期刊
FOOD CHEMISTRY-X
卷 20, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.fochx.2023.100902
关键词
Fruit spirits; SVM; PLS-DA; Raman spectroscopy; Recognition models
This study aimed to test the efficiency of FT-Raman spectroscopy for fruit spirits discrimination by developing differentiation models. Different preprocessing methods and feature selection steps helped to construct classification models with accuracy scores greater than 90%.
The present work aimed to test the efficiency of FT-Raman spectroscopy for fruit spirits discrimination by developing differentiation models based on two approaches, namely a supervised statistical method (Partial Least Squares Discriminant Analysis), and a Machine Learning technique (Support Vector Machines). For this purpose, a data set comprising 86 Romanian distillate samples was used, which aimed to be differentiated in terms of the raw material used for production (plum, apple, pear and grape) and county of origin (Cluj, Satu Mare and Salaj). Eight distinct preprocessing methods (autoscale, mean center, variance scaling, smoothing, 1st derivative, 2nd derivative, standard normal variate and Pareto) followed by a feature selection step were applied to identify the meaningful input data based on which the most efficient classification models can be constructed. Both types of models led to accuracy scores greater than 90% in differentiating the distillate samples in terms of geographical and botanical origin.
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