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Review
Chemistry, Multidisciplinary
Yuanyuan Wang et al.
Summary: Transition metal carbides/nitrides (MXenes) are emerging two-dimensional (2D) materials obtained from MAX phase ceramics. MXenes have been widely investigated due to their unique structure, synthesis method, and functionalization method. MXene-based membranes show excellent gas separation performances due to their high permeability, fine sieving ability, and diverse processability. This review provides insights into the structure-property relationship of MXene-based membranes and outlines their outstanding carbon dioxide (CO2) capture performance, as well as discussing the challenges and future prospects of MXene materials in the field of gas separation.
Review
Biochemistry & Molecular Biology
Jong Sung Won et al.
Summary: MXenes are a new class of two-dimensional materials that have been widely utilized in various fields due to their controlled characteristics. In cellulose research, MXene hybrids are effective composites that improve the mechanical properties and prevent MXene accumulation. Cellulose/MXene composites have applications in electrical, materials, chemical, mechanical, environmental, and biomedical engineering.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2023)
Article
Engineering, Chemical
Hongli Zhang et al.
Summary: Two-dimensional (2D) nanomaterial-based membranes hold great promise for various applications due to their attractive properties in molecular separation and transport. However, the swelling problem of 2D membranes has hindered their performance. In this study, the insertion of flexible and hydrophilic carboxylated cellulose nanofibers (CNFs) effectively stabilized the Ti3C2Tx MXene laminar architecture, enhancing mechanical strength, fixing interlayer distance, and improving anti-swelling properties. Furthermore, the intercalation of nanocelluloses increased interlayer spacing and created open gaps for fast and selective molecular transport. When applied in antibiotics separative filtration process, the resulting membrane exhibited excellent anti-swelling properties and high selectivity of antibiotics, making it ideal for various applications.
SEPARATION AND PURIFICATION TECHNOLOGY
(2023)
Article
Engineering, Chemical
Peng Xu et al.
Summary: MXene-based membranes with an ultrathin layer of ionic liquid show enhanced gas separation performance, with the thickness of the ionic liquid film affecting the selectivity. The MXene-slit width has less influence on gas permeance but affects the CO2/N2 selectivity. A composite membrane composed of MXene with an 8 angstrom slit and 40 pairs of ionic liquid exhibits the best CO2/N2 separation performance.
SEPARATION AND PURIFICATION TECHNOLOGY
(2023)
Article
Nanoscience & Nanotechnology
Bencheng Zhao et al.
Summary: Facing the complex and deteriorated environment, wearable materials with integrated functions have rapidly progressed. In this study, a laminated MXene foam/cellulose@LDH composite membrane was fabricated for personal thermal management and electromagnetic interference shielding. The membrane exhibited excellent optical properties, radiative thermal management performances, stain resistance, and electromagnetic interference shielding performance, providing a promising strategy for comfortable living.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Applied
Shuwei Tang et al.
Summary: In this study, a flexible gas barrier film with a nacre-like layered structure was developed. The film exhibited superior mechanical properties, acid-base stability, and barrier properties to gases and volatile organic compounds. It also possessed antibacterial properties, biocompatibility, and degradability.
CARBOHYDRATE POLYMERS
(2023)
Article
Engineering, Environmental
Yin Zhang et al.
Summary: This study reports a bioinspired and stable multifunctional coating based on Ti3C2TX MXene network intercalated with cellulose nanocrystals for scalable construction of smart wood. The optimized CNC/MXene coating exhibits high adhesion, sensitive fire response time, superior flame retardancy, and excellent smoke suppression. It also has the potential photocatalysis oxidation capacity for volatile organic compounds removal.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Environmental
Chae-Young Park et al.
Summary: This article investigates an energy-efficient and eco-friendly membrane-based CO2 separation process. Thin-film composite (TFC) membranes with a defect-free, ultra-thin, and highly permeable selective layer were successfully manufactured through transient-filler (TF) treatment. The resulting TFC membrane showed significantly improved gas permeance, making it a promising material for CO2 separation.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Engineering, Environmental
Zhanghui Wang et al.
Summary: Nanocellulose-based membranes, with their unique structure and properties, have shown great potential in molecular separation in various fields. This paper reviews the recent advancements in the application of nanocellulose membranes in water treatment, chemical industries, seawater desalination, and battery fields, providing insights into their separation mechanisms.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Nanoscience & Nanotechnology
Bencheng Zhao et al.
Summary: This work utilizes a laminated MXene foam/cellulose@LDH composite membrane for personal thermal management and electromagnetic interference shielding. The membrane exhibits excellent optical properties, radiative thermal management performances, and electromagnetic interference shielding performance.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Nanoscience & Nanotechnology
Yawen Zhang et al.
Summary: In this study, stable lamellar membranes were prepared by electrostatic attraction and hydrogen bond formation between polycation polyethyleneimine (PEI) and negatively charged MXene. The interlayer d-spacing of the membrane could be changed by adjusting the suspension pH, allowing for precise molecular separation and high organic solvent penetration. Moreover, the insertion of PEI did not hinder the passage of water molecules. The optimized MXene-PEI membranes showed excellent channel stability.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Materials Science, Paper & Wood
Zhongguo Wang et al.
Summary: Designing gas separation membranes from natural resources such as clay and cellulose is important. In this study, natural clay attapulgite nanorods were integrated into cellulose nanofibers to create organic/inorganic composite membranes. These membranes exhibited effective CO2/N-2 separation due to the sealing of non-selective interfacial voids/defects by flexible cellulose nanofibers.
Article
Engineering, Environmental
Jian Li et al.
Summary: The study utilized MXene nanosheets and polyamide to construct high rejection thin film nanocomposite membrane, which exhibited excellent pure water permeability, high rejection towards dyes.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Nanoscience & Nanotechnology
Jie Yang et al.
Summary: This study presents a highly sensitive and waterproof flexible pressure sensor using a free-standing hydrophobic bacterial cellulose/Ti3C2Tx MXene (HBT) hybrid film as a sensing layer. The sensor exhibits high sensitivity, fast response, wide linear sensing range, low detection limit, and excellent repeatability, while maintaining outstanding sensing features even after being immersed in water multiple times.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Chemistry, Multidisciplinary
Xinpeng Che et al.
Summary: Combining rigid biological nanofibrils and mild manual shake, an efficient and nondestructive method of liquid exfoliation was developed for obtaining large lateral size MXene nanosheets. The resulting MXene nanosheets exhibited high yield, excellent chemical stability, and wide applications in solar-thermal evaporation and energy harvest.
Article
Chemistry, Multidisciplinary
Yanmei Zhang et al.
Summary: In this study, an advanced membrane with a stable interlayer spacing was developed using MXene for water purification. The membrane showed outstanding anti-swelling property and anti-fouling ability, offering a promising approach for precise water purification.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Physical
Wenjia Luo et al.
Summary: Membrane separation systems have gained significant attention in the gas separation field due to their cost-effectiveness, high efficiency, and eco-friendly advantages. In this study, a high-performance CO2-philic MXene/PEG mixed matrix membrane was prepared through a simple vacuum filtration process, displaying excellent CO2 permeance and selectivity in the separation of CO2/N2 and CO2/CH4. The study demonstrates a new strategy for the design and fabrication of CO2-philic MXene-based membranes for highly efficient CO2 separation from natural gas and flue gas.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2022)
Article
Engineering, Chemical
Renhao Li et al.
Summary: This study presents a method for constructing a composite membrane based on MXene and MOF-801. By in situ synthesis of MOF-801@MXene nanosheets at room temperature and fabrication of membranes, composite membranes with significantly enhanced gas permeance and selectivity were obtained.
JOURNAL OF MEMBRANE SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Mingliang Cheng et al.
Summary: In this study, a sandwich composite was constructed by coating the core material of transparent wood with silver nanowire@MXene, which achieved high-performance EMI shielding while maintaining high transparency and flexibility. The composite exhibited high EMI shielding effectiveness in the X-band and large-scale production feasibility, providing inspiration for the development of advanced EMI shielding materials for wide applications.
Article
Chemistry, Multidisciplinary
Youyu Jia et al.
Summary: This study successfully intercalated an ionic liquid into a two-dimensional lamellar membrane and enhanced the immobilization and separation performance through modifying the nanochannel walls. The optimal membrane exhibited larger interlayer spacing and higher ionic liquid uptake, demonstrating excellent CO2 permeance and CO2/N2 selectivity.
Review
Engineering, Chemical
Ali Pournaghshband Isfahani et al.
Summary: Gas separation membranes incorporating two-dimensional materials, especially MXenes, have shown outstanding physical properties and have great potential in energy-efficient gas separation. This Review summarizes recent advances in the field, discussing research opportunities, modification approaches, transport mechanisms, and future prospects.
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
(2022)
Article
Polymer Science
Wenjia Luo et al.
Summary: This study presents the preparation of a high-performance self-supporting Pebax/CMCp MXene mixed matrix membrane (MMM) for CO2 gas separation. The experimental results show that the prepared membrane exhibits high gas permeability and selectivity, as well as excellent thermal stability and long-term durability.
Review
Chemistry, Multidisciplinary
Ajit Khosla et al.
Summary: This article introduces the use and potential of MXene-polymer hybrid membranes in environmental remediation, emphasizing their excellent physicochemical properties and adsorptive behavior. The paper reviews the fabrication routes of these hybrid membranes and their applications in water purification, gas separation, radiation shielding, and more.
Article
Chemistry, Multidisciplinary
Akira Isogai
Summary: Nanocelluloses have unique morphologies, characteristics, and surface nanostructures, and can be prepared from abundant and renewable plant biomass resources. They have the potential to contribute to the establishment of a sustainable society and help overcome global environmental issues. However, overcoming fundamental and application-related issues is necessary for the further expansion of nanocelluloses.
ADVANCED MATERIALS
(2021)
Article
Engineering, Chemical
Kai Qu et al.
Summary: The study successfully fabricated self-crosslinked MXene hollow fiber membranes using a simple thermal treatment process, demonstrating improved molecular sieving performance.
JOURNAL OF MEMBRANE SCIENCE
(2021)
Article
Engineering, Chemical
Qingwu Long et al.
Summary: In this study, high-performance MXene membranes with stable and tunable nanochannels were prepared by self-assembly, allowing for precise control of internal nanochannels and surface properties, resulting in excellent water permeability and molecular separation performance.
JOURNAL OF MEMBRANE SCIENCE
(2021)
Article
Engineering, Environmental
Shoaib Anwer et al.
Summary: A novel and facile synthesis strategy was introduced to design 2D MXene nanosheets coated cellulose fibers based 3D nanostructures, overcoming the drawbacks in commonly used CDI electrodes and MXene based electrodes. The CLF@Ti3C2Tx based active electrodes exhibited good specific capacitance and high salt adsorption capacitance in 1M sodium chloride electrolyte, with considerable cycling stability.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Engineering, Chemical
Feng Shi et al.
Summary: The study found that MXene-filled membranes allow for much higher loading (up to 20 wt%) compared to GO-filled membranes (up to 5 wt%). Interestingly, dry-state membranes exhibit optimal CO2 separation performance at low loading (1 wt%), while wet-state membranes show increased permeability and CO2/N-2 selectivity at higher filler loadings, contrasting with results obtained under dry conditions. The enhanced CO2 separation performance at high loading under humidification can be attributed to the hydrated interlayer channels of MXene/GO, indicating unique characteristics of MXene in wet-state mixed matrix membranes for CO2 separation.
JOURNAL OF MEMBRANE SCIENCE
(2021)
Article
Engineering, Chemical
D. Petukhov et al.
Summary: The specific properties of O- and OH-terminated Ti3C2Tx nanosheets contribute to the permeance and sorption type selectivity of MXene membranes. These membranes demonstrate high separation factors and permeances for ammonia and water vapors, with strong sorption capacities and labyrinthine transport. The diffusion coefficient of strongly absorbed gases increases with pressure, and the interlayer distance expands, reducing activation barriers for hopping diffusion. Demonstrated characteristics make Ti3C2Tx nanosheets a promising candidate for developing ammonia selective membranes.
JOURNAL OF MEMBRANE SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Yizao Wan et al.
Summary: Ultrathin, strong, and highly flexible Ti3C2Tx MXene/bacterial cellulose (BC) composite films were successfully fabricated using a scalable in situ biosynthesis method. The composite films exhibited excellent mechanical properties and specific EMI shielding efficiency, making them promising materials for addressing EMI problems in modern society.
Article
Engineering, Environmental
Dechao Wang et al.
Summary: The study introduces a strategy to transform Ti3C2Tx MXene into a novel MX-fluid, which exhibits stable antioxidant ability and improved processability. The MX-fluid shows macroscopic flow behavior at room temperature and addresses dispersion issues when blending with other polymer matrices.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Multidisciplinary
Hengfei Qin et al.
Summary: The dual ice-templating assembly (DITA) strategy can control the assembly of cellulose nanofibrils (CNF) into elastic aerogels with interconnected sub-micron fibers, exhibiting excellent superelastic behavior and multifunctional properties.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Zong Lu et al.
Summary: The study involves the creation of a 2D laminar membrane with Li+ selective transport channels by stacking MXene nanosheets with poly(sodium 4-styrene sulfonate) (PSS) containing active sulfonate sites. This membrane shows excellent Li+ selectivity in ionic mixture solutions and high Li+ permeation rate. The selective and rapid transport of partially dehydrated Li+ within subnanochannels is attributed to precisely controlled interlayer spacing and weaker ion-terminal interaction.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Guozhen Liu et al.
CHEMISTRY-AN ASIAN JOURNAL
(2020)
Article
Nanoscience & Nanotechnology
Ahmad Arabi Shamsabadi et al.
ACS APPLIED MATERIALS & INTERFACES
(2020)
Article
Engineering, Chemical
Mingmin Jia et al.
JOURNAL OF MEMBRANE SCIENCE
(2020)
Article
Nanoscience & Nanotechnology
Canghai Ma et al.
ACS APPLIED MATERIALS & INTERFACES
(2020)
Article
Chemistry, Multidisciplinary
Yuhang Ye et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Review
Chemistry, Multidisciplinary
Huseyin Enis Karahan et al.
ADVANCED MATERIALS
(2020)
Review
Chemistry, Multidisciplinary
Qihui Qian et al.
Article
Chemistry, Physical
Mingmei Ding et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Review
Chemistry, Multidisciplinary
Jian Li et al.
ENVIRONMENTAL SCIENCE-NANO
(2020)
Article
Multidisciplinary Sciences
Tian Li et al.
Article
Multidisciplinary Sciences
Hao Yang et al.
NATURE COMMUNICATIONS
(2019)
Article
Chemistry, Multidisciplinary
Weiqian Tian et al.
ADVANCED MATERIALS
(2019)
Article
Engineering, Chemical
Yiyi Fan et al.
JOURNAL OF MEMBRANE SCIENCE
(2019)
Article
Chemistry, Multidisciplinary
Jie Shen et al.
ADVANCED FUNCTIONAL MATERIALS
(2018)
Article
Multidisciplinary Sciences
Li Ding et al.
NATURE COMMUNICATIONS
(2018)
Article
Engineering, Chemical
Xiong-Fei Zhang et al.
JOURNAL OF MEMBRANE SCIENCE
(2018)
Article
Chemistry, Multidisciplinary
Xiaoqin Zou et al.
ADVANCED MATERIALS
(2018)
Article
Chemistry, Physical
M. Karunakaran et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2017)
Article
Chemistry, Multidisciplinary
Shu Huang et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2017)
Review
Chemistry, Multidisciplinary
Beatriz Seoane et al.
CHEMICAL SOCIETY REVIEWS
(2015)
Review
Chemistry, Multidisciplinary
Jianfeng Yao et al.
CHEMICAL SOCIETY REVIEWS
(2014)
Article
Multidisciplinary Sciences
Michael Ghidiu et al.
