☆ 4.8 Review

Ferromagnetic Elements in Two-Dimensional Materials: 2D Magnets and Beyond

ADVANCED FUNCTIONAL MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Electrochemically exfoliated Ni-doped MoS2 nanosheets for highly efficient hydrogen evolution and Zn-H2O battery

Hao Wei et al.

Summary: In this research, a one-step electrochemical exfoliation strategy was developed to fabricate Ni-doped MoS2 nanosheets with high electrical conductivity and abundant active sites. The Ni-EX-MoS2 catalyst exhibited excellent electrocatalytic performance for the hydrogen evolution reaction and showed potential for applications in energy conversion.

CHINESE CHEMICAL LETTERS (2023)

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Article Green & Sustainable Science & Technology

Heterostructure of amorphous nickel boride anchored 2D-layered cobalt selenide nanosheets as a disposable strip sensor for detection of toxic pollutant 5-nitroquinoline in aquatic samples

Ramaraj Sukanya et al.

Summary: A distinctive approach was taken to develop an electrochemical heterostructure sensor with chemically reduced nickel boride (Ni3B) nanoparticles anchored in two-dimensional (2D) layered cobalt selenide (CoSe) nanosheets for the electrochemical monitoring of water pollutant 5-nitroquinoline (5-NQ). The fabricated hybrid 2D CoSe/Ni3B/SPCE disposable sensor showed excellent electrocatalytic activity, a wide linear range, and a low detection limit for 5-NQ. This work provides a clear idea for the fabrication of transition metal-based metal boride and selenide heterostructures with excellent catalytic activity for the electrochemical detection of various pollutants in real-time monitoring.

JOURNAL OF CLEANER PRODUCTION (2023)

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Article Chemistry, Physical

Rational design of hollow rice-grained α-Fe2O3/carbon nanofibers with optimized impedance matching for electromagnetic wave absorption enhanced

Jingshen Xu et al.

Summary: In this study, Fe2O3/CNFs composites were prepared by the in-situ transformation method, combining carbon nanofibers (CNFs) with hollow rice-grained alpha-Fe2O3 nanoparticles. The rational microstructure design reduced the filling ratio, optimized impedance matching, and improved electromagnetic wave absorption performance. The Fe2O3/CNFs composites achieved strong reflection loss (-38.1 dB) and broad effective absorption bandwidth (4.6 GHz) at a low filling ratio (20 wt.%), and analysis of electromagnetic parameters confirmed the crucial role of the microstructure in the performance improvement. With optimized impedance matching and a simple preparation method, Fe2O3/CNFs have broad application prospects in electromagnetic wave absorption.

NANO RESEARCH (2023)

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Article Chemistry, Multidisciplinary

Room-temperature spin-valve devices based on Fe3GaTe2/MoS2/Fe3GaTe2 2D van der Waals heterojunctions

Wen Jin et al.

Summary: This study presents a two-dimensional spin valve device based on a two-dimensional ferromagnetic crystal, which exhibits a stable spin-valve effect at room temperature with high magnetoresistance. The research provides a new approach to develop room-temperature two-dimensional spin valve devices.

NANOSCALE (2023)

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Article Chemistry, Physical

Submonolayer Eu superstructures-A class of 2D magnets

Dmitry Averyanov et al.

Summary: The study demonstrates that regular Eu lattices form a class of 2D magnets with different structures, stoichiometries, and chemical bonding. The magnetic properties of the Eu superstructures show ferromagnetic or ferrimagnetic behavior. Control over the magnetic transition temperature by weak magnetic fields further confirms the 2D nature of the magnetism.

NANO RESEARCH (2023)

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Article Chemistry, Physical

Terbium-modified two-dimensional zirconium-based metal-organic frameworks for photoluminescence detection of nitrite

You-Liang Chen et al.

Summary: This study demonstrates the post-synthetic installation of terbium ions on a 2D water-stable zirconium-based metal-organic framework. The loading of terbium ions can be adjusted by tuning the synthetic temperature. The energy transfer from the framework to the terbium sites can be highly tunable, making it suitable for nitrite quantification.

MOLECULAR SYSTEMS DESIGN & ENGINEERING (2023)

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Article Engineering, Electrical & Electronic

Magnetism modulation in Co3Sn2S2 by current-assisted domain wall motion

Qiuyuan Wang et al.

Summary: The efficiency of spintronic devices can be improved by generating higher effective magnetic fields with lower working currents. Spin-transfer torques can drive magnetic domain wall motion in a device composed of a single material. Here, we report magnetism modulation in Co3Sn2S2-a magnetic Weyl semimetal-via spin-transfer-torque-driven domain wall motion. The threshold current density for driving domain wall motion is less than 5.1 x 10(5) A cm(-2) at zero external field and less than 1.5 x 10(5) A cm(-2) at a moderate external field (0.2 kOe). The spin-transfer-torque effective field can reach as high as 2.4-5.6 kOe MA(-1) cm(2) at 150 K.

NATURE ELECTRONICS (2023)

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Article Electrochemistry

Facile synthesis of Ni doped BiOBr nanosheets as efficient photo-assisted charging supercapacitors

Amornrat Khampunbut et al.

Summary: Enhanced visible light-driven pseudocapacitance response is achieved by synthesizing Ni-doped BiOBr nanosheets via a facile precipitation method. The doping of Ni atoms onto the BiOBr structure expands the light absorption range and improves photogenerated carrier separation efficiency. The Ni-BiOBr photoelectrode exhibits a significantly higher specific capacitance under UV light compared to dark conditions. Moreover, the Ni-BiOBr//reduced graphene oxide asymmetric supercapacitors demonstrate excellent energy density and capacitance retention under light irradiation.

ELECTROCHIMICA ACTA (2023)

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Article Engineering, Chemical

High permeability dual-channel membranes based on porous Fluorine-Cerium nanosheets for molecular sieving

Shurui Han et al.

Summary: Two-dimensional membranes based on fluorine-cerium nanosheets offer great potential for molecular separation. By adjusting pore size, surface structure, and loading amounts, these membranes achieve high regularity separation channels and precise molecular separation ability. They demonstrate stable long-term use and promising repeatability, as well as good chemical and mechanical stability.

JOURNAL OF MEMBRANE SCIENCE (2023)

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Article Chemistry, Multidisciplinary

A Room-Temperature Spin-Valve with van der Waals Ferromagnet Fe5GeTe2/Graphene Heterostructure

Bing Zhao et al.

Summary: This article demonstrates the robust room-temperature operation of lateral spin-valve devices using the vdW ferromagnet Fe5GeTe2 in heterostructures with graphene. Spin-dynamics measurements reveal multidirectional spin polarization at the Fe5GeTe2/graphene interface. Density functional theory calculations and Monte Carlo simulations reveal significantly canted Fe magnetic moments in Fe5GeTe2 along with the presence of negative spin polarization at the interface. These findings open opportunities for vdW interface design and applications of vdW-magnet-based spintronic devices at ambient temperatures.

ADVANCED MATERIALS (2023)

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Article Chemistry, Physical

Improving performances of Lithium-Sulfur cells via regulating of VSe2 functional mediator with Doping-Defect engineering and Electrode-Separator integration strategy

Yumiao Han et al.

Summary: In this study, a nickel-doped vanadium selenide/reduced graphene oxide (NiVSe2/rGO) composite was prepared and used as a modified separator in lithium-sulfur batteries. The composite material adsorbed lithium polysulfides and catalyzed their conversion reaction, effectively reducing their diffusion and suppressing the shuttle effect. Additionally, the integration of the electrode and separator improved the performance of the battery, allowing for high sulfur loading and low electrolyte/sulfur ratio.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2023)

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Article Nanoscience & Nanotechnology

Room-Temperature and Tunable Tunneling Magnetoresistance in Fe3GaTe2-Based 2D van der Waals Heterojunctions

Wen Jin et al.

Summary: This study demonstrates a room-temperature magnetic tunnel junction (MTJ) based on a Fe3GaTe2/WS2/Fe3GaTe2 heterostructure, which exhibits a tunneling magnetoresistance (TMR) ratio of up to 213% and a high spin polarization of 72% at 10 K, the highest reported in Fe3GaTe2-based MTJs so far. The MTJ also maintains a robust tunneling spin-valve signal at room temperature (300 K) with low bias currents, offers potential for low-energy consumption in all-2D vdW spintronics and provides alternative routes for electronic control of spintronic devices.

ACS APPLIED MATERIALS & INTERFACES (2023)

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Article Multidisciplinary Sciences

Ferromagnetism emerged from non-ferromagnetic atomic crystals

Cheng Gong et al.

Summary: The isolation of graphene has sparked interest in two-dimensional materials, and recently, ferromagnetism has been observed in several. Gong et al. have found a ferromagnetic state at the interface of antiferromagnetic FePS3 and non-magnetic WS2, providing an alternative approach to achieve two-dimensional ferromagnetism.

NATURE COMMUNICATIONS (2023)

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Article Environmental Sciences

Insight into the improved photocatalytic removal of tetracycline hydrochloride by constructing cobalt doping in 2D/2D (BiO)2CO3/BiOCl type-II heterojunctions

Honghong Wang et al.

Summary: Element doping coupled with heterojunction construction and morphology control is an efficient way to improve the properties of photocatalytic materials. In this study, a thiourea-modified 2D/2D cobalt-doped (BiO)2CO3/BiOCl heterojunction photocatalyst (Co-(BC/BL)Tu) was constructed using a simple one-pot hydrothermal method. The Co-(BC/BL)Tu product exhibited outstanding visible-light-driven photodegradation property, with a photodegradation rate constant k value 5.2 times higher than that of pure (BiO)2CO3, attributed to the synergistic effect of the 2D/2D structure, cobalt doping, and type-II heterostructures. This study provides a facile and promising strategy for constructing a high-effective photocatalytic system by combining morphology control engineering, doping engineering, and heterostructure engineering.

CHEMOSPHERE (2023)

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Article Chemistry, Multidisciplinary

Spin-Orbit Torque Switching in an All-Van der Waals Heterostructure

Inseob Shin et al.

Summary: The study explores the control of magnetization in ferromagnets using spin-orbit torque, highlighting the use of vdW topological materials WTe2 and ferromagnet Fe3GeTe2 to meet the requirements for energy-efficient spintronic devices. By engineering vdW-type materials, a significantly reduced switching current density is achieved, offering a promising approach for energy-efficient magnetization control in SOT-based spintronics.

ADVANCED MATERIALS (2022)

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Article Chemistry, Physical

Co-anion exchange prepared 2D structure Ni(Co,Fe)PS for efficient overall water electrolysis

Yongjae Jeung et al.

Summary: In this study, 2D-structured Ni(Co,Fe) PS catalysts were synthesized to achieve efficient HER and OER processes through the combination of sulfide and phosphide. The synthesized catalysts exhibited lower overpotentials and Tafel slope values, as well as significantly reduced charge transfer resistance, contributing to the improved efficiency of an overall water splitting system.

APPLIED SURFACE SCIENCE (2022)

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Article Chemistry, Physical

Governing the Ni content and size of 2D layered C/Ni nanoparticle composites for enhanced electromagnetic wave absorption

Minmin Liu et al.

Summary: Control of size and dispersity is critical for magnetic metal absorbents to inhibit eddy currents and enhance electromagnetic wave absorption performance (EMWAP). Layered C/Ni nano particle (NP) composites were developed with controlled size and dispersity for excellent EMWAP. The synthetic method via one-step calcination process allows for adjustment of electric/magnetic properties and EMWAP, showing high absorption rate, thin thickness, and wide bandwidth.

APPLIED SURFACE SCIENCE (2022)

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Article Materials Science, Multidisciplinary

Edge ferromagnetism of graphene oxide

Roman Strzelczyk et al.

Summary: The intrinsic ferromagnetism in graphene oxide is related to the zigzag edges created during the exfoliation process, with spin-flip transitions of protons from hydroxyl groups enhancing spin fluctuations. This results in superferromagnetism below a specific temperature range, with residual ferromagnetism observed in GO paper due to surviving magnetic moments in closed pores.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2022)

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Article Chemistry, Physical

Monolayer gadolinium halides, GdX2 (X = F, Cl, Br): intrinsic ferrovalley materials with spontaneous spin and valley polarizations

Kang Sheng et al.

Summary: The monolayers (MLs) GdX2, where X = F, Cl, Br, have been predicted to be rare and excellent materials with high stability, magnetic anisotropy, Curie temperature, and spontaneous valley polarization. These unique properties make them promising candidates for experimental studies and practical applications in spintronics and valleytronics.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2022)

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Review Materials Science, Multidisciplinary

Recent advances in two-dimensional ferromagnetism: strain-, doping-, structural- and electric field-engineering toward spintronic applications

Sheng Yu et al.

Summary: Since 2017, a wide range of 2D magnetic materials with unusual physical characteristics have been discovered, providing a platform for exploring novel 2D spintronic devices. Significant progress has been made in both theoretical and experimental studies. Various engineering strategies, such as strain, doping, structure, and electric field manipulation, have been applied to practical spintronic applications.

SCIENCE AND TECHNOLOGY OF ADVANCED MATERIALS (2022)

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Article Materials Science, Multidisciplinary

2D Van der Waals Rare Earth Material Based Ratiometric Luminescence Thermography Integrated on Micro-Nano Devices Vertically

Ping Chen et al.

Summary: This study demonstrates a ratiometric luminescence thermography technique based on 2D van der Waals rare earth material. It enables vertical integration of micro-nano devices and provides real-time temperature estimation during operation. The technology shows potential for wide application, providing high-resolution temperature distribution information and facilitating the development of high-performance electronic devices.

ADVANCED OPTICAL MATERIALS (2022)

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Article Chemistry, Applied

Electronic structure modulation with ultrafine Fe3O4 nanoparticles on 2D Ni-based metal-organic framework layers for enhanced oxygen evolution reaction

Wei Huang et al.

Summary: In this study, ultrafine Fe3O4 nanoparticles were immobilized on 2D Ni-based MOFs to enhance OER stability and catalytic activity. The optimal Fe3O4/Ni-BDC composite showed the best OER performance with higher overpotential, lower Tafel slope, and considerable durability, facilitated by Fe species with a higher oxidation state for the formation of adsorbed O* species.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Analytical

All-Electrical Control of Compact SOT-MRAM: Toward Highly Efficient and Reliable Non-Volatile In-Memory Computing

Huai Lin et al.

Summary: This study reports on a new type of non-volatile spin-orbit torque magnetic tunnel junction (MTJ) device based on 2D material Fe3GeTe2, which demonstrates uni-polar and high-speed field-free magnetization switching. Compared to conventional structures, this device shows improved data storage features and larger sensing margin, and can be used for Boolean logic operations with faster latency and lower power consumption.

MICROMACHINES (2022)

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Review Chemistry, Multidisciplinary

Surface Functionalization for Magnetic Property Tuning of Nonmagnetic 2D Materials

Serrae N. Reed-Lingenfelter et al.

Summary: Surface functionalization with organic molecules has been effective in modulating the electronic properties of 2D materials and inducing magnetic behaviors in nonmagnetic 2D materials. Key studies have shown that graphene, layered topological insulators, and transition metal dichalcogenides can be functionalized with different molecules to impart magnetic properties, opening up exciting opportunities for future research and applications.

ADVANCED MATERIALS INTERFACES (2022)

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Article Chemistry, Physical

Heterogeneous Activation of Persulfate by LaMO3 (M=Co, Fe, Cu, Mn, Ni) Perovskite Catalysts for the Degradation of Organic Compounds

Donatos Manos et al.

Summary: Sulfate radical-based advanced oxidation processes (SR-AOPs) have been used for degrading pollutants by generating reactive oxidant species (ROS) through the activation of oxidants. In this study, a series of LaMO3 (M=Co, Fe, Cu, Mn, Ni) perovskite catalysts were synthesized and tested for their activity in activating persulfate for the degradation of phenolic pollutants. The results showed that the catalytic activity depended on the structure facilitating electron transfer between the perovskite and oxidant, with LaNiO3 and LaCoO3 as the most active catalysts.

CATALYSTS (2022)

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Article Nanoscience & Nanotechnology

Few-Layered WS2 Anchored on Co, N-Doped Carbon Hollow Polyhedron for Oxygen Evolution and Hydrogen Evolution

Liangbin Xia et al.

Summary: WS2@Co9S8, prepared by inhibiting WS2 growth using Co-based zeolite imidazole framework (ZIF-67), showed excellent catalytic activity for OER and HER, with an OER potential only 15 mV higher than that of RuO2.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Review Pharmacology & Pharmacy

2D materials-based nanomedicine: From discovery to applications

Jiang Ouyang et al.

Summary: Due to their unique physicochemical characteristics, 2D materials have attracted increasing attention in the field of biomedicine. Nanomedicines based on 2D materials have been extensively applied in various diseases, showing great potential in therapeutic and imaging applications, as well as in biological functionalization.

ADVANCED DRUG DELIVERY REVIEWS (2022)

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Article Chemistry, Analytical

Design and fabrication of novel flexible sensor based on 2D Ni-MOF nanosheets as a preliminary step toward wearable sensor for onsite Ni (II) ions detection in biological and environmental samples

Sally E. A. Elashery et al.

Summary: In this study, an innovative and sensitive flexible sensor for efficient potentiometric monitoring of Ni (II) ions has been designed and developed. The flexible sensor shows rapid, accurate and stable response in monitoring Ni (II) ions in biological and environmental samples.

ANALYTICA CHIMICA ACTA (2022)

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Review Chemistry, Multidisciplinary

Electrochemistry in Magnetic Fields

Songzhu Luo et al.

Summary: Developing new strategies in magnetoelectrochemistry is crucial to control and understand electrochemical reactions. It combines concepts from multiple disciplines and explores the effects of magnetic fields on fundamental electrochemical principles.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Education, Scientific Disciplines

Hybridization bond states and band structure of graphene: a simple approach

Mario Perez et al.

Summary: This article reviews the basic theoretical aspects of graphene and presents a simplified and understandable approach to its structure and band properties. It aims to show that the abstract nature of graphene is not as daunting as it may seem.

EUROPEAN JOURNAL OF PHYSICS (2022)

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Article Chemistry, Physical

Emerging 2D magnetic states in a graphene-based monolayer of EuC6

Ivan S. Sokolov et al.

Summary: Recent discoveries of intrinsic two-dimensional magnets have opened up vast opportunities in addressing fundamental problems in condensed matter physics, with potential applications ranging from ultra-compact spintronics to quantum computing. However, the ever-growing material landscape of 2D magnets lacks carbon-based systems, which are prominent in other areas of 2D research. Investigations on monolayer EuC6 have revealed emergence of 2D ferromagnetism, but detailed studies on competing magnetic states are still needed.

NANO RESEARCH (2022)

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Article Chemistry, Physical

Ultra-broadband, fast, and polarization-sensitive photoresponse of low-symmetry 2D NdSb2

Gang Li et al.

Summary: Broadband photodetectors with polarization-sensitive ability have attracted significant attention for their potential use in optoelectronic devices. In this work, a low-symmetry two-dimensional material, neodymium diantimonides (NdSb2), is introduced as a highly anisotropic material for broadband detection. The photodetector demonstrates high responsivity and fast response time at 532 nm, as well as stable performance over a long period of time. The polarization sensitivity and anisotropic factor of the detector are also investigated, revealing its potential for high-performance polarized photodetectors.

NANO RESEARCH (2022)

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Review Chemistry, Physical

A Review of the Synthesis, Properties, and Applications of 2D Materials

Vigneshwaran Shanmugam et al.

Summary: With the discovery of graphene, the study and development of novel 2D materials have been made possible, offering unique properties that surpass traditional bulk materials. This article provides an overview of the intrinsic properties of 2D materials, as well as reviews and discusses their synthesis, applications, and future prospects. Intensive research in this area is expected to lead to the discovery of new materials with enhanced properties, benefiting both industries and society.

PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION (2022)

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Article Multidisciplinary Sciences

Designing of two dimensional lanthanum cobalt hydroxide engineered high performance supercapacitor for longer stability under redox active electrolyte

Deepa B. Bailmare et al.

Summary: This study investigates the influence of rare earth elements on the stability of layered double hydroxides (LDHs) in redox active electrolyte supercapacitors. The choice of rare earth element (such as lanthanum) is found to have a significant impact on the stability of La-Co LDHs electrode in redox electrolyte. This highlights the importance of considering rare earth elements in the design of LDH systems for redox active supercapacitor development.

SCIENTIFIC REPORTS (2022)

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Article Chemistry, Physical

In situ preparation of two-dimensional ytterbium ions doped all-inorganic perovskite nanosheets for high-performance visual dual-bands photodetectors

Rui Sun et al.

Summary: This study presents the synthesis of 2D all-inorganic perovskite nanosheets doped with rare earth ions, demonstrating excellent optical and electrical properties. The morphology of the nanosheets can be adjusted by changing ligand ratios, resulting in high-performance photodetectors with dual-band detection capabilities. The passivation effect of Yb3+ ions enhances the photostability of the nanosheets, leading to a high responsivity and dual-band detection capability in photodetectors.

NANO ENERGY (2022)

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Article Chemistry, Physical

Computation-Aided Discovery and Synthesis of 2D PrOBr Photocatalyst

Rongyan Wang et al.

Summary: This study reports the discovery and synthesis of a new photocatalyst, PrOBr, which shows high efficiency and stability. The 2D material exhibits high catalytic activity in water splitting and carbon dioxide reduction, outperforming traditional 2D photocatalysts.

ACS ENERGY LETTERS (2022)

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Article Materials Science, Multidisciplinary

Two-dimensional ferromagnetism detected by proximity-coupled quantum Hall effect of graphene

Tuan Khanh Chau et al.

Summary: The recent discovery of a two-dimensional van der Waals magnet has opened up new possibilities for understanding two-dimensional magnetic systems. By coupling monolayer graphene with the two-dimensional ferromagnet CGT, we are able to electrically monitor the magnetic phase transition of the CGT layer.

NPJ QUANTUM MATERIALS (2022)

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Article Chemistry, Physical

Exfoliated Fe3GeTe2 and Ni3GeTe2 materials as water splitting electrocatalysts

Filipa M. Oliveira et al.

Summary: It has been found that two-dimensional layered metallic materials Fe3GeTe2 and Ni3GeTe2 have stable water- and air-stability. Fe3GeTe2 has shown excellent oxygen evolution reaction (OER) activity, while the electrochemical catalytic performance of Ni3GeTe2 has not been reported. Single-layered FGT was obtained through exfoliation, showing superior catalytic activity in alkaline media. FGT achieved the best performance in OER, consistent with theoretical predictions.

FLATCHEM (2022)

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Article Multidisciplinary Sciences

Breaking through the Mermin-Wagner limit in 2D van der Waals magnets

Sarah Jenkins et al.

Summary: This study demonstrates that magnetic ordering can be stabilized at finite temperatures in finite-size 2D van der Waals magnets with short-range interactions, independent of magnetic anisotropy and lattice symmetry.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Physical

Boosting charge transfers in cadmium sulfide nanorods with a few layered Ni-doped MoS2 nanosheets for enhanced photocatalytic hydrogen evolution

D. Praveen Kumar et al.

Summary: This article introduces a method of improving the activity of MoS2 by transition metal (Ni) doping and exfoliation, enhancing its performance in hydrogen production photocatalytic reactions. The results of the study show that the modified MoS2/CdS composite has 70 times higher activity in hydrogen production compared to pure CdS, with stable hydrogen production ability. Metal doping and exfoliation improve the conductivity, surface area, and active sites of MoS2, while promoting catalytic kinetics and effective utilization of photogenerated charges.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Chemistry, Physical

Samarium hydroxide nanorolls anchored graphitic carbon nitride nanosheets: An active electrode material for supercapacitors

E. Vivek et al.

Summary: This study developed a novel nanocomposite material for supercapacitors, comprised of samarium hydroxide nanorolls attached to the surface of graphitic carbon nitride nanosheets. The unique morphology of the nanocomposite aids in creating active sites during redox reactions, resulting in high specific capacitance and cyclability. An asymmetric supercapacitor device constructed using this nanocomposite exhibited high energy density and power density. The investigation highlights the exciting morphology of the nanocomposites and their synergetic reaction, providing insights for the nanoengineering of active materials in supercapacitor applications.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Chemistry, Physical

Fe-MOFs derived porous Fe4N@carbon composites with excellent broadband electromagnetic wave absorption properties

Xuechen Liang et al.

Summary: Designing components and optimizing structure is an effective strategy to enhance the electromagnetic wave absorption of materials. This study successfully fabricated Fe-metal-organic framework derived iron nitride and carbon-based composites using a two-step method, combining the porous structure of metal-organic frameworks with the excellent electromagnetic properties of Fe4N. The formation of the Fe4N phase and the porous structure optimize impedance matching, significantly enhancing the electromagnetic wave absorption capacity of the composite.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Chemistry, Physical

Tunable spin injection and detection across a van der Waals interface

Keun-Hong Min et al.

Summary: The authors investigate the tunnelling magnetoresistance in Fe3GeTe2/hBN(WSe2)/Fe3GeTe2 magnetic tunnel junctions and report strong variations including polarization reversals with bias. Using van der Waals heterostructures with two-dimensional magnets, they demonstrate electrically tunable spin injection and detection, as well as modulated and reversed net spin polarization of the injected carriers, leading to changes in tunnelling magnetoresistance. The authors attribute the spin polarization reversals to contributions from high-energy localized spin states in the metallic ferromagnet, which is inaccessible in conventional magnetic junctions.

NATURE MATERIALS (2022)

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Article Chemistry, Physical

Deterministic switching of a perpendicularly polarized magnet using unconventional spin-orbit torques in WTe2

I-Hsuan Kao et al.

Summary: This paper demonstrates the experimental realization of field-free deterministic magnetic switching using the out-of-plane antidamping spin-orbit torque in the quantum material WTe2, and confirms this phenomenon through numerical simulations. This is of great importance for next-generation spintronic applications.

NATURE MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Single-atom lanthanum on 2D N-doped graphene oxide as a novel bifunctional electrocatalyst for rechargeable zinc-air battery

Z. Yang et al.

Summary: In this study, a rare-earth lanthanum (La) was introduced into N-doped graphene oxide (NGO) to form the single-atom 2D La@NGO, which exhibited excellent oxygen reduction reaction performances and methanol tolerance. The 7%La@NGO showed the best performance among the La@NGO series, surpassing the commercial Pt/C electrocatalyst, and also exhibited good bifunctional electrocatalytic behaviors. The rechargeable zinc-air battery assembled with 7%La@NGO demonstrated high power density, large specific capacity, high rechargeable efficiency, and excellent cycling stability.

MATERIALS TODAY CHEMISTRY (2022)

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Article Chemistry, Physical

??????????????Redox regulation of photocatalytic nitrogen reduction reaction by gadolinium doping in two-dimensional bismuth molybdate nanosheets

Hongda Li et al.

Summary: In this study, a novel Gd-doped 2D Bi2MoO6 nanosheet photocatalyst was designed and prepared, which showed improved nitrogen reduction performance by increasing reaction sites and promoting the separation and transfer of photogenerated carriers. This work proves that the lanthanide ion Gd3+ can be used to regulate the nitrogen reduction reaction and enhance its performance.

APPLIED SURFACE SCIENCE (2022)

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Review Materials Science, Multidisciplinary

A review on two-dimensional (2D) magnetic materials and their potential applications in spintronics and spin-caloritronic

Ehsan Elahi et al.

Summary: This review article summarizes recent progress in the research of van der Waals 2D ferromagnetic materials, including intrinsic magnetism, interlayer coupling effect, and device structures for spintronics. The effects of Anomalous Hall Effect, Anomalous Nernst Effect, and Spin Seebeck Effect on spin transport are described, as well as the challenges, applications, and perspectives of 2D ferromagnetic materials.

COMPUTATIONAL MATERIALS SCIENCE (2022)

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Article Materials Science, Multidisciplinary

Two-dimensional NiO nanosheets for efficient Congo red adsorption removal

Giovana M. Galvani et al.

Summary: In this study, NiO nanosheets with excellent adsorption performance were successfully synthesized by adjusting the synthesis parameters. The nanosheets showed a high adsorption capacity for Congo red dye, with the best performance achieved at a calcination temperature of 300℃.

MATERIALS CHEMISTRY AND PHYSICS (2022)

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Article Chemistry, Analytical

Graphene frameworks-confined synthesis of 2D-layered NiCoP for the electrochemical sensing of H2O2 at lower overpotential

Yanyan Zhu et al.

Summary: A highly efficient and durable 2D-layered nickel cobalt phosphide nanosheet, confined by 3D graphene frameworks, exhibits remarkable electroactivity towards hydrogen peroxide and has broad prospects in the field of electrochemistry, especially in biosensing applications.

MICROCHIMICA ACTA (2022)

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Article Multidisciplinary Sciences

Above-room-temperature strong intrinsic ferromagnetism in 2D van der Waals Fe3GaTe2 with large perpendicular magnetic anisotropy

Gaojie Zhang et al.

Summary: We report a two-dimensional intrinsic ferromagnetic crystal Fe3GaTe2 with strong ferromagnetism above room temperature and large perpendicular magnetic anisotropy. This crystal exhibits record-high Curie temperature, high saturation magnetic moment, large PMA energy density, and large anomalous Hall angle at room temperature. Room-temperature anomalous Hall devices and direct magnetic domains imaging based on Fe3GaTe2 nanosheet have been realized.

NATURE COMMUNICATIONS (2022)

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Article Nanoscience & Nanotechnology

Spin filtering effect in all-van der Waals heterostructures with WSe2 barriers

Yuanhui Zheng et al.

Summary: Utilizing van der Waals heterostructures with WSe2 barriers has demonstrated the spin-filtering effect, allowing for manipulation of magnetoresistance through changing the thickness of WSe2. A spin-filtering model based on Delta-symmetry electrons tunneling explains the transition from negative to positive MR signal. These findings highlight the potential of TMDC materials in controlling spin currents in 2D spintronic devices.

NPJ 2D MATERIALS AND APPLICATIONS (2022)

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Review Chemistry, Multidisciplinary

Application of 2D Materials for Adsorptive Removal of Air Pollutants

Jun Tae Kim et al.

Summary: Air pollution is a major global safety issue, and 2D materials with their unique properties and advantages have the potential to be used as adsorbent materials for environmental decontamination. Graphene oxide and reduced graphene oxide have attracted attention due to their low cost synthesis and high performance, and different material designs have been proposed to enhance their filtration capabilities.

ACS NANO (2022)

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Article Chemistry, Physical

Efficient photocatalytic CO2 conversion over 2D/2D Ni-doped CsPbBr3/Bi3O4Br Z-scheme heterojunction: Critical role of Ni doping, boosted charge separation and mechanism study

Xiaotian Wang et al.

Summary: In this study, a novel ultrathin Ni-doped CsPbBr3/Bi3O4Br Z-scheme heterostructure was constructed, which showed enhanced CO2 adsorption and activation ability. The synergistic effect between doping and heterostructure significantly improved the efficiency of photocatalytic CO2 reduction.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Physics, Multidisciplinary

Large Room-Temperature Magnetoresistance in van der Waals Ferromagnet/Semiconductor Junctions

Wenkai Zhu et al.

Summary: A large tunnel magnetoresistance (TMR) has been achieved at room temperature in magnetic tunnel junctions (MTJs) based on two-dimensional van der Waals (vdW) heterostructures, which opens up new possibilities for low power consumption and miniaturization of spintronic devices.

CHINESE PHYSICS LETTERS (2022)

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Article Chemistry, Physical

Designing In Situ Grown Ternary Oxide/2D Ni-BDC MOF Nanocomposites on Nickel Foam as Efficient Electrocatalysts for Electrochemical Water Splitting

Ebrahim Sadeghi et al.

Summary: In this study, a series of nanocomposites based on two-dimensional metal-organic frameworks were developed on nickel foam using a facile and scalable method, for the purpose of overall water splitting. The researchers found that different types of nanocomposites exhibited distinct catalytic activities for the hydrogen and oxygen evolution reactions, leading to improved efficiency of overall water splitting.

ACS MATERIALS AU (2022)

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Article Chemistry, Physical

Perspective Boosting electrocatalytic water splitting by magnetic fields

Xiaoning Li et al.

Summary: This article comprehensively discusses the various effects of magnetic fields on the oxygen evolution reaction, highlighting the importance of the type/setup of the magnetic field and the magnetism of electrocatalysts for its real effectiveness.

CHEM CATALYSIS (2022)

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Article Engineering, Electrical & Electronic

Gadolinium Halide Monolayers: A Fertile Family of Two-Dimensional 4f Magnets

Haipeng You et al.

Summary: Two-dimensional (2D) magnets have great potentials for next-generation information devices. This mini-review introduces recent progress in 2D Gd halides from a theoretical aspect. It highlights the key roles of Gd's 4f and 5d orbitals in these materials.

ACS APPLIED ELECTRONIC MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Synthesis of porphyrin-based 2D ytterbium metal organic frameworks for efficient photodynamic therapy

Xiang Zheng et al.

Summary: In this study, 2D Yb-TCPP MOFs with a size of around 200 nm were synthesized using a wet chemical method. These MOFs exhibited high efficiency in generating singlet oxygen species (O-1(2)) and low cytotoxicity, showing promising potential as anticancer agents in vitro.

RSC ADVANCES (2022)

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Review Chemistry, Inorganic & Nuclear

Two-dimensional materials for electrocatalysis and energy storage applications

Tingting Li et al.

Summary: This paper discusses in detail the use of 2D materials beyond graphene in electrocatalysis and energy storage. The properties related to the electronic and structural features of these materials are explored and recent research results are analyzed. The paper also highlights the potential and future challenges of these materials in the fields of energy conversion and storage.

INORGANIC CHEMISTRY FRONTIERS (2022)

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Article Nanoscience & Nanotechnology

Recent advances in graphene and other 2D materials

Pablo Ares et al.

Summary: The isolation and study of graphene as the first two-dimensional material has opened up new possibilities in the field of condensed matter physics and materials. Its stable and outstanding properties have led to the exploration of a whole new family of materials known as two-dimensional materials or 2D materials. The combination of 2D crystals allows the creation of composite materials with unique functionalities, enabling the study of new challenges in fundamental physics and the development of novel applications.

NANO MATERIALS SCIENCE (2022)

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Article Chemistry, Multidisciplinary

A cobalt-doped WS2/WO3 nanocomposite electrocatalyst for the hydrogen evolution reaction in acidic and alkaline media

Sunil R. Kadam et al.

Summary: The development of earth-abundant and green electrocatalysts for efficient hydrogen evolution is an important research field. In this study, WS2/WO3 hybrid catalysts were synthesized and it was found that the 5% Co-WS2/WO3 composite showed the most promising electrocatalytic activity among the doped catalysts.

NEW JOURNAL OF CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

2D magnetic phases of Eu on Ge(110)

Dmitry Averyanov et al.

Summary: 2D magnetic materials are at the forefront of magnetism research, exhibiting unconventional phases and properties controlled by external stimuli. This study reports 2D magnetic phases of Eu on the Ge(110) surface, with different surface densities of Eu atoms. The phases exhibit in-plane magnetic ordering at low temperatures, with a strong dependence of the effective magnetic transition temperature on weak magnetic fields. The study suggests that a variety of substrates can host submonolayer 2D magnetic phases.

NANOSCALE (2022)

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Article Chemistry, Inorganic & Nuclear

Tandem ZnCo-porphyrin metal-organic frameworks for enhanced photoreduction of CO2

Xuyang Chen et al.

Summary: A bimetallic ZnCo-porphyrin metal-organic framework (ZnCo-BMOF) nanosheet was developed for efficient photoreduction of CO2 to CO. The ZnCo-BMOF nanosheet combines photosensitizers (Zn porphyrin) and catalysts (Co porphyrin) to enable fast electron transfer and effective catalytic activity.

INORGANIC CHEMISTRY FRONTIERS (2022)

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Article Chemistry, Multidisciplinary

Two-dimensional cobalt telluride as a piezo-tribogenerator

Solomon Demiss Negedu et al.

Summary: This study successfully generates electricity using waste heat through the piezoelectric and triboelectric properties of 2D cobalt telluride. The 2D piezo-tribogenerator shows excellent characteristics with high voltage, fast response time, and high responsivity. Density functional theory is used to validate the experimental results.

NANOSCALE (2022)

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Review Pharmacology & Pharmacy

Two-dimensional (2D) materials beyond graphene in cancer drug delivery, photothermal and photodynamic therapy, recent advances and challenges ahead: A review

Mohammad Jafar Molaei

Summary: Various 2D materials with superior properties have been developed for biomedical and cancer therapy applications, such as TMDs, BN, MXenes, LDHs, and BP nanosheets. These materials are used for drug delivery, bioimaging, photothermal therapy, and other applications in cancer treatment.

JOURNAL OF DRUG DELIVERY SCIENCE AND TECHNOLOGY (2021)

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Article Chemistry, Physical

Ni-Fe-Co based mixed metal/metal-oxides nanoparticles encapsulated in ultrathin carbon nanosheets: A bifunctional electrocatalyst for overall water splitting

Waleed Yaseen et al.

Summary: This study presents a highly efficient Ni-Fe-Co-based mixed metal/metal-oxides nanoparticles encapsulated in ultrathin carbon nanosheets (NFC@CNSs) catalyst, which exhibits remarkable activity in 1.0 M KOH with superior specific surface area and microstructure. In an alkaline media, the catalyst can achieve a high current density of 10 mA cm(-2) with a low applied voltage, demonstrating excellent catalytic efficiency.

SURFACES AND INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Ferromagnetism in 2D Vanadium Diselenide

Xiong Wang et al.

Summary: This study reports a 2D ferromagnetic semiconductor material, 2H-phase vanadium diselenide (VSe2), showing enhanced magnetic ordering due to structural anisotropy at the 2D limit. This material only exhibits ferromagnetism in its 2D form, making it a promising candidate for miniature spintronics and information storage devices.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Large Tunneling Magnetoresistance in van der Waals Ferromagnet/Semiconductor Heterojunctions

Wenkai Zhu et al.

Summary: This study reports all-2D van der Waals vertical spin-valve devices with two distinct transport behaviors and reveals the critical role of pinholes in the magnetoresistance of such devices.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Defect Engineering of Two-Dimensional Transition-Metal Dichalcogenides: Applications, Challenges, and Opportunities

Qijie Liang et al.

Summary: This review article highlights the role of chalcogen atomic defects in engineering 2D TMDs, particularly focusing on device performance improvements. Various approaches for creating chalcogen atomic defects and their effects on optical, electrical, and magnetic properties are systematically overviewed. The dynamic evolution and repair of chalcogen atomic defects are also discussed, along with perspectives on challenges and opportunities in the field.

ACS NANO (2021)

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Article Electrochemistry

Double metal-organic frameworks derived Fe-Co-Ni phosphides nanosheets as high-performance electrocatalyst for alkaline electrochemical water splitting

Xiaolong Zhang et al.

Summary: An efficient bi-functional electrocatalyst FeCoNiP@C/NF has been developed for electrochemical overall water-splitting. The catalyst exhibited excellent OER, HER, and overall water-splitting abilities in 1.0 M KOH to reach a current density of 100 mA/cm(2).

ELECTROCHIMICA ACTA (2021)

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Article Engineering, Environmental

2D bimetallic RuNi alloy Co-catalysts remarkably enhanced the photocatalytic H2 evolution performance of g-C3N4 nanosheets

Xin Han et al.

Summary: The bimetallic RuNi alloys with a 2D structure can serve as a co-catalyst for g-C3N4 nanosheets, improving photocatalytic hydrogen production performance.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Multidisciplinary

2D organic-α-Co(OH)2 material and derived Co/C composites with bifunctions of anti-corrosion and microwave absorption

Jianwen Ge et al.

Summary: This article successfully fabricated alpha-Co(OH)(2) lamellae as the precursor of Co/C composites and investigated the microstructures and absorption properties. The in situ polymerization and subsequent calcination process suggested that decorated carbon plays a crucial role in tuning the microstructure, leading to high absorption performance and corrosion resistance for the samples. Additionally, the ring-shaped Co/C composites generated at relatively low temperature exhibited outstanding microwave absorption characteristics, providing an opportunity for the design of absorbent materials with commercial value.

COMPOSITES PART B-ENGINEERING (2021)

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Review Chemistry, Analytical

Two-dimensional inorganic nanosheets: production and utility in the development of novel electrochemical (bio)sensors and gas-sensing applications

Alexandros Ch. Lazanas et al.

Summary: This review focuses on the application of inorganic layered materials in developing novel electrochemical sensors, analytical devices, and gas-phase sensing applications using two-dimensional nanosheets, discussing various families of ILMs and production methods while evaluating their utility in contemporary analysis and potential for further improvement.

MICROCHIMICA ACTA (2021)

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Article Nanoscience & Nanotechnology

The effects of substitutional Fe-doping on magnetism in MoS2 and WS2 monolayers

Kyungnam Kang et al.

Summary: Substitutional Fe-doping of MoS2 and WS2 monolayers induces different magnetic properties, with Fe dopants in WS2 assuming deep-level trap states compared to shallow states in Fe:MoS2. Unlike Fe:MoS2, Fe:WS2 does not show a magnetic phase transition to ferromagnetism, as confirmed by density functional theory calculations.

NANOTECHNOLOGY (2021)

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Article Chemistry, Physical

Two-dimensional ferromagnetism in Eu-intercalated few-layer graphene

Ivan S. Sokolov et al.

Summary: 2D magnets show potential for unconventional quantum phases, exploration of fundamental physics of magnetism, and ultra-compact devices. By encapsulating a monolayer Eu lattice between graphene monolayers, a chemically inert van der Waals 2D ferromagnet is formed. The results expand the family of 2D magnets and establish a versatile platform for synthesis of new members by metal intercalation.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Materials Science, Multidisciplinary

Magnetic properties of devicelike cobalt/2D materials interfaces

Jacko Rastikian et al.

Summary: The magnetism of a cobalt ultrathin film deposited on different two-dimensional (2D) materials was studied using the Brillouin light scattering technique. The results showed enhanced perpendicular magnetic anisotropy in the Co/2D systems compared to the reference layer (Co/SiO2), along with an increase in magnetic damping and a small Dzyaloshinskii-Moriya interaction in the samples. These findings were discussed in comparison with ab initio calculations and recent literature.

PHYSICAL REVIEW MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A Multifunctional Dysprosium-Carboxylato 2D Metall-Organic Framework

Jonay Gonzalez et al.

Summary: This study reported the microwave assisted synthesis of a bidimensional (2D) metal–organic framework (MOF). The material exhibits single-ion magnet behavior and can be exfoliated into stable nanosheets by sonication.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Analytical

An ultrathin 2D Yb(III) metal-organic frameworks with strong electrochemiluminescence as a on-off-on platform for detection of picric acid and berberine chloride form

Xiao Yan Wang et al.

Summary: This study explores the strong electrochemiluminescence behavior of ultrathin two-dimensional metal-organic frameworks, showing that thinner 2D Yb-MOFs exhibit stronger ECL signals. The ECL intensity is enhanced by increasing the specific surface area and fluorescence quantum yield. The ultrathin 2D Yb-MOF-1 is selected as a new ECL emitter for picric acid and berberine chloride form detection, demonstrating promising analytical performance.

TALANTA (2021)

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Article Multidisciplinary Sciences

Current-induced switching of proximity-induced ferromagnetic surface states in a topological insulator

Masataka Mogi et al.

Summary: Efficient current-induced switching of surface ferromagnetism in hetero-bilayers of topological insulator (Bi1-xSbx)(2)Te-3 and ferromagnetic insulator Cr2Ge2Te6 demonstrates the potential for electrical control of dissipationless topological-current circuits, showing efficient charge-to-spin current conversion and large anomalous Hall effect.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Strong intrinsic room-temperature ferromagnetism in freestanding non-van der Waals ultrathin 2D crystals

Hao Wu et al.

Summary: A scalable method has been developed to prepare freestanding non-van der Waals ultrathin 2D crystals, leading to the discovery of strong, ambient-air-robust room-temperature ferromagnetism in freestanding non-van der Waals 2D CrTe crystals. These freestanding 2D CrTe crystals show comparable or even better ferromagnetic properties than commonly used Fe, Co, Ni, and BaFe12O19, making them promising as new platforms for intrinsically ferromagnetic 2D crystals at room temperature and integrated 2D devices.

NATURE COMMUNICATIONS (2021)

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Article Engineering, Environmental

Erbium-doped tungsten selenide nanosheets with near-infrared II emission and photothermal conversion

Youqiang Huang et al.

Summary: By doping Er ions, the luminescence of 2D nanosheets is extended to the NIR II window, with a high photothermal conversion efficiency. This suggests that the prepared nanosheets may be promising for dual-functionality in bioimaging and photothermal therapy.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Excellent electromagnetic wave absorption of Co/Fe2O3 composites by additional activated carbon for tuning the optical and the magnetic properties

Dahlang Tahir et al.

Summary: The study successfully achieved a composite Co/Fe2O3/AC material with excellent electromagnetic wave absorption performance, attributed to conductivity loss, multiple reflections, electron hoping, and scattering caused by the unique arrangement of atoms. This material shows great potential for the development of absorbing materials for electromagnetic waves.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Review Engineering, Environmental

Magnetic field assisted adsorption of pollutants from an aqueous solution: A review

Jianran Ren et al.

Summary: The magnetic field serves as a special substance that objectively exists and transmits magnetic force between objects, providing enhancement for pollutant adsorption. By adjusting the type and parameters of the magnetic field, adsorption efficiency and selectivity can be improved. Currently, there is a research gap in the area of pollutant enhanced-adsorption technique using magnetic fields.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Physics, Applied

Magnetic Properties and Microstructures of Fe-Doped (Ti1-xFex)3AlC2 MAX Phase and Their MXene Derivatives

Shengyu Sun et al.

Summary: The effects of Fe substitution for Ti on the (Ti1-xFex)(3)AlC2 MAX phases result in structural expansion, contraction, and a change in ferromagnetic state. Exfoliation leads to paramagnetic two-dimensional MXenes, with broken exchange coupling along c-axis. The (Ti0.975Fe0.025)(3)C2T delta free-standing paper exhibits excellent electromagnetic interference properties with a wide frequency range.

JOURNAL OF SUPERCONDUCTIVITY AND NOVEL MAGNETISM (2021)

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Article Chemistry, Physical

Spin-induced linear polarization of photoluminescence in antiferromagnetic van der Waals crystals

Xingzhi Wang et al.

Summary: This study successfully demonstrates the optical detection of Neel vector orientation in the van der Waals antiferromagnet NiPS3, and reveals a strong correlation between photoluminescence polarization and spin orientation in the crystal. By applying an in-plane magnetic field, manipulation of the photoluminescence polarization is achieved.

NATURE MATERIALS (2021)

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Article Materials Science, Multidisciplinary

Room-temperature ferromagnetism enhancement in Fe-doped VSe2 nanosheets synthesized by a chemical method

Li-Yan Hu et al.

Summary: Two-dimensional VSe2 and V1-xFexSe2 nanosheets were synthesized using a high-temperature organic solution method, with tunable thickness and room-temperature ferromagnetism. The enhancement of magnetization in V0.8Fe0.2Se2 nanosheets is attributed to the coupling interaction of 3d orbits between V and Fe atoms, showing 5 times higher coercivity and magnetization compared to pure VSe2 nanosheets.

RARE METALS (2021)

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Article Multidisciplinary Sciences

Embedding atomic cobalt into graphene lattices to activate room-temperature ferromagnetism

Wei Hu et al.

Summary: Embedding Cobalt atoms in graphene lattice can achieve robust room-temperature ferromagnetism, facilitated by the formation of square-planar Co-N-4 moieties and local magnetic moments provided by atomically dispersed Co atoms.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Physical

Atomically Thin Nanosheets Confined in 2D Heterostructures: Metal-Ion Batteries Prospective

Abbas Khan et al.

Summary: This article discusses the significance and characteristics of graphene-based and beyond-graphene 2D heterostructures as electrode materials for various ion batteries, along with the challenges and future research directions in developing these materials.

ADVANCED ENERGY MATERIALS (2021)

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Article Physics, Applied

Exchange bias and spin-orbit torque in the Fe3GeTe2-based heterostructures prepared by vacuum exfoliation approach

Yu Zhang et al.

Summary: This study demonstrates the importance of high-quality interfaces in achieving exchange bias and SOT effect in 2D van der Waals materials-based magnetic heterostructures. The results show significant out-of-plane exchange bias and improved SOT-driven switching performance, paving the way for the implementation of 2D van der Waals materials in spintronic devices.

APPLIED PHYSICS LETTERS (2021)

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Article Chemistry, Inorganic & Nuclear

Iron Phthalocyanine/Two-Dimensional Metal-Organic Framework Composite Nanosheets for Enhanced Alkaline Hydrogen Evolution

Xiaoyin Zhang et al.

Summary: A study on the development of two-dimensional metal-organic framework (2D MOF) composite nanosheets for enhanced performance in alkaline hydrogen evolution reaction (HER) was reported. The nanosheets, consisting of ultrathin Ni-MOF with uniformly anchored FePc molecules, exhibited significantly increased current density, improved activity, and enhanced durability. The resulting nanosheet catalyst FePc@Ni-MOF demonstrated low overpotential and satisfactory long-term stability, outperforming pristine FePc, Ni-MOF, and a counterpart FePc@bulk-MOF.

INORGANIC CHEMISTRY (2021)

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Article Chemistry, Analytical

Building CoP/Co-MOF heterostructure in 2D nanosheets for improving electrocatalytic hydrogen evolution over a wide pH range

Qiling Li et al.

Summary: This study proposed a facile method to fabricate a self-supported electrode with excellent hydrogen evolution reaction (HER) activities. The optimized 2D CoP/Co-MOF exhibits outstanding HER performance over a wide pH range, with fast charge-transfer rate and abundant exposed active sites. This work provides an effective strategy to design pH-universal HER activity of MOF-based electrocatalysts.

JOURNAL OF ELECTROANALYTICAL CHEMISTRY (2021)

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Article Materials Science, Multidisciplinary

Magnetism and microwave absorption properties of two-dimensional layered ferromagnetic metal Fe3GeTe2

Ying Ji et al.

Summary: Two-dimensional van der Waals ferromagnetic material Fe3GeTe2 (FGT) with high Curie temperature shows potential for overcoming microwave pollution and radiation. FGT nanosheets exhibit low reflection loss in microwave absorption, which is further improved by introducing graphene nanosheets (GNS). FGT@GNS 1-2 composites demonstrate excellent microwave absorption performance, meeting the requirements for strong absorption and thin thickness of microwave absorption materials.

JOURNAL OF MATERIALS SCIENCE (2021)

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Review Green & Sustainable Science & Technology

Hydrogen energy systems: A critical review of technologies, applications, trends and challenges

Meiling Yue et al.

Summary: This paper reviews the current progress and outlook of hydrogen technologies and their application in power systems, highlighting the importance of hydrogen in clean energy and pointing out the technical and economic challenges that need to be addressed.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2021)

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Article Chemistry, Multidisciplinary

CO2-Induced 2D Ni-BDC Metal-Organic Frameworks with Enhanced Photocatalytic CO2 Reduction Activity

Hongwei Chang et al.

Summary: The design and fabrication of 2D metal-organic framework nanosheets with high activity for CO2 reduction is a critical issue. CO2 molecules play a key role in helping break interlayer hydrogen bonds and exposing active planes, leading to high efficiency in CO2-to-CO conversion. This strategy based on strong interaction between metal centers and reactive molecules provides a novel model for obtaining high-quality and active 2D MOFs.

ADVANCED MATERIALS INTERFACES (2021)

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Review Physics, Applied

Recent progress on 2D magnets: Fundamental mechanism, structural design and modification

Xue Jiang et al.

Summary: This review summarizes the recent progress on 2D magnets, focusing on magnetic exchange interaction, databases, and modification strategies. It presents various types of 2D magnetic materials and their interaction mechanisms.

APPLIED PHYSICS REVIEWS (2021)

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Article Physics, Multidisciplinary

Magnetic and f-electron effects in LaNiO2 and NdNiO2 nickelates with cuprate-like 3dx2-y2 band

Ruiqi Zhang et al.

Summary: By comparing the electronic structures of LaNiO2 and NdNiO2, the role of Nd 4f electrons in shaping the ground state of NdNiO2 is revealed, showing strong similarities between the two compounds except for the effects of the 4f electrons. The hybridization between Nd 4f and Ni 3d orbitals significantly modifies the Fermi surfaces of different magnetic states, and the competition between magnetically ordered phases mainly depends on the gaps in the Ni 3d(x2-y2) band. The study also found similarities in the on-site Hubbard U values between nickelates and cuprates, but the value of the Hund's coupling J(H) is sensitive to the Nd magnetic moment. Additionally, NdNiO2 exhibits 3D magnetism with competing antiferromagnetic and (interlayer) ferromagnetic exchange, contributing to the lower Tc compared to cuprates.

COMMUNICATIONS PHYSICS (2021)

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Article Chemistry, Physical

Prediction of 2D ferromagnetism and monovalent europium ions in EuBr/graphene heterojunctions

Haoyi Tan et al.

Summary: The study predicted that 2D ferromagnetic EuBr/graphene heterojunctions exhibit metallicity and intrinsic ferromagnetism, with Eu playing a key role. Monte Carlo simulations can estimate the Curie temperature, which can be further modulated by external strains and charge-carrier doping.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Article Materials Science, Multidisciplinary

Critical behavior in the van derWaals itinerant ferromagnet Fe4GeTe2

Suchanda Mondal et al.

Summary: The critical phenomenon of magnetic phase transition in the van der Waals itinerant ferromagnet Fe4GeTe2 was investigated, revealing specific critical exponents during the continuous paramagnetic to ferromagnetic transition. The analysis suggests a quasi-two-dimensional itinerant magnetism in Fe4GeTe2 single crystal, with a certain magnetic anisotropy present.

PHYSICAL REVIEW B (2021)

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Proceedings Paper Materials Science, Multidisciplinary

Ferromagnetism in graphene oxide

Apurva Sinha et al.

Summary: The presence of d and/or f electrons is essential for the formation of localized magnetic moments in material systems, and the exchange interaction between these moments is crucial for observing an ordered magnetic ground state. While ferromagnetism has been reported in carbon-based materials in the past, it is impossible to generate localized magnetic moments in systems with exclusively pure sp(3), sp(2), or sp carbons. However, the presence of mixed hybridization like sp(2)-sp(3) character can favor the formation of such moments.

MATERIALS TODAY-PROCEEDINGS (2021)

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Review Materials Science, Multidisciplinary

Transition-Metal (Fe, Co, and Ni)-Based Nanofiber Electrocatalysts for Water Splitting

Xuejie Cao et al.

Summary: Electrochemical water splitting is a promising technology for sustainable hydrogen production that relies on efficient electrocatalysts like transition-metal-based materials. Fibrous electrocatalysts, with their unique structure and advantages, have shown great potential in accelerating hydrogen and oxygen evolution reactions. Iron, cobalt, and nickel-based nanofiber electrocatalysts are particularly promising for future applications in water splitting.

ADVANCED FIBER MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Femtosecond laser-induced spin dynamics in single-layer graphene/CoFeB thin films

Surya Narayan Panda et al.

Summary: This study investigates the magnetization dynamics in graphene/ferromagnet hybrid heterostructures and reveals an inverse relationship between ultrafast demagnetization time and Gilbert damping parameter, induced by interfacial spin accumulation and pure spin-current transport. The findings can contribute to the understanding of magnetic damping and aid in the design of graphene-based ultrahigh-speed spintronic devices.

NANOSCALE (2021)

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Review Chemistry, Multidisciplinary

Recent progress in water-splitting electrocatalysis mediated by 2D noble metal materials

Lin Tian et al.

Summary: Two-dimensional nanostructures have enabled noble-metal-based nanomaterials to be promising electrocatalysts towards overall water splitting, with inherent structural advantages and beneficial electronic and strain effects. The review highlights the recent progress in advanced electrocatalysts based on 2D noble-metal-based nanomaterials and discusses water-splitting mechanisms, engineering strategies, challenges, and structural merits of 2D nanostructures. Additionally, representative water-splitting electrocatalysts are discussed to showcase the superiorities of 2D noble-metal-based nanomaterials for electrochemical water splitting, while also addressing underlying challenges and future opportunities.

NANOSCALE (2021)

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Review Materials Science, Multidisciplinary

Recent developments on 2D magnetic materials: challenges and opportunities

Shalini Kumari et al.

Summary: Two-dimensional magnetic materials show strong magnetization at ultrathin limits above room temperature, promising for miniaturization of future energy efficient nanoelectronic devices beyond Moore's law. These materials have various promising applications, including spintronics devices.

EMERGENT MATERIALS (2021)

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Review Energy & Fuels

2D materials and their heterostructures for photocatalytic water splitting and conversion of CO2 to value chemicals and fuels

G. Shiva Shanker et al.

Summary: The rapid increase in global energy consumption from conventional polluting fuels has put tremendous pressure on the environment, highlighting the urgent need to transition to environment-friendly, renewable energy sources. Producing hydrogen energy from water using sunlight appears to be a promising approach, while 2D materials and heterostructures are attracting attention for their potential in efficient hydrogen production and CO2 conversion. Efforts are being made to design high-performance photocatalysts based on emergent functional materials to address the challenges in advancing this energy technology.

JOURNAL OF PHYSICS-ENERGY (2021)

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Review Chemistry, Multidisciplinary

Two-Dimensional Magnets: Forgotten History and Recent Progress towards Spintronic Applications

David L. Cortie et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Physical

Electronic structure tailoring of BiOBr (010) nanosheets by cobalt doping for enhanced visible-light photocatalytic activity

Luhua Shao et al.

APPLIED SURFACE SCIENCE (2020)

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Article Materials Science, Multidisciplinary

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Density functional theory prediction on magnetism in Gd-doped monolayer MoS2

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SOLID STATE COMMUNICATIONS (2015)

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Defects induced ferromagnetism in plasma-enabled graphene nanopetals

Z. J. Yue et al.

APPLIED PHYSICS LETTERS (2014)

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Structural! spectroscopic analyses and H2/O2/CO responses of thulium(III) oxide nanosquare sheets

Sung Woo Lee et al.

APPLIED SURFACE SCIENCE (2014)

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Magnetic entrapment for fast and sensitive determination of metronidazole with a novel magnet-controlled glassy carbon electrode

Guangming Yang et al.

ELECTROCHIMICA ACTA (2014)

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Optical and electrical properties of MoS2 and Fe-doped MoS2

Song Yu Wang et al.

JAPANESE JOURNAL OF APPLIED PHYSICS (2014)

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Facile synthesis of hierarchical Fe4(P2O7)3 for removal of U(VI)

Xia Liu et al.

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High densities of magnetic nanoparticles supported on graphene fabricated by atomic layer deposition and their use as efficient synergistic microwave absorbers

Guizhen Wang et al.

NANO RESEARCH (2014)

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Obtaining High Localized Spin Magnetic Moments by Fluorination of Reduced Graphene Oxide

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ACS NANO (2013)

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Review Chemistry, Multidisciplinary

Alternative Plasmonic Materials: Beyond Gold and Silver

Gururaj V. Naik et al.

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Photocatalytic reduction of CO2 for fuel production: Possibilities and challenges

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Microwave absorption response of nickel/graphene nanocomposites prepared by electrodeposition

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JOURNAL OF MATERIALS SCIENCE (2013)

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Electrical Transport Measured in Atomic Carbon Chains

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NANO LETTERS (2013)

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Graphene-ferromagnet interfaces: hybridization, magnetization and charge transfer

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NANOSCALE (2013)

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Vertical graphene spin valve with Ohmic contacts

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NANOSCALE (2013)

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Prediction of two-dimensional diluted magnetic semiconductors: Doped monolayer MoS2 systems

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PHYSICAL REVIEW B (2013)

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Electrosynthesis of Iron, Cobalt, and Zinc Microcrystals and Magnetic Enhancement of the Oxygen Reduction Reaction

Lorena M. A. Monzon et al.

CHEMISTRY OF MATERIALS (2012)

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Metals on graphene: correlation between adatom adsorption behavior and growth morphology

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PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2012)

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Synthesis, structural determination and spectroscopic analysis of a novel 2D terbium coordination network with ethyleneglycol-bis-(2-aminoethylether)-N,N,N′,N′-tetraacetic acid

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SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY (2012)

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The surface science of graphene: Metal interfaces, CVD synthesis, nanoribbons, chemical modifications, and defects

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SURFACE SCIENCE REPORTS (2012)

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Perpendicular Magnetic Anisotropy of Full-Heusler Films in Pt/Co2FeAl/MgO Trilayers

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APPLIED PHYSICS EXPRESS (2011)

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Direct study of the f-electron configuration in lanthanide systems

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JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY (2011)

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2D materials: to graphene and beyond

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NANOSCALE (2011)

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Induced magnetism of carbon atoms at the graphene/Ni(111) interface

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APPLIED PHYSICS LETTERS (2010)

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Enhanced microwave performance of cobalt nanoflakes with strong shape anisotropy

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APPLIED PHYSICS LETTERS (2010)

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Nickel/carbon hybrid nanostructures as microwave absorbers

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MATERIALS LETTERS (2010)

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A perpendicular-anisotropy CoFeB-MgO magnetic tunnel junction

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NATURE MATERIALS (2010)

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Quantum anomalous Hall effect in graphene from Rashba and exchange effects

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PHYSICAL REVIEW B (2010)

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Limits on Intrinsic Magnetism in Graphene

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PHYSICAL REVIEW LETTERS (2010)

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Room-Temperature Ferromagnetism of Graphene

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Diamagnetism in disordered graphene

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PHYSICAL REVIEW B (2007)

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The rise of graphene

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NATURE MATERIALS (2007)

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Defect-induced magnetism in graphene

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PHYSICAL REVIEW B (2007)

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Ferromagnetism and superconductivity in carbon-based systems

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JOURNAL OF LOW TEMPERATURE PHYSICS (2007)

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Challenges for semiconductor spintronics

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NATURE PHYSICS (2007)

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Orbital ordering phenomena in d- and f-electron systems

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REPORTS ON PROGRESS IN PHYSICS (2006)

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Contact induced magnetism in carbon nanotubes

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JOURNAL OF PHYSICS-CONDENSED MATTER (2004)

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Direct observation of local ferromagnetism on carbon in C/Fe multilayers

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EUROPHYSICS LETTERS (2004)

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Metallic behavior of the Zintl phase EuGe2:: combined structural studies, property measurements, and electronic structure calculations

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Magnetic properties and diffusion of adatoms on a graphene sheet

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PHYSICAL REVIEW LETTERS (2003)

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Magnetism in photopolymerized fullerenes

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CARBON (2003)

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Ferromagnetism in oriented graphite samples -: art. no. 024429

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PHYSICAL REVIEW B (2002)

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Thickness-dependent Curie temperatures of ultrathin magnetic films: Effect of the range of spin-spin interactions

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PHYSICAL REVIEW LETTERS (2001)

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