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Article
Engineering, Environmental
Soyoung Park et al.
Summary: In this study, cobalt doped/ZnTiO3/Ti3C2Tx MXene material was synthesized and found to have excellent performance in the adsorption and photocatalytic degradation of tetracycline antibiotics. The material showed high adsorption capacity and degradation rate, suggesting its potential application in removing tetracycline antibiotics widely used in animal husbandry.
JOURNAL OF HAZARDOUS MATERIALS
(2023)
Article
Chemistry, Analytical
Fuqiang Guo et al.
Summary: In this study, Ti3C2Tx/CuO nanocomposites were successfully prepared through an environmentally friendly and simple hydrothermal method. The synthesized materials were characterized using various techniques, including XRD, SEM, TEM, XPS, FTIR, UV-vis, and BET. The results showed that Ti3C2Tx/CuO nanocomposites exhibited a mesoporous structure and a higher specific surface area compared to Ti3C2Tx, indicating the presence of more gas adsorption/diffusion regions. The introduction of CuO led to Ti3C2Tx having rich oxygen vacancies and adsorbed oxygen. The Ti3C2Tx/CuO sensor showed superior gas sensing performance, including a significantly higher response to 50 ppm NO2, ultra-fast response/recovery time, great reversibility, outstanding selectivity to NO2, and desirable long-term stability. The enhanced gas sensing performance can be attributed to the hybrid heterojunctions formed between CuO and Ti3C2Tx, which facilitate carrier migration and accelerate the redox reaction. The presence of more oxygen vacancies and adsorbed oxygen in Ti3C2Tx/CuO further enhances the gas sensing performance. These improved gas sensing performance indicators modified with CuO are expected to be advantageous for the development of Ti3C2Tx-based sensors for commercial NO2 detection in the future.
SENSORS AND ACTUATORS B-CHEMICAL
(2023)
Article
Chemistry, Physical
Siwei Liu et al.
Summary: In this work, a ZnO1-x/Ti3C2 composite with rich oxygen vacancies was prepared by a hydrothermal process and subsequent annealing in a hydrogen atmosphere, showing high responses to low concentrations of NO2 at room temperature. The excellent sensing properties of the ZnO1-x/Ti3C2 composite are attributed to the presence of abundant oxygen vacancies and the formation of a ZnO1-x/Ti3C2 Schottky barrier. The composite also demonstrates high selectivity to NO2 compared to other gases. This study provides new insights into enhancing the room-temperature gas sensitivity of MOS-containing composites by constructing oxygen vacancies and heterojunctions.
APPLIED SURFACE SCIENCE
(2023)
Article
Chemistry, Analytical
Yutong Han et al.
Summary: Transition metal carbides/nitrides (MXenes) and transition metal dichalcogenides (TMDs) have shown great potential in gas sensors due to their surface properties. In this study, SnS2 nanoflakes were integrated with Ti3C2Tx skeleton platforms for VOC detection. The SnS2/Ti3C2Tx sensor exhibited fast response/recovery times, excellent selectivity, and reliable long-term stability, making it a promising option for VOC detection at room temperature.
SENSORS AND ACTUATORS B-CHEMICAL
(2023)
Article
Chemistry, Physical
Jingyu Shi et al.
Summary: In this study, a facile synthesis method was used to prepare ZnO@Co3O4 single-shelled hollow cubes with porous surfaces. The resulting HCs exhibited excellent gas sensing performance and stability due to their larger surface area and catalytic effect.
APPLIED SURFACE SCIENCE
(2023)
Article
Engineering, Environmental
Yu Yao et al.
Summary: In this study, MnO2 with high catalytic activity was introduced onto MXene material, improving the sensitivity and selectivity of the gas sensor. The composite material exhibited a 10-20 times higher response to different volatile organic compounds compared to the pristine MXene-based sensor, and showed a unique and stable response to the lung cancer marker hexanal.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Nanoscience & Nanotechnology
Yanjie Wang et al.
Summary: In this study, mixed-dimensional heterostructures of two-dimensional (2D) black phosphorus (BP) nanosheet-templated zero-dimensional (0D) SnO2 quantum dots (QDs) (BP/SnO2) were prepared for trace H2S detection. The optimized BP/SnO2 sensors showed high response (233.8) and fast response/recovery speeds (16.4/9.5 s) towards 5 ppm H2S at a relatively low operation temperature. The sensors demonstrated excellent repeatability, long-term stability, selectivity, and favorable humidity tolerance.
ACS APPLIED NANO MATERIALS
(2023)
Article
Engineering, Environmental
Qikun Xu et al.
Summary: This study successfully achieved high selectivity and fast response detection of H2S using MXene sensors. A novel self-calibration strategy was introduced to eliminate the influence of humidity in gas detection, offering a viable solution for addressing real-world humidity effects on gas sensors.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Xue Bai et al.
Summary: In this study, a N-doped three-dimensional needle bridge connection core-shell structure material was synthesized, showing excellent NO2 sensing performance. The material possesses a unique porous and bridge connection core-shell structure with high specific surface area and abundant active sites, and the catalytic performance is promoted by N-doping, demonstrating good stability.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Yali Guo et al.
Summary: Nickel@MXene quantum dots (Ni@MQDs) were successfully prepared and showed outstanding catalytic performance for Cr (VI) reduction in the presence of formic acid. Density functional theory calculations revealed that Ni@MQDs exhibited an upshift of D-band center of active Ni atoms, leading to improved catalytic reaction kinetics. This work may pave the way for the design and synthesis of novel MQDs-based hybrid catalysts for wastewater treatment.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Chemistry, Analytical
G. Mathankumar et al.
Summary: Nanostructured transition metal oxides have gained much attention in gas sensing applications due to their superior size-dependent adsorption and catalytic properties. Pure and yttrium-doped WO3 nanoplates were prepared by one-step hydrothermal method and their gas sensing performance was studied. The Y-doped samples exhibited excellent selectivity towards NO2 and showed significantly enhanced gas sensitivity, response time, and recovery time compared to the pure sample. The enhancement in gas sensing performance has been explained by the gas sensing mechanism and work function measurement. Y-doped WO3 nanostructures provide a new pathway for improving the performance of transition metal oxide-based gas sensors.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Chemistry, Physical
Xiaonan Wu et al.
Summary: The study focuses on the development of high-performance chemiresistive gas sensors at room temperature by combining MXene with SMO. The SnO2-TiO2-Ti3C2Tx heterostructure sensor exhibits excellent sensitivity, selectivity, and stability for NO2 detection. The improved sensing performance is attributed to the synergic effects of three phases, which form functionalized surfaces and multiple-type heterojunctions, resulting in enhanced electrical transduction function.
APPLIED SURFACE SCIENCE
(2022)
Article
Engineering, Environmental
Xiang Li et al.
Summary: In this study, MoO3 microporous nanoflowers were synthesized and showed excellent gas sensing performance to H2S. This work provides a reference for the design of high-performance gas sensors based on metal oxides.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Kedhareswara Sairam Pasupuleti et al.
Summary: In this study, a high-performance langasite-based surface acoustic wave (SAW) gas sensor for nitrogen dioxide (NO2) at room temperature was developed. The sensor exhibited excellent selectivity, sensitivity, and response time, as well as stability in various relative humidity conditions. The integration of 2D materials with metal oxides shows promise for environmental protection.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Shuaishuai Man et al.
Summary: In this study, a highly conductive MXene (Ti3C2Tx) was fabricated for the first time using electrophoretic deposition (EPD) as an interlayer to prepare a novel PbO2 electrode. The Ti3C2Tx interlayer significantly improved the electrochemical performance of the EPD-2.0/PbO2 electrode, reducing the charge transfer resistance, increasing the number of active sites, and enhancing the generation ability of ·OH radicals. Experimental results showed that the EPD-2.0/PbO2 electrode exhibited promising potential for the electrochemical degradation of basic fuchsin (BF).
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Chemistry, Analytical
Xiaowei Ren et al.
Summary: In this study, an ultrahigh sensitive and selective NO2 gas sensor based on porous ZnO nanocubes derived from metal organic frameworks (MOFs) was reported. The fabricated gas sensor demonstrated excellent selectivity to NO2 over other gases, attributed to the unique structure after pyrolysis which provides more exposed active sites and connected pore channels.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Chemistry, Analytical
Jie Hu et al.
Summary: In this article, a novel flower-like WO3-In2O3 hollow heterostructure was successfully constructed and its gas sensing performance was systematically investigated. The results showed that the WO3-In2O3 structure achieved higher sensing performance compared to other sensing materials, attributed to the synergistic effect of its excellent structure and heterojunction configuration. This study provides new insights and strategies for improving the sensing performance of metal oxide semiconductor-based gas sensing materials.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Nanoscience & Nanotechnology
Utkarsh Kumar et al.
Summary: This work presents the design of novel 2D-material/0D-quantum dot heterostructures using a chemical method, and demonstrates their enhanced NO2 gas-sensing capability. Advanced characterization techniques were used to confirm the formation of MoS2/SnS heterojunction nanomaterials. The sensing characterization showed excellent response time and low limit of detection for NO2 using the MoSiSnS heterostructures.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Engineering, Environmental
Yajie Zhang et al.
Summary: In this study, In2O3/MoS2 composite sensor was synthesized to improve the sensitivity and selectivity of NO2 detection at room temperature.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Chemistry, Analytical
Hao Ren et al.
Summary: This study successfully improved the gas sensing capability of black phosphorus (BP) for NH3 detection by incorporating SnO quantum dots, demonstrating the great potential of BP as a universal gas sensor.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Chemistry, Analytical
Chengyu Yang et al.
Summary: In-doped SnO2 nanofibers were prepared by electrospinning method and showed high response and selectivity to NOX. The gas-sensing mechanism was investigated and it was found that the polycrystalline structure and In dopant played important roles in the excellent sensing performance.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Chemistry, Analytical
Run-Hui Wang et al.
Summary: In this study, a layered mesoporous aggregate of tin oxide nanocrystals with high specific surface area and mesoporous structure was synthesized. The tin oxide showed high ethanol sensing performance at low temperatures, with high selectivity and stability. The ethanol sensing mechanism changed with increasing operating temperature.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Engineering, Environmental
Dandan Huang et al.
Summary: This study successfully prepared [MIL-125(Ti)/ FexTiyOz]T-X (MFTT-X) gas-sensitive materials, and demonstrated their significantly enhanced sensitivity and fast response and recovery time towards acetone.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Engineering, Environmental
Xue Bai et al.
Summary: The N-doped three-dimensional needle bridge connection core-shell structure N-CoS2@Co3O4 synthesized in this work exhibits excellent NO2 sensing performance, attributed to its unique structural features and high catalytic performance promoted by N-doping.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Yong Zhou et al.
Summary: In this study, nitrogen-functionalized heterophase TiO2 homojunctions (N-MXene) derived from MXene Ti3C2Tx were prepared and utilized as a sensing layer to detect trace NH3 gas at room temperature. The sensors exhibited improved detection limits and performance compared to existing MXene-involved reports, showing strong responses, sufficient recovery, and fast response/recovery speeds under humid conditions. The incorporation of nitrogen doping and TiO2 homojunctions played a key role in enhancing the performance of the sensors.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Physical
Siwei Liu et al.
Summary: In this study, Ti3C2/TiO2 nanocomposites were synthesized through in-situ growth of TiO2 on the surface of multilayer Ti3C2 MXene, showing improved response to NO2 gas and excellent gas-sensing performance. The formation of a Schottky barrier at the Ti3C2/TiO2 interface contributed to the outstanding response and selectivity of the composites. This work provides a simple method to enhance the gas-sensing performance of MXene materials in practical applications.
APPLIED SURFACE SCIENCE
(2021)
Article
Environmental Sciences
Marco Travaglio et al.
Summary: The study reveals a positive relationship between air pollutant concentrations, particularly nitrogen oxides, and COVID-19 mortality and infectivity. PM2.5 was identified as a major contributor to COVID-19 cases in England, with a 12% increase in cases linked to a 1 m³ increase in the long-term average of PM2.5. The findings suggest that even a small increase in air pollution could lead to a significant rise in COVID-19 infectivity and mortality rates in England.
ENVIRONMENTAL POLLUTION
(2021)
Article
Environmental Sciences
Zohar Barnett-Itzhaki et al.
Summary: The study found that long-term exposure to air pollutants concentrations exceeding WHO guidelines, such as PM2.5 and NOx, may exacerbate morbidity and mortality rates from COVID-19. The models also highlighted the importance of the relative number of hospital beds in decreasing the morbidity and mortality of COVID-19.
ENVIRONMENTAL RESEARCH
(2021)
Article
Engineering, Environmental
Arunkumar Shanmugasundaram et al.
Summary: Researchers have developed a new sensor NSC@ZNS with excellent sensing characteristics for NO2, with high sensitivity and rapid response. The sensor has a detection limit of 21 ppb at ambient temperature, and demonstrates superior selectivity to NO2.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Engineering, Environmental
Qui Thanh Hoai Ta et al.
Summary: Si@TiO2/Ti3C2Tx heterostructures were synthesized in situ from Ti3AlC2 MAX phase by combining high-temperature Si diffusion and HF etching. The optimal heterostructure showed semiconductor behavior with enhanced surface area due to the distribution of small TiO2 particles over Ti3C2Tx MXene. The heterostructure exhibited excellent 2,4-Dinitrophenol photodegradation and room-temperature NO2-sensing capabilities, with the photocatalytic degradation attributed to broad light absorption and efficient carrier separation by Schottky contact. Density-functional theory calculations suggested that Si atoms could facilitate NO2 adsorption, highlighting the multi-functionality potential of Si@TiO2/Ti3C2Tx heterostructure.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Optics
G. L. Whitworth et al.
Summary: Researchers have successfully achieved a solution-processed infrared laser that operates at room temperature using colloidal quantum dots, with tunable wavelength and low linewidth. These lasers have advantages such as high integration capability and low cost, making them suitable for various applications.
Article
Chemistry, Analytical
Yajie Zhang et al.
Summary: Alkalized V2CTx MXene material, synthesized with abundant surface functional groups, suitable interlayer spacing, and appropriate Na+ intercalation, exhibits excellent gas sensing performance, especially high sensitivity and response to NO2.
SENSORS AND ACTUATORS B-CHEMICAL
(2021)
Article
Chemistry, Analytical
Orhan Sisman et al.
Summary: A novel organic-inorganic hybrid conductometric NO2 sensor was introduced by depositing liquid crystalline zinc oktakisalkylthiophthalocyanine on the surface of Cu2O nanowires. The sensing properties towards NO2 under different conditions were investigated, and the structures and performances of materials were characterized by SEM and UV-vis spectrophotometer.
SENSORS AND ACTUATORS B-CHEMICAL
(2021)
Article
Chemistry, Physical
Dongyue Wang et al.
Summary: In this paper, a PVA/Ag nanofibers-based TENG was developed for human respiration, movement, and harmful gas monitoring, achieving high voltage and power density outputs. By integrating a voltage regulator module, stable voltage output from the wind-driven TENG was achieved, providing a feasible solution for different wind conditions. A self-powered sensor system was developed by integrating TENGs and a gas sensor, offering a sustainable detection platform for tracking the source of harmful gases.
Article
Chemistry, Multidisciplinary
Fei Li et al.
Summary: A coordination-engineering strategy is proposed for finely adjusting the matrix thickness around conductive PbS quantum dots, resulting in improved performance of the QD film. This approach significantly enhances the power-conversion efficiency of QD solar cells.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Physical
Ahmed A. Abokifa et al.
Summary: In this study, room temperature sensing of chloroform gas using SnO2 nanostructured thin films synthesized via a single-step ACVD process is demonstrated. Theoretical calculations and simulations show that chloroform molecules have a thermodynamically favorable adsorption on the SnO2 surface, leading to a drop in surface resistance and a sensing response. Long-range dispersive interactions account for a significant portion of the adsorption energies, highlighting the stronger binding of chloroform on metal-oxides compared to carbon-based materials.
APPLIED SURFACE SCIENCE
(2021)
Article
Engineering, Environmental
Jingjing Liu et al.
Summary: A high-response formaldehyde gas sensor based on Ag-ZnO/In2O3 nanofibers was successfully fabricated, showing superior sensitivity, selectivity and stability, with an ultra-high response value towards formaldehyde. The low detection limit of the sensor can be mainly attributed to the proper design of multi-level heterojunctions, which significantly enhance the sensing performance.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Chemistry, Analytical
Miao Liu et al.
Summary: In this study, a high-performance room temperature gas-sensing material was successfully developed by utilizing MXene and reduced graphene oxide as building blocks. The resulting 3D aerogel shows excellent acetone-sensing performance at room temperature, with fast response and recovery times, as well as good reproducibility and selectivity. This strategy of composite 3D graphene/MXene architectures with metal oxide semiconductors provides a new pathway for future development of room temperature gas sensors.
SENSORS AND ACTUATORS B-CHEMICAL
(2021)
Article
Chemistry, Analytical
Xiqi Chen et al.
Summary: The study demonstrated a fully recoverable WS2-based gas sensor with enhanced anti-humidity ability by incorporating zero-dimensional PbS nanoparticles and UV light. The optimized WS2/PbS (molar ratio of 10:1) gas sensor showed significantly improved recovery rate from 33.4% to 99.8% with almost no baseline drift compared to the pure WS2 gas sensor, attributing to the irradiation of UV that accelerated the desorption of water molecules.
SENSORS AND ACTUATORS B-CHEMICAL
(2021)
Article
Chemistry, Analytical
Qianqiong Zhu et al.
Summary: The Au modified SnS2 nano-flowers show improved gas-sensing characteristics at low temperatures, with higher response values and shorter response and recovery times. The enhanced sensing properties can be attributed to the catalytic effect of Au NPs and the Schottky contact formed between Au NPs and SnS2.
SENSORS AND ACTUATORS B-CHEMICAL
(2021)
Article
Chemistry, Physical
Baihe Sun et al.
Summary: Co3O4 nanocrystals were effectively attached to branched polyethylenimine (PEI) functionalized Ti3C2Tx MXene sheets to fabricate composites with enhanced sensing performance towards NOx gas. The heterogeneous structure with improved electron transfer channels and diffusion capacity contributed to the high sensitivity and selectivity of Co3O4@PEI/Ti3C2Tx MXene composites, making them promising candidates for high-sensitivity NOx gas sensors.
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