4.7 Article

Graphdiyne and Nitrogen-Doped Graphdiyne Nanotubes as Highly Efficient Electrocatalysts for Oxygen Reduction Reaction

相关参考文献

注意:仅列出部分参考文献,下载原文获取全部文献信息。
Article Chemistry, Multidisciplinary

Directly Growing Graphdiyne Nanoarray Cathode to Integrate an Intelligent Solid Mg-Moisture Battery

Xinlong Fu et al.

Summary: A continuous humidity and solar-light dual responsive intelligent solid Mg-moisture battery (SMB) with a graphdiyne nanosheets array as a new generation cathode for high-performance intelligent SMB was fabricated. The battery can be continuously tuned by humidity and solar-light and shows ultrafast response time, recovery time, and sensitive respiratory sensing performance, making it a promising self-power humidity monitor.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2023)

Article Chemistry, Multidisciplinary

Energy Storage Mechanism in Supercapacitors with Porous Graphdiynes: Effects of Pore Topology and Electrode Metallicity

Tangming Mo et al.

Summary: Porous graphdiynes are a class of 2D materials with tunable electronic structures and various pore structures, which can be used as nanostructured electrodes and provide understanding of energy storage mechanisms in supercapacitors. This study investigates the effects of stacking structure and metallicity on energy storage with porous graphdiyne electrodes. The simulations show that supercapacitors based on porous graphdiynes with AB stacking structure achieve higher double-layer capacitance and ionic conductivity compared to AA stacking. The enhanced quantum capacitance of doped porous graphdiynes enables them to deliver outstanding gravimetric and volumetric energy and power densities. These findings pave the way for designing high-performance supercapacitors by controlling pore topology and metallicity of electrode materials.

ADVANCED MATERIALS (2023)

Review Chemistry, Multidisciplinary

Graphynes and Graphdiynes for Energy Storage and Catalytic Utilization: Theoretical Insights into Recent Advances

Hao Li et al.

Summary: Carbon allotropes have played an important role in people's lives throughout history. Graphyne family materials, especially graphdiyne, have a wide range of potential applications due to their superior properties. GYF-based materials still have many potential applications, especially in energy storage and catalytic utilization, which need further development.

CHEMICAL REVIEWS (2023)

Review Chemistry, Multidisciplinary

Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design

Yonggui Zhao et al.

Summary: The oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) are critical steps in energy conversion and storage systems, but their slow kinetics and the complexity of catalyst-electrolyte interfaces limit their practical applications. Recent advances in in situ/operando characterization techniques have enabled the monitoring of catalysts under reaction conditions, providing valuable insights into the mechanistic studies of OER/ORR catalysts. This review highlights the determination of active species, identification of active sites, and monitoring of reactive intermediates, and discusses strategies for rational catalyst design.

CHEMICAL REVIEWS (2023)

Review Chemistry, Multidisciplinary

Graphdiyne-Based Single-Atom Catalysts with Different Coordination Environments

Xinliang Fu et al.

Summary: As a special carbon material, graphdiyne (GDY) provides an ideal platform for constructing single-atom catalysts (ACs) due to its incomplete charge transfer effect, tunable electronic structure, and ability to anchor metal atoms directly. This mini-review highlights recent progress in the rational design and application of GDY-based ACs, and examines the relationship between coordination engineering of these catalysts and their catalytic performance. Prospects for the future development of GDY-based ACs in energy conversion are also discussed.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

Review Chemistry, Multidisciplinary

Two-Dimensional Carbon Graphdiyne: Advances in Fundamental and Application Research

Xuchen Zheng et al.

Summary: Graphdiyne (GDY), a two-dimensional all-carbon network with sp/sp(2)-hybridized structure, has shown great potential for innovation and development in various fields. GDY has attracted extensive attention from scientists due to its controlled growth, chemical and physical properties, and mechanisms that differ from traditional carbon materials. It has become one of the frontiers of chemistry and materials science and has generated numerous research achievements in the fundamental and applied study of carbon materials. The applications of GDY in catalysis, energy storage, photoelectronic, biomedicine, environmental science, life science, detectors, and material separation are comprehensively introduced in this review.

ACS NANO (2023)

Article Chemistry, Analytical

Smart enzyme-free amplification dual-mode self-powered platform designed on two-dimensional networked graphdiyne and DNA nanorods for ultra-sensitive detection of breast cancer biomarkers

Yunzhi Ma et al.

Summary: Research has shown that microRNAs can be used as potential biomarkers for cancer diagnosis due to their regular dysregulation in cancers. This study presents a new approach for ultra-responsive dual-mode detection of miRNA-141, a breast cancer biomarker, using a self-powered biosensor fabricated with two-dimensional networked graphdiyne.

ANALYTICA CHIMICA ACTA (2023)

Article Chemistry, Multidisciplinary

Engineering Dual Single-Atom Sites on 2D Ultrathin N-doped Carbon Nanosheets Attaining Ultra-Low-Temperature Zinc-Air Battery

Tingting Cui et al.

Summary: The novel dual single-atom catalyst FeMn-DSAC exhibits remarkable bifunctional activities for ORR and OER, enabling efficient operation of the ZAB at ultra-low temperature of -40 degrees C with peak power density of 30 mW cm(-2) and up to 86% specific capacity retention compared to room temperature.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

Review Engineering, Environmental

Defect engineering of graphynes for energy storage and conversion

Jialu Wang et al.

Summary: Defect engineering of graphynes is a complex technique that can improve their energy storage and catalytic performance by altering their geometry and chemical environment through introducing defects. This review paper discusses the progress in defect engineering of graphynes for energy storage, electrocatalysis, and photocatalysis, and explores the opportunities and challenges for future research on defective graphynes.

CHEMICAL ENGINEERING JOURNAL (2022)

Review Chemistry, Multidisciplinary

Graphdiyne Electrochemistry: Progress and Perspectives

Xinyue Chen et al.

Summary: This review provides an overview of the development history, structural and electrochemical features of graphdiyne materials, summarizes recent progress in the synthesis of graphdiyne materials and their composites, and covers various electrochemical applications in fields such as energy conversion, energy storage, and sensing.
Article Chemistry, Multidisciplinary

A Simple Preheating-Pyrolysis Strategy Leading to Superior Oxygen Reduction Reaction Activity in Fe-N/Carbon Black

Chen Ouyang et al.

Summary: Controlling pyrolysis conditions enhances the catalytic activity of the oxygen reduction reaction (ORR) and can produce low-cost catalysts.

ADVANCED MATERIALS (2022)

Review Chemistry, Multidisciplinary

Understanding of Oxygen Redox in the Oxygen Evolution Reaction

Xiaopeng Wang et al.

Summary: This article provides a comprehensive review of the oxygen redox process in the oxygen evolution reaction (OER) through lattice oxygen oxidation mechanism (LOM), and discusses the characterization techniques used to identify the oxygen redox. It explains the critical advantage and underlying science of LOM compared to the traditional adsorbate evolution mechanism (AEM) in generating higher OER activities. The article also provides insights into future developments in LOM electrocatalysts.

ADVANCED MATERIALS (2022)

Article Chemistry, Physical

Regulating symmetry of organic precursors for mechanochemical synthesizing rich pyridonic-/pyridinic-nitrogen doped graphyne

Yuxuan Lu et al.

Summary: This study successfully synthesized graphyne material with rich pyridinic- and pyridonic-nitrogen doping via a mechanochemical route. The introduction of symmetric hexabromobenzene was found to suppress the formation of graphitic carbon impurities. By optimizing the material ratio, the obtained graphyne material exhibited higher energy storage capacity and structural stability.

CARBON (2022)

Article Multidisciplinary Sciences

Graphdiyne-based metal atomic catalysts for synthesizing ammonia

Huidi Yu et al.

Summary: Researchers have successfully synthesized a novel catalyst Pd-GDY, showing excellent electrocatalytic performance in nitrogen reduction with high yield and selectivity. The catalyst exhibits extremely high NH3 yield and reaction selectivity in neutral media, with minimal performance degradation.

NATIONAL SCIENCE REVIEW (2021)

Review Chemistry, Multidisciplinary

Single Atom Catalysts for Fuel Cells and Rechargeable Batteries: Principles, Advances, and Opportunities

Yuchao Wang et al.

Summary: This paper discusses the importance of developing efficient and robust electrochemical energy storage systems, as well as the role of single atom catalysts in improving device performance. Additionally, it summarizes the working principles and challenges of next-generation electrochemical energy storage and conversion devices.

ACS NANO (2021)

Article Chemistry, Multidisciplinary

Co-Zn-MOFs Derived N-Doped Carbon Nanotubes with Crystalline Co Nanoparticles Embedded as Effective Oxygen Electrocatalysts

Wendi Zhang et al.

Summary: This study successfully synthesized cobalt-embedded N-doped carbon nanotubes with excellent ORR activity, exhibiting a half wave potential comparable to Pt/C. The three-dimensional network formed by crystalline Co@CNTs-T facilitates electron migration and ion diffusion, contributing to its stability as an electrocatalyst.

NANOMATERIALS (2021)

Article Chemistry, Physical

Theoretical investigation of CO2 electroreduction on N (B)-doped graphdiyne mononlayer supported single copper atom

Zhen Feng et al.

Summary: This study systematically investigated the geometric structures, electronic properties, and catalytic performance of boron- and nitrogen-doped graphdiyne complexes anchored with a single copper atom for CO2 electrochemical reduction reaction (CO2RR). The nitrogen-doped graphdiyne monolayers exhibited more efficient catalytic performance compared to the boron-doped ones, attributed to differences in adsorption energies and charge transfer. The findings suggest that electronegativity of coordinated elements plays a crucial role in designing atomic metal catalysts for CO2RR.

APPLIED SURFACE SCIENCE (2021)

Article Chemistry, Multidisciplinary

Efficient Hydrogen Evolution on Nanoscale Graphdiyne

Lan Hui et al.

Summary: The unique nanostructure of GDY provides active sites for hydrogen adsorption and facilitates the electron-transfer process, making it a superior metal-free efficient HER electrocatalyst with long-term durability compared to Pt/C.
Article Chemistry, Physical

Acidic Water Oxidation on Quantum Dots of IrOx/Graphdiyne

Zhongqiang Wang et al.

Summary: A controllable graphdiyne induced growth strategy prepared oxidized iridium quantum dots with highly uniform size distribution, showing superior activity and durability for acidic OER compared to previous electrocatalysts. The graphdiyne effectively increased catalytically active sites and protected metal catalysts from corrosion, demonstrating advantages in charge transfer behavior.

ADVANCED ENERGY MATERIALS (2021)

Review Chemistry, Physical

Engineering Carbon Materials for Electrochemical Oxygen Reduction Reactions

Liangxu Lin et al.

Summary: The electrochemical oxygen reduction reaction is crucial in energy conversion technologies, and the use of low-cost and durable carbon materials as efficient catalysts shows promise for future applications. Research efforts are focusing on understanding catalytic mechanisms and engineering techniques to improve the performance and selectivity of these carbon catalysts. Future improvements in carbon catalysts are expected to lead to more efficient and reliable energy conversion technologies.

ADVANCED ENERGY MATERIALS (2021)

Article Chemistry, Physical

Aqueous/solid state Zn-air batteries based on N doped graphdiyne as efficient metal-free bifunctional catalyst

Tiantian Lu et al.

Summary: The study demonstrates the use of N-doped graphdiyne (GDY) as an efficient metal-free bifunctional catalyst for stable aqueous and solid-state ZABs, showing high catalytic performance and long-term stability. The findings suggest the potential of N-doped GDY as an effective and ultra-stable catalyst for ZABs, especially in solid-state ZABs for wearable electronics applications.

NANO ENERGY (2021)

Review Chemistry, Multidisciplinary

Recent advances of graphdiyne: synthesis, functionalization, and electrocatalytic applications

Xiaojie Chen et al.

Summary: Graphdiyne (GDY) with unique structure and properties shows great application prospects in various fields. Recent research has focused on the synthesis, structural modification, and practical applications of GDY, with significant progress in the field of electrocatalysis.

MATERIALS CHEMISTRY FRONTIERS (2021)

Article Chemistry, Multidisciplinary

N-Doped Graphdiyne Coating for Dendrite-Free Lithium Metal Batteries

Hong Shang et al.

CHEMISTRY-A EUROPEAN JOURNAL (2020)

Article Nanoscience & Nanotechnology

Highly Lithiophilic Graphdiyne Nanofilm on 3D Free-Standing Cu Nanowires for High-Energy-Density Electrodes

Hong Shang et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

Article Chemistry, Physical

Graphdiyne-engineered heterostructures for efficient overall water-splitting

Huidi Yu et al.

NANO ENERGY (2019)

Review Chemistry, Inorganic & Nuclear

Graphdiyne applied for electrochemical energy storage

Jianjiang He et al.

DALTON TRANSACTIONS (2019)

Article Chemistry, Physical

N-doped graphdiyne for high-performance electrochemical electrodes

Hong Shang et al.

NANO ENERGY (2018)

Article Multidisciplinary Sciences

Selectively nitrogen-doped carbon materials as superior metal-free catalysts for oxygen reduction

Qing Lv et al.

NATURE COMMUNICATIONS (2018)

Article Chemistry, Multidisciplinary

Ultrathin Graphdiyne Nanosheets Grown InSitu on Copper Nanowires and Their Performance as Lithium-Ion Battery Anodes

Hong Shang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

Review Chemistry, Physical

Redox-Active Polymers for Energy Storage Nanoarchitectonics

Jeonghun Kim et al.

Review Chemistry, Multidisciplinary

Nanostructured material-based biofuel cells: recent advances and future prospects

Cui-e Zhao et al.

CHEMICAL SOCIETY REVIEWS (2017)

Article Nanoscience & Nanotechnology

Activity targets for nanostructured platinum group-metal-free catalysts in hydroxide exchange membrane fuel cells

Brian P. Setzler et al.

NATURE NANOTECHNOLOGY (2016)

Review Chemistry, Multidisciplinary

Metal-Free Catalysts for Oxygen Reduction Reaction

Liming Dai et al.

CHEMICAL REVIEWS (2015)

Review Multidisciplinary Sciences

Graphene-supported platinum catalysts for fuel cells

Nedjeljko Seselj et al.

SCIENCE BULLETIN (2015)

Article Chemistry, Physical

Improved electrocatalytic activity of carbon materials by nitrogen doping

Awan Zahoor et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2014)

Article Chemistry, Multidisciplinary

Architecture of graphdiyne nanoscale films

Guoxing Li et al.

CHEMICAL COMMUNICATIONS (2010)