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Article
Polymer Science
Lei Du et al.
Summary: In this study, a high-performance and self-healing bio-based polyurethane hot-melt adhesive (DPU) was successfully developed. The adhesive showed high lap shear strength and biomass content, along with excellent self-healing and repeatable adhesion properties. It also exhibited excellent resistance to low temperatures and solvents, making it a promising alternative to conventional PU-HMAs.
EUROPEAN POLYMER JOURNAL
(2023)
Article
Agricultural Engineering
Xiao-Li Zhao et al.
Summary: Biobased epoxy covalent adaptable networks (ECANs) were prepared using glycerol triglycidyl ether (GTE), vanillin (VA), and diamines. The ECANs exhibited excellent mechanical and thermal properties due to the introduction of rigid imine bonds and aromatic groups. They also showed reprocessability and can be used as high-performance recoverable adhesives.
INDUSTRIAL CROPS AND PRODUCTS
(2023)
Article
Polymer Science
Peng Sun et al.
Summary: Supramolecular adhesives with dynamic and reversible bonding properties have attracted significant attention, but developing high-performance adhesives remains a challenge. Recent research has successfully constructed strong and functional supramolecular adhesives by combining noncovalent interactions with rational design strategies. These studies have focused on improving adhesion strength and achieving special functionalities, such as underwater adhesion and conductivity. Future research should address current challenges and further enhance the performance and explore new applications of supramolecular adhesives.
MACROMOLECULAR CHEMISTRY AND PHYSICS
(2023)
Article
Polymer Science
Lin Wang et al.
Summary: In this study, a series of vitrimer networks were designed and synthesized by incorporating multiple hydrogen bonds and boronic ester bonds into styrene butadiene rubber (SBR). The aggregated 2-ureido-4-[1H]-pyrimidinone (UPy) rings enhanced the strength and durability of the rubber through reversible breaking and reforming events. The UPy aggregations also improved the dimensional stability of the rubber at elevated temperatures.
Article
Engineering, Environmental
Shengdu Yang et al.
Summary: In this study, a strong and stable supramolecular adhesive material was realized through a facile and powerful noncovalent bonding strategy, integrating natural thioctic acid and mono-hydroxylated adamantane-functionalized poly(disulfide) backbone. The optimized supramolecular adhesive showed fascinating reconfigurable ability upon repeated cooling and heating, thanks to the dynamic covalent poly(disulfides) network and reversible nanoconfined effect. This work provides valuable guidance for further developing rational theories of adhesive action mechanism and constructing high-performance adhesives based on small molecules.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Environmental
Ying Zhou et al.
Summary: A tough, strong, and recyclable soybean protein isolate (SPI)-based adhesive, SPI/BP@mica, was developed by co-assembly of mica and SPI via dynamic boron-nitrogen (B-N) coordinated catechol-derived boronic ester (B-O) interfacial bonding. The adhesive showed improved cohesive strength and energy dissipation capacity due to the dynamic covalent B-O, imine, and hydrogen bonds. It also exhibited excellent mold resistance, flame retardancy, and cost effectiveness compared to conventional adhesives.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Multidisciplinary
Bixia Zheng et al.
Summary: Introducing microphase separation and dynamic bonds into polyurethane improves performance. A modified lignin-based polyol (MLOH) was developed, which greatly improved reactivity and dispersibility compared to virgin lignin. A high-performance modified lignin-based dynamic covalent polyurethane (MLPU) with lignin enhanced microphase separation was fabricated, demonstrating excellent adhesive performance, shape memory capability, solvent resistance, temperature tolerance, durability, debonding ability, and reusability.
COMPOSITES PART B-ENGINEERING
(2023)
Article
Chemistry, Multidisciplinary
Aleix Costa Cornella et al.
Summary: Self-healing polymers improve sustainability by recovering their properties, and can be recycled. However, there are still sustainability issues, including the use of fossil-derived materials and hazardous chemicals.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2023)
Article
Engineering, Environmental
Nicole Tratnik et al.
Summary: In this study, a novel epoxy vitrimer with a higher renewable content was designed using renewable materials. The epoxy vitrimer exhibited self-strengthening effect and improved mechanical and thermal properties after multiple recycling cycles.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Polymer Science
Danielle M. Fitzgerald et al.
Summary: Pressure sensitive adhesives are widely used in everyday products and have the potential for greater use in medicine. The strength of adhesion depends on the chemical and material properties of the adhesive formulation and its interaction with the surface. This review focuses on the structure-property relationships of polymer architecture and pressure sensitive adhesion, specifically in the context of durable, removable, and biocompatible adhesion to wet surfaces like tissue. Challenges in biomedical wound closure are also discussed, along with innovative strategies to address them.
PROGRESS IN POLYMER SCIENCE
(2023)
Article
Polymer Science
Zhiyong Liu et al.
Summary: In this study, a recyclable adhesive was developed by incorporating dynamic boronic esters into epoxy resin derived from soybean oil. The successful synthesis of epoxidized soybean oil and boronic esters was confirmed through the analysis of proton nuclear magnetic resonance spectra and differential scanning calorimetry results. Swelling tests and tensile curves demonstrated the presence of covalently cross-linked networks. Self-healing and reprocessing experiments indicated that the cross-linked network topology could be re-assembled under mild conditions.
Review
Materials Science, Biomaterials
Yongping Lu et al.
Summary: Adhesive materials, both natural and synthetic, have the ability to stick to mucus or epithelial cells. They are widely used in biomedicine due to their unique properties, such as adhesion, biocompatibility, and surface characteristics. They can target specific areas in the human body, improving therapeutic effects and preventing bacterial infections. This review systematically introduces the properties and mechanisms of different types of adhesive materials and explores their applications in drug delivery, antibacterials, tissue repair, and other biomedical fields. The prospects and challenges of using adhesive materials in biomedicine are also discussed.
JOURNAL OF MATERIALS CHEMISTRY B
(2023)
Review
Polymer Science
Yulei Tian et al.
Summary: Adhesives are important bridging substances with wide applications, especially in the textile industry. Textile-related adhesives are classified into natural, synthetic, and natural/synthetic composite categories, with diverse synthesis methods and application characteristics. Understanding the role of adhesives in textile development can facilitate the future of functional, intelligent, and versatile textiles.
EUROPEAN POLYMER JOURNAL
(2022)
Article
Polymer Science
Pierre Berto et al.
Summary: This paper investigates a new route to synthesize reversibly cross-linked rubber based on the Diels-Alder chemistry. By grafting furan groups onto the polymer backbone and adding bis-maleimide compound, a thermo-reversible cross-linked elastomer is formed. The resulting rubber has easily tunable mechanical properties and exhibits good reprocessability.
Article
Polymer Science
Qinggeng Jiang et al.
Summary: In this paper, biodegradable epoxidized natural rubber containing cyclic carbonate groups (CNR) was synthesized. The material exhibited high self-healing efficiency due to the double dynamic covalent structure. Additionally, it was confirmed to be biodegradable according to biodegradable measurement. This is the first time that natural rubber with biodegradable and self-healing characteristics has been obtained.
Review
Chemistry, Multidisciplinary
Ziyang Liu et al.
Summary: This article discusses the demand for adhesives with changeable adhesion capabilities and how to meet these requirements. It mainly focuses on current research and design and manufacturing techniques of stimuli-responsive material-based adhesives. Additionally, critical suggestions are made for the potential applications and future development of smart adhesives.
Article
Chemistry, Physical
Yifei Wang et al.
Summary: A new approach to fabricating responsive capsules by incorporating hindered poly(urea-urethane) chemistry into capsule shells is reported. These capsules can be destroyed to release a payload or fused together to create a monolith.
CHEMISTRY OF MATERIALS
(2022)
Article
Biochemistry & Molecular Biology
Zheng Liu et al.
Summary: In this study, a reusable and degradable 100% bio-based wood adhesive was developed by incorporating dynamic covalent/hydrogen hybrid networks into the adhesive system. The adhesive exhibited high bonding performance, water resistance, flame retardancy, mold resistance, and antibacterial properties.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2022)
Article
Polymer Science
Seppe Terryn et al.
Summary: The effect of Diels-Alder reaction on material properties was investigated, and the design parameters were tuned to meet different application requirements and achieve control over material properties.
Article
Polymer Science
Selene Chappuis et al.
Summary: The curing process of epoxy-anhydride vitrimers involves the formation of a poly(ester-co-ether) network through anionic copolymerization and homopolymerization reactions. By controlling the curing conditions and adding DHEBA, the yield of esters and hydroxides can be improved without compromising the thermal properties of the network.
Article
Engineering, Environmental
Dong-Mei Xie et al.
Summary: The study presents a method to fabricate sustainable polyurethanes from renewable castor oil, which exhibit good mechanical properties, reprocessability, and recyclability.
CHEMICAL ENGINEERING JOURNAL
(2022)
Review
Agricultural Engineering
Caoxing Huang et al.
Summary: Adhesives traditionally made from fossil-based polymers have issues of toxicity, environmental pollution, and non-renewable raw materials. Therefore, research on environmentally friendly and renewable adhesives from bio-based materials has gained attention. Lignin, a natural and renewable phenolic polymer with various functional groups, has been extensively studied for its exploitation. Despite some progress, developing lignin-based adhesives with performances surpassing fossil-based adhesives remains challenging.
INDUSTRIAL CROPS AND PRODUCTS
(2022)
Article
Chemistry, Multidisciplinary
Karen P. Cortes-Guzman et al.
Summary: In this study, biobased thermoset materials with self-healing abilities were synthesized through Transimination reactions and successfully 3D-printed. The resulting materials exhibited a range of mechanical properties and potential applications. The ability to be reprocessed makes these materials significant in promoting the use of renewable resources in polymer production.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2022)
Article
Polymer Science
Chao Liu et al.
Summary: A novel type of self-healing waterborne polyurethane (HSPU) film with dynamic quadrupolar hydrogen (UPy) and aromatic disulfide bonds was developed. The film exhibits excellent mechanical properties, self-healing abilities, and wear resistance. It can be reprocessed under pressure or recycled in solvent, making it a promising coating material for sustainable applications.
Review
Polymer Science
Chunyan Cui et al.
Summary: This review discusses the development and various types of wet adhesives, including catechol-based wet adhesives and non-catechol-based wet adhesives, as well as their adhesion mechanisms and advantages and disadvantages.
PROGRESS IN POLYMER SCIENCE
(2021)
Article
Nanoscience & Nanotechnology
Huiwen Pang et al.
Summary: The study developed an inorganic crystal cross-linked hybrid soy protein adhesive that showed excellent performance in plywood manufacturing, providing a novel and effective preparation strategy for high-performance SP-based adhesives.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Review
Chemistry, Multidisciplinary
Hailong Fan et al.
Summary: Underwater adhesives are in high demand due to their specific challenges in development and performance on wet or submerged surfaces. Current strategies include different types of underwater adhesives and their development and performance based on various mechanisms and strategies. Possible research directions and prospects for underwater adhesives are also discussed.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Sidi Li et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Article
Chemistry, Multidisciplinary
Weifeng Liu et al.
Article
Polymer Science
Zhiyong Liu et al.
Article
Chemistry, Physical
Fei Song et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2019)
Article
Polymer Science
Zhiyong Liu et al.
Article
Polymer Science
Longhe Zhang et al.
Review
Chemistry, Multidisciplinary
Wim Denissen et al.
Article
Chemistry, Multidisciplinary
Wim Denissen et al.
ADVANCED FUNCTIONAL MATERIALS
(2015)
Article
Multidisciplinary Sciences
Damien Montarnal et al.
