期刊
ADVANCED OPTICAL MATERIALS
卷 4, 期 4, 页码 608-619出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adom.201500670
关键词
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资金
- Air Force Office of Scientific Research (Synthetic photonics multidisciplinary university research initiative, synthesis, fabrication, and development) [FA9550-14-1-0037]
- U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-09ER46604]
- UES-AFRL [S-977-022-001]
- Office of Secretary Defense-Test and Evaluation (OSD-TE)
- National Defense Education Program (NDEP)/BA-1 [Defense-Wide/PE0601120D8Z]
- Basic Research, SMART Program office Grant [N00244-09-1-0081]
A facile one-step fabrication of large-area multicolored emissive photopatterns in mixed quantum dot-polymer films is demonstrated. This is in sharp contrast to the current photopatterning approaches that utilize only a single quantum dot (QD) component for single-color patterns. Strategies are presented that allow for either selective or collective modification of specific predetermined photoluminescent peaks of green and red QDs during photopattern development. These strategies yield novel patterns and allow for unprecedented control over how the color contrast of the photopattern evolves with continuous light illumination. These results clearly show that the evolution of the emission spectra of a multicolor mixed QD-polymer film can be readily tailored during pattern development, either by careful selection of the excitation wavelength or through combinations of controllably unstable and stable QDs with different recovery rates. Notably, these strategies are simple, fast, and robust, yielding high-resolution microscopic patterns over large areas (up to fractions of a cm(2)). Furthermore, the flexibility and capabilities of these strategies greatly expand the potential applications of multicolor emissive photopatterns, particularly in the areas of sensing, imaging, and lasing systems where it is important to exert delicate control over the intensity of selected colors within specific spatial regions.
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