期刊
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
卷 4, 期 11, 页码 6186-6192出版社
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.6b01779
关键词
Biomass conversion; Multifunctional catalysis; Hydrodeoxygenation; Continuous flow; Ruthenium; Eucalyptol
资金
- Excellence Initiative of the German federal and state government
- Deutscher Akademischer Austaush Dienst (DAAD)
- Alexander von Humboldt Foundation
Ruthenium nanoparticles immobilized on acidfunctionalized supported ionic liquid phases (RuNPs@SILPs) were applied in the hydrodeoxygenation of eucalyptol. RuNPs@SILPs were highly effective and selective catalysts toward the synthesis of the deoxygenation product p-menthane, in which the catalytic properties of the bifunctional catalysts was dependent on the acidity of the SILP. Integration of the acid and metal catalytic species onto a single-support allowed for the implementation of RuNPs@SILP into a continuous flow process. The modular synthesis of these bifunctional catalysts also allowed for an investigation into the roles of the individual and combined acid and metal functionalities in the hydrodeoxygenation of eucalyptol.
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