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Cu2ZnSnS4 monograin layer solar cells for flexible photovoltaic applications

JOURNAL OF MATERIALS CHEMISTRY A (2023)

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Article Energy & Fuels

Efficiency enhancement of Cu2ZnSnS4 monograin layer solar cells via absorber post-growth treatments

K. Timmo et al.

Summary: The efficiency of CZTS monograin layer solar cells is limited by recombination losses, which can be reduced by post-treating the surfaces of monograin powder crystals. This study optimized two sequential post-treatment steps and found that secondary phases were formed on the crystals' surfaces in the thermal annealing process. The study also showed that adjusting the annealing temperature can modify the Cu/Zn+Sn ratio in the CZTS crystals and improve the performance of monograin layer solar cells.

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2023)

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Article Multidisciplinary Sciences

Flexible solar cells based on foldable silicon wafers with blunted edges

Wenzhu Liu et al.

Summary: Flexible solar cells have great potential in photovoltaic applications for buildings and wearable electronics due to their lightweight, shockproof, and self-powered properties. Despite 50 years of effort, the development of flexible silicon solar cells has been stagnant due to their rigidity. This study presents a strategy for fabricating large-scale, foldable silicon wafers and manufacturing flexible solar cells with improved flexibility. These cells demonstrate high efficiency and durability, making them suitable for commercial production in flexible modules.

NATURE (2023)

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Article Energy & Fuels

Solar cell efficiency tables (version 62)

Martin A. A. Green et al.

Summary: This article presents consolidated tables showing the highest independently confirmed efficiencies for solar cells and modules. The guidelines for including results into these tables are outlined, and new entries since January 2023 are reviewed.

PROGRESS IN PHOTOVOLTAICS (2023)

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Article Energy & Fuels

Kesterite based monograin photovoltaics: The ideal solution for sustainable power supply

Dieter Meissner et al.

Summary: The growth of PV installations using highly efficient monocrystalline silicon modules is progressing well in developed countries, but the progress of electrification in cities and poor countries is lagging behind the targets set by the UN Sustainable Development Goals. Over 40% of the world population still lacks access to clean fuels and technologies for cooking. Low-cost decentralized and flexible PV technology, such as monograin technology, offers a solution for harvesting solar energy in densely populated regions and remote areas. This technology is sustainable, with low material losses and energy input, making it suitable for developing countries interested in decentralized power production.

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2023)

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Article Energy & Fuels

Impact of Li and K co-doping on the optoelectronic properties of CZTS monograin powder

Katri Muska et al.

Summary: This study investigated the effects of Li and K co-doping on the properties of Cu2ZnSnS4 (CZTS) monograin powders used in monograin layer (MGL) solar cells. CZTS powders were grown using different LiI-KI ratios in the synthesis-growth process. The Li concentration in the synthesized CZTS varied depending on the initial amount of LiI, while the amount of K remained constant. The addition of Li in CZTS resulted in the formation of a solid solution and an increase in the effective bandgap energy. Solar cells using Li and K co-doped CZTS powder showed the highest performance with a power conversion efficiency of 9.4%.

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2023)

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Article Energy & Fuels

Control of the phase evolution of kesterite by tuning of the selenium partial pressure for solar cells with 13.8% certified efficiency

Jiazheng Zhou et al.

Summary: The phase evolution during selenization of CZTSSe is controlled to improve efficiency of solar cells. By applying positive pressure in the reaction chamber, the formation of secondary phases is prevented, resulting in high-crystallinity kesterite films. Solar cells with 13.8% certified efficiency are achieved. This work provides insights into the phase evolution and mechanism of kesterite absorbers.

NATURE ENERGY (2023)

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Article Chemistry, Physical

Flexible Perovskite Solar Cells: From Materials and Device Architectures to Applications

Yuanji Gao et al.

Summary: In this article, recent progress in flexible perovskite solar cells (f-PSCs) is reviewed, including flexible substrates, flexible transparent electrodes, performance optimization, large-scale fabrication techniques, and flexibility enhancement strategies. The potential applications and future development prospects of f-PSCs are also discussed.

ACS ENERGY LETTERS (2022)

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Article Energy & Fuels

Reduced recombination through CZTS/CdS interface engineering in monograin layer solar cells

M. Kauk-Kuusik et al.

Summary: The efficiency of CZTS solar cells can be improved by controlling the intermixing of Cd and Cu at the CZTS/CdS interface. Cd diffusion into the CZTS surface after CdS air-annealing forms an ultra-thin Cu2Zn (x) Cd1-x SnS4 layer, reducing interface recombination and enhancing the performance of the cell.

JOURNAL OF PHYSICS-ENERGY (2022)

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Article Engineering, Environmental

Highly efficient flexible organic photovoltaic modules for sustainable energy harvesting under low-light condition via suppressing voltage-drop by metal-mediated cross-linkable polymer interfacial layer

Muhammad Jahandar et al.

Summary: This study aims to improve the efficiency and stability of large-area flexible organic photovoltaics (OPV) by developing a novel interfacial layer (c-PEIE CIL) and non-fullerene acceptor material. The research found that OPV cells based on c-PEIE CIL achieved high efficiency and stability, especially in cloudy weather conditions.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Materials Science, Multidisciplinary

Characterization of tetrahedrite Cu10Cd2Sb4S13 monograin materials grown in molten CdI2 and LiI

Fairouz Ghisani et al.

Summary: Cd-substituted tetrahedrite Cu10Cd2Sb4S13 (TH-Cd) monograin powders were synthesized using the molten salt synthesis-growth method with CdI2 and LiI as fluxes. XRD data showed formation of single phase tetrahedrite Cu10Cd2Sb4S13 in both fluxes, with differences in lattice parameters and composition. Energy dispersive X-ray spectroscopy and Atomic Absorption Spectroscopy confirmed stoichiometry and Li incorporation in the crystals, while photoluminescence study revealed different PL bands and activation energies for crystals grown in CdI2 and LiI. Li incorporation from LiI into the crystal lattice of TH-Cd forming a solid solution was evidenced by the changes observed.

THIN SOLID FILMS (2021)

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Article Chemistry, Physical

Detailed Insight into the CZTS/CdS Interface Modification by Air Annealing in Monograin Layer Solar Cells

Marit Kauk-Kuusik et al.

Summary: Research has shown that the temperature and duration of air annealing play a crucial role in the performance of CZTS/CdS heterojunction devices, with different annealing methods having varying effects on device efficiency. Through effects such as elemental intermixing and Cu-Zn ordering, the performance of the CZTS/CdS interface can be improved, but the issue of copper enrichment at the interface still needs to be addressed.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Band Tails and Cu-Zn Disorder in Cu2ZnSnS4 Solar Cells

J. K. Larsen et al.

ACS APPLIED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Upper limit to the photovoltaic efficiency of imperfect crystals from first principles

Sunghyun Kim et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Article Energy & Fuels

All-solution-processed transparent front contact for monograin layer kesterite solar cells

Stefan Edinger et al.

PROGRESS IN PHOTOVOLTAICS (2019)

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Article Physics, Applied

Observation of band gap fluctuations and carrier localization in Cu2CdGeSe4

Juri Krustok et al.

JOURNAL OF PHYSICS D-APPLIED PHYSICS (2019)

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Article Energy & Fuels

Cd-Free Cu(In,Ga)(Se,S)2 Thin-Film Solar Cell With Record Efficiency of 23.35%

Motoshi Nakamura et al.

IEEE JOURNAL OF PHOTOVOLTAICS (2019)

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Article Chemistry, Physical

The effect of Ag alloying of Cu2(Zn,Cd)SnS4 on the monograin powder properties and solar cell performance

Kristi Timmo et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Article Energy & Fuels

The electrical and optical properties of kesterites

Maarja Grossberg et al.

JOURNAL OF PHYSICS-ENERGY (2019)

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Article Energy & Fuels

Doping and alloying of kesterites

Yaroslav E. Romanyuk et al.

JOURNAL OF PHYSICS-ENERGY (2019)

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Article Energy & Fuels

Back and front contacts in kesterite solar cells: state-of-the-art and open questions

Charlotte Platzer-Bjorkman et al.

JOURNAL OF PHYSICS-ENERGY (2019)

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Article Chemistry, Physical

Understanding the Effects of Cd and Ag Doping in Cu2ZnSnS4 Solar Cells

Gopalakrishnan Sai Gautam et al.

CHEMISTRY OF MATERIALS (2018)

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Article Materials Science, Multidisciplinary

Study of Cu2CdGeSe4 monograin powders synthesized by molten salt method for photovoltaic applications

M. Kauk-Kuusik et al.

THIN SOLID FILMS (2018)

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Article Chemistry, Physical

Synergistic Effects of Double Cation Substitution in Solution-Processed CZTS Solar Cells with over 10% Efficiency

Shreyash H. Hadke et al.

ADVANCED ENERGY MATERIALS (2018)

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Article Chemistry, Inorganic & Nuclear

Substitution of Li for Cu in Cu2ZnSnS4: Toward Wide Band Gap Absorbers with Low Cation Disorder for Thin Film Solar Cells

A. Lafond et al.

INORGANIC CHEMISTRY (2017)

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Article Chemistry, Physical

Modification of the optoelectronic properties of Cu2CdSnS4 through low-temperature annealing

M. Pilvet et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2017)

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Article Materials Science, Multidisciplinary

Influence of order-disorder in Cu2ZnSnS4 powders on the performance of monograin layer solar cells

K. Timmo et al.

THIN SOLID FILMS (2017)

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Article Chemistry, Physical

Investigation of rough surfaces on Cu2ZnSn(SxSe1-x)4 monograin layers using light beam induced current measurements

Christian Neubauer et al.

APPLIED SURFACE SCIENCE (2017)

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Article Nanoscience & Nanotechnology

New Insight of Li-Doped Cu2ZnSn(S,Se)4 Thin Films: Li-Induced Na Diffusion from Soda Lime Glass by a Cation-Exchange Reaction

Yanchun Yang et al.

ACS APPLIED MATERIALS & INTERFACES (2017)

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Article Nanoscience & Nanotechnology

Tuning the Band Gap of Cu2ZnSn(S,Se)4 Thin Films via Lithium Alloying

Yanchun Yang et al.

ACS APPLIED MATERIALS & INTERFACES (2016)

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Article Chemistry, Physical

Germanium Alloyed Kesterite Solar Cells with Low Voltage Deficits

A. D. Collord et al.

CHEMISTRY OF MATERIALS (2016)

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Article Chemistry, Physical

Ag2ZnSn(S,Se)4: A highly promising absorber for thin film photovoltaics

Evgueni Chagarov et al.

JOURNAL OF CHEMICAL PHYSICS (2016)

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Article Chemistry, Physical

Is the Cu/Zn Disorder the Main Culprit for the Voltage Deficit in Kesterite Solar Cells?

Stephane Bourdais et al.

ADVANCED ENERGY MATERIALS (2016)

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Article Chemistry, Physical

Nanoscale Microstructure and Chemistry of Cu2ZnSnS4/CdS Interface in Kesterite Cu2ZnSnS4 Solar Cells

Fangyang Liu et al.

ADVANCED ENERGY MATERIALS (2016)

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Proceedings Paper Physics, Applied

Comparative study of SnS recrystallization in molten CdI2, SnCl2 and KI

Kristi Timmo et al.

PHYSICA STATUS SOLIDI C: CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 13, NO 1 (2016)

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Engineering Solar Cell Absorbers by Exploring the Band Alignment and Defect Disparity: The Case of Cu- and Ag-Based Kesterite Compounds

Zhen-Kun Yuan et al.

ADVANCED FUNCTIONAL MATERIALS (2015)

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p-n junction improvements of Cu2ZnSnS4/CdS monograin layer solar cells

M. Kauk-Kuusik et al.

APPLIED SURFACE SCIENCE (2015)

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Article Materials Science, Multidisciplinary

Compositionally tunable structure and optical properties of Cu1.85(CdxZn1-x)1.1SnS4.1 (0 ≤ x ≤ 1) monograin powders

M. Pilvet et al.

THIN SOLID FILMS (2015)

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Article Physics, Applied

A low-temperature order-disorder transition in Cu2ZnSnS4 thin films

Jonathan J. S. Scragg et al.

APPLIED PHYSICS LETTERS (2014)

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Fast and reliable calculation of the two-diode model without simplifications

Stephan Suckow et al.

PROGRESS IN PHOTOVOLTAICS (2014)

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Review Chemistry, Multidisciplinary

Classification of Lattice Defects in the Kesterite Cu2ZnSnS4 and Cu2ZnSnSe4 Earth-Abundant Solar Cell Absorbers

Shiyou Chen et al.

ADVANCED MATERIALS (2013)

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Post-growth annealing effect on the performance of Cu2ZnSnSe4 monograin layer solar cells

M. Kauk-Kuusik et al.

THIN SOLID FILMS (2013)

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Article Physics, Applied

Impact of KCN etching on the chemical and electronic surface structure of Cu2ZnSnS4 thin-film solar cell absorbers

M. Baer et al.

APPLIED PHYSICS LETTERS (2011)

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The crystal structure of kesterite type compounds: A neutron and X-ray diffraction study

Susan Schorr

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2011)

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Influence of compositional deviations on the properties of Cu2ZnSnSe4 monograin powders

K. Muska et al.

EUROPEAN MATERIALS RESEARCH SOCIETY CONFERENCE SYMPOSIUM: ADVANCED INORGANIC MATERIALS AND CONCEPTS FOR PHOTOVOLTAICS (2011)

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Synthesis of Cu2ZnSnS4 monograin powders with different compositions

K. Muska et al.

EUROPEAN MATERIALS RESEARCH SOCIETY CONFERENCE SYMPOSIUM: ADVANCED INORGANIC MATERIALS AND CONCEPTS FOR PHOTOVOLTAICS (2011)

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Proceedings Paper Energy & Fuels

Effects of sulphur and tin disulphide vapour treatments of Cu2ZnSnS(Se)4 absorber materials for monograin solar cells

M. Kauk et al.

EUROPEAN MATERIALS RESEARCH SOCIETY CONFERENCE SYMPOSIUM: ADVANCED INORGANIC MATERIALS AND CONCEPTS FOR PHOTOVOLTAICS (2011)

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Sulfur-containing Cu2ZnSnSe4 monograin powders for solar cells

K. Timmo et al.

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2010)

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Article Physics, Applied

Crystal and electronic band structure of Cu2ZnSnX4 (X=S and Se) photovoltaic absorbers: First-principles insights

Shiyou Chen et al.

APPLIED PHYSICS LETTERS (2009)

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Cu2Zn1-xCdxSn(Se1-ySy)(4) solid solutions as absorber materials for solar cells

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PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE (2008)

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Stability issues of Cu(In,Ga)Se2-based solar cells

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