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Minireview on Metal-Chalcogenide Cathode Materials with Dual-Redox Centers for Magnesium-Metal-Anode-Based Batteries: Recent Progress and Future Directions

ENERGY & FUELS (2023)

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Engineering Pocket-Like Graphene-Shell Encapsulated FeS2: Inhibiting Polysulfides Shuttle Effect in Potassium-Ion Batteries

Bochao Chen et al.

Summary: A graphene-shell-encapsulated FeS2 embedded in N/S codoped 3D hollow carbon spheres is developed to address the issue of polysulfides dissolution in potassium-ion batteries. Experimental and computational results demonstrate that the graphene-shell promotes K ion mobility, enhancing cycle stability and rate performance of the electrode. These findings provide insights for designing metal-based sulfide electrodes for PIBs.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Multifunctional Hyphae Carbon Powering Lithium-Sulfur Batteries

Lei Huang et al.

Summary: Biotechnology is utilized to develop a novel biological self-assembly technology for the large-scale preparation of multifunctional Rhizopus hyphae carbon fiber (RHCF) and its derivatives. The designed RHCF derivatives exhibit powerful multifunctionality in lithium-sulfur batteries, showing excellent cycling performance and high-rate capacity. This work provides a new method for advanced energy storage and conversion using hollow carbon fibers and their derivatives.

ADVANCED MATERIALS (2022)

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Article Electrochemistry

Revealing the electrochemical mechanism of the conversion-type Co3S4 in a novel high-capacity Mg-Li hybrid battery

Xing Cai et al.

Summary: In this study, an ultrahigh-capacity Mg-Li hybrid battery was assembled for the first time using spinel Co3S4 cathode and Mg anode. The Co3S4-F particles delivered high discharge capacity and energy density, outperforming reported chalcogenides. The synergistic effect of Co3S4-F micro/nano particles and APC-LiCl hybrid electrolyte promoted outstanding electrochemical performance.

ELECTROCHIMICA ACTA (2022)

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Article Energy & Fuels

Nanostructures of Carbon Nanofiber-Constrained Stannous Sulfide with High Flexibility and Enhanced Performance for Sodium-Ion Batteries

Long Qing et al.

Summary: A nanostructure of SnS/N-CNFs was constructed by embedding SnS nanoparticles in nitrogen-doped carbon nanofibers (N-CNFs), which were used as anodes for SIBs. The SnS/N-CNFs structure can restrict the volume changes of SnS, improve the cycling performance of the batteries, and exhibit outstanding flexibility.

ENERGY & FUELS (2022)

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Article Materials Science, Ceramics

CoS2 as Cathode Material for Magnesium Batteries with Dual-salt Electrolytes

Li Wenbo et al.

Summary: The influence of Li+/Mg2+ dual-salt electrolytes on the electrochemical performance of CoS2 as a conversion cathode for MMBs is studied, and it is found that Li-salt additives can significantly enhance the conversion kinetics of CoS2 and improve the cycling stability of the battery.

JOURNAL OF INORGANIC MATERIALS (2022)

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Article Chemistry, Physical

VS4 anchored on Ti3C2 MXene as a high-performance cathode material for magnesium ion battery

Jinglian Zhu et al.

Summary: Rechargeable magnesium batteries face challenges due to strong coulombic effects, but this study presents a high-performance system using hierarchical nano-micro hybrids to improve accessibility and reduce charge transfer resistance, achieving high discharge capacity, outstanding rate performance, and excellent cycling performance.

JOURNAL OF POWER SOURCES (2022)

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Article Chemistry, Physical

Structure adapting of bulk FeS2 micron particles and the corresponding anode for high performance sodium-ion batteries

Yong Li et al.

Summary: In this work, a novel FeS2-PANI-SWCNTs electrode structure was successfully designed to address the issues of low conductivity and large volume changes of FeS2 in sodium-ion batteries. The dual protection of PANI and SWCNTs resulted in excellent rate capability and long cycling stability of the electrode, while also suppressing the shuttle effect of polysulfides and reducing capacity loss.

JOURNAL OF MATERIOMICS (2022)

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Article Engineering, Environmental

Large-scale sodiophilic/buffered alloy architecture enables deeply cyclable Na metal anodes

Qianwen Chen et al.

Summary: By constructing a Cu6Sn5 alloy layer on commercial Cu foils, the deposition behavior of Na can be significantly improved, reducing nucleation overpotential and dendrite formation, while mitigating stress and volume change caused by the alloy reaction.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Revealing the Reaction and Fading Mechanism of FeSe2 Cathodes for Rechargeable Magnesium Batteries

Donggang Tao et al.

Summary: The study synthesized nanorod-like FeSe2 as a cathode for rechargeable Mg batteries, demonstrating high capacity and good rate capability. In situ characterizations revealed the Mg2+ intercalation mechanism for FeSe2 and considered the fading mechanism caused by the dissolution of Fe2+ and selenium in the electrolyte during cycling.

CHEMPHYSCHEM (2022)

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Review Energy & Fuels

Lithium-Free Batteries: Needs and Challenges

Srikanth Ponnada et al.

Summary: This paper investigates lithium-free metal batteries and aims to bridge the gap between academia and industry by advocating best practices and recommendations for measuring performance and key parameters, in order to promote the commercial application of these batteries for large-scale energy storage.

ENERGY & FUELS (2022)

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Article Chemistry, Applied

Highly active cobalt-doped nickel sulfide porous nanocones for high-performance quasi-solid-state zinc-ion batteries

Xin Tong et al.

Summary: A highly active cobalt-doped Ni3S2 porous nanocone framework designed as a zinc-ion battery electrode demonstrates excellent battery performance and cycling stability, along with high energy density. The results not only provide new insights into cathode materials design for zinc-based batteries, but also suggest their commercial potential in portable and wearable electronics.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Physical

Insight into the coordinating mechanism of multi-electron reaction and structural stability induced by K plus pre-intercalation for magnesium ions batteries

Shiqi Ding et al.

Summary: The application of K+ pre-intercalation strategy successfully enables high specific capacity and excellent cycling stability in cathode materials for magnesium ion batteries, shedding light on the viability of multi-electron reaction without compromising structural stability.

NANO ENERGY (2022)

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Article Chemistry, Multidisciplinary

Size-Controllable Nickel Sulfide Nanoparticles Embedded in Carbon Nanofibers as High-Rate Conversion Cathodes for Hybrid Mg-Based Battery

Guilei Zhu et al.

Summary: This article develops a size-controllable cathode material called nickel sulfide nanoparticles embedded in carbon nanofibers (NiS@C) for hybrid Mg2+/Li+ batteries. The optimized design of the material shows superior electrochemical performance, including high discharge capacity, excellent rate performance, and remarkable cycle life. Furthermore, the conversion mechanism of NiS in MLIBs is demonstrated for the first time, affirming the involvement of both Mg2+ and Li+ at the cathodic side.

ADVANCED SCIENCE (2022)

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Article Chemistry, Multidisciplinary

In Situ Anchoring Anion-Rich and Multi-Cavity NiS2 Nanoparticles on NCNTs for Advanced Magnesium-Ion Batteries

Zisen Ye et al.

Summary: In this paper, NiS2 and its composite with Ni-based carbon nanotubes (NiS2/NCNTs) are explored as cathode materials for Mg-ion batteries. NiS2/NCNTs with excellent Mg2+ storage property is synthesized by growing NiS2 nanoparticles on NCNTs. NiS2 with a large regular cavity structure and abundant sulfur-sulfur (S-S) bonds can provide active sites and unobstructed transport paths for the insertion-disinsertion of Mg2+. NiS2/NCNTs exhibit high capacity and outstanding rate performance.

ADVANCED SCIENCE (2022)

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Article Chemistry, Physical

Highly reversible Mg metal anodes enabled by interfacial liquid metal engineering for high-energy Mg-S batteries

Chuanliang Wei et al.

Summary: Metallic Mg is a promising anode material for rechargeable magnesium-ion batteries, but low Mg2+ conductivity caused by liquid electrolyte passivation hinders its development. This study found that Mg dendrites can be formed in Mg metal anodes, and these nanoscale dendrites can pierce through separators and cause short circuits. By painting a liquid metal Ga layer on Mg foil, the issues of Mg metal anodes can be addressed and a high-performance Mg metal anode can be obtained.

ENERGY STORAGE MATERIALS (2022)

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Article Chemistry, Physical

PVP-induced synergistic engineering of interlayer, self-doping, active surface and vacancies in VS4 for enhancing magnesium ions storage and durability

Shiqi Ding et al.

Summary: In this study, PVP was innovatively incorporated with VS4 to improve the kinetic performance, cycling life, and specific capacities of magnesium-ion batteries. The novel design of PVP-VS4 exhibited long-term cycling stability and exceptional high-rate capability. The reaction kinetics and energy storage mechanism were further analyzed using experimental techniques and computational calculations.

ENERGY STORAGE MATERIALS (2022)

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Understanding the Electrochemical Performance of FeS2 Conversion Cathodes

David S. Ashby et al.

Summary: Conversion cathodes have the potential to improve energy densities in rechargeable Li+ batteries, but their limited electrochemical stability and power density have hindered their practical use. In this study, we investigate the effects of cell fabrication, electrolyte interaction, and current density on the electrochemical performance of FeS2/Li batteries. The capacity loss is primarily attributed to the large volume changes during (de)lithiation, leading to the degradation of the conductive matrix. However, by applying external pressure and increasing current density, the capacity loss and polysulfide loss can be minimized.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Engineering, Environmental

Strategy of cation/anion co-doping for potential elevating of VS4 cathode for magnesium ion batteries

Shiqi Ding et al.

Summary: VS4 modified with cation/anion co-doping (MVSO) shows enhanced electrical conductivity and improved cycle and rate performance. MVSO exhibits excellent electrochemical properties, including high specific capacity, ultralong cycling life, superior rate capability, and low self-discharge ratio. The fast reaction kinetics and high capacitive process contribution of MVSO are highlighted.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Core-Shell-Structured Carbon Nanotube@VS4 Nanonecklaces as a High-Performance Cathode Material for Magnesium-Ion Batteries

Jianbo Li et al.

Summary: In this study, a betaine-assisted solvothermal strategy was used to improve the electronic conductivity and polarization effect of VS4. By coating VS4 nanoblocks onto carbon nanotubes (CNTs), the contact between the electrode and electrolyte was promoted, and the uniform distribution of nanoblocks was ensured. The as-synthesized CNT@VS4 nanonecklaces exhibited excellent performance for magnesium-ion batteries, thanks to their abundant active sites and electron-conductive highways.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2022)

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Article Chemistry, Multidisciplinary

TiVCTx MXene/Chalcogenide Heterostructure-Based High-Performance Magnesium-Ion Battery as Flexible Integrated Units

Yuming Zhang et al.

Summary: Magnesium-ion batteries have attracted attention due to their high theoretical capacity, high safety, and low cost. This study presents a high-performance, stable cycling NiSe2-CoSe2@TiVCTx heterostructure magnesium-ion battery cathode, prepared using a bimetallic metal-organic framework and co-assembly strategy. The cathode exhibits high discharge-specific capacity and cycling stability, and has practical applications as a flexible integrated unit for self-powered systems.

SMALL (2022)

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Article Nanoscience & Nanotechnology

FeS2 Nanoparticle/Graphene Composites for Lithium-Ion Storage with Enhanced Anode Performances

Tongjun Li et al.

Summary: This study aims to improve the capacity loss and electrochemical performance issues in marcasite (FeS2) as an anode material for lithium-ion batteries (LIBs) by introducing sulfur vacancy structure. By using L-cysteine as the sulfur source and reducing GO to rGO sheets with NaBH4, FeS2 nanoparticles with S-vacancy 3D structure were successfully synthesized. Through DFT calculations and systematic characterization, it is shown that the S-vacancies enhance the binding energy and charge-transfer rate of the FeS2/rGO composite, resulting in superior performance as a LIBs anode material.

ACS APPLIED NANO MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Cooperative Cationic and Anionic Redox Reactions in Ultrathin Polyvalent Metal Selenide Nanoribbons for High-Performance Electrochemical Magnesium-Ion Storage

Xiaolan Xue et al.

Summary: The ultrathin CoSe2 nanoribbons are proven to be a robust cathode material for rechargeable magnesium batteries, with a Mg2+ storage mechanism based on cooperative cationic and anionic redox processes, contributing to improved specific capacity and electrochemical kinetics.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Physical

Using amorphous CoSx hollow nanocages as cathodes for high-performance magnesium-lithium dual-ion batteries

Haoyuan Chen et al.

Summary: In this study, amorphous hollow cobalt sulfide nanocages were prepared as cathode materials for high performance magnesium-lithium dual-ion batteries (MLDBs), resulting in high specific capacities and short activation processes. This work provides valuable insights into the development of high-performance MLDBs.

APPLIED SURFACE SCIENCE (2022)

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Article Energy & Fuels

Electrospinning Preparation of a High-Rate Self-Supported Cathode for Rechargeable Aqueous Zinc-Ion Batteries

Jie Liu et al.

Summary: This study presents a solution for the preparation of a self-supported cathode for aqueous zinc-ion batteries. The cathode material, fabricated through electrospinning, consists of vanadium oxide nanodots encapsulated in carbon nanofibers. This unique nanostructure not only inhibits element dissolution but can also be directly used as the cathode, without the need for extra additives. The self-supported cathode exhibits high specific capacity, rate performance, and outstanding cycle ability.

ENERGY & FUELS (2022)

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Article Chemistry, Physical

Benzoate anion derived carbon-encapsulated NiS nanoparticles as a freestanding cathode for magnesium-based batteries

Guilei Zhu et al.

Summary: A facile approach is designed to fabricate carbon encapsulated NiS nanoparticles for binder-free cathode material. The resulting material exhibits enhanced electrochemical performance and long lifespan in hybrid Mg2+/Li+ batteries.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Chemistry, Multidisciplinary

A Molybdenum Polysulfide In-Situ Generated from Ammonium Tetrathiomolybdate for High-Capacity and High-Power Rechargeable Magnesium Cathodes

Dong Chen et al.

Summary: Rechargeable magnesium batteries (RMBs) are a promising energy-storage technology, but the development of high-performance cathode materials is a major challenge. This study demonstrates the high performance of ammonium tetrathiomolybdate as an RMB cathode material, which forms an amorphous structure with efficient magnesium-storage active sites and open transport pathways through ammonium extraction. The covalent-like molybdenum-sulfur bond weakens the interaction with magnesium ions and promotes simultaneous redox of molybdenum and sulfur, leading to high capacity.

ACS NANO (2022)

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Review Electrochemistry

Boron-Based Electrolytes for Rechargeable Magnesium Batteries: Biography and Perspective

Wen Ren et al.

Summary: This article reviews the origin and development process of boron-magnesium electrolyte, and focuses on several representative applications. It also briefly discusses the fundamental understandings and typical concerns related to the design of magnesium-boron electrolytes. Finally, future directions and possible proposals for practical magnesium-boron electrolytes are put forward.

BATTERIES & SUPERCAPS (2022)

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Review Chemistry, Physical

Status and perspectives of hierarchical porous carbon materials in terms of high-performance lithium-sulfur batteries

Yinyu Xiang et al.

Summary: Lithium-sulfur (Li-S) batteries face challenges in their commercialization due to poor electrical and ionic conductivity, dissolution of polysulfide ions, and volume change. Hierarchical porous carbon (HPC) materials have been investigated as a solution to these issues. This review presents recent progress in the synthesis and application of HPC materials in various components of Li-S batteries, and discusses the correlation between the structural features of HPC and the electrochemical performance of Li-S batteries. Challenges and future perspectives of HPCs for Li-S batteries are also discussed.

CARBON ENERGY (2022)

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Review Chemistry, Physical

Oxide cathodes for sodium-ion batteries: Designs, challenges, and perspectives

Tao Chen et al.

Summary: This article summarizes the research progress of transition-metal oxides in sodium-ion batteries and discusses the existing challenges and strategies to overcome them. It aims to provide guidance for the development of metal oxides in the next stage.

CARBON ENERGY (2022)

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Article Chemistry, Physical

Benzoate anion derived carbon-encapsulated NiS nanoparticles as a freestanding cathode for magnesium-based batteries

Guilei Zhu et al.

Summary: The research successfully designed and prepared a new type of cathode material by carbon-encapsulated nickel sulfide nanoparticles, which were applied in hybrid magnesium-ion/lithium-ion batteries, achieving high reversible capacity and long lifespan characteristics.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Nanoscience & Nanotechnology

Synergy Strategy of Electrical Conductivity Enhancement and Vacancy Introduction for Improving the Performance of VS4 Magnesium-Ion Battery Cathode

Shiqi Ding et al.

Summary: The introduction of Mo doping and N-TG in VS4 as a cathode for MIBs increases electrical conductivity, improves adsorption of Mg2+ ions, and enhances the electrochemical properties of the battery.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Engineering, Environmental

High-performance heterojunction Ti3C2/CoSe2 with both intercalation and conversion storage mechanisms for magnesium batteries

Fanfan Liu et al.

Summary: The construction of a novel Ti3C2/CoSe2 heterostructure as a cathode for rechargeable magnesium batteries shows significantly improved electrochemical performance and capacity retention. Mechanisms and dynamics of magnesium storage were analyzed, demonstrating impressive potential for application in high-performance energy storage devices.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

A hybrid Mg2+/Li+ battery based on high-capacity conversion-type cobalt disulfide cathodes with ultralong cycle life and high energy density

Chao Liu et al.

Summary: The study utilizes a novel self-supported CoS2/carbon composite nanotube arrays electrode as the cathode for MLIB, delivering high specific capacity, impressive long cycling life, superior energy density, and good rate capability. The even distribution of active nanoparticles in nanotube arrays and the inhibition of polysulfide intermediates dissolution by N-doped amorphous carbon contribute to the excellent performance of the cathodes.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Mo-doped VS4 with interlayer-expanded and engineering sulfur vacancies as cathode for advanced magnesium storage

Shiqi Ding et al.

Summary: Mo-doping in VS4 shortens the diffusion path for fast reaction kinetics, maintains the structure stability, and provides more active sites for increasing reversible capacity, resulting in excellent electrochemical properties. This design strategy of metal ion doping provides a favorable reference for developing various alkali metal ion batteries.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

A Polymorphic FeS2 Cathode Enabled by Copper Current Collector Induced Displacement Redox Mechanism

Lulu Tan et al.

Summary: In this work, a composite of pyrite (P-FeS2) and marcasite (M-FeS2) was fabricated for high-performance Li-FeS2 battery, with a high specific capacity of 894 mAh/g and specific energy over 1300 Wh/kg. The electrochemical irreversibility was found to be primarily caused by the shuttle effect, which was addressed by using a Cu current collector to chemically immobilize lithium polysulfides and fundamentally alter the reaction pathway, leading to superior rate capability and long lifespan of the composite.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

A Pyrite Iron Disulfide Cathode with a Copper Current Collector for High-Energy Reversible Magnesium-Ion Storage

Yinlin Shen et al.

Summary: Pyrite FeS2 shows great promise as a cathode material in high-energy metal-anode-based rechargeable batteries due to its low cost, high theoretical capacity, and environmentally friendly characteristics. The use of a copper current collector in FeS2 cathodes for rechargeable magnesium batteries enables significantly enhanced reversible capacity and superior energy density compared to previously reported metal chalcogenide cathodes. This high-performance FeS2 cathode can operate over 1000 cycles with good capacity retention, demonstrating its potential for practical applications in energy storage systems.

ADVANCED MATERIALS (2021)

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Article Energy & Fuels

Rational Synthesis of Fern Leaf-like FeS2@Sulfur-Doped Carbon as an Anode for Superior Lithium-Ion Batteries

Wen Chen et al.

Summary: The fern leaf-like FeS2@ sulfur-doped carbon composite shows enhanced electrochemical performance in lithium-ion batteries due to the synergistic effect of the hierarchical microstructure of FeS2 and the sulfur-doped carbon coating layer, delivering high initial discharge capacities and superior rate capability and cyclability.

ENERGY & FUELS (2021)

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Review Chemistry, Physical

A Brief Review on Solid Electrolyte Interphase Composition Characterization Technology for Lithium Metal Batteries: Challenges and Perspectives

Xinyi Shan et al.

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Amorphous Redox-Rich Polysulfides for Mg Cathodes

Minglei Mao et al.

Summary: The article proposes a strategy of utilizing amorphization and anion enrichment in cathode materials to enhance the performance of Mg batteries. The designed amorphous titanium polysulfides show significant advantages in energy density, demonstrating competitive potential.

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Article Chemistry, Physical

Polyaniline-coated VS4@rGO nanocomposite as high-performance cathode material for magnesium batteries based on Mg2+/Li+ dual ion electrolytes

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IONICS (2020)

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Morphology-dependent electrochemical performance of VS4 for rechargeable magnesium battery and its magnesiation/demagnesiation mechanism

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JOURNAL OF POWER SOURCES (2020)

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Nanosized FeS2 Particles Caged in the Hollow Carbon Shell as a Robust Polysulfide Adsorbent and Redox Mediator

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NATURE ENERGY (2020)

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Joint Cationic and Anionic Redox Chemistry for Advanced Mg Batteries

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NANO LETTERS (2020)

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Studies of FeSe2Cathode Materials for Mg-Li Hybrid Batteries

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ENERGIES (2020)

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Self-supported PPy-encapsulated CoS2 nanosheets anchored on the TiO2-x nanorod array support by Ti-S bonds for ultra-long life hybrid Mg2+/Li+ batteries

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JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Exploring Cation-Anion Redox Processes in One-Dimensional Linear Chain Vanadium Tetrasulfide Rechargeable Magnesium Ion Cathodes

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Electrochemical intercalations of divalent ions inside Ni/Zn co-doped cobalt sulfide nanoparticle decorated carbon spheres with superior capacity

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Interchain-Expanded Vanadium Tetrasulfide with Fast Kinetics for Rechargeable Magnesium Batteries

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ACS APPLIED MATERIALS & INTERFACES (2019)

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A Crosslinked Polytetrahydrofuran-Borate-Based Polymer Electrolyte Enabling Wide-Working-Temperature-Range Rechargeable Magnesium Batteries

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Hybrid Mg/Li-ion batteries enabled by Mg2+/L+ co-intercalation in VS4 nanodendrites

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CoSe2 hollow microspheres, nano-polyhedra and nanorods as pseudocapacitive Mg-storage materials with fast solid-state Mg2+ diffusion kinetics

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Cobalt Disulfide Nanoparticles Embedded in Porous Carbonaceous Micro-Polyhedrons Interlinked by Carbon Nanotubes for Superior Lithium and Sodium Storage

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Aobing Du et al.

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Article Chemistry, Physical

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Highly active electrolytes for rechargeable Mg batteries based on a [Mg2(μ-Cl)2]2+ cation complex in dimethoxyethane

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A comparison between the electrochemical behavior of reversible magnesium and lithium electrodes

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