND ENGINEERING (2021)

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Review Engineering, Chemical

An overview and recent advances in electrocatalysts for direct seawater splitting

Hao-Yu Wang et al.

Summary: Compared to pure water, seawater is considered an unlimited resource for direct electrolysis. However, challenges such as chlorine-related competing reactions and various impurities hinder its practical application. The development of efficient electrocatalysts is crucial for addressing these challenges and advancing the technology of direct seawater splitting.

FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING (2021)

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Article Chemistry, Physical

Boron-modified cobalt iron layered double hydroxides for high efficiency seawater oxidation

Libo Wu et al.

Summary: A novel hierarchical nanosheet-nanoflake-structured B-Co2Fe LDH catalyst has been developed with excellent OER catalytic activity, stability, and corrosion resistance in seawater electrolysis, showing promising potential for selective seawater oxidation.

NANO ENERGY (2021)

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Article Chemistry, Physical

Doping modification, defects construction, and surface engineering: Design of cost-effective high-performance electrocatalysts and their application in alkaline seawater splitting

Xiao Hu Wang et al.

Summary: Studies have shown that doping and defects can promote water dissociation and hydrogen desorption, accelerating the hydrogen evolution reaction and improving the oxygen evolution reaction kinetics. Asymmetric electrodes exhibit good stability and efficiency in alkaline seawater electrolysis.

NANO ENERGY (2021)

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Article Nanoscience & Nanotechnology

Fe2O3/NiO Interface for the Electrochemical Oxygen Evolution in Seawater and Domestic Sewage

Lu Li et al.

Summary: The study presents an efficient method for hydrogen production through electrolysis of seawater and domestic sewage, utilizing a surface-engineered FeNi oxide layer on Ni foam (NF) to achieve exceptional oxygen evolution reaction (OER) performance. The electrocatalyst shows significantly lower overpotentials and high current densities in 1M KOH, with satisfactory stability during practical electrolysis. This work provides a facile approach to fabricate an electrocatalyst for seawater and domestic sewage electrolysis, with great significance for the synergetic development of hydrogen economy and environmental science.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Multidisciplinary

Clean and Affordable Hydrogen Fuel from Alkaline Water Splitting: Past, Recent Progress, and Future Prospects

Zi-You Yu et al.

Summary: The hydrogen economy has emerged as a promising alternative to the current hydrocarbon economy, involving the use of renewable energy to split water into hydrogen and oxygen for further utilization as clean fuel. Among various water electrolysis technologies, alkaline water splitting has been commercialized for over 100 years and is considered the most mature and economic option. Advanced nonprecious metal electrocatalysts have shown potential for improving the efficiency and stability of alkaline water splitting processes, with a focus on catalyst synthesis and performance improvement.

ADVANCED MATERIALS (2021)

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Energy-saving hydrogen production by chlorine-free hybrid seawater splitting coupling hydrazine degradation

Fu Sun et al.

Summary: A potential solution to grid-scale production of carbon-neutral hydrogen energy without reliance on freshwater is demonstrated through chlorine-free hydrogen production by hybrid seawater splitting coupling hydrazine degradation. The electrolyzer achieves a high hydrogen production rate at low electricity expense and avoids chlorine electrochemistry in complex chemical environments. By integrating low-voltage direct hydrazine fuel cells or solar cells, self-powered hybrid seawater electrolysis is realized, enabling efficient conversion of ocean resources to hydrogen fuel while removing harmful pollutants.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Physical

The electronic structure of transition metal oxides for oxygen evolution reaction

Hongxia Wang et al.

Summary: Electrolysis of water for hydrogen and oxygen production is crucial for storing renewable energy in chemical fuels. The efficiency is often limited by the oxygen evolution reaction kinetics, requiring efficient electrocatalysts. Understanding the electronic structure and its relationship with catalytic activity has led to strategies like doping and defect engineering to enhance activity. Challenges and future perspectives in the field are also discussed.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Review Chemistry, Multidisciplinary

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Fanghao Zhang et al.

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TRENDS IN CHEMISTRY (2021)

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NixFeyN@C microsheet arrays on Ni foam as an efficient and durable electrocatalyst for electrolytic splitting of alkaline seawater

Boran Wang et al.

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Cheng Wang et al.

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NANOSCALE (2021)

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Review Chemistry, Physical

Seawater electrocatalysis: activity and selectivity

Sakila Khatun et al.

Summary: Seawater is considered a major hydrogen reservoir, but the presence of multielements and interference in electrochemistry, particularly chlorine chemistry, make electrocatalytic water splitting challenging. To achieve sustainable seawater electrolysis, focus should not only on electrocatalyst activity but also on selective oxygen evolution reaction to suppress corrosive chlorine chemistry.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Seawater electrocatalysis: activity and selectivity

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Summary: Seawater is considered a major hydrogen reservoir, but the presence of multiple elements and interference in electrochemistry, especially chlorine chemistry, make seawater electrolysis challenging. To make seawater electrolysis sustainable, efficient oxygen evolution reaction and suppression of corrosive chlorine chemistry by electrocatalysts are highly desirable.

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Heterogeneous lamellar-edged Fe-Ni(OH)2/Ni3S2 nanoarray for efficient and stable seawater oxidation

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Article Electrochemistry

Anodically deposited manganese molybdenum tungsten oxide anodes for oxygen evolution in seawater electrolysis

T Matsui et al.

JOURNAL OF APPLIED ELECTROCHEMISTRY (2002)

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Article Electrochemistry

The durability of manganese-molybdenum oxide anodes for oxygen evolution in seawater electrolysis

K Fujimura et al.

ELECTROCHIMICA ACTA (2000)

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